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"Southwestern" boundary of the $$N = 40$$ island of inversion; First study of low-lying bound excited states in $$^{59}$$V and $$^{61}$$V

Elekes, Z.*; Juh$'a$sz, M. M.*; Sohler, D.*; Sieja, K.*; 吉田 数貴; 緒方 一介*; Doornenbal, P.*; Obertelli, A.*; Achouri, N. L.*; 馬場 秀忠*; et al.

Physical Review C, 106(6), p.064321_1 - 064321_10, 2022/12


$$^{59}$$Vと$$^{61}$$Vの低励起準位構造を初めて探索した。$$^{61}$$Vについては中性子ノックアウト反応と陽子非弾性散乱が、$$^{59}$$Vについては中性子ノックアウト反応データが得られた。$$^{59}$$Vについては4つ、$$^{61}$$Vについては5つの新たな遷移が確認された。Lenzi-Nowacki-Poves-Sieja (LNPS)相互作用に基づく殻模型計算との比較によって、それぞれの同位体について確認されたガンマ線のうち3つが、first 11/2$$^{-}$$状態とfirst 9/2$$^{-}$$状態からの崩壊と決定された。$$^{61}$$Vについては、($$p$$,$$p'$$)非弾性散乱断面積は四重極変形と十六重極変形を想定したチャネル結合法により解析されたが、十六重極変形の影響により、明確に反転の島に属するとは決定できなかった。


Extended $$p_{3/2}$$ neutron orbital and the $$N = 32$$ shell closure in $$^{52}$$Ca

Enciu, M.*; Liu, H. N.*; Obertelli, A.*; Doornenbal, P.*; Nowacki, F.*; 緒方 一介*; Poves, A.*; 吉田 数貴; Achouri, N. L.*; 馬場 秀忠*; et al.

Physical Review Letters, 129(26), p.262501_1 - 262501_7, 2022/12

 被引用回数:0 パーセンタイル:0(Physics, Multidisciplinary)



A First glimpse at the shell structure beyond $$^{54}$$Ca; Spectroscopy of $$^{55}$$K, $$^{55}$$Ca, and $$^{57}$$Ca

小岩井 拓真*; Wimmer, K.*; Doornenbal, P.*; Obertelli, A.*; Barbieri, C.*; Duguet, T.*; Holt, J. D.*; 宮城 宇志*; Navr$'a$til, P.*; 緒方 一介*; et al.

Physics Letters B, 827, p.136953_1 - 136953_7, 2022/04

 被引用回数:2 パーセンタイル:67.14(Astronomy & Astrophysics)

中性子過剰核$$^{54}$$Caでは、新魔法数34が発見されて以来、その構造を知るために多くの実験がなされてきたが、それを超える中性子過剰核の情報は全く知られてこなかった。本論文では、理化学研究所RIBFにて$$^{55}$$K, $$^{55}$$Ca, $$^{57}$$Caの励起状態から脱励起するガンマ線を初めて観測した結果を報告した。それぞれ1つのガンマ線しか得られなかったものの、$$^{55}$$Kおよび$$^{55}$$Caのデータは、それぞれ、陽子の$$d_{3/2}$$$$s_{1/2}$$軌道間のエネルギー差、中性子の$$p_{1/2}$$$$f_{5/2}$$軌道間のエネルギー差を敏感に反映し、両方とも最新の殻模型計算によって200keV程度の精度で再現できることがわかった。また、1粒子状態の程度を特徴づける分光学的因子を実験データと歪曲波インパルス近似による反応計算から求め、その値も殻模型計算の値と矛盾しないことがわかった。


The $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe cross section from the surrogate ratio method and its effect on the $$^{60}$$Fe nucleosynthesis

Yan, S. Q.*; Li, X. Y.*; 西尾 勝久; Lugaro, M.*; Li, Z. H.*; 牧井 宏之; Pignatari, M.*; Wang, Y. B.*; Orlandi, R.; 廣瀬 健太郎; et al.

Astrophysical Journal, 919(2), p.84_1 - 84_7, 2021/10

 被引用回数:1 パーセンタイル:17.16(Astronomy & Astrophysics)

The long-lived $$^{60}$$Fe (with a half-life of 2.62 Myr) is a crucial diagnostic of active nucleosynthesis in the Milky Way galaxy and in supernovae near the solar system. The neutron-capture reaction $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe on $$^{59}$$Fe (half-life=44.5 days) is the key reaction for the production of $$^{60}$$Fe in massive stars. This reaction cross section has been previously constrained by the Coulomb dissociation experiment, which offered partial constraint on the E1 $$gamma$$-ray strength function but a negligible constraint on the M1 and E2 components. In this work, for the first time, we use the surrogate ratio method to experimentally determine the $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe cross sections in which all the components are included. We derived a Maxwellian-averaged cross section of 27.5$$pm$$3.5 mb at $$kT$$ = 30 keV and 13.4$$pm$$1.7 mb at $$kT$$ = 90 keV, roughly 10%-20% higher than previous estimates. We analyzed the impact of our new reaction rates in nucleosynthesis models of massive stars and found that uncertainties in the production of $$^{60}$$Fe from the $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe rate are at most 25$$%$$. We conclude that stellar physics uncertainties now play a major role in the accurate evaluation of the stellar production of $$^{60}$$Fe.


Investigation of the ground-state spin inversion in the neutron-rich $$^{47,49}$$Cl isotopes

Linh, B. D.*; Corsi, A.*; Gillibert, A.*; Obertelli, A.*; Doornenbal, P.*; Barbieri, C.*; Chen, S.*; Chung, L. X.*; Duguet, T.*; G$'o$mez-Ramos, M.*; et al.

Physical Review C, 104(4), p.044331_1 - 044331_16, 2021/10


 被引用回数:2 パーセンタイル:32.08(Physics, Nuclear)



OECD/NEA benchmark on pellet-clad mechanical interaction modelling with fuel performance codes; Influence of pellet geometry and gap size

Soba, A.*; Prudil, A.*; Zhang, J.*; Dethioux, A.*; Han, Z.*; Dostal, M.*; Matocha, V.*; Marelle, V.*; Lasnel-Payan, J.*; Kulacsy, K.*; et al.

Proceedings of TopFuel 2021 (Internet), 10 Pages, 2021/10

The NEA Expert Group on Reactor Fuel Performance (EGRFP) proposed a benchmark on fuel performance codes modeling of pellet-cladding mechanical interation (PCMI). The aim of the benchmark was to improve understanding and modeling of PCMI amongst NEA member organizations. This was achieved by comparing PCMI predictions for a number of specified cases. The results of the two hypothetical cases (1 and 2) were presented earlier. The two final cases (3 and 4) are comparison between calculations and measurements, which will be published as NEA reports. This paper focuses on Case 3, which consists of eight beginning of life (BOL) sub-cases (3a to 3h) each with different pellet designs that have undergone ramping in the Halden Reactor. The aforementioned experiments are known as the IFA-118 experiments and were performed from 1969 to 1970. The variations between cases include four different pellets dimensions (7, 14, 20 and 30 mm of height), two different gapsizes between pellet-cladding (40 and 100 microns) and three variations on pellet face geometry (flat, dishing and dishing with chamfer). Such diversity has allowed exploring the codes sensitivity to these individual factors.


Pairing forces govern population of doubly magic $$^{54}$$Ca from direct reactions

Browne, F.*; Chen, S.*; Doornenbal, P.*; Obertelli, A.*; 緒方 一介*; 宇都野 穣; 吉田 数貴; Achouri, N. L.*; 馬場 秀忠*; Calvet, D.*; et al.

Physical Review Letters, 126(25), p.252501_1 - 252501_7, 2021/06

 被引用回数:4 パーセンタイル:45.66(Physics, Multidisciplinary)



First spectroscopic study of $$^{51}$$Ar by the ($$p$$,2$$p$$) reaction

Juh$'a$sz, M. M.*; Elekes, Z.*; Sohler, D.*; 宇都野 穣; 吉田 数貴; 大塚 孝治*; 緒方 一介*; Doornenbal, P.*; Obertelli, A.*; 馬場 秀忠*; et al.

Physics Letters B, 814, p.136108_1 - 136108_8, 2021/03


 被引用回数:2 パーセンタイル:32.08(Astronomy & Astrophysics)

($$p$$,$$2p$$)反応と$$gamma$$線分光を用いて$$^{51}$$Arの束縛状態と非束縛状態の核構造研究を行った。実験結果と殻模型計算を比較することで、2つの束縛状態と6つの非束縛状態を決定した。$$^{51}$$Arの束縛状態を生成する反応断面積が小さいことから、これは中性子数32, 34の顕著なsub-shell closureが存在している確かな証拠と解釈できる。


General synthesis of single-atom catalysts for hydrogen evolution reactions and room-temperature Na-S batteries

Lai, W.-H.*; Wang, H.*; Zheng, L.*; Jiang, Q.*; Yan, Z.-C.*; Wang, L.*; 吉川 浩史*; 松村 大樹; Sun, Q.*; Wang, Y.-X.*; et al.

Angewandte Chemie; International Edition, 59(49), p.22171 - 22178, 2020/12

 被引用回数:56 パーセンタイル:96.11(Chemistry, Multidisciplinary)

Herein, we report a comprehensive strategy to synthesize a full range of single-atom metals on carbon matrix, including V, Mn, Fe, Co, Ni, Cu, Ge, Mo, Ru, Rh, Pd, Ag, In, Sn, W, Ir, Pt, Pb, and Bi. The extensive applications of various single-atom catalysts (SACs) are manifested via their ability to electro-catalyze typical hydrogen evolution reactions (HER) and conversion reactions in novel room-temperature sodium sulfur batteries (RT-Na-S). The enhanced performances for these electrochemical reactions arisen from the ability of different single active atoms on local structures to tune their electronic configuration. Significantly, the electrocatalytic behaviors of diverse SACs, assisted by density functional theory calculations, are systematically revealed by in situ synchrotron X-ray diffraction and in situ transmission electronic microscopy, providing a strategic library for the general synthesis and extensive applications of SACs in energy conversion and storage.


$$N$$ = 32 shell closure below calcium; Low-lying structure of $$^{50}$$Ar

Cort$'e$s, M. L.*; Rodriguez, W.*; Doornenbal, P.*; Obertelli, A.*; Holt, J. D.*; Men$'e$ndez, J.*; 緒方 一介*; Schwenk, A.*; 清水 則孝*; Simonis, J.*; et al.

Physical Review C, 102(6), p.064320_1 - 064320_9, 2020/12


 被引用回数:7 パーセンタイル:71.34(Physics, Nuclear)

理化学研究所RIBFにおいて、$$N$$=32同位体である$$^{50}$$Arの低励起構造を陽子・中性子ノックアウト反応,多核子剥離反応,陽子非弾性散乱と$$gamma$$線分光によって調査した。すでに知られていた2つに加えて、3$$^{-}$$状態の候補を含む5つの状態を新たに確認した。$$gamma$$ $$gamma$$ coincidenceによって得られた準位図は$$sd-pf$$模型空間での殻模型計算やカイラル2体・3体力による第一原理計算と比較した。陽子・中性子ノックアウト反応断面積の理論との比較により、新たに発見された2つの状態は2$$^{+}$$状態であり、また以前に4$$^{+}_{1}$$とされていた状態も2$$^{+}$$であることが示唆された。


First- and second-order topological superconductivity and temperature-driven topological phase transitions in the extended Hubbard model with spin-orbit coupling

Kheirkhah, M.*; Yan, Z.*; 永井 佑紀; Marsiglio, F.*

Physical Review Letters, 125(1), p.017001_1 - 017001_8, 2020/07

 被引用回数:29 パーセンタイル:93.03(Physics, Multidisciplinary)



Shell evolution of $$N$$ = 40 isotones towards $$^{60}$$Ca; First spectroscopy of $$^{62}$$Ti

Cort$'e$s, M. L.*; Rodriguez, W.*; Doornenbal, P.*; Obertelli, A.*; Holt, J. D.*; Lenzi, S. M.*; Men$'e$ndez, J.*; Nowacki, F.*; 緒方 一介*; Poves, A.*; et al.

Physics Letters B, 800, p.135071_1 - 135071_7, 2020/01

 被引用回数:22 パーセンタイル:96.25(Astronomy & Astrophysics)

ガンマ線分光による$$N$$=40同調体である$$^{62}$$Tiの分光学研究を$$^{63}$$V($$p$$,$$2p$$)$$^{62}$$TiをRIBFで行った。今回初めて測定された$$2_1^+ rightarrow 0_{rm gs}^+$$$$4_1^+ rightarrow 2_1^+$$の遷移はTiの基底状態が変形していることを示唆した。これらのエネルギーは近傍核の$$^{64}$$Crや$$^{66}$$Feと比較して大きく、したがって四重極集団運動が小さくなっていることが示唆される。今回の結果は大規模殻模型計算によって良く再現される一方、第一原理計算や平均場模型では今回の結果は再現されなかった。


Quasifree neutron knockout from $$^{54}$$Ca corroborates arising $$N=34$$ neutron magic number

Chen, S.*; Lee, J.*; Doornenbal, P.*; Obertelli, A.*; Barbieri, C.*; 茶園 亮樹*; Navr$'a$til, P.*; 緒方 一介*; 大塚 孝治*; Raimondi, F.*; et al.

Physical Review Letters, 123(14), p.142501_1 - 142501_7, 2019/10


 被引用回数:37 パーセンタイル:92.75(Physics, Multidisciplinary)

$$^{54}$$Caでは中性子魔法数34が現れると考えられているが、その直接的な実験的証拠を得るため、$$^{54}$$Caからの中性子ノックアウト反応$$^{54}$$Ca($$p,pn$$)$$^{53}$$Caによって生成される状態を理化学研究所のRI Beam Factoryによって調べた。基底状態および2.2MeVの励起状態が強く生成され、1.7MeVの励起状態の生成量は小さかった。$$^{53}$$Caの運動量分布から、基底状態および2.2MeVの励起状態は$$p$$軌道の中性子を叩き出して得られた状態であることが明らかになった。DWIA計算によって得られた分光学的因子から、$$^{54}$$Caは$$p$$軌道がほぼ完全に占有された閉殻構造を持つことが明らかになり、中性子魔法数34の出現が確実なものとなった。


The $$^{95}$$Zr($$n, gamma$$)$$^{96}$$Zr cross section from the surrogate ratio method and its effect on $$s$$-process nucleosynthesis

Yan, S. Q.*; Li, Z. H.*; Wang, Y. B.*; 西尾 勝久; Lugaro, M.*; Karakas, A. I.*; 牧井 宏之; Mohr, P.*; Su, J.*; Li, Y. J.*; et al.

Astrophysical Journal, 848(2), p.98_1 - 98_8, 2017/10

 被引用回数:5 パーセンタイル:24.24(Astronomy & Astrophysics)

The $$^{95}$$Zr($$n, gamma$$)$$^{96}$$Zr reaction cross section is crucial in the modelling of $$s$$-process nucleosynthesis in asymptotic giant branch stars because it controls the operation of the branching point at the unstable $$^{95}$$Zr and the subsequent production of $$^{96}$$Zr. We have carried out the measurement of the $$^{90}$$Zr($$^{18}$$O,$$^{16}$$O) and $$^{94}$$Zr($$^{18}$$O,$$^{16}$$O) reactions and obtained the $$gamma$$-decay probability ratio of $$^{92}$$Zr$$^{*}$$ and $$^{96}$$Zr$$^{*}$$ to determine the $$^{95}$$Zr($$n, gamma$$)$$^{96}$$Zr reaction cross sections with the surrogate ratio method. We tested our deduced maxwellian-averaged cross section in stellar models with masses between 2 and 6 $$M_{odot}$$ and metallicities 0.014 and 0.03. The largest changes - up 80 % variations in $$^{96}$$Zr - are seen in the models of 3-4 $$M_{odot}$$, where the $$^{22}$$Ne neutron source is mildly activated. The new rate can still provide a match to data from meteoritic stardust silicon carbide grains, provided the maximum mass of the parent stars is below 4 $$M_{odot}$$, for a metallicity of 0.03.


Examination of the surrogate ratio method for the determination of the $$^{93}$$Zr(n,$$gamma$$)$$^{94}$$Zr cross section with $$^{90,92}$$Zr($$^{18}$$O,$$^{16}$$O)$$^{92,94}$$Zr reactions

Yan, S. Q.*; Li, Z. H.*; Wang, Y. B.*; 西尾 勝久; 牧井 宏之; Su, J.*; Li, Y. J.*; 西中 一朗; 廣瀬 健太郎; Han, Y. L.*; et al.

Physical Review C, 94(1), p.015804_1 - 015804_5, 2016/07

 被引用回数:6 パーセンタイル:47.4(Physics, Nuclear)

The relative $$gamma$$-decay probability ratios of the neutron resonance states in $$^{94}$$Zr and $$^{92}$$Zr populated via two neutron transfer reactions, $$^{92}$$Zr($$^{18}$$O,$$^{16}$$O)$$^{94}$$Zr and $$^{90}$$Zr($$^{18}$$O,$$^{16}$$O)$$^{92}$$Zr, have been measured to test the validity of the surrogate ratio method (SRM) in determining the (n,$$gamma$$) reaction cross section. The cross sections of the $$^{93}$$Zr(n,$$gamma$$)$$^{94}$$Zr reaction are derived from the experimentally obtained ratios and the cross sections of the $$^{91}$$Zr(n,$$gamma$$)$$^{92}$$Zr reaction in the equivalent neutron energy range of $$E_{rm n}$$ = 0 - 8 MeV. The deduced cross sections of $$^{93}$$Zr(n,$$gamma$$)$$^{94}$$Zr reaction agree with the directly measured ones in the low-energy region, and with the evaluated ENDF/B-VII.1 data at higher energies of $$E_{rm n} >$$ 3 MeV. The agreement supports the concept of the SRM method to indirectly determine the (n,$$gamma$$) reaction cross sections.


Energetic ion transport by microturbulence is insignificant in tokamaks

Pace, D. C.*; Austin, M. E.*; Bass, E. M.*; Budny, R.*; Heidbrink, W. W.*; Hillesheim, J. C.*; Holcomb, C. T.*; Gorelenkova, M.*; Grierson, B. A.*; McCune, D. C.*; et al.

Physics of Plasmas, 20(5), p.056108_1 - 056108_18, 2013/05

 被引用回数:32 パーセンタイル:82.82(Physics, Fluids & Plasmas)



Signature splitting inversion and backbending in $$^{80}$$Rb

He, C.*; Shen, S.*; Wen, S.*; Zhu, L.*; Wu, X.*; Li, G.*; Zhao, Y.*; Yan, Y.*; Bai, Z.*; Wu, Y.*; et al.

Physical Review C, 87(3), p.034320_1 - 034320_10, 2013/03

 被引用回数:5 パーセンタイル:40.17(Physics, Nuclear)

High-spin states of $$^{80}$$Rb are studied via the fusion-evaporation reactions $$^{65}$$Cu+$$^{19}$$F, $$^{66}$$Zn+$$^{18}$$O, and $$^{68}$$Zn+$$^{16}$$O with the beam energies of 75 MeV, 76 MeV, and 80 MeV, respectively. Twenty-three states with twenty-eight $$gamma$$ transitions are added to the previously proposed level scheme, where the second negative-parity band is significantly pushed up to spins of 22$$^-$$ and 15$$^-$$ and two sidebands are built on the known first negative-parity band. Two successive band crossings with frequencies 0.51 MeV and 0.61 MeV in the $$alpha$$ = 0 branch as well as another one in the $$alpha$$ =1 branch of the second negative-parity band are observed. Signature inversions occur in the positive-parity and first negative-parity bands at the spins of 11$$hbar$$ and 16$$hbar$$, respectively. The signature splitting is seen obviously in the second negative-parity band, but the signature inversion is not observed. It is also found that the structure of the two negative-parity bands is similar to that of its isotone $$^{82}$$Y. Signature inversion in the positive-parity yrast band with configuration $$pi$$g9/2 $$otimes$$ $$nu$$g9/2 in this nucleus is discussed using the projected shell model.


The Spectra of the multicharged argon hollow ions; Observation, modeling and using for diagnostics of the early stage of the heating of clusters by a supper high contrast femtosecond laser pulses

Pikuz, T.; Faenov, A.*; Skobelev, I.*; Fortov, V. E.*; Boldarev, A.*; Gasilov, V.*; Chen, L. M.*; Zhang, L.*; Yan, W.*; Yuan, D.*; et al.

AIP Conference Proceedings 1465, p.181 - 201, 2012/07

 被引用回数:0 パーセンタイル:0.13

A study is made of the ultra-short laser pulse irradiation of Ar cluster targets. Experiments have been performed with large cluster sizes and using very high laser contrasts, which have allowed clear and unambiguous observation of exotic inner-shell transitions in near-neutral Ar ions. The interaction of the main laser pulse with the unperturbed target is a necessary requirement for observing these lines. Our measurements are supported by kinetics calculations in which a very detailed atomic model is used. X-ray spectral methods have been proposed to determine the parameters of the appearing plasma at the early stages of its evolution. It has been shown that the spectra of hollow ions are the most informative in the first moments of the heating of a cluster, whereas the diagnostics of the late stages can be performed using the conventional lines of multicharged ions.


From a single-band metal to a high-temperature superconductor via two thermal phase transitions

He, R.-H.*; 橋本 真*; Karapetyan, H.*; Koralek, J. D.*; Hinton, J. P.*; Testaud, J. P.*; Nathan, V.*; 吉田 良行*; Yao, H.*; 田中 清尚*; et al.

Science, 331(6024), p.1579 - 1583, 2011/03

 被引用回数:265 パーセンタイル:98.75(Multidisciplinary Sciences)



Aqueous chemistry with seaborgium (element 106)

Br$"u$chle, W.*; Andrassy, M.*; Angert, R.*; Eberhardt, K.*; Fricke, B.*; Gregorich, K. E.*; G$"u$nther, R.*; Hartmann, W.*; Heimann, R.*; Hoffman, D. C.*; et al.

1st International Conference on the Chemistry and Physics of the Transactinide Elements; Extended Abstracts, 4 Pages, 1999/00


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