検索対象:     
報告書番号:
※ 半角英数字
 年 ~ 
 年
検索結果: 12 件中 1件目~12件目を表示
  • 1

発表形式

Initialising ...

選択項目を絞り込む

掲載資料名

Initialising ...

発表会議名

Initialising ...

筆頭著者名

Initialising ...

キーワード

Initialising ...

使用言語

Initialising ...

発行年

Initialising ...

開催年

Initialising ...

選択した検索結果をダウンロード

論文

Direct observation of topological magnon polarons in a multiferroic material

Bao, S.*; Gu, Z.-L.*; Shangguan, Y.*; Huang, Z.*; Liao, J.*; Zhao, X.*; Zhang, B.*; Dong, Z.-Y.*; Wang, W.*; 梶本 亮一; et al.

Nature Communications (Internet), 14, p.6093_1 - 6093_9, 2023/09

Magnon polarons are novel elementary excitations possessing hybrid magnonic and phononic signatures, and are responsible for many exotic spintronic and magnonic phenomena. Despite long-term sustained experimental efforts in chasing for magnon polarons, direct spectroscopic evidence of their existence is hardly observed. Here, we report the direct observation of magnon polarons using neutron spectroscopy on a multiferroic Fe$$_{2}$$Mo$$_{3}$$O$$_{8}$$ possessing strong magnon-phonon coupling. Specifically, below the magnetic ordering temperature, a gap opens at the nominal intersection of the original magnon and phonon bands, leading to two separated magnon-polaron bands. Each of the bands undergoes mixing, interconverting and reversing between its magnonic and phononic components. We attribute the formation of magnon polarons to the strong magnon-phonon coupling induced by Dzyaloshinskii-Moriya interaction. Intriguingly, we find that the band-inverted magnon polarons are topologically nontrivial. These results uncover exotic elementary excitations arising from the magnon-phonon coupling, and offer a new route to topological states by considering hybridizations between different types of fundamental excitations.

論文

Two-step Mott transition in Ni(S,Se)$$_2$$; $$mu$$SR studies and charge-spin percolation model

Sheng, Q.*; 金子 竜也*; Yamakawa, Kohtaro*; Guguchia, Z.*; Gong, Z.*; Zhao, G.*; Dai, G.*; Jin, C.*; Guo, S.*; Fu, L.*; et al.

Physical Review Research (Internet), 4(3), p.033172_1 - 033172_14, 2022/09

A pyrite system NiS$$_{2-x}$$Se$$_x$$ exhibits a bandwidth controlled Mott transition via (S,Se) substitutions in a two-step process: the antiferromagnetic insulator (AFI) to antiferromagnetic metal (AFM) transition at $$xsim$$0.45 followed by the AFM to paramagnetic metal (PMM) transition at $$xsim$$1.0. Among a few other Mott systems which exhibit similar two-step transitions, Ni(S,Se)$$_2$$ is of particular interest because a large intermediate AFM region in the phase diagram would provide unique opportunities to study the interplay between the spin and charge order. By comparing and combining our muon spin relaxation studies and previous neutron scattering studies, here we propose a picture where the spin order is maintained by the percolation of "nonmetallic" localized and dangling Ni moments surrounded by S, while the charge transition from AFI to AFM is caused by the percolation of the conducting paths generated by the Ni-Se-Ni bonds.

論文

Field-tuned magnetic structure and phase diagram of the honeycomb magnet YbCl$$_3$$

Hao, Y. Q.*; Wo, H. L.*; Gu, Y. M.*; Zhang, X. W.*; Gu, Y. Q.*; Zheng, S. Y.*; Zhao, Y.*; Xu, G. Y.*; Lynn, J. W.*; 中島 健次; et al.

Science China; Physics, Mechanics & Astronomy, 64(3), p.237411_1 - 237411_6, 2021/03

 被引用回数:3 パーセンタイル:62.6(Physics, Multidisciplinary)

We report thermodynamic and neutron diffraction measurements on the magnetic ordering properties of the honeycomb lattice magnet YbCl$$_3$$. We find YbCl$$_3$$ exhibits a N${'e}$el type long-range magnetic order at the wavevector (0, 0, 0) below T$$_N$$ = 600 mK. This magnetic order is associated with a small sharp peak in heat capacity and most magnetic entropy release occurs above the magnetic ordering temperature. The magnetic moment lies in-plane, parallel to the monoclinic a-axis, whose magnitude m$$_{rm Yb}$$ = 0.86(3) $$mu_B$$ is considerably smaller than the expected fully ordered moment of 2.24 $$mu_B$$ for the doublet crystal-field ground state. The magnetic ordering moment gradually increases with increasing magnetic field perpendicular to the ab-plane, reaching a maximum value of 1.6(2) $$mu_B$$ at 4 T, before it is completely suppressed above $$sim$$9 T. These results indicate the presence of strong quantum fluctuations in YbCl$$_3$$.

論文

Coordination number regulation of molybdenum single-atom nanozyme peroxidase-like specificity

Wang, Y.*; Jia, G.*; Cui, X.*; Zhao, X.*; Zhang, Q.*; Gu, L.*; Zheng, L.*; Li, L. H.*; Wu, Q.*; Singh, D. J.*; et al.

Chem, 7(2), p.436 - 449, 2021/02

 被引用回数:147 パーセンタイル:99.8(Chemistry, Multidisciplinary)

Nanozymes are promising alternatives to natural enzymes, but their use remains limited owing to poor specificity. Overcoming this is extremely challenging due to the intrinsic structural complexity of these systems. We report theoretical design and experimental realization of a series of heterogeneous molybdenum single-atom nanozymes (named Mo$$_{rm{SA}}$$-N$$_{x}$$-C), wherein we find that the peroxidase-like specificity is well regulated by the coordination numbers of single Mo sites. The resulting Mo$$_{rm{SA}}$$-N$$_{3}$$-C catalyst shows exclusive peroxidase-like behavior. It achieves this behavior via a homolytic pathway, whereas Mo$$_{rm{SA}}$$-N$$_{2}$$-C and Mo$$_{rm{SA}}$$-N$$_{4}$$-C catalysts have a different heterolytic pathway. The mechanism of this coordination-number-dependent enzymatic specificity is attributed to geometrical structure differences and orientation relationships of the frontier molecular orbitals.

論文

General synthesis of single-atom catalysts for hydrogen evolution reactions and room-temperature Na-S batteries

Lai, W.-H.*; Wang, H.*; Zheng, L.*; Jiang, Q.*; Yan, Z.-C.*; Wang, L.*; 吉川 浩史*; 松村 大樹; Sun, Q.*; Wang, Y.-X.*; et al.

Angewandte Chemie; International Edition, 59(49), p.22171 - 22178, 2020/12

 被引用回数:64 パーセンタイル:95.63(Chemistry, Multidisciplinary)

Herein, we report a comprehensive strategy to synthesize a full range of single-atom metals on carbon matrix, including V, Mn, Fe, Co, Ni, Cu, Ge, Mo, Ru, Rh, Pd, Ag, In, Sn, W, Ir, Pt, Pb, and Bi. The extensive applications of various single-atom catalysts (SACs) are manifested via their ability to electro-catalyze typical hydrogen evolution reactions (HER) and conversion reactions in novel room-temperature sodium sulfur batteries (RT-Na-S). The enhanced performances for these electrochemical reactions arisen from the ability of different single active atoms on local structures to tune their electronic configuration. Significantly, the electrocatalytic behaviors of diverse SACs, assisted by density functional theory calculations, are systematically revealed by in situ synchrotron X-ray diffraction and in situ transmission electronic microscopy, providing a strategic library for the general synthesis and extensive applications of SACs in energy conversion and storage.

論文

Diluted ferromagnetic semiconductor Li(Zn,Mn)P with decoupled charge and spin doping

Deng, Z.*; Zhao, K.*; Gu, B.; Han, W.*; Zhu, J. L.*; Wang, X. C.*; Li, X.*; Liu, Q. Q.*; Yu, R. C.*; 後神 達郎*; et al.

Physical Review B, 88(8), p.081203_1 - 081203_5, 2013/08

 被引用回数:71 パーセンタイル:91.9(Materials Science, Multidisciplinary)

We report the discovery of a diluted magnetic semiconductor, Li(Zn,Mn)P, in which charge and spin are introduced independently via lithium off-stoichiometry and the isovalent substitution of Mn$$^{2+}$$ for Zn$$^{2+}$$, respectively. Isostructural to (Ga,Mn)As, Li(Zn,Mn)P was found to be a ${it p}$-type ferromagnetic semiconductor with excess lithium providing charge doping. First-principles calculations indicate that excess Li is favored to partially occupy the Zn site, leading to hole doping. Ferromagnetism with Curie temperature up to 34 K is achieved while the system still shows semiconducting transport behavior.

論文

Anisotropic two-dimensional electron gas at the LaAlO$$_{3}$$/SrTiO$$_{3}$$ (110) interface

Annadi, A.*; Zhang, Q.*; Renshaw Wang, X.*; Tuzla, N.*; Gopinadhan, K.*; L$"u$, W. M.*; Roy Barman, A.*; Liu, Z. Q.*; Srivastava, A.*; Saha, S.*; et al.

Nature Communications (Internet), 4, p.1838_1 - 1838_7, 2013/05

 被引用回数:94 パーセンタイル:94.71(Multidisciplinary Sciences)

We report the observation of unexpected conductivity at the LaAlO$$_{3}$$/SrTiO$$_{3}$$ interface prepared on (110)-oriented SrTiO$$_{3}$$, with a LaAlO$$_{3}$$-layer thickness-dependent metal-insulator transition. Density functional theory calculation reveals that electronic reconstruction, and thus conductivity, is still possible at this (110) interface by considering the energetically favourable (110) interface structure, that is, buckled TiO$$_{2}$$/LaO, in which the polarization discontinuity is still present. The conductivity was further found to be strongly anisotropic along the different crystallographic directions with potential for anisotropic superconductivity and magnetism, leading to possible new physics and applications.

論文

Li(Zn,Mn)As as a new generation ferromagnet based on a I-II-V semiconductor

Deng, Z.*; Jin, C. Q.*; Liu, Q. Q.*; Wang, X. C.*; Zhu, J. L.*; Feng, S. M.*; Chen, L. C.*; Yu, R. C.*; Arguello, C.*; 後神 達郎*; et al.

Nature Communications (Internet), 2, p.1425_1 - 1425_5, 2011/08

 被引用回数:150 パーセンタイル:93.71(Multidisciplinary Sciences)

(Ga,Mn)Asは典型的な強磁性III-V族半導体として知られている。これは3価のGa原子を2価のMnで置き換えたものであるが、化学的溶解度が限られているため準安定であり、薄膜でしか製作できないものであった。また電子ドープも行うことができなかった。この困難な条件を超えるため、Masekらは理論的にI-II-V族半導体LiZnAsを提案した。この物質では原子価が等しい(Zn,Mn)の置き換えによる磁性の発現とLi濃度を過剰あるいは不足させることによるキャリアードープを独立に制御可能である。本研究では世界で初めてバルクな状態でのLi$$_{1+y}$$(Zn$$_{1-x}$$Mn$$_x$$)Asの合成に成功した。わずかにLiを過剰にすることで、50Kまでの温度で強磁性が現れること、またp型のキャリアーを持つことが観測され、これらの結果を報告した。

論文

Elongation of plasma channel for electron acceleration

Chen, L.-M.; 中島 一久; Hong, W.*; Hua, J. F.*; 亀島 敬; 小瀧 秀行; 杉山 精博*; Wen, X.*; Wu, Y.*; Tang, C.*; et al.

Chinese Optics Letters, 5(S1), p.S133 - S135, 2007/05

Experiments for the laser guiding studies has been carried out with the 30 fs, 100 TW laser pulse interaction with the long slab and discharged capillary of underdense plasma. Formation of extremely long plasma channel with its length 10 times above the Rayleigh length is observed when the laser pulse power is much higher than the critical power for relativistic self-focusing. The long self-guiding channel formation is accompanied by the quasi-monoenergetic electron acceleration with a low transverse emittance and high electric current (10 nC/shot). In order to continuously elongate plasma channel, a 4 cm-scale discharged capillary was used. We successfully demonstrated laser-plasma acceleration of high-quality electron beams up to nearly GeV. Our results exactly verified the prediction of laser-wakefield acceleration through a cm-scale plasma channel in the blowout bubble regime.

論文

Self-guiding of 100 TW femtosecond laser pulses in centimeter-scale underdense plasma

Chen, L.-M.; 小瀧 秀行; 中島 一久*; Koga, J. K.; Bulanov, S. V.; 田島 俊樹; Gu, Y. Q.*; Peng, H. S.*; Wang, X. X.*; Wen, T. S.*; et al.

Physics of Plasmas, 14(4), p.040703_1 - 040703_4, 2007/04

 被引用回数:36 パーセンタイル:75.67(Physics, Fluids & Plasmas)

レーザーの自己導波の調査のため、長いunderdenseのプラズマと100TWレーザーパルスの相互作用実験を行い、レイリー長の約20倍の10mmという非常に長いプラズマチャネルを観測した。レーザーパルスがチャネル中で曲がること、及び電子キャビティ形成が実験的に初めて観測された。

口頭

Guiding of 100 TW Relativistic Laser Pulses by 10 mm Plasma Channels

Koga, J. K.; Chen, L.-M.; 小瀧 秀行; 中島 一久; Bulanov, S. V.; 田島 俊樹; Gu, Y. Q.*; Peng, H. S.*; Hua, J. F.*; An, W. M.*; et al.

no journal, , 

100TW, 30fsの相対論的強度のレーザーを長いスリットガスジェット(1.2$$times$$10mm$$^{2}$$)へ集光し、レーザー・プラズマ相互作用により電子を発生させる最初の実験を行った。10mmの、レイリー長の20倍となるプラズマチャネルの形成が確認された。このチャネルの特長として、レーザーの偏向,ホース効果,キャビティの形成が確認された。この長いチャネルの形成と同時にコリメートされた(エミッタンス0.8$$pi$$mm mrad),高エネルギーの準単色電子($$sim$$70MeV)の発生が確認された。このときの1MeV以上の電子の電荷量は 10nC/shotであり、これは長いチャネル形成の効果によるものと考えられる。

口頭

センチメートルスケールのキャピラリー放電プラズマチャネルを用いたレーザー電子加速

亀島 敬; 小瀧 秀行; 神門 正城; 大東 出; 川瀬 啓悟; 福田 祐仁; Chen, L. M.*; 本間 隆之; 近藤 修司; Esirkepov, T. Z.; et al.

no journal, , 

レーザープラズマ電子加速は非常に高い電場を持っているが、加速空間が非常に短いという問題点を持っているため、その電子ビームの加速エネルギーは100MeV程度に制限されていた。近年、このレーザープラズマ電子加速が抱える問題点をキャピラリー放電管を用いることで大幅に解決がなされた。プラズマは密度が高いほど屈折率が低くなる特徴を利用して放電管の中でプラズマ密度を中心で薄く、その外周を高く分布させれば光ファイバーと同じ原理でレーザーは放電管内のプラズマ中を集光伝搬しながら相互作用する。ゆえに、加速空間を大幅に拡張することができる。この実験を2006年に中国工程物理研究院とKEK、及び原子力機構で共同実験を行い、キャピラリ放電管を用いて4.4Jのレーザーパルスの集光伝搬及び0.56GeVの電子ビームの生成に成功した。加えて、JAEAにて同様の実験を2007年に行い、1Jのレーザーパルスの集光伝搬及び電子ビームの発生に成功した。

12 件中 1件目~12件目を表示
  • 1