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magnetic order with spatially alternating spin scalar chirality in overdoped Co
TaS
Cho, W.*; Park, P.*; Kim, C.*; An, Y.*; 飯田 一樹*; 梶本 亮一; Matin, S.*; Sibille, R.*; Crooker, S. A.*; Park, J.-G.*
Physical Review B, 113(17), p.174410_1 - 174410_14, 2026/05
被引用回数：0 パーセンタイル：0.00(Materials Science, Multidisciplinary)Co
TaS (
) exhibits a spontaneous Hall effect from spin texture in antiferromagnets, with a tetrahedral triple-Q () order and uniform spin scalar chirality. Upon Co overdoping (
), it undergoes a shift in magnetic ordering vectors from 
to 
. Interestingly, the spontaneous Hall effect disappeared in the overdoped regime, which was originally attributed to the loss of order. However, a question remains whether a new type of order can exist with alternating chirality in the overdoped regime. To address this, we investigated CoTaS using inelastic neutron scattering (INS), neutron diffraction, and optical dichroism, and found that INS data and spin-wave simulations support a order with alternating chirality. Moreover, neutron diffraction data show field-independent Bragg peaks, while linear dichroism detects no in-plane anisotropy, consistent with threefold rotation symmetry. Our data support the scenario of an alternating-chirality order in CoTaS, cancelling the spontaneous Hall effect. This study highlights a combined neutron-optical approach to identify complex spin textures.
magnetic orderings in a triangular lattice; Implications for multi- orderings in general two-dimensional latticesPark, P.*; Cho, W.*; Kim, C.*; An, Y.*; 飯田 一樹*; 梶本 亮一; Matin, S.*; Zhang, S.-S.*; Batista, C. D.*; Park, J.-G.*
Physical Review X, 15(3), p.031032_1 - 031032_29, 2025/07
被引用回数：5 パーセンタイル：74.19(Physics, Multidisciplinary)Multi- magnetic structures on two-dimensional (2D) lattices provide a key route to realizing topological physics in 2D magnetism. A major experimental challenge is to unambiguously confirm their formation by excluding the possibility of topologically trivial multi-domain single- or double- magnetic orders, which cannot be distinguished using conventional diffraction techniques. Here, we propose that long-wavelength spin dynamics offers a universal diagnostic for triangular lattices: triple- orders that preserve rotational symmetry and single- or double- orders that break it exhibit qualitatively distinct anisotropies in their Goldstone mode velocities, stemming from fundamental differences in their underlying spin configurations. We validate this concept using the metallic triangular-lattice antiferromagnet Co
TaS, which hosts both a stripe-type single- state and a triple- tetrahedral ordering at different temperatures. Using inelastic neutron-scattering and spin dynamics simulations, we first refine the spin Hamiltonian by fitting the paramagnetic excitation spectra, allowing us to develop an unbiased model independent of magnetic ordering. We then show that the observed velocity profiles of the Goldstone modes agree with the high-temperature model's predictions: markedly anisotropic for the single- phase and near isotropic for the triple- phase. Importantly, this contrast persists across various exchange parameters, highlighting its model-independent nature and suggesting potential applicability to other 2D lattice systems. Beyond the long-wavelength regime, we present a substantial discrepancy between the measured and simulated magnon spectra exclusively in the triple- phase. We attribute this discrepancy to magnon energy renormalization arising from order-of-magnitude-enhanced magnon-magnon interactions in the triple- phase, due to its noncollinear configuration. This work provides universal insight into the dynamical properties of topological multi- magnetic orderings in 2D lattice structures, offering a broadly applicable diagnostic to distinguishing them from topologically trivial single- or double- counterparts. The unequivocal confirmation of the triple- structure in CoTaS further establishes it as a prominent material platform for exploring topological spin textures in the genuine 2D limit.
河合 優作*; Park, J.*; 元川 竜平; 以倉 崚平*; 村山 駿介*; 山岡 賢司*; 藤井 義久*; 池本 夕佳*; 田中 賢*; 松葉 豪*; et al.
ACS Applied Polymer Materials (Internet), 7(12), p.7767 - 7776, 2025/06
被引用回数：2 パーセンタイル：48.04(Materials Science, Multidisciplinary)The material properties of polymeric materials in aqueous environments are significantly influenced by water content. It is widely recognized that polymeric materials become more brittle with increased water content. However, the specific relationship between hydration levels and polymer chains has not been fully elucidated, leaving many uncertainties. Conversely, intermediate water (IMW), which refers to adsorbed water, plays an active role in influencing the biocompatibility and antifouling properties of these materials. In this study, we examined the correlation between IMW and toughness (Gf) / Youngs modulus (E). We synthesized dual cross-network (DC) elastomers through the bulk copolymerization of cyclodextrin (CD) monomers and vinyl monomers in the presence of movable cross-linked elastomers. The resulting DC elastomers exhibited both high Gf and high E. We used poly(2-methoxyethyl acrylate) (PMEA) as the primary polymer and poly(N,N-dimethyl acrylamide) (PDMAA) as the secondary polymer. The DC materials were formulated as DC(MEA-DMAA)(100-w:w)(Wc), where w and Wc represent the weight percentage of the secondary polymer (PDMAA) and the water content, respectively. The mechanical properties of the DC materials mostly decreased with increasing amounts of the secondary polymer. However, DC(MEA-DMAA)(90:10)(22), which contained 10 wt percent of PDMAA, exhibited the highest Gf and E among all samples. Differential scanning calorimetry (DSC) measurements indicated the presence of IMW in DC(MEA-DMAA)(90:10)(22). We propose that the IMW in this sample facilitates the formation of crosslinks between polymer chains and water molecules, contributing to the observed enhancements in E and Gf.
Go, J.*; Park, M.-H.*; Gao, S.*; 松宮 久*; Gong, W.; 辻 伸泰*
Journal of Alloys and Compounds, 1014, p.178749_1 - 178749_10, 2025/02
被引用回数：14 パーセンタイル：96.39(Chemistry, Physical)In Mg alloys, basal dislocation slip is the preferential slip system that is activated at room temperature, while non-basal slips are typically difficult to activate owing to their high critical resolved shear stress. Until now, minimal focus has been directed towards the influence of loading direction on slip behavior in pre-twinned AZ31 alloys. This study employed transmission electron microscopy to demonstrate that non-basal slips, specifically prismatic and pyramidal I slips, are activated under deformation conditions where de-twinning is difficult in a pre-twinned AZ31 Mg alloy. When the tensile loading direction is parallel to the precompression direction, de-twinning and basal slip are the primary deformation modes. Conversely, when the tensile loading direction is perpendicular to the precompression direction, where de-twinning is challenging to activate, both basal and non-basal slips, such as prismatic and pyramidal I slips, emerge as the primary deformation modes. These results indicate that the pre-twinned AZ31 Mg alloy cannot deform solely through basal slips, and the activation of either de-twinning or non-basal slips is necessary to satisfy the von Mises criterion. Our findings in this study demonstrate the impact of non-basal slip activity on macroscopic yield stress and overall deformation, hence enhancing the understanding of magnesium alloy deformation mechanisms.
TaSPark, P.*; Cho, W.*; Kim, C.*; An, Y.*; Avdeev, M.*; 飯田 一樹*; 梶本 亮一; Park, J.-G.*
Physical Review B, 109(6), p.L060403_1 - L060403_7, 2024/02
被引用回数：27 パーセンタイル：94.25(Materials Science, Multidisciplinary)Spontaneous Hall conductivity has recently been reported in the triangular lattice antiferromagnet CoTaS under a zero magnetic field. This phenomenon originates from the distinctive noncoplanar triple- magnetic ground state, possessing uniform real-space Berry curvature characterized by scalar spin chirality. We investigated the physical properties of CoTaS by judiciously controlling the composition, revealing a drastic change in its bulk properties, even by slight variations in cobalt composition, despite the same crystal structure. For 
, CoTaS keeps all the characteristics of the ground state consistent with the previous studies - two antiferromagnetic phase transitions at 
and 
(
), a large spontaneous Hall conductivity [
], and a weak ferromagnetic moment along the 
axis. However, samples with 
exhibit distinct bulk properties, including the absence of both and the weak ferromagnetic moment. Our neutron diffraction data reveal that CoTaS with develops coplanar helical magnetic order with 
. This is entirely different from what has been seen in 
, explaining the observed composition dependence.
Park, Y.-J.*; 澤田 淳; 小堤 健紀*; 田中 達也*; 橋本 秀爾*; 森田 豊*
Proceedings of 3rd International Conference on Discrete Fracture Network Engineering (DFNE 2022) (Internet), 8 Pages, 2022/00
高レベル放射性廃棄物の地層処分の安全評価には地層中の長期にわたる地下水流動と核種移行プロセスの把握が求められる。沿岸部地下環境において、地下水流動は海水起源の塩水と陸水起源の淡水の密度差による複雑な相互作用の影響を受ける。加えて、数百万年の長期においては、海進・海退に伴う海水準変動の影響を受ける。本研究では、そのような沿岸域における亀裂性の結晶質岩を対象とした処分場の地下水流動と核種移行を評価するため、塩分濃度と地下水流速などの地下水環境の長期的な変遷を評価するための広域スケールとブロックスケールを組み合わせた評価フレームを構築した。
Park, J. S.*; 原田 正英; 長谷川 勝一; 春日井 好己; 明午 伸一郎; 酒井 健二; 鈴谷 賢太郎; 他55名*
Progress of Theoretical and Experimental Physics (Internet), 2021(6), p.063C01_1 - 063C01_12, 2021/06
被引用回数：2 パーセンタイル：18.32(Physics, Multidisciplinary)The Sterile Neutrino Search at the J-PARC Spallation Neutron Source (JSNS) experiment aims to search for sterile neutrino oscillations using a neutrino beam from muon decays at rest. The JSNS2 detector contains 17 tons of 0.1
gadolinium (Gd) loaded liquid scintillator (LS) as a neutrino target. Detector construction was completed in the spring of 2020. A slow control and monitoring system (SCMS) was implemented for reliable control and quick monitoring of the detector operational status and environmental conditions. It issues an alarm if any of the monitored parameters exceed a preset acceptable range. The SCMS monitors the high voltage of the photomultiplier tubes, the LS level in the detector, possible LS overflow and leakage, the temperature and air pressure in the detector, the humidity of the experimental hall, and the LS flow rate during filling and extraction. An initial 10 days of data-taking with a neutrino beam was done following a successful commissioning of the detector and SCMS in 2020 June. In this paper, we present a description of the assembly and installation of the SCMS and its performance.
Kim, J. G.*; Bae, J. W.*; Park, J. M.*; Woo, W.*; Harjo, S.; Lee, S.*; Kim, H. S.*
Metals and Materials International, 27(2), p.376 - 383, 2021/02
被引用回数：11 パーセンタイル：40.28(Materials Science, Multidisciplinary)Heterogeneous structured materials achieve a combination of high strength and extreme ductility due to synergetic strengthening driven by conditions in the interfacial region. Although the origin of synergetic strengthening has been revealed to be strain incompatibility in the interfacial region, the effect of the strength difference between hard and soft phases on strengthening has not been investigated well. In the work reported in the present paper, the effect of the difference in strength of the hard and soft phases on synergetic strengthening was investigated by conducting in situ neutron diffraction tensile tests. As a result, it was determined that the dislocation density in a layered sheet of high Mn (HMn) steel/interstitial free (IF) steel is higher than that in a layered sheet of HMn/low carbon steel. The big difference in mechanical properties between HMn steel and IF steel induces a high stress gradient and results in additional dislocations.
Kim, S.*; Lee, B.*; Reeder, J. T.*; Seo, S. H.*; Lee, S.-U.*; Hourlier-Fargette, A.*; Shin, J.*; 関根 由莉奈; Jeong, H.*; Oh, Y. S.*; et al.
Proceedings of the National Academy of Sciences of the United States of America, 117(45), p.27906 - 27915, 2020/11
被引用回数：132 パーセンタイル：94.58(Multidisciplinary Sciences)本研究では、汗のコルチゾール分析のための流動イムノアッセイ、グルコースとアスコルビン酸(ビタミンC)分析のための蛍光測定イメージング、および電極を使用した発汗速度のデジタルトラッキングを組み合わせた、ワイヤレス,バッテリー不要の皮膚インターフェースマイクロ流体システムを実現した。運動している被験者を対象とした体系的なテストにより、本開発デバイスが物理的ストレスと生化学的相関を追跡可能であることが示された。
田屋 英俊*; Park, A.*; Cho, S.*; Gubler, P.; 服部 恒一*; Hong, J.*; Huang, X.-G.*; Lee, S. H.*; 門内 明彦*; 大西 明*; et al.
Physical Review C, 102(2), p.021901_1 - 021901_6, 2020/08
被引用回数：8 パーセンタイル：54.27(Physics, Nuclear)We investigate the hadron production from the vortical quark-gluon plasma created in heavy-ion collisions. Based on the quark-coalescence and statistical hadronization models, we show that total hadron yields summed over the spin components are enhanced by the local vorticity with quadratic dependence. The enhancement factor amounts to be a few percent and may be detectable within current experimental sensitivities. We also show that the effect is stronger for hadrons with larger spin, and thus propose a new signature of the local vorticity, which may be detected by the yield ratio of distinct hadron species having different spins such as 
and 
. The vorticity dependence of hadron yields seems robust, with consistent predictions in both of the hadron production mechanisms for reasonable values of the vorticity strength estimated for heavy-ion collisions.
Bae, J. W.*; Jung, J.*; Kim, J. G.*; Park, J. M.*; Harjo, S.; 川崎 卓郎; Woo, W.*; Kim, H. S.*
Materialia, 9, p.100619_1 - 100619_15, 2020/03
In the present study, an integrated experimental-numerical analysis on ferrous medium-entropy alloy (FMEA) was conducted to understand the micromechanical response of the constituent phases in the FMEA at -137
C. The initial face-centered cubic (FCC) single phase microstructure of the FMEA was transformed to body-centered cubic (BCC) martensite during tensile deformation at -137C, resulting in improved low-temperature mechanical properties. The microstructure evolution due to deformation-induced phase transformation mechanism and strain partitioning behavior was analyzed using 
electron backscatter diffraction. The mechanical responses related to the stress partitioning between constituent phases and deformation-induced transformation rate were measured using 
neutron diffraction in combination with the nanoindentation analysis.
Zhang, Y.*; Guo, H.*; Kim, S. B.*; Wu, Y.*; Ostojich, D.*; Park, S. H.*; Wang, X.*; Weng, Z.*; Li, R.*; Bandodkar, A. J.*; et al.
Lab on a Chip, 19(9), p.1545 - 1555, 2019/05
被引用回数：224 パーセンタイル：99.73(Biochemical Research Methods)汗中のバイオマーカーおよび非侵襲的な方法で汗を集める方法は、健康および生理学的状態の評価のための汗利用の関心を生み出し、スポーツから臨床医学までの範囲の潜在的用途がある。本論文は、皮膚密着型のマイクロ流体システムを用いた2つの結果について述べる。(1)簡易な身体的および心理的刺激による汗の採取、(2)酵素化学および比色アプローチによる汗中のクレアチニンおよび尿素の濃度の検出。結果、乳児や高齢者などを対象に日常的で非薬理学的な汗の捕捉が可能になり、腎臓疾患のスクリーニング/モニタリングに汗を使用する可能性が示された。
neutron diffraction study of phase stress evolution in a ferrous medium-entropy alloy under low-temperature tensile loadingBae, J. W.*; Kim, J. G.*; Park, J. M.*; Woo, W.*; Harjo, S.; Kim, H. S.*
Scripta Materialia, 165, p.60 - 63, 2019/05
被引用回数：49 パーセンタイル：87.59(Nanoscience & Nanotechnology)Phase stress evolution of face-centered cubic (FCC) and deformation-induced body-centered cubic (BCC) phases was measured in recently developed ferrous medium-entropy alloy. This was done during tensile deformation at -137C using neutron diffraction measurement for the quantitative interpretation of the role of martensitic transformation on the improved low-temperature tensile properties. The strain-hardening rate curve exhibits two-stage hardening behavior, and the phase stress and stress contribution from the BCC phase increases significantly while that from FCC phase decreases during plastic deformation. This is a direct demonstration that BCC phase contributes significantly to the increase in strength and strain hardening.
Oh, J.*; Le, M. D.*; Nahm, H.-H.*; Sim, H.*; Jeong, J.*; Perring, T. G.*; Woo, H.*; 中島 健次; 河村 聖子; Yamani, Z.*; et al.
Nature Communications (Internet), 7, p.13146_1 - 13146_6, 2016/10
被引用回数：72 パーセンタイル：87.53(Multidisciplinary Sciences)(Y,Lu)MnOにおいて、磁気励起とフォノンが結合する磁気弾性励起を中性子散乱により観測し、その量子的振る舞いを調べた。
Polevoi, A. R.*; Loarte, A.*; 林 伸彦; Kim, H. S.*; Kim, S. H.*; Koechl, F.*; Kukushkin, A. S.*; Leonov, V. M.*; Medvedev, S. Yu.*; 村上 匡且*; et al.
Nuclear Fusion, 55(6), p.063019_1 - 063019_8, 2015/06
被引用回数：49 パーセンタイル：88.92(Physics, Fluids & Plasmas)The operational space (
-
) for long pulse scenarios of ITER was assessed by 1.5D core transport modelling with pedestal parameters predicted by the EPED1 code. The analyses include the majority of transport models presently used for interpretation of experiments and ITER predictions. The EPED1 code was modified to take into account boundary conditions predicted by SOLPS for ITER. In contrast with standard EPED1 assumptions, EPED1 with the SOLPS boundary conditions predicts no degradation of the pedestal pressure as density is reduced. Lowering the plasma density to 
5-6 
10
m
leads to an increased plasma temperature (similar pedestal pressure), which reduces the loop voltage and increases the duration of the burn phase to 
1000 s with Q 
5 for 
13 MA at moderate normalised pressure (
2). These ITER plasmas require the same level of additional heating power as the reference Q = 10 inductive scenario at 15 MA. However, unlike the "hybrid" scenarios considered previously, these H-mode plasmas do not require specially shaped q profiles nor improved confinement in the core for the transport models considered in this study. Thus, these medium density H-mode plasma scenarios with 13 MA present an attractive alternative to hybrid scenarios to achieve ITER's long pulse Q 5 and deserve further analysis and experimental demonstration in present tokamaks.
Luce, T. C.*; Challis, C. D.*; 井手 俊介; Joffrin, E.*; 鎌田 裕; Politzer, P. A.*; Schweinzer, J.*; Sips, A. C. C.*; Stober, J.*; Giruzzi, G.*; et al.
Nuclear Fusion, 54(1), p.013015_1 - 013015_15, 2013/12
被引用回数：55 パーセンタイル：89.66(Physics, Fluids & Plasmas)The ITPA IOS group has coordinated experimental and modeling activity on the development of advanced inductive scenarios for applications in the ITER tokamak. This report documents the present status of the physics basis and the prospects for applications in ITER. The key findings are: (1) inductive scenarios capable of higher 
than the ITER baseline scenario (
) with normalized confinement at or above the standard H-mode scaling have been established under stationary conditions on the four largest diverted tokamaks (AUG, DIII-D, JET, JT-60U) in a broad range in 
and density; (2) MHD modes can play a key role in reaching stationary high performance, but also define the stability and confinement limits; (3) the experiments have yielded clearer measurements of the normalized gyroradius scalin; and (4) coordinated modeling activity supports the present research by clarifying the most significant uncertainties in the projections to ITER.
Park, J.*; 高山 俊雄*; 浅野 雅春; 前川 康成; 工藤 一秋*; 高山 俊雄*
Polymer, 54(17), p.4570 - 4577, 2013/08
被引用回数：7 パーセンタイル：20.27(Polymer Science)芳香族ポリベンズイミダゾール(PBI)膜に匹敵する耐熱性と機械特性を示す脂環式PBI(ChPBI)への放射線グラフト重合及びその後のスルホン化処理によりグラフト型ポリベンズイミダゾール電解質膜(sPBI)を作製した。ChPBIは、
-1,4-cyclohexanedicarboxylic acidと3,3'-diaminobenzidineの縮合反応より合成した。合成したChPBIは塩化リチウム含有のジメチル酢酸溶液から製膜することで結晶性を示し、
線の照射によりグラフト重合の開始種となる長寿命ラジカルが生成することがわかった。得られた結晶性ChPBI膜を220kGy照射後スチレン/1-プロピルアルコール(50/50)中でのグラフト重合とスルホン化処理により、イオン交換容量が2.1
2.9mmol/gのsPBI膜が調製できた。sPBI膜は1010
S/cmと従来のPBI膜よりも高いプロトン伝導度を示した。走査電子顕微鏡/エネルギー分散型X線分析(SEM-EDX分析)より、sPBI膜中の1
m径のグラフトドメインの形成が高イオン導電性に重要であることがわかった。このsPBI膜は、120C熱水中で600時間後においてもプロトン伝導度の減少を起こさないことから、これまで作製したグラフト型電解質膜よりも耐熱性に優れていることを明らかにした。
Polevoi, A. R.*; 林 伸彦; Kim, H. S.*; Kim, S. H.*; Koechl, F.*; Kukushkin, A. S.*; Leonov, V. M.*; Loarte, A.*; Medvedev, S. Yu.*; 村上 匡且*; et al.
Europhysics Conference Abstracts (Internet), 37D, p.P2.135_1 - P2.135_4, 2013/07
Long-pulse operation 
1000 s with 
5 is foreseen in ITER to demonstrate high neutron fluence scenarios which can be of use for the nuclear technology and for the TBM. In this study we address the viability of achieving ITER's long-pulse scenario in plasma regimes with H-mode confinement level by characterizing the current-density operational space and the achievable Q with long pulse burning phases. The EPED1 model with boundary conditions from SOLPS predicts no degradation of pedestal pressure with decreasing density in ITER. Modelling of core transport with 1.5D transport models carried out with pedestal parameters predicted by EPED1+SOLPS indicate that there is a large operational space for long pulse plasma operation with high fusion gain 5. Reducing the plasma density to 5-6 10m leads to an increased plasma temperature (similar pedestal pressure) which reduces the loop voltage and increases the duration of the burn phase to 1000 s with 5 for 13 MA at moderate normalised pressure, 2. Unlike the "hybrid" scenarios, these H-mode plasmas do not require specially shaped q profiles nor improved confinement in the core for the majority of the transport models considered in this study. Thus, these medium density H-mode plasma scenarios present an attractive alternative to hybrid scenarios to achieve ITER's long pulse.
Park, J.; 榎本 一之; 山下 俊*; 高木 康行*; 戸高 勝則*; 前川 康成
Journal of Membrane Science, 438, p.1 - 7, 2013/07
被引用回数：15 パーセンタイル：41.38(Engineering, Chemical)芳香族ポリイミド膜と同等の耐熱性,機械特性を示す脂環式ポリイミド膜(A-PI膜)への放射線グラフト重合による燃料電池用電解質膜の作製とそのグラフト重合機構の解析を試みた。芳香族ポリイミドが放射線グラフト重合性を示さないのに対し、その一部を脂環式構造に置換したA-PI膜は放射線グラフト重合性を示した。得られたグラフト膜をスルホン化することで、ナフィオンより高いイオン伝導度と機械・熱的安定性を示す電解質膜が作製できた。照射A-PI膜の紫外・可視光分光(UV-VIS)スペクトルより、420, 600nmに吸収極大を持つ長寿命中間体の存在が確認できた。UV-VISスペクトルの減衰と電子スピン共鳴によるラジカルの減衰の比較から、この中間体が脂環式部位に生じたアルキルラジカルであり、A-PI膜の放射線グラフト重合における開始部位であることが確定できた。
Jeong, J. H.*; Bae, Y. S.*; Joung, M.*; Kim, H. J.*; Park, S. I.*; Han, W. S.*; Kim, J. S.*; Yang, H. L.*; Kwak, J. G.*; 坂本 慶司; et al.
Fusion Engineering and Design, 88(5), p.380 - 387, 2013/06
被引用回数：4 パーセンタイル：29.04(Nuclear Science & Technology)A 3.6 MW DC power supply system was developed for the 170 GHz EC H&CD system in KSTAR. It consists of a cathode power supply (CPS), an anode power supply (APS) and a body power supply (BPS). The CPS is capable of supplying a voltage of -66 kV and a current of 55 A to the cathode with respect to the collector using pulse step modulation (PSM). The APS is a voltage divider system consisting of a fixed resistor and zener diode units with the capability of 60 kV stand-off voltage. For high frequency current modulation, the parallel discharge switch is introduced between the cathode and anode. The BPS is a DC power supply with 50 kV/160 mA. The series MOS-FET solid-state switch is used for on/off modulation in the body voltage sychronizing with anode voltage. The parallel discharge switch is also introduced between the body and collector for high frequency RF modulation. This paper describes the key features of the high voltage power supply system as well as the test results.
