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Noseck, U.*; Sch
fer, T.*; Alonso, U.*; 浜本 貴史*; Havlova, V.*; Hibberd, R.*; 石寺 孝充; 北村 暁; Klajmon, M.*; Missana, T.*; et al.
Applied Geochemistry, 201, p.106762_1 - 106762_23, 2026/04
被引用回数:0 パーセンタイル:0.00グリムゼル試験場(GTS)での長期原位置試験(LIT)および対応するモックアップ実験において、地球化学的条件が変化する環境での
Se(VI)、
Tc(VII)、
U(VI)、
Np(V)、
Am(III)、Th(IV)および
Pu(IV)の挙動をより深く理解するために、熱力学ベンチマーク計算を実施した。本計算では、これらの元素の地球化学的な溶存状態評価モデルとデータベースの状況を確認することも目的としている。これらの実験は、結晶質岩石中に設置されたベントナイト人工バリアを含む放射性廃棄物処分場概念における廃棄体近傍の場をシミュレートしており、その知見は放射性廃棄物処分場の長期安全性評価に貢献する。
Jiang, L.*; Wang, H. H.*; Su, Y. H.; 徐 平光; 篠原 武尚; Xia, B.*; Wang, Y. W.*
Journal of Materials Science, 61(14), p.9754 - 9775, 2026/04
被引用回数:0 パーセンタイル:0.00In this study, pulsed neutron Bragg-edge transmission imaging was employed to characterize plastic deformation of high-manganese austenitic steel during cryogenic impact fracture. Electron backscatter diffraction was used to examine the microstructural evolution. The results reveal that the Bragg-edge width was identified as the critical value for large plastic deformation. Both crack initiation and stable crack growth regions exhibited higher levels of plastic deformation, twin density, and dislocation density compared to unstable crack growth regions. As the test temperature decreased from 273 K to 77 K, the transition point from stable to unstable crack growth occurred earlier. This is responsible for the reduction in impact absorbed energy. These findings provide new insights into the cryogenic toughening mechanism of high-manganese steel.
Mohamad, A. B.; Chen, J.*; 井岡 郁夫*; 鈴木 恵理子; 近藤 啓悦; 阿部 陽介; 山下 真一郎; 大久保 成彰; 根本 義之; 岡田 裕史*; et al.
Journal of Nuclear Materials, 625, p.156513_1 - 156513_9, 2026/04
被引用回数:0 パーセンタイル:0.00(Materials Science, Multidisciplinary)Ion irradiation was carried out on Cr coating Zry cladding to investigate their microstructure evolution and mechanical properties. The sample was irradiated at reactor normal operation conditions. Microstructural observation and mechanical testing of non-irradiated samples and irradiated samples were performed to understand irradiation damage to the Cr-coated Zry cladding. Results of High Resolution Transmission Electron Microscopy and chemical analysis revealed Fe enrichment at the Cr coating and Zr substrate interface of irradiated samples due to irradiation enhanced diffusion or irradiation induced mixing. Irradiation led to the formation of Fe enrichment at the Cr Zr interface approximately 15nm. Moreover, hardening of the Cr coating and Zr substrate regions was observed in the irradiated sample.
J-PARCセンター 安全ディビジョン
JAEA-Review 2025-056, 145 Pages, 2026/03
本報告書は、大強度陽子加速器施設(J-PARC)の安全管理(放射線安全及び一般安全)について2024年度の活動をとりまとめたものである。放射線管理については、施設及び周辺環境の放射線管理、個人線量の管理、放射線安全管理設備の維持・管理等の業務の概要、その他の関連業務について記述した。一般安全については、検討会及び各種専門部会、安全衛生会議、教育・講習会、訓練、さらに安全巡視等について記述した。また、安全文化醸成活動及び安全管理業務に関連して行った技術開発・研究についても、章を分けて記述した。
O
precursors on solid-state formation reactions of (K
Na
)NbO
庄司 琢磨*; Nam, H.*; Ye, J.*; Ito, Daiki*; 高木 優香*; 米田 安宏; 永田 肇*
Journal of the American Ceramic Society, 109(3), p.e70657_1 - e70657_9, 2026/03
被引用回数:0 パーセンタイル:0.00(K,Na)NbO
(KNN)系セラミックスは、優れた圧電特性を有するにもかかわらず、化学的均質性が低いことから、実用的な圧電デバイスへの応用には躊躇されてきた。本研究では、Nb
O
前駆体の役割が製造手法によって異なり、KNNの化学的均質性と強く相関していることを軟X線吸収分光を用いて明らかにした。したがって、Nb
O
前駆体の選択はKNN製造における支配的要因である。
Glazyrin, K.*; Spektor, K.*; Bykov, M.*; Carvalho, P. H. B.*; Dong, W.*; K
rmann, F.*; 佐野 亜沙美; 服部 高典; Beyer, D. C.*; Sahlberg, M.*; et al.
Nature Communications (Internet), 17, p.2622_1 - 2622_10, 2026/03
被引用回数:0 パーセンタイル:0.00高エントロピー材料の研究は様々な科学分野に貢献し、応用面で興味深い特性を次々と明らかにしている。本研究では、高温高圧下におけるX線・中性子飛行時間法実験および第一原理計算により、カンター合金(CoCrFeNiMn)の水素抵抗性を調査した。我々は、カンター合金組成に基づく面心立方(fcc)型水素化物の形成を報告する。さらに、水素含有量の推定を含むその特性評価を提供する。これらの知見は、高エントロピー合金および高エントロピー水素化物の複雑な化学に関する知見の蓄積に貢献するものである。
Zn
Mo
O
Bao, S.*; Liao, J.*; Huang, Z.*; Shangguan, Y.*; Ma, Z.*; Zhang, B.*; Cheng, S.*; Xu, H.*; Song, Z.*; Dong, S.*; et al.
Physical Review Letters, 136(9), p.096502_1 - 096502_8, 2026/03
被引用回数:0 パーセンタイル:0.00Lattice vibrations can carry angular momentum and magnetic moments under broken inversion or time-reversal symmetry, forming so-called chiral phonons. While such excitations have been explored in nonmagnetic systems via optical probes, their direct detection in magnetic materials and coupling to spin excitations remain largely unexplored. Here, using neutron spectroscopy, sensitive to both nuclear and magnetic scattering, we reveal the magnetic signature of chiral phonons in ferrimagnetic Fe
Zn
Mo
O
with Curie temperature
K. Below
, we observe enhanced magnetic scattering of phonons at small momenta, arising from strong magnon-phonon coupling. In addition, out-of-plane intensity modulation, phonon mode splitting, and field-induced Zeeman shifts are observed, all closely associated with the ferrimagnetic order. These features vanish above
, where phonon spectra are dominated by nuclear scattering. These observations demonstrate the existence of chiral phonons carrying substantial magnetic moments that directly contribute to magnetic scattering, and establish neutron spectroscopy as a powerful, momentum-resolved probe of their magnetic character.
Cr
S
Zhao, G.*; Li, J.*; Zhang, J.*; 小嶋 健児*; Cai, Y.*; 伊藤 孝; Yoon, S. W.*; Wang, X.*; 前川 禎通*; Su, G.*; et al.
Physical Review Research (Internet), 8(1), p.013331_1 - 013331_10, 2026/03
Ferrotoroidic materials, which break both time- and space-reversal symmetries to enhance magnetoelectric responses, are of great interest for applications. Ba
Cr
S
, a recently synthesized quasi-one-dimensional ferrotoroidic candidate, combines polarization, magnetization, and toroidal moment, yet its electronic band structure, magnetic evolution, and phase transitions remain incompletely understood to date. Here, we investigate Ba
Cr
S
, using electrical transport, direct current magnetization, alternating current susceptibility, specific heat, and muon spin rotation (
SR) measurements, along with various first-principles calculations. Electrical transport measurements and density functional theory confirm a narrow band gap (
0.707~eV, experimentally;
0.680~eV, theoretically).
SR measurements reveal that static magnetism dominates down to 2~K, with an ordered volume fraction of
89% at this temperature. Two distinct transitions are identified: one around the N
el temperature [
~K] and another corresponding to a phase transition near 30~K, as consistently indicated by our complementary experimental techniques. The absence of dynamic critical behaviors and the lack of a
-type specific heat anomaly are consistent with a first-order-like transition at
. Based on various complementary experimental results and theoretical calculations, we propose a hypothesis that the
30~K broad feature arises from the complex interplay between crystal structure distortion and magnetic coupling, which is potentially directly linked to ferrotoroidicity. As the first study integrating
SR with complementary experiments and first-principles calculations to explore ferrotoroidicity, this work provides key insights into the underlying physics of Ba
Cr
S
and related compounds in this area.
伊東 達矢; 小川 祐平*; Gong, W.; 川崎 卓郎; 柴田 曉伸*; Harjo, S.
Scripta Materialia, 273, p.117084_1 - 117084_6, 2026/03
被引用回数:0 パーセンタイル:0.00(Nanoscience & Nanotechnology)The effect of solute hydrogen on stacking fault evolution in austenitic steels remains debated. In this study, the changes in stacking fault probability in the
111
//loading direction grains family (
) of hydrogen-charged and non-charged Fe-24Cr-19Ni austenitic steels were evaluated using
neutron diffraction during tensile deformation at 223 and 177 K. When
values were plotted against macroscopic strain, hydrogen apparently enhanced stacking fault evolution. However, when identical data were translated into the form of
versus stress, the superficial hydrogen-effect on
notably disappeared. Rather, deformation temperature played more predominant role - lower temperature led to higher
regardless of hydrogen-charging, reflecting the reduction of stacking fault energy with decreasing temperature. These findings demonstrate that hydrogen has a minor effect on stacking fault evolution compared with temperature and applied stress.
Li, H.*; Gong, W.; 川崎 卓郎; Harjo, S.; Zheng, R.*; 他6名*
Acta Materialia, 305, p.121884_1 - 121884_10, 2026/02
被引用回数:0 パーセンタイル:0.00(Materials Science, Multidisciplinary)The quest for lightweight and highly formable magnesium (Mg) alloys has drawn significant attention due to the growing demand for energy-efficient structural materials. Achieving high ductility in Mg at room temperature, which is critical for mass production of structural components, remains a formidable challenge despite decades of research. In this study, we demonstrate super-ductility in an ultrafine-grained (UFG) Mg alloy at room temperature. By microalloying with trace manganese (Mn) and reducing the grain size to sub-micron scale, Mg-0.3Mn binary alloy achieves an exceptional room temperature tensile elongation of 135% at a quasi-static strain rate. Detailed microstructural analysis reveals that grain boundary (GB) sliding, rather than intragranular dislocation slip, is the dominant deformation mechanism in the UFG Mg-0.3Mn alloy. Unlike conventional alloying strategies that lead to GB pinning, the segregation of Mn element along GBs in a manner of nano-clusters could reduce interfacial bonding strength, acting as a lubricant to facilitate GB sliding and thus dramatically boost the ductility. This innovative GB engineering approach unlocks unprecedentedly remarkable deformability of Mg-based alloys at room temperature, paving the way for next-generation lightweight structural applications.
Bess, J. D.*; Shepherd, D.*; McSpaden, A. T.*; 福島 昌宏; 大泉 昭人
International Criticality Safety Benchmark Evaluation Project (ICSBEP) Handbook (2025 edition); NEA/NSC/DOC(95)03/I, Vol.I; PU-MET-FAST-050 (Internet), 544 Pages, 2026/02
本報告は、加速器駆動システム(ADS)の設計において重要となる鉛断面積の積分検証データを取得することを目的としたシリーズ実験に関するものである。本実験キャンペーンでは、高濃縮ウラン、低濃縮ウラン、プルトニウムなど、種々の燃料組成を用い、鉛による高速中性子スペクトル場における系統的なデータが取得された。すべての実験は、JAEAと米国ロスアラモス国立研究所(LANL)の共同研究により国立臨界実験研究センター(NCERC)で実施された。プルトニウム燃料を用いた実験として2種類の炉心が構築され、Jupiter炉心では95wt.%
Puおよび4.5wt.%
Puのプルトニウム金属燃料が使用され、High-240 Pu Jupiter炉心では
Pu高含有のプルトニウム金属燃料(72.8wt.%
Pu, 22wt.%
Pu)が使用された。本ベンチマークレポートは、このうちHigh-240 Pu Jupiter炉心構成に基づく高中性子スペクトル臨界実験の結果を、国際臨界安全評価プロジェクト(ICSBEP)への登録のためにまとめたものである。
Pd in concrete rubble太田 祐貴; Do, V.-K.; Banjarnahor, I. M.; 岩橋 弘之; 古瀬 貴広; 田中 康介
Journal of Radioanalytical and Nuclear Chemistry, 335(1), p.939 - 948, 2026/02
被引用回数:0 パーセンタイル:0.00(Chemistry, Analytical)This paper presents an analytical method for detecting
Pd in concrete using inductively coupled plasma tandem mass spectrometry (ICP-MS/MS). Palladium was purified through an HCl-free chromatographic process utilizing Ni-resin, which was optimized for high and stable chemical recovery. Palladium was effectively retained on the Ni-resin when treated with dilute nitric acid and was subsequently eluted with hot concentrated nitric acid. This approach improved elution efficiency and increased the recovery rate to over 90%. The determination of
Pd via ICP-MS/MS was performed using NH
as a reaction gas. By measuring the mass shift of 51, corresponding to Pd(NH
)
product ions, we successfully eliminated interference from the isobar
Ag. The total interference removal factor for
Ag reached approximately 10,000, demonstrating that the method is highly selective and reliable for quantifying
Pd. The method detection limit for 107Pd in concrete matrices was estimated to be 0.05 Bq g
, indicating its sensitivity to detect low levels of the radionuclide, in compliance with environmental safety regulations. This method is now routinely used to monitor
Pd in concrete samples collected from the Fukushima Daiichi Nuclear Power Station.
underwater radiation monitoring detectorJi, W.*; Lee, E.*; Ji, Y.-Y.*; 越智 康太郎; 吉村 和也; 舟木 泰智; 眞田 幸尚
Nuclear Engineering and Technology, 58(2), p.103933_1 - 103933_6, 2026/02
被引用回数:0 パーセンタイル:0.00(Nuclear Science & Technology)汚染予測地点の河川や貯水池の堆積物中の
Cs放射能濃度を推定するために、水中放射線in-situ検出器MARK-U1(Monitoring of Ambient Radiation of KAERI - Underwater)の性能を検証することを目的とした。さらに、高純度ゲルマニウム(HPGe)半導体検出器を用いて放射能を測定するため、コアサンプルを採取した。放射能を推定するために、測定されたスペクトルと試料中の
Cs放射能を比較して換算係数を導き出した。モンテカルロN粒子(MCNP)シミュレーションを実施し、in-situ測定に有効な線源形状を決定した。シミュレーション結果は、31.62%の偏差で、現場のMARK-U1モニタリング結果とよく相関した。これらの結果は、in-situ検出器の性能を検証するものである。したがって、この装置は、試料採取を必要とせず、in-situモニタリングによって水底堆積物中の
Cs放射能濃度を推定するために使用することができる。
-decay strength of
VDahl, J. K.*; Larsen, A. C.*; 清水 則孝*; 宇都野 穣
Physical Review C, 113(2), p.024328_1 - 024328_16, 2026/02
被引用回数:0 パーセンタイル:0.00
Vに対する核準位密度とガンマ線強度関数を、
-
-
殻をバレンス殻にとった大規模殻模型計算によって調べた。オスロ法による実験データを全体的によく説明し、特に、低エネルギーの
遷移の強度が増大するという特徴を再現することに成功した。そのメカニズムを解明するために、
遷移の行列要素を軌道角運動量部分とスピン角運動量部分に分け、その干渉項の符号の分布を調べた。その結果、低エネルギーガンマ崩壊に対しては、正の干渉が主であるという新しい知見が得られた。
Chen, J.*; 山本 慧; 他13名*
Physical Review Letters, 136(5), p.056702_1 - 056702_8, 2026/02
被引用回数:0 パーセンタイル:0.00(Physics, Multidisciplinary)The recently developed van der Waals magnets provide a promising platform for spintronics and magnonics. Here, we report the observation of surface magnon propagation in the van der Waals antiferromagnet CrSBr. We find a nearly unidirectional propagation of antiferromagnetic magnon modes, which emerge near the anticrossing of the optical and acoustic magnon bands, in agreement with our theory of magnetostatic waves in antiferromagnets. The propagation direction can be reversed by switching the magnetic field. The observed antiferromagnetic magnons operate in the gigahertz regime due to the weak interlayer exchange coupling. Our results open the pathway for nonreciprocal magnonic applications based on van der Waals antiferromagnets at easily-accessible microwave frequencies.
Yao, X.*; Chen, P.*; Verma, R.*; Zhao, X.*; Yang, H.-Y.*; DeBeer-Schmitt, L.*; Aczel, A. A.*; Wu, C.-M.*; Alba-Venero, D.*; 大原 高志; et al.
Physical Review Letters, 136(8), p.086702_1 - 086702_6, 2026/02
We demonstrate that a multi-k incommensurate magnetic state in the Weyl semimetal CeAlGe gives rise to a singular angular magnetoresistance (SAMR), which is an electrical transport signature capable of detecting magnetic field direction with exceptional precision. In contrast, its sister compound CeAlSi is devoid of both multi-k order and SAMR. We reveal that both phenomena appear upon 57% Ge substitution in CeAlSi1-xGex and coincide with electronic structure changes that soften the single-ion in-plane anisotropy and enhance Weyl-mediated magnetic interactions. These results unveil a remarkable connection between band topology, electronic transport, and collective magnetism in Weyl semimetals.
RhZhang, J. Z.*; Chen, Z. Q.*; Qu, T.*; Wang, Y. K.*; Li, Z. H.*; Orlandi, R.; 他62名*
Physics Letters B, 873, p.140144_1 - 140144_9, 2026/02
被引用回数:0 パーセンタイル:0.00(Astronomy & Astrophysics)At the RIKEN,
-delayed
-ray spectroscopy studies were conducted on
Rh and
Rh, resulting in the world's first successful identification of a 1/2
isomer in these isotope, extending the energy difference between the 9/2
and 1/2
states up to neutron number
=74. Comparison of the new results with state-of-the-art calculations suggests that triaxial deformation plays a significant role in the evolution of the energy difference, indicating a shape transition from axially symmetric to triaxial deformation within the Rh isotopic series. These findings provide new insights into the structure of neutron-rich nuclei in the atomic number
region, elucidating the interplay between triaxial deformation and shell evolution.
Ji, Y.-Y.*; Ji, W.*; Kim, K.*; Kim, M. J.*; 越智 康太郎; 森下 祐樹; 眞田 幸尚
Radiation Physics and Chemistry, 244, p.113781_1 - 113781_12, 2026/02
被引用回数:0 パーセンタイル:0.00UAVによる空中
線スペクトロメトリは迅速な放射線マッピングを可能にするが、飛行高度による減衰、視野効果、汚染の不均一性、地形条件により地上線量率の定量評価は難しい。本研究では福島第一原子力発電所周辺でホバリング飛行による校正と地上測定を組み合わせた実用的手法を開発した。二重指数モデルで高度補正係数を導出し、三脚およびバックパック測定と比較した結果、不均一サイトでの補正は系統誤差を生むが、均一サイトでの校正により一致が改善された。適切な補正を用いれば、UAV空中測定は信頼できる線量率分布評価が可能である。
Cho, K.*; 山下 葵平*; 角谷 心之輔*; 齊藤 拓馬*; 佐々木 泰祐*; 澤泉 克彦*; 奥川 将行*; 小泉 雄一郎*; 眞山 剛*; 菊川 泰地*; et al.
Acta Materialia, 303, p.121696_1 - 121696_18, 2026/01
被引用回数:3 パーセンタイル:61.18(Materials Science, Multidisciplinary)The deformation behavior and strengthening mechanism of Inconel 718 with a hierarchical structure composed of microscale crystallographic lamellar microstructure (CLM) and nanoscale cellular structure, fabricated by laser powder bed fusion, were clarified via nanoscale microstructural and in-situ neutron diffraction analyses. The CLM is a layered structure parallel to the building direction (BD) and consists of relatively wide main and narrow sub-layers with
110
and
100
orientations, respectively, with respect to BD. This is the first study to demonstrate that the yield stress of the alloys depends strongly on deformation stresses of the sub-layers, even though Schmid factors of the primary slip system for both layers are the same. The sub-layer continues to deform elastically even beyond the micro-yield point of the main layer, which results in the macroscopic strengthening at an early stage of deformation. On the other hand, the cellular structure is formed in both layers, associated with a dendritic cell growth along
100
direction, Nb segregation between the cells and an accumulation of dislocations to decrease a residual stress. The cell boundaries with numerous dislocations and Nb segregation act as a strong barrier to dislocation motion resulting in a stress increase through the Hall-Petch law, even though they are low-angle grain boundaries. The spacing and morphology of the cell boundary depend strongly on fabrication conditions. The optimized cellular structure provides significant strengthening comparable to or greater than that caused by large-angle grain boundaries, thereby increasing the macroscopic strength of the alloys through hardening of the sub-layer.
Zhu, L.*; Dong, W.*; Naeem, M.*; Kong, H.*; Hu, C.*; Fan, Z.*; Gong, W.; Harjo, S.; Lan, S.*; Wu, Y.*; et al.
Acta Materialia, 303, p.121734_1 - 121734_10, 2026/01
被引用回数:1 パーセンタイル:40.12(Materials Science, Multidisciplinary)Body-centered cubic (BCC) metals typically exhibit high yield strength but limited work hardening and uniform elongation, especially at low temperatures. High-entropy alloys (HEAs) offer opportunities to overcome these limitations, though their deformation mechanisms remain unclear. Using in situ neutron diffraction and microstructural analysis, this study identifies the origin of the exceptionally large uniform elongation at liquid nitrogen temperature in a single-phase BCC (TiZrHf)
Al
Nb
HEA. Initial plastic deformation is governed by a BCC-to-orthorhombic (
") transformation, followed by
" twinning and deformation-induced amorphization at later stages. The cooperation of these mechanisms suppresses work softening from dislocation plasticity, enabling high yield strength with large uniform elongation and providing a viable strategy for designing cryogenic structural materials.