Refine your search:     
Report No.
 - 
Search Results: Records 1-20 displayed on this page of 48

Presentation/Publication Type

Initialising ...

Refine

Journal/Book Title

Initialising ...

Meeting title

Initialising ...

First Author

Initialising ...

Keyword

Initialising ...

Language

Initialising ...

Publication Year

Initialising ...

Held year of conference

Initialising ...

Save select records

Journal Articles

Study on heat transfer behavior of a rectangular particle bed with volumetric heating

Wen, J.*; Kamada, Yuto*; Yokoyama, Kosei*; Matsumoto, Tatsuya*; Liu, W.*; Morita, Koji*; Imaizumi, Yuya; Tagami, Hirotaka; Matsuba, Kenichi; Kamiyama, Kenji

Proceedings of 31st International Conference on Nuclear Engineering (ICONE31) (Internet), 8 Pages, 2024/08

Journal Articles

Lanthanide extraction using a thiodiglycolamic acid extractant; Effect of S-donor on lanthanide separation

Shimojo, Kojiro; Fujiwara, Iori*; Oshima, Tatsuya*; Yokoyama, Keiichi; Yaita, Tsuyoshi

Analytical Sciences, 38(7), p.1003 - 1006, 2022/07

 Times Cited Count:0 Percentile:0.00(Chemistry, Analytical)

Liquid-liquid extraction of lanthanide (Ln) ions was investigated using $$N,N$$-dioctylthiodiglycolamic acid (DOTDGAA), which is a sulfur donor ligand with an amide group and a carboxyl group connected by a thioether chain. The extraction performance and selectivity of DOTDGAA for Ln ions were compared with those of $$N,N$$-dioctyldiglycolamic acid (DODGAA), which is also an oxygen donor ligand with a similar chemical structure, to assess the effect of the soft/hard donor atom on Ln separation. DOTDGAA quantitatively extracted all Ln ions while being selective toward light and middle Ln ions, in contrast to the selectivity of DODGAA for heavier Ln ions. Slope analysis demonstrated that the Ln$$^{3+}$$ transfer using DOTDGAA proceeded through a proton-exchange reaction, forming a 1:3 complex, Ln(DOTDGAA)$$_{3}$$. The back-extraction of Ln ions from the extracting phase was successfully achieved under acidic conditions.

Journal Articles

Isotope-selective ionization utilizing field-free alignment of isotopologues with a train of femtosecond laser pulses

Akagi, Hiroshi; Kasajima, Tatsuya*; Kumada, Takayuki; Itakura, Ryuji; Yokoyama, Atsushi; Hasegawa, Hirokazu*; Oshima, Yasuhiro*

Physical Review A, 91(6), p.063416_1 - 063416_7, 2015/06

 Times Cited Count:7 Percentile:38.53(Optics)

We propose a strategy of isotope-selective ionization for a binary mixture of isotopologues of homonuclear diatomic molecules, utilizing field-free alignment with a train of femtosecond laser pulses. Field-free alignment can be achieved simultaneously for two isotopologues consisting of two atoms with the same atomic mass number $$alpha$$ or $$beta$$, utilizing a pulse train with their time interval of T$$_{com}$$ = $$beta$$ T($$alpha$$) = $$alpha$$ T($$beta$$), where T($$alpha$$) and T($$beta$$) are the rotational revival times of the isotopologues. We demonstrate experimentally that a train of four alignment pulses with their interval of T$$_{com}$$ ($$alpha$$ = 14, $$beta$$ = 15) creates transiently aligned $$^{14}$$N$$_{2}$$ and anti-aligned $$^{15}$$N$$_{2}$$ just before T$$_{com}$$/2 after the last pulse, and vice versa just after T$$_{com}$$/2. Highly isotope-selective N$$_{2}$$ ionization is achieved at these timings with another femtosecond laser pulse, which induces the non-resonant multiphoton ionization with the cross section remarkably depending on the angle between the molecular axis and the laser electric field direction. The ion yield ratio I($$^{15}$$N$$_{2}$$$$^{+}$$)/I($$^{14}$$N$$_{2}$$$$^{+}$$) ranges from 0.49 to 2.00, which is wider than the range obtained with single alignment pulse.

Journal Articles

X-ray backscattering study of crystal lattice distortion in hidden order of URu$$_2$$Si$$_2$$

Tabata, Chihiro*; Inami, Toshiya; Michimura, Shinji*; Yokoyama, Makoto*; Hidaka, Hiroyuki*; Yanagisawa, Tatsuya*; Amitsuka, Hiroshi*

Philosophical Magazine, 94(32-33), p.3691 - 3701, 2014/00

 Times Cited Count:16 Percentile:59.53(Materials Science, Multidisciplinary)

Journal Articles

In-situ stress measurement in the Mizunami Underground Research Laboratory; A New test of strain sensitivity method applying to CCBO

Tanno, Takeo; Sato, Toshinori; Sanada, Hiroyuki; Hikima, Ryoichi*; Yokoyama, Tatsuya*; Shimoyama, Masahiro*

Heisei-25 Nendo (2013 Nen) Shigen, Sozai Gakkai Shuki Taikai Koenshu, p.255 - 256, 2013/09

${it In-situ}$ rock stresses were measured by Compact Conical-ended Borehole Overcoring (CCBO) technique in the 300m depth gallery at the Mizunami Underground Research Laboratory and the measurement results were evaluated using a conventional method and a new test of strain sensitivity method. To compare the ${it in-situ}$ rock stress evaluated by both methods, the new test of strain sensitivity method resulted in more accurate evaluation than the conventional method, because of its improved stress deviations.

Journal Articles

In situ stress measurement by CCBO in Mizunami Underground Researh Laboratory

Sato, Toshinori; Tanno, Takeo; Sanada, Hiroyuki; Yokoyama, Tatsuya*; Shimoyama, Masahiro*

Heisei-25 Nendo (2013 Nen) Shigen, Sozai Gakkai Shuki Taikai Koenshu, p.257 - 258, 2013/09

Japan Atomic Energy Agency is operating underground research laboratory projects in order to establish a firm scientific basis for safe geological disposal of HLW. One of these is the Mizunami Underground Research Laboratory (MIU) project focused on crystalline rock. In situ stress measurement by Compact Conical-ended Borehole Overcoring (CCBO) are conducted to understand in situ stress state at 300 m depth.

Journal Articles

Change of Si(110) reconstructed structure by Ge nanocluster formation

Yokoyama, Yuta; Yamazaki, Tatsuya; Asaoka, Hidehito

Journal of Crystal Growth, 378, p.230 - 232, 2013/09

 Times Cited Count:2 Percentile:23.49(Crystallography)

The initial processes of Ge nano cluster formation on Si(110)-16$$times$$2 reconstructed structure were investigated via scanning tunneling microscopy. For a small amount of Ge deposited on Si(110)-16$$times$$2 single-domain structure at room temperature, the surface structure did not change significantly. After direct current heating at 973 K for 20 min, the striped structure almost broken and disordered-like structure was formed on the terrace. With increasing the annealing time, the surface structure changed from disordered-like structure to the 16$$times$$2 double-domain structure and pyramidal nano clusters were formed at the domain boundary. These results suggest that the surface stress was induced by Ge nano cluster formation and the double-domain structure was formed in order to relax the stress.

Journal Articles

Direct stress measurement of Si(111) 7$$times$$7 reconstruction

Asaoka, Hidehito; Yamazaki, Tatsuya; Yokoyama, Yuta; Yamaguchi, Kenji

Journal of Crystal Growth, 378, p.37 - 40, 2013/09

 Times Cited Count:3 Percentile:31.80(Crystallography)

We have focused on stress measurements of the reconstructed Si(111) 7$$times$$7 and the H-terminated Si(111) 1$$times$$1 surfaces. In order to obtain information on both the surface stress and the surface structure simultaneously, we have combined the surface-curvature and the reflection-high-electron-energy-diffraction instrumentations in an identical ultrahigh vacuum system. At the beginning of Ge wetting layer growth on H-terminated Si(111), the stress gradient drastically changes accompanied by change in the surface structure resulting from the H desorption. Comparison of the surface stress behaviors between Ge wetting layer growth on the H-terminated Si(111) 1$$times$$1 and the Si(111) 7$$times$$7 surfaces reveals that the Si(111) 1$$times$$1 surface releases 1.6 N/m (=J/m$$^{2}$$), or (1.3 eV/(1$$times$$1 unit cell)), of the surface energy from the strong tensile Si(111) 7$$times$$7 reconstruction.

Journal Articles

Isotope-selective ionization utilizing molecular alignment and non-resonant multiphoton ionization

Akagi, Hiroshi; Kasajima, Tatsuya; Kumada, Takayuki; Itakura, Ryuji; Yokoyama, Atsushi; Hasegawa, Hirokazu*; Oshima, Yasuhiro*

Applied Physics B, 109(1), p.75 - 80, 2012/10

 Times Cited Count:16 Percentile:61.14(Optics)

We demonstrate a laser nitrogen isotope separation, which is based on field-free alignment and angular dependent ionization of $$^{14}$$N$$_{2}$$ and $$^{15}$$N$$_{2}$$ isotopomers. A linearly-polarized short laser pulse ($$lambda$$$$sim$$795 nm, $$Delta$$$$tau$$$$sim$$60 fs) creates rotational wave packets in the isotopomers, which periodically revive with different revival times as a result of different moments of inertia. Another linearly-polarized short laser pulse ($$lambda$$$$sim$$795 nm, $$Delta$$$$tau$$$$sim$$60 fs) ionizes one of the isotopomers selectively as a result of their different angular distributions. In the present experiments, the ion yield ratio $$R$$ [= $$I$$($$^{15}$$N$$_{2}$$$$^{+}$$)/$$I$$($$^{14}$$N$$_{2}$$$$^{+}$$)] can be changed in the range from 0.85 to 1.22, depending on the time delay between the two laser pulses.

Journal Articles

Numerical study on quantum walks implemented on the cascade rotational transitions in a diatomic molecule

Matsuoka, Leo; Kasajima, Tatsuya; Hashimoto, Masashi; Yokoyama, Keiichi

Journal of the Korean Physical Society, 59(4), p.2897 - 2900, 2011/10

 Times Cited Count:13 Percentile:62.04(Physics, Multidisciplinary)

Journal Articles

Numerical study on quantum walks implemented on the cascade rotational transitions in a diatomic molecule

Matsuoka, Leo; Kasajima, Tatsuya; Hashimoto, Masashi; Yokoyama, Keiichi

arXiv.org (Internet), 5 Pages, 2011/04

Journal Articles

Observation of ion cyclotron emission owing to DD fusion product H ions in JT-60U

Sato, Shoichi*; Ichimura, Makoto*; Yamaguchi, Yusuke*; Katano, Makoto*; Imai, Yasutaka*; Murakami, Tatsuya*; Miyake, Yuichiro*; Yokoyama, Takuro*; Moriyama, Shinichi; Kobayashi, Takayuki; et al.

Plasma and Fusion Research (Internet), 5, p.S2067_1 - S2067_4, 2010/12

Ion cyclotron emissions (ICEs) due to deuterium-deuterium fusion-product (FP) ions on JT-60U are studied. ICE due to H-ions is identified from the difference of the toroidal wave number of 2nd ICE(D). The parameter dependence for the appearance of ICE(H) is investigated from the experimental conditions and also is studied by using "Escape Particle Orbit analysis Code (EPOC)".

Journal Articles

Vibration-selective coherent anti-Stokes Raman scattering with linearly chirped white-light pulses

Kasajima, Tatsuya; Yokoyama, Keiichi; Matsuoka, Leo; Yokoyama, Atsushi

Chemical Physics Letters, 485(1-3), p.45 - 48, 2010/01

 Times Cited Count:1 Percentile:3.00(Chemistry, Physical)

Journal Articles

Quantum control of molecular vibration and rotation toward the isotope separation

Yokoyama, Keiichi; Matsuoka, Leo; Kasajima, Tatsuya; Tsubouchi, Masaaki; Yokoyama, Atsushi

Proceedings of 5th Asian Symposium on Intense Laser Science (ASILS-5), p.113 - 119, 2009/05

The current status of the fundamental research for the quantum control conducted at Kansai Photon Science Institute are reported. In particular, the experimental studies on vibrational control of diatomic molecules, the nitrogen molecules and the iodine molecules, and the theoretical study on the rotational control of the diatomic molecule, the cesium iodide molecule (CsI), are introduced. For the study of vibrational control of N$$_{2}$$, the vibration selective excitation with extremely broadband white light pulses is demonstrated by tuning the time interval of a linearly chirped white light pulse pair. For the study of vibrational control of I$$_{2}$$, the direction control of stimulated impulsive Raman transition is demonstrated by changing the sign of the chirp rate. For the study of rotational control of CsI, the isotope-selective population distribution transfer is demonstrated numerically using frequency comb in the terahertz-wave region.

Oral presentation

Studies for isotope separation of radioactive waste

Yokoyama, Keiichi; Kasajima, Tatsuya; Matsuoka, Leo; Hashimoto, Masashi; Tsubouchi, Masaaki; Sugiyama, Akira; Yokoyama, Atsushi

no journal, , 

Technological innovation in the isotope separation of long-lived fission products is demanded. Quantum control may provide a breakthrough in such technology. Recently, we proposed a novel scheme based on cascaded excitation of rotation in diatomic molecules. Both (1) demonstration of quantum walk by Raman transition using a conventional Ti:Sapphire laser and (2) development of high-power terahertz-wave source are concurrently proceeded. (1) Cascaded excitation of rotation in the nitrogen molecule N$$_{2}$$ will be induced by impulsive Raman transitions. At present, we are developing a method to observe the incoherent population distribution among rotational states, which involves femotosecond coherent anti-Stokes Raman scattering. Also, current status of (2) development of high-power terahertz-wave source will be briefly introduced, including optical rectification in ZnTe and LiNbO$$_{3}$$ crystals and a plan for construction of a high-power, picosecond laser as a driver laser.

Oral presentation

Study on quantum walks by rotational transitions in diatomic molecules

Matsuoka, Leo; Kasajima, Tatsuya; Yokoyama, Keiichi

no journal, , 

no abstracts in English

Oral presentation

Study of the ion cyclotron emission due to D-D fusion-product H-ions on JT-60U

Sato, Shoichi*; Ichimura, Makoto*; Yamaguchi, Yusuke*; Katano, Makoto*; Imai, Yasutaka*; Murakami, Tatsuya*; Miyake, Yuichiro*; Yokoyama, Takuro*; Moriyama, Shinichi; Kobayashi, Takayuki; et al.

no journal, , 

Ion cyclotron emissions (ICEs) due to deuterium-deuterium fusion-product (FP) ions on JT-60U are studied. ICE due to H-ions is identified from the difference of the toroidal wave number of 2nd ICE(D). The parameter dependence for the appearance of ICE(H) is investigated from the experimental conditions and also is studied by using "Escape Particle Orbit analysis Code (EPOC)".

Oral presentation

Impulsive stimulated Raman transition of I$$_2$$ in the B $$^3$$$$Pi$$(0$$^+_u$$) state

Matsuoka, Leo; Yokoyama, Keiichi; Kasajima, Tatsuya; Yokoyama, Atsushi

no journal, , 

no abstracts in English

Oral presentation

A New scheme for the laser isotope separation applicable to heavy elements

Yokoyama, Keiichi; Matsuoka, Leo; Kasajima, Tatsuya; Tsubouchi, Masaaki; Hashimoto, Masashi

no journal, , 

Recent progress in laser science enables us precise manipulation of molecules by taking advantages of the wave nature of matter. These techniques are called coherent quantum control. Using coherent quantum control, a breakthrough in laser isotope separation may be realized. Actually, we proposed a novel scheme of isotope selective excitation, which is based on cascaded excitation of rotation in diatomic molecules. A numerical simulation done by solving a coupled Schroedinger equation for the cesium iodide molecule has shown that the separation factor reaches three orders of magnitude higher than that by the conventional scheme. The current status of the experimental demonstration undergoing in our institute will be introduced.

Oral presentation

Time-resolved vibrational CARS for measurement of rotational state distribution

Kasajima, Tatsuya; Yokoyama, Keiichi

no journal, , 

no abstracts in English

48 (Records 1-20 displayed on this page)