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Journal Articles

Conceptual design of the iodine-sulfur process flowsheet with more than 50% thermal efficiency for hydrogen production

Kasahara, Seiji; Imai, Yoshiyuki; Suzuki, Koichi*; Iwatsuki, Jin; Terada, Atsuhiko; Yan, X.

Nuclear Engineering and Design, 329, p.213 - 222, 2018/04

 Times Cited Count:21 Percentile:90.58(Nuclear Science & Technology)

A conceptual design of a practical large scale plant of the thermochemical water splitting iodine-sulfur (IS) process flowsheet was carried out as a heat application of JAEA's commercial high temperature gas cooled reactor GTHTR300C plant design. Innovative techniques proposed by JAEA were applied for improvement of hydrogen production thermal efficiency; depressurized flash concentration H$$_{2}$$SO$$_{4}$$ using waste heat from Bunsen reaction, prevention of H$$_{2}$$SO$$_{4}$$ vaporization from a distillation column by introduction of H$$_{2}$$SO$$_{4}$$ solution from a flash bottom, and I$$_{2}$$ condensation heat recovery in an HI distillation column. Hydrogen of about 31,900 Nm$$^{3}$$/h would be produced by 170 MW heat from the GTHTR300C. A thermal efficiency of 50.2% would be achievable with incorporation of the innovative techniques and high performance HI concentration and decomposition components and heat exchangers expected in future R&D.

Journal Articles

Research on PARC process for future reprocessing

Asakura, Toshihide; Hotoku, Shinobu; Ban, Yasutoshi; Matsumura, Masakazu*; Kim, S.-Y.; Mineo, Hideaki; Morita, Yasuji

Proceedings of International Conference ATALANTE 2004 Advances for Future Nuclear Fuel Cycles, 5 Pages, 2004/06

In JAERI, PARC process based on PUREX technique has been studied to as the basis of future reprocessing. The key of concept is to obtain the products, U and Pu, within only a single extraction cycle by separating Np and Tc from U and Pu before U/Pu partition. Two flow-sheet tests on the process were performed with 44 GWd/t PWR spent-fuel solutions. It was demonstrated that remaining Np in raffinate from co-extraction could be decreased to 13 % compared to the dissolver solution with increased solvent flow rate and with increased nitric acid concentration of FP scrubbing solution. It was demonstrated that Np separation (selective reduction by n-butyraldehyde) efficiency could be improved from 36 % to 78 % by flow-sheet modification; increasing reductant concentration and scrubbing solution flow rate. The feasibility of the Tc separation technique by high acid scrubbing was demonstrated.

Journal Articles

Spent fuel test of an advanced PUREX process:PARC

Mineo, Hideaki; Uchiyama, Gunzo; Hotoku, Shinobu; Asakura, Toshihide; Kihara, Takehiro; ; ; Kimura, Shigeru; ; ; et al.

Proc. of Int. Conf. on Future Nuclear Systems (GLOBAL'99)(CD-ROM), 7 Pages, 1999/00

no abstracts in English

Journal Articles

Visualization of buoyancy-driven exchange flow between helium and air through a small opening

; ; ; ; Fumizawa, Motoo

The 4th Triennial Int. Symp. on Fluid Control,Fluid Measurement,and Visualization; FLUCOME 94, 0, p.691 - 695, 1994/00

no abstracts in English

Journal Articles

Studies on the nickel・iodine・sulfur process for hydrogen production

; Shimizu, Saburo; Nakajima, Hayato; ; Ikezoe, Yasumasa;

Int.J.Hydrogen Energy, 9(3), p.191 - 196, 1984/00

 Times Cited Count:6 Percentile:75.27(Chemistry, Physical)

no abstracts in English

Journal Articles

A Nickel-iodine-sulfur process for hydrogen production

Sato, Shoichi; Shimizu, Saburo; Nakajima, Hayato; Ikezoe, Yasumasa

Int.J.Hydrogen Energy, 8(1), p.15 - 22, 1983/00

 Times Cited Count:13 Percentile:85.63(Chemistry, Physical)

no abstracts in English

JAEA Reports

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