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論文

Producing gold at ISOLDE-CERN

Barzakh, A. E.*; Andreyev, A. N.; Atanasov, D.*; Cubiss, J. G.*; Harding, R. D.*; Al Monthery, M.*; Althubiti, N. A.*; Andel, B.*; 他38名*

Nuclear Instruments and Methods in Physics Research B, 513, p.26 - 32, 2022/02

 被引用回数:0 パーセンタイル:0.02(Instruments & Instrumentation)

The yield of 18 beams of radioactive gold nuclei produced by irradiating the ISOLDE uranium target with 1.4-GeV protons was measured. The production-efficiency dependence on the half-life was derived using the in-target production calculations. Three release models were tested to describe the results. Irregularities in the efficiency curve for 3 long-lived high-spin gold isomers ($$^{187,191,193}$$Au$$^m$$) were found, which require further investigation.

論文

Laser-assisted nuclear decay spectroscopy of $$^{176,177,179}$$Au

Harding, R. D.*; Andreyev, A. N.; Barzakh, A. E.*; Cubiss, J. G.*; Van Duppen, P.*; Al Monthery, M.*; Althubiti, N. A.*; Andel, B.*; 他26名*

Physical Review C, 104(2), p.024326_1 - 024326_16, 2021/08

 被引用回数:3 パーセンタイル:48.27(Physics, Nuclear)

A detailed nuclear spectroscopy study of $$^{176,177,179}$$Au was performed at ISOLDE, CERN. This work provides new insights into the low-lying levels in the daughter nuclei $$^{172,173,175}$$Ir. For $$^{176}$$Au, the nuclear magnetic moments of a high spin and low spin state were determined and used to predict the most likely configuration of each level. Their $$alpha$$-decay branching ratios were also extracted: a 58(5)% branching for the low-spin state, and 29(5)% for the high-spin state.

論文

Laser-assisted decay spectroscopy and mass spectrometry of $$^{178}$$Au

Cubiss, J. G.*; Andreyev, A. N.; Barzakh, A. E.*; Manea, V.*; Al Monthery, M.*; Althubiti, N. A.*; Andel, B.*; Antalic, S.*; 他39名*

Physical Review C, 102(4), p.044332_1 - 044332_12, 2020/10

 被引用回数:5 パーセンタイル:53.56(Physics, Nuclear)

A comprehensive study of the isotope $$^{178}$$Au has been made at the CERN-ISOLDE facility, using resonance laser ionization. Two long-lived states in $$^{178}$$Au were identified - a low-spin ground state and a high-spin isomer - each of which were produced as pure beams. Using the ISOLTRAP precision Penning trap, the excitation energy of the isomeric state in $$^{178}$$Au was determined to be $$E^{*} = $$ 189(14) keV. The $$alpha$$-decay fine structure patterns of the two states were studied using the Windmill decay station, providing information on the low-lying states in the daughter nucleus $$^{174}$$Ir. Nuclear spin assignments of $$I(^{178}$$Au$$^{g}) = (2,3)$$ and $$I(^{178}$$Au$$^{m}) = (7,8)$$ are made based on the observed $$beta$$-decay feeding and hyperfine structure intensity patterns.

論文

Shape coexistence in $$^{187}$$Au studied by laser spectroscopy

Barzakh, A. E.*; Atanasov, D.*; Andreyev, A. N.; Al Monthery, M.*; Althubiti, N. A.*; Andel, B.*; Antalic, S.*; Blaum, K.*; 他34名*

Physical Review C, 101(6), p.064321_1 - 064321_7, 2020/06

 被引用回数:10 パーセンタイル:77.42(Physics, Nuclear)

Hyperfine-structure parameters and isotope shift of the $$9/2^{-}$$ isomeric state in $$^{187}$$Au relative to $$^{197}$$Au for the 267.6-nm atomic transition have been measured for the first time using the in-source resonance-ionization spectroscopy technique. The magnetic dipole moment and change in the mean-square charge radius for this $$9/2^{-}$$ isomer have been deduced. The observed large isomer shift relative to the $$1/2^{+}$$ ground state in $$^{187}$$Au confirms the occurrence of the shape coexistence in $$^{187}$$Au proposed earlier from the analysis of the nuclear spectroscopic data and particle plus triaxial rotor calculations. The analysis of the magnetic moment supports the previously proposed $$9/2^{-}$$, $$1/2^{-}$$[541] assignment at moderate prolate deformation for $$^{187}$$Au$$^{m}$$.

論文

Hyperfine anomaly in gold and magnetic moments of $$I^{pi}$$ = 11/2$$^{-}$$ gold isomers

Barzakh, A. E.*; Atanasov, D.*; Andreyev, A. N.; Al Monthery, M.*; Althubiti, N. A.*; Andel, B.*; Antalic, S.*; Blaum, K.*; 他39名*

Physical Review C, 101(3), p.034308_1 - 034308_9, 2020/03

 被引用回数:20 パーセンタイル:93.27(Physics, Nuclear)

Hyperfine-structure constants for the $$I^{pi}$$ = 11/2$$^{-}$$ gold isomers $$^{177,191,193,195}$$Au$$^{m}$$ have been measured at CERN-ISOLDE, using the in-source laser resonance-ionization spectroscopy technique. From the measured hyperfine constants the differences between hyperfine anomalies have been deduced. These differential hyperfine anomaly values have been used to determine the hyperfine anomaly relative to the stable $$^{197}$$Au with advanced atomic calculations. Magnetic dipole moments for the gold isomers in question have been deduced, taking into account the corresponding relative hyperfine-anomaly values. It has been shown that the commonly used prescription for the extraction of the magnetic moment values for the gold isotopes should be reconsidered. The magnetic moments calculated by this prescription have been reevaluated by properly accounting for the hyperfine anomaly, which is as large as 10% for several gold isotopes.

論文

$$alpha$$-decay branching ratio of $$^{180}$$Pt

Cubiss, J. G.*; Harding, R. D.*; Andreyev, A. N.; Althubiti, N.*; Andel, B.*; Antalic, S.*; Barzakh, A. E.*; Cocolios, T. E.*; Day Goodacre, T.*; Farooq-Smith, G. J.*; et al.

Physical Review C, 101(1), p.014314_1 - 014314_4, 2020/01

 被引用回数:5 パーセンタイル:53.56(Physics, Nuclear)

$$^{180}$$Ptの基底状態から娘核$$^{176}$$Osの基底状態への$$alpha$$崩壊分岐比を0.52(5)%と、過去の値と比較してより高精度で再決定した。$$^{180}$$PtはCERN-ISOLDE実験施設において$$^{180}$$Hgを単離し、その$$beta$$崩壊孫核種として生成した。今回の結果を用いて導出した$$alpha$$崩壊の換算崩壊幅は、中性子欠損Pt同位体の$$alpha$$崩壊幅の系統性について新しい描像を与えることとなった。

論文

Shape staggering of midshell mercury isotopes from in-source laser spectroscopy compared with density-functional-theory and Monte Carlo shell-model calculations

Sels, S.*; Day Goodacre, T.*; Marsh, B. A.*; Pastore, A.*; Ryssens, W.*; 角田 佑介*; Althubiti, N.*; Andel, B.*; Andreyev, A. N.; 他39名*

Physical Review C, 99(4), p.044306_1 - 044306_17, 2019/04

 被引用回数:32 パーセンタイル:95.84(Physics, Nuclear)

Neutron-deficient $$^{177-185}$$Hg isotopes were studied using in-source laser resonance-ionization spectroscopy at the CERN-ISOLDE radioactive ion-beam facility. The endpoint of the odd-even nuclear shape staggering in mercury was observed directly by measuring the isotope shifts and hyperfine structures of $$^{177-185}$$Hg. Changes in the mean-square charge radii for all mentioned isotopes, magnetic dipole, and electric quadrupole moments of the odd-$$A$$ isotopes and arguments in favor of $$I = 7/2$$ spin assignment for $$^{177,179}$$Hg were deduced. Experimental results are compared with density functional theory (DFT) and Monte Carlo shell model (MCSM) calculations. DFT calculations using Skyrme parametrizations predict a jump in the charge radius around the neutron $$N = 104$$ midshell, with an odd-even staggering pattern related to the coexistence of nearly degenerate oblate and prolate minima. This near-degeneracy is highly sensitive to many aspects of the effective interaction, a fact that renders perfect agreement with experiments out of reach for current functionals. MCSM calculations of states with the experimental spins and parities show good agreement for both electromagnetic moments and the observed charge radii. A clear mechanism for the origin of shape staggering within this context is identified: a substantial change in occupancy of the proton $${pi}h_{9/2}$$ and neutron $${nu}i_{13/2}$$ orbitals.

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