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論文

Spin and lattice dynamics in the van der Waals antiferromagnet MnPSe$$_{3}$$

Liao, J.*; Huang, Z.*; Shangguan, Y.*; Zhang, B.*; Cheng, S.*; Xu, H.*; 梶本 亮一; 蒲沢 和也*; Bao, S.*; Wen, J.*

Physical Review B, 109(22), p.224411_1 - 224411_10, 2024/06

https://doi.org/10.1103/PhysRevB.109.224411
 被引用回数：0 パーセンタイル：0.00(Materials Science, Multidisciplinary)

Antiferromagnetic van der Waals family $$M$$P$$X_{3}$$ ($$M$$ = Fe, Mn, Co, and Ni; $$X$$ = S and Se) have attracted significant research attention due to the possibility of realizing long-range magnetic order down to the monolayer limit. Here, we perform inelastic neutron scattering measurements on single-crystal samples of MnPSe$$_{3}$$, a member of the $$M$$P$$X_{3}$$ family, to study the spin dynamics and determine the effective spin model. The excited magnon bands are well characterized by a spin model, which includes a Heisenberg term with three intraplane exchange parameters ($$J_{1} = -0.73$$ meV, $$J_{2} = -0.014$$ meV, $$J_{3} = -0.43$$ meV) and one interplane parameter ($$J_{c} = -0.054$$ meV), and an easy-plane single-ion anisotropy term ($$D = -0.035$$ meV). Additionally, we observe the intersection of the magnon and phonon bands but no anomalous spectral features induced by the formation of magnon-phonon hybrid excitations at the intersecting region. We discuss possible reasons for the absence of such hybrid excitations in MnPSe$$_{3}$$.

論文

Microscopic origin of the spin-reorientation transition in the kagome topological magnet TbMn$$_{6}$$Sn$$_{6}$$

Huang, Z.*; Wang, W.*; Ye, H.*; Bao, S.*; Shangguan, Y.*; Liao, J.*; Cao, S.*; 梶本 亮一; 池内 和彦*; Deng, G.*; et al.

Physical Review B, 109(1), p.014434_1 - 014434_9, 2024/01

https://doi.org/10.1103/PhysRevB.109.014434
 被引用回数：0 パーセンタイル：0.00(Materials Science, Multidisciplinary)

TbMn$$_{6}$$Sn$$_{6}$$ is a correlated topological magnet with a Mn-based kagome lattice, in which a Chern gap opens at the Dirac point at low temperatures. The magnetic moment direction of the ferrimagnetic order changes from in the kagome plane to the out-of-plane upon cooling, which is essential for generating the Chern gap, but the underlying mechanism for the spin reorientation remains elusive. Here, we investigate the spin-reorientation transition in TbMn$$_{6}$$Sn$$_{6}$$ using neutron scattering. We provide direct evidence for the spin-reorientation transition and unveil the coexistence of two Tb modes at 200 K. To account for these results, we put forward a model based on SU(N) spin-wave theory, in which there is a temperature evolution of the ground state Tb $$4f$$ orbitals, driven by the crystalline electric field, single-ion anisotropy, and exchange interactions between Tb and Mn ions. Our findings shed light on the complex magnetism of TbMn$$_{6}$$Sn$$_{6}$$, despite its relatively simple ground state magnetic structure, and provide insights into the mechanisms for tuning magnetic topological materials.

論文

Valley-selective phonon-magnon scattering in magnetoelastic superlattices

Liao, L.*; Puebla, J.*; 山本 慧; Kim, J.*; 前川 禎通*; Hwang, Y.*; Ba, Y.*; 大谷 義近*

Physical Review Letters, 131(17), p.176701_1 - 176701_6, 2023/10

https://doi.org/10.1103/PhysRevLett.131.176701
 被引用回数：6 パーセンタイル：80.90(Physics, Multidisciplinary)

Phonons and magnons are engineered by periodic potential landscapes in phononic and magnonic crystals, and their combined studies may enable valley phonon transport tunable by the magnetic field. Through nonreciprocal surface acoustic wave transmission, we demonstrate valley-selective phonon-magnon scattering in magnetoelastic superlattices. The lattice symmetry and the out-of-plane magnetization component control the sign of nonreciprocity. The phonons in the valleys play a crucial role in generating nonreciprocal transmission by inducing helical strains that couple with the magnons. The transmission spectra show a nonreciprocity peak near a transmission gap, matching the phononic band structure. Our results open the way for manipulating valley phonon transport through periodically varying magnon-phonon coupling.

論文

Direct observation of topological magnon polarons in a multiferroic material

Bao, S.*; Gu, Z.-L.*; Shangguan, Y.*; Huang, Z.*; Liao, J.*; Zhao, X.*; Zhang, B.*; Dong, Z.-Y.*; Wang, W.*; 梶本 亮一; et al.

Nature Communications (Internet), 14, p.6093_1 - 6093_9, 2023/09

https://doi.org/10.1038/s41467-023-41791-9
 被引用回数：12 パーセンタイル：92.34(Multidisciplinary Sciences)

Magnon polarons are novel elementary excitations possessing hybrid magnonic and phononic signatures, and are responsible for many exotic spintronic and magnonic phenomena. Despite long-term sustained experimental efforts in chasing for magnon polarons, direct spectroscopic evidence of their existence is hardly observed. Here, we report the direct observation of magnon polarons using neutron spectroscopy on a multiferroic Fe$$_{2}$$Mo$$_{3}$$O$$_{8}$$ possessing strong magnon-phonon coupling. Specifically, below the magnetic ordering temperature, a gap opens at the nominal intersection of the original magnon and phonon bands, leading to two separated magnon-polaron bands. Each of the bands undergoes mixing, interconverting and reversing between its magnonic and phononic components. We attribute the formation of magnon polarons to the strong magnon-phonon coupling induced by Dzyaloshinskii-Moriya interaction. Intriguingly, we find that the band-inverted magnon polarons are topologically nontrivial. These results uncover exotic elementary excitations arising from the magnon-phonon coupling, and offer a new route to topological states by considering hybridizations between different types of fundamental excitations.

論文

Evidence for strong correlations at finite temperatures in the dimerized magnet Na$$_{2}$$Cu$$_{2}$$TeO$$_{6}$$

Shangguan, Y.*; Bao, S.*; Dong, Z.-Y.*; Cai, Z.*; Wang, W.*; Huang, Z.*; Ma, Z.*; Liao, J.*; Zhao, X.*; 梶本 亮一; et al.

Physical Review B, 104(22), p.224430_1 - 224430_8, 2021/12

https://doi.org/10.1103/PhysRevB.104.224430
 被引用回数：1 パーセンタイル：5.86(Materials Science, Multidisciplinary)

Dimerized magnets forming alternating Heisenberg chains exhibit quantum coherence and entanglement and thus can find potential applications in quantum information and computation. However, magnetic systems typically undergo thermal decoherence at finite temperatures. Here, we show inelastic neutron scattering results on an alternating antiferromagnetic-ferromagnetic chain compound Na$$_{2}$$Cu$$_{2}$$TeO$$_{6}$$ that the excited quasiparticles can counter thermal decoherence and maintain strong correlations at elevated temperatures. At low temperatures, we observe clear dispersive singlet-triplet excitations arising from the dimers formed along the crystalline $$b$$-axis. The excitation gap is of $$sim$$18 meV and the bandwidth is about half of the gap. The band top energy has a weak modulation along the [100] direction, indicative of a small interchain coupling. The gap increases while the bandwidth decreases with increasing temperature, leading to a strong reduction in the available phase space for the triplons. As a result, the Lorentzian-type energy broadening becomes highly asymmetric as the temperature is raised. These results are associated with a strongly correlated state resulting from hard-core constraint and quasiparticle interactions. We consider these results to be not only evidence for strong correlations at finite temperatures in Na$$_{2}$$Cu$$_{2}$$TeO$$_{6}$$, but also for the universality of the strongly correlated state in a broad range of quantum magnetic systems.

口頭

ダイヤモンド薄膜の同位体濃縮

寺地 徳之*; 小野田 忍; 小泉 聡*; Liao, M.*; 谷口 尚*; 大島 武; Jelezko, F.*; Wrachtrup, J.*; 磯谷 順一*

no journal, , 

炭素を同位体濃縮させることで、ダイヤモンドのさまざまな物性が向上することが知られている。たとえば、量子計算応用における窒素-空孔複合欠陥(NVセンター)に局在する電子のスピン緩和時間も、同位体濃縮することで改善する。つまり、スピン緩和時間を向上させるため、結晶内の窒素低減や$$^{13}$$C炭素存在比を天然存在比のものより小さくすることが求められる。本研究では、窒素濃度低減に加え、$$^{13}$$Cを低減した$$^{12}$$C同位体濃縮ダイヤモンド薄膜を化学気相合成し、その特性評価を行った。その結果、気相での同位体濃縮度が固相変換後も保たれ、窒素不純物などが少ないダイヤモンド薄膜を成長することに成功した。

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