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論文

Phonon softening in Lu(Pt$$_{1-x}$$Pd$$_x$$)$$_2$$In close to a zero-temperature structural instability

Gruner, T.*; Lucas, S.*; Geibel, C.*; 金子 耕士; 筒井 智嗣*; Schmalzl, K.*; Stockert, O.*

Physical Review B, 106(11), p.115142_1 - 115142_6, 2022/09

 被引用回数:1 パーセンタイル:18.86(Materials Science, Multidisciplinary)

The disappearance of a charge-density-wave (CDW) transition in Lu(Pt$$_{1-x}$$Pd$$_x$$)$$_2$$In is thought to be closely linked to a maximum of the superconducting transition temperature in the system. We studied the superstructure and the phonon softening in Lu(Pt$$_{0.5}$$Pd$$_{0.5}$$)$$_2$$In by means of neutron and high-resolution inelastic X-ray scattering. A full phonon softening at $$q_{textrm{CDW}}$$ = (0.5, 0.5, 0) with the appearance of superstructure peaks could be clearly identified. The large tail of the superstructure intensity above the CDW transition indicates the importance of critical fluctuations.

論文

Photoelectron diffraction for probing valency and magnetism of 4$$f$$-based materials; A View on valence-fluctuating EuIr$$_2$$Si$$_2$$

Usachov, D. Yu*; Tarasov, A. V.*; Schulz, S.*; Bokai, K. A.*; Tupitsyn, I. I.*; Poelchen, G.*; Seiro, S.*; Caroca-Canales, N.*; Kliemt, K.*; Mende, M.*; et al.

Physical Review B, 102(20), p.205102_1 - 205102_11, 2020/11

 被引用回数:9 パーセンタイル:54.31(Materials Science, Multidisciplinary)

Using photoelectron diffraction (PED) and magnetic dichroism measurements, we explore the electronic and magnetic properties of the near-surface region of the valence-fluctuating material EuIr$$_2$$Si$$_2$$. We present and discuss the methodology for modeling of the 4$$f$$ photoemission spectra, PED patterns and magnetic dichroism for rare-earth-based materials. For the Eu-terminated surface we found that the topmost Eu layer is divalent and exhibits a ferromagnetic order below 10 K. The valency of the next Eu layer, that is the 5th atomic layer, is about 2.8 at low temperature that is close to the valency in the bulk. The properties of the Si-terminated surface are drastically different. The first subsurface Eu layer (4th atomic layer below the surface) behaves divalently and orders ferromagnetically at much higher temperature. Experimental data indicate, however, that there is an admixture of trivalent Eu in this layer, resulting in its valency of about 2.1. The next deeper lying Eu layer (8th atomic layer below the surface) behaves mixed-valently, but the estimated valency of 2.4 is notably lower than the value in the bulk. The obtained results create a background for further studies of exotic surface properties of 4$$f$$-based materials, and allow to derive information related to valency and magnetism of individual rare-earth layers in a rather extended area near the surface.

論文

Electromagnetic properties of low-lying states in neutron-deficient Hg isotopes; Coulomb excitation of $$^{182}$$Hg, $$^{184}$$Hg, $$^{186}$$Hg and $$^{188}$$Hg

Wrzosek-Lipska, K.*; Rezynkina, K.*; Bree, N.*; Zieli$'n$ska, M.*; Gaffney, L. P.*; Petts, A.*; Andreyev, A. N.; Bastin, B.*; Bender, M.*; Blazhev, A.*; et al.

European Physical Journal A, 55(8), p.130_1 - 130_23, 2019/08

 被引用回数:10 パーセンタイル:75.05(Physics, Nuclear)

The neutron-deficient mercury isotopes serve as a classical example of shape coexistence, whereby at low energy near-degenerate nuclear states characterized by different shapes appear. The electromagnetic structure of even-mass $$^{182-188}$$Hg isotopes was studied using safe-energy Coulomb excitation of neutron-deficient mercury beams delivered by the REX-ISOLDE facility at CERN. The population of 0$$^{+}_{1,2}$$, 2$$^{+}_{1,2}$$, and 4$$^{+}_{1}$$ states was observed in all nuclei under study. Reduced $$E2$$ matrix elements coupling populated yrast and non-yrast states were extracted, including their relative signs. These are a sensitive probe of shape coexistence and may be used to validate nuclear models. The experimental results are discussed in terms of mixing of two different configurations and are compared with three different model calculations: the Beyond Mean Field model, the Interacting Boson Model with configuration mixing and the General Bohr Hamiltonian. Partial agreement with experiment was observed, hinting to missing ingredients in the theoretical descriptions.

論文

Divalent EuRh$$_2$$Si$$_2$$ as a reference for the Luttinger theorem and antiferromagnetism in trivalent heavy-fermion YbRh$$_2$$Si$$_2$$

G$"u$ttler, M.*; Generalov, A.*; 藤森 伸一; Kummer, K.*; Chikina, A.*; Seiro, S.*; Danzenb$"a$cher, S.*; Koroteev, Yu. M.*; Chulkov, E. V.*; Radovic, M.*; et al.

Nature Communications (Internet), 10, p.796_1 - 796_7, 2019/02

 被引用回数:9 パーセンタイル:59.99(Multidisciplinary Sciences)

Application of the Luttinger Theorem (LT) to the canonical heavy-fermion Kondo Lattice (KL) material YbRh$$_2$$Si$$_2$$ suggests that its large 4f-derived Fermi surface (FS) in the paramagnetic (PM) regime should be similar in shape and volume to that of the divalent local moment anti-ferromagnet (AFM) EuRh$$_2$$Si$$_2$$ in its PM regime. This leads to the tempting opportunity to explore a new experimental realization of the LT in general and how the large FS may change upon the AFM transition below 70 mK in YbRh$$_2$$Si$$_2$$ in particular. A detailed knowledge of the FS reconstruction might be essential to disclose the properties of this phase, which is a precursor of quantum criticality and superconductivity. Using angle-resolved photoemission spectroscopy (ARPES), we observe a large FS for PM EuRh$$_2$$Si$$_2$$ essentially the same as the one seen in YbRh$$_2$$Si$$_2$$ in the KL state at a temperature of 1 K. Across the EuRh$$_2$$Si$$_2$$ AFM transition we found an extensive fragmentation of the FS due to Brillouin zone folding, intersection and resulting hybridization of the Doughnut and Jungle gym Fermi-surface sheets. Our results on EuRh$$_2$$Si$$_2$$ indicate that the formation of the AFM state in YbRh$$_2$$Si$$_2$$ is very likely also connected with large changes in the FS, which have to be taken into account in the controversial analysis and discussion of anomalies observed at the quantum critical point in this system.

論文

Collectivity in the light radon nuclei measured directly via Coulomb excitation

Gaffney, L. P.*; Robinson, A. P.*; Jenkins, D. G.*; Andreyev, A. N.; Bender, M.*; Blazhev, A.*; Bree, N.*; Bruyneel, B.*; Butler, P.*; Cocolios, T. E.*; et al.

Physical Review C, 91(6), p.064313_1 - 064313_11, 2015/06

 被引用回数:8 パーセンタイル:51(Physics, Nuclear)

Radioactive ion beams of $$^{202,204}$$Rn were studied by means of low-energy Coulomb excitation at REX-ISOLDE, CERN. The electric-quadrupole (E2) matrix elements connecting the first excited 2$$^+$$ to the ground state of these nuclei was extracted, which permits to determine the collectivity of these isotopes, which in both cases is deduced to be weak, as expected from the low-lying level-energy scheme. Comparisons were also made with beyond-mean-field model calculations and the magnitude of the transitional quadrupole moments are well reproduced.

論文

Magnetic transitions in YbCo$$_2$$Si$$_2$$

金子 耕士; Stockert, O.*; Mufti, N.*; Kiefer, K.*; Klingner, C.*; Krellner, C.*; Geibel, C.*; Steglich, F.*

Journal of Physics; Conference Series, 200, p.032031_1 - 032031_4, 2010/02

 被引用回数:5 パーセンタイル:84.54

YbCo$$_2$$Si$$_2$$ with the tetragonal ThCr$$_2$$Si$$_2$$-type structure is an isoelectronic compound to YbRh$$_2$$Si$$_2$$. At zero magnetic field YbCo$$_2$$Si$$_2$$ undergoes two magnetic transitions at $$T_{rm N, L}$$=0.9,K and $$T_{rm N, H}$$=1.7,K,and exhibits a complex magnetic phase diagram for small applied fields, lower than ${textit{textbf{B}}}$=2,T. Therefore, YbCo$$_2$$Si$$_2$$ is not only a good reference to YbRh$$_2$$Si$$_2$$ but also an interesting system in its own to study its magnetic properties. In order to reveal the magnetic structure of YbCo$$_2$$Si$$_2$$, a neutron powder diffraction experiment was carried out. At zero field, several superlattice reflections were clearly observed at 0.5,K. By heating up to 1.1,K, to the intermediate phase, a substantial change in both, the peak position and the intensity ratio of the magnetic reflection was found. We will propose a possible magnetic structure for both phases.

口頭

YbCo$$_2$$Si$$_2$$における磁気転移

金子 耕士; Stockert, O.*; Mufti, N.*; Kiefer, K.*; Klingner, C.*; Krellner, C.*; Geibel, C.*; Steglich, F.*

no journal, , 

YbCo$$_2$$Si$$_2$$は、$$T_{rm N,L}$$=0.9K, $$T_{rm N,H}$$=1.7Kの2段の磁気転移を示すことが明らかとなった。また2T以下の低磁場で多段の磁気転移を示す、複雑な磁気相図が報告された。YbCo$$_2$$Si$$_2$$の磁気構造の決定とともに、この系の磁気相互作用を明らかにする目的で、中性子回折実験を行った。実験は、ベルリンのBER-II原子炉に設置されたE2において行った。粉末中性子回折パターンから、常磁性状態(2.0K)の結果を差し引いたものにおいて、明瞭な磁気反射の観測に成功した。0.48Kで観測された磁気反射は、1.1Kへの昇温に伴い、低角側にシフトするとともに、その強度比が大きく変化することを見いだした。今回観測された磁気反射は、磁気秩序を示す他の$$R$$Co$$_2$$Si$$_2$$($$R$$=希土類)において観測される100, 001とは異なっており、YbCo$$_2$$Si$$_2$$の磁気秩序相は、単純な整合反強磁性構造ではないことを示している。当日は単結晶の結果と合わせて、その磁気構造について報告する。

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