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Sato, Takumi; Shibata, Hiroki; Hayashi, Hirokazu; Takano, Masahide; Kurata, Masaki
Journal of Nuclear Science and Technology, 52(10), p.1253 - 1258, 2015/10
Times Cited Count:6 Percentile:45.29(Nuclear Science & Technology)In order to explore the applicability of the chlorination by MoCl as a potential pretreatment technique for waste treatment of fuel debris by pyrochemical methods, chlorination experiments of UO
and (U
Zr
)O
simulated fuel debris were carried out in two steps: the first one is a chlorination reaction by homogeneous heating, the second one is a volatilization of molybdenum by-product by heating under temperature gradient condition. Most of UO
and (U
Zr
)O
powder were converted to UCl
or UCl
and ZrCl
mixture at 573 K, respectively. In the case of (U
Zr
)O
sintered particle, most of sample was converted to the chlorides because the products evaporated and be separated from sample surface at 773 K, while only the surface of the sample disk was converted to the chlorides at 573 and 673 K. Most of molybdenum by-product and ZrCl
were separated from UCl
by volatilization at 573 K.
Wu, G.; Baba, Yuji; Sekiguchi, Tetsuhiro; Shimoyama, Iwao
Journal of Synchrotron Radiation, 8(Part.2), p.469 - 471, 2001/03
no abstracts in English
Ugajin, Mitsuhiro; Shiba, Koreyuki
Journal of Nuclear Materials, 105(2), p.211 - 218, 1982/00
Times Cited Count:12 Percentile:75.22(Materials Science, Multidisciplinary)no abstracts in English
Katsuta, Hiroji; R.B.McLellan*; Furukawa, Kazuo
Journal of Physics and Chemistry of Solids, 43(6), p.533 - 538, 1982/00
Times Cited Count:39 Percentile:88.17(Chemistry, Multidisciplinary)no abstracts in English
; ;
Physica Status Solidi (B), 113, p.647 - 655, 1982/00
Times Cited Count:17 Percentile:63.75(Physics, Condensed Matter)no abstracts in English