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論文

Changes in mean-squared charge radii and magnetic moments of $$^{179-184}$$Tl measured by in-source laser spectroscopy

Barzakh, A.*; Andreyev, A. N.; Cocolios, T. E.*; de Groote, R. P.*; Fedorov, D. V.*; Fedosseev, V. N.*; Ferrer, R.*; Fink, D. A.*; Ghys, L.*; Huyse, M.*; et al.

Physical Review C, 95(1), p.014324_1 - 014324_12, 2017/01

 被引用回数:22 パーセンタイル:86.87(Physics, Nuclear)

Hyperfine structure and isotope shifts have been measured for the ground and isomeric states in the neutron deficient isotopes $$^{179-184}$$Tl using the 276.9 nm transition. The experiment has been performed at the CERN Isotope Separator On-Line facility using the in-source resonance-ionization laser spectroscopy technique. Spins for the ground states in $$^{179,181,183}$$Tl have been determined as $$I$$ = 1/2. Magnetic moments and changes in the nuclear mean-square charge radii have been deduced. By applying the additivity relation for magnetic moments of the odd-odd Tl nuclei the leading configuration assignments were confirmed. A deviation of magnetic moments for isomeric states in $$^{182,184}$$Tl from the trend of the heavier Tl nuclei is observed. The charge radii of the ground states of the isotopes $$^{179-184}$$Tl follow the trend for isotonic (spherical) lead nuclei. The noticeable difference in charge radii for ground and isomeric states of $$^{183,184}$$Tl has been observed, suggesting a larger deformation for the intruder-based 9/2$$^{-}$$ and 10$$^{-}$$ states compared to the ground states. An unexpected growth of the isomer shift for $$^{183}$$Tl has been found.

論文

Measurement of the first ionization potential of astatine by laser ionization spectroscopy

Rothe, S.*; Andreyev, A. N.*; Antalic, S.*; Borschevsky, A.*; Capponi, L.*; Cocolios, T. E.*; De Witte, H.*; Eliav, E.*; Fedorov, D. V.*; Fedosseev, V. N.*; et al.

Nature Communications (Internet), 4, p.1835_1 - 1835_6, 2013/05

 被引用回数:79 パーセンタイル:94.43(Multidisciplinary Sciences)

The radioactive element astatine exists only in trace amounts in nature. Its properties can therefore only be explored by study of smallest quantities of artificially produced isotopes or by performing theoretical calculations. One of the most important properties influencing the chemical behaviour is the energy required to remove one electron from the valence shell, referred to as the ionization potential (IP). Here we use laser spectroscopy to probe the optical spectrum of astatine near the ionization threshold. The observed series of Rydberg states allowed the deduction of the IP of the astatine atom for the first time. New ab initio calculations were performed to support the experimental result. The measured value of IP(At) serves as a benchmark for quantum chemistry calculations of the properties of astatine as well as for the theoretical prediction of the ionization potential of super-heavy element 117, the heaviest homologue of astatine.

論文

Results of aerosol code comparisons with releases from ACE MCCI tests

Fink, J. K.*; Corradini, M.*; 日高 昭秀; Honta$~n$$'o$n, E.*; Mignanelli, M. A.*; Schr$"o$dl, E.*; Strizhov, V.*

KfK-5108; NEA/CSNI/R(92)10, p.533 - 546, 1992/00

米国EPRIが主催する先進格納容器実験ACE計画では、シビアアクシデントの影響評価とアクシデントマネジメント対策の検討に資するため、その一環として溶融炉心/コンクリート反応に関する実験と計算コードの比較を行った。計算コードの比較は、制御棒材を含むコリウム溶融物とケイ土系コンクリートとの相互作用を調べたL6実験に対するブラインド計算として行われ、英国,ドイツ,スペイン,日本,ロシア,米国がSOLGASMIX, VANESA1.01, CORCON2.04/VANESA1.01, CORCON.UW等の各コードを用いて参加した。日本からは、JAERIがVANESA1.01コードを用いて参加した。その結果、高揮発性のAg, In, Teについては、計算結果と実験結果の差が1桁以内でほぼ一致した。しかしながら、中揮発性のBa, Srでは1桁から3桁の差が生じ、低揮発性のMoでは約5桁の差が見られた。FP以外では、特にSiの放出において、Zr-Si間の化学反応を適切に考慮しているSOLGASMIXコードの方が、その一部しか考慮していないVANESAコードよりも実験結果との差が小さかった。

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