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論文

Continuum excitations in a spin supersolid on a triangular lattice

Zhu, M.*; Romerio, V.*; Steiger, N.*; Nabi, S. D.*; 村井 直樹; 河村 聖子; Povarov, K. Y.*; Skourski, Y.*; Sibille, R.*; Keller, L.*; et al.

Physical Review Letters, 133(18), p.186704_1 - 186704_6, 2024/11

https://doi.org/10.1103/PhysRevLett.133.186704
 被引用回数：5 パーセンタイル：72.87(Physics, Multidisciplinary)

Magnetic, thermodynamic, neutron diffraction and inelastic neutron scattering are used to study spin correlations in the easy-axis XXZ triangular lattice magnet K$$_{2}$$Co(SeO$$_{3}$$)$$_{2}$$. Despite the presence of quasi-2D supersolid magnetic order, the low-energy excitation spectrum contains no sharp modes and is instead a broad and structured multiparticle continuum. Applying a weak magnetic field drives the system into an m = 1/3 fractional magnetization plateau phase and restores sharp spin wave modes. To some extent, the behavior at zero field can be understood in terms of spin wave decay. However, the presence of clear excitation minima at the M points of the Brillouin zone suggest that the spinon language may provide a more adequate description, and signals a possible proximity to a Dirac spin liquid state.

論文

Antiferromagnetism and phase stability of CrMnFeCoNi high-entropy alloy

Zhu, L.*; He, H.*; Naeem, M.*; Sun, X.*; Qi, J.*; Liu, P.*; Harjo, S.; 中島 健次; Li, B.*; Wang, X.-L.*

Physical Review Letters, 133(12), p.126701_1 - 126701_6, 2024/09

https://doi.org/10.1103/PhysRevLett.133.126701
 被引用回数：1 パーセンタイル：53.15(Physics, Multidisciplinary)

It has long been suspected that magnetism could play a vital role in the phase stability of multi- component high-entropy alloys. However, the nature of the magnetic order, if any, has remained elusive. Here, by using elastic and inelastic neutron scattering, we demonstrate evidence of antiferromagnetic order below $$sim$$80 K and strong spin fluctuations persisting to room temperature in a single-phase face-centered cubic (fcc) CrMnFeCoNi high-entropy alloy. Despite the chemical complexity, the magnetic structure in CrMnFeCoNi can be described as $$gamma$$-Mn-like, with the magnetic moments confined in alternating (001) planes and pointing toward the $$langle$$111$$rangle$$ direction. Combined with first-principles calculation results, it is shown that the antiferromagnetic order and spin fluctuations help stabilized the fcc phase in CrMnFeCoNi high-entropy alloy.

論文

Microscopic insights of the extraordinary work-hardening due to phase transformation

Ma, Y.*; Naeem, M.*; Zhu, L.*; He, H.*; Sun, X.*; Yang, Z.*; He, F.*; Harjo, S.; 川崎 卓郎; Wang, X.-L.*

Acta Materialia, 270, p.119822_1 - 119822_13, 2024/05

https://doi.org/10.1016/j.actamat.2024.119822
 被引用回数：9 パーセンタイル：94.10(Materials Science, Multidisciplinary)

We report an in situ neutron diffraction study of 316 L that reveals an extraordinary work-hardening rate (WHR) of $$sim$$7 GPa at 15 K. Detailed analyses show that the major contribution to the excellent strength and ductility comes from the transformation-induced plasticity (TRIP) effect, introduced by the austenite-to-martensite ($$gamma$$-to-$$alpha$$') phase transition. A dramatic increase in the WHR is observed along with the transformation; the WHR declined when the austenite phase is exhausted. During plastic deformation, the volume-fraction weighted phase stress and stress contribution from the $$alpha$$'-martensite increase significantly. The neutron diffraction data further suggest that the $$gamma$$-to-$$alpha$$' phase transformation was mediated by the $$varepsilon$$-martensite, as evidenced by the concurrent decline of the $$varepsilon$$ phase with the $$gamma$$ phase.

論文

Low spin spectroscopy of neutron-rich $$^{43,44,45}$$Cl via $$beta^-$$ and $$beta n$$ decay

Tripathi, V.*; Bhattacharya, S.*; Rubino, E.*; Benetti, C.*; Perello, J. F.*; Tabor, S. L.*; Liddick, S. N.*; Bender, P. C.*; Carpenter, M. P.*; Carroll, J. J.*; et al.

Physical Review C, 109(4), p.044320_1 - 044320_15, 2024/04

https://doi.org/10.1103/PhysRevC.109.044320
 被引用回数：0 パーセンタイル：0.00(Physics, Nuclear)

ミシガン州立大学の国立超伝導サイクロトロン研究所において$$^{48}$$Caのフラグメンテーション反応によって中性子過剰核$$^{43,45}$$Sを生成し、そこからのベータ崩壊および遅発中性子放出ベータ崩壊によって$$^{43,44,45}$$Clの励起状態を得た。得られた実験データをSDPFSDG-MU相互作用を用いた大規模殻模型計算と比較し、よい一致を得た。

論文

Crystal-liquid duality driven ultralow two-channel thermal conductivity in $$alpha$$-MgAgSb

Li, J.*; Li, X.*; Zhang, Y.*; Zhu, J.*; Zhao, E.*; 古府 麻衣子; 中島 健次; Avdeev, M.*; Liu, P.-F.*; Sui, J.*; et al.

Applied Physics Reviews (Internet), 11(1), p.011406_1 - 011406_8, 2024/03

https://doi.org/10.1063/5.0173680
 被引用回数：7 パーセンタイル：92.96(Physics, Applied)

The desire for intrinsically low lattice thermal conductivity ($$kappa_L$$) in thermoelectrics motivates numerous efforts on understanding the microscopic mechanisms of heat transport in solids. Here, based on theoretical calculations, we demonstrate that $$alpha$$-MgAgSb hosts low-energy localized phonon bands and avoided crossing of the rattler modes, which coincides with the inelastic neutron scattering result. Using the two-channel lattice dynamical approach, we find, besides the conventional contribution ($$sim$$70% at 300 K) from particlelike phonons propagating, the coherence contribution dominated by the wavelike tunneling of phonons accounts for $$sim$$30% of total $$kappa_L$$ at 300 K. By considering dual contributions, our calculated room-temperature $$kappa_L$$ of 0.64 Wm$$^{-1}$$K$$^{-1}$$ well agrees with the experimental value of 0.63 Wm$$^{-1}$$K$$^{-1}$$. More importantly, our computations give a nonstandard $$kappa_L propto T^{-0.61}$$ dependence, perfectly explaining the abnormal temperature-trend of $$sim T^{-0.57}$$ in experiment for $$alpha$$-MgAgSb. By molecular dynamics simulation, we reveal that the structure simultaneously has soft crystalline sublattices with the metavalent bonding and fluctuating liquid-like sublattices with thermally induced large amplitude vibrations. These diverse forms of chemical bonding arouse mixed part-crystal part-liquid state, scatter strongly heat-carrying phonons, and finally produce extremely low $$kappa_L$$. The fundamental research from this study will accelerate the design of ultralow-$$kappa_L$$ materials for energy-conversion applications.

論文

Phase transformation and equation of state in Ti-45Al alloy under high pressure

Li, X.*; Zhu, R.*; Xin, J.*; Luo, M.*; Shang, S.-L.*; Liu, Z.-K.*; Yin, C.*; 舟越 賢一*; Dippenaar, R. J.*; 肥後 祐司*; et al.

CALPHAD; Computer Coupling of Phase Diagrams and Thermochemistry, 84, p.102641_1 - 102641_6, 2024/03

https://doi.org/10.1016/j.calphad.2023.102641
 被引用回数：0 パーセンタイル：0.00(Thermodynamics)

The phase transformations and pressure-volume dependencies of the Ti-45Al alloy with respect to pressure have been investigated by means of in-situ observation using multi anvil-type high-pressure devices and synchrotron radiation. Under hydrostatic compression from 0 to 10.1 GPa, about 2.3 vol. % of $$gamma$$ transforms continuously to $$alpha$$2. Lattice parameters as well as volume fractions of these two phases have been determined as a function of pressure. Bulk moduli estimated using Birch-Murnaghan's equation of state are 148 GPa for the $$gamma$$ phase, 138 GPa for the $$alpha$$2 phase, and 149 GPa for their two-phase mixture of Ti-45Al alloy. First-principles have also applied to investigate bulk moduli of two single phases, and the deviation between calculations and measurements is discussed and attributed to mainly phase transformation. The presently study provides useful insights into thermodynamics of $$alpha$$2 and $$gamma$$ phases under high pressure.

論文

Extreme phonon anharmonicity underpins superionic diffusion and ultralow thermal conductivity in argyrodite Ag$$_{8}$$SnSe$$_{6}$$

Ren, Q.*; Gupta, M. K.*; Jin, M.*; Ding, J.*; Wu, J.*; Chen, Z.*; Lin, S.*; Fabelo, O.*; Rodriguez-Velamazan, J. A.*; 古府 麻衣子; et al.

Nature Materials, 22(8), p.999 - 1006, 2023/08

https://doi.org/10.1038/s41563-023-01560-x
 被引用回数：72 パーセンタイル：99.21(Chemistry, Physical)

Ultralow thermal conductivity and fast ionic diffusion endow superionic materials with excellent performance both as thermoelectric converters and as solid-state electrolytes. Yet the correlation and interdependence between these two features remain unclear owing to a limited understanding of their complex atomic dynamics. Here we investigate ionic diffusion and lattice dynamics in argyrodite Ag$$_{8}$$SnSe$$_{6}$$ using synchrotron X-ray and neutron scattering techniques along with machine-learned molecular dynamics. We identify a critical interplay of the vibrational dynamics of mobile Ag and a host framework that controls the overdamping of low-energy Ag-dominated phonons into a quasi-elastic response, enabling superionicity. Concomitantly, the persistence of long-wavelength transverse acoustic phonons across the superionic transition challenges a proposed 'liquid-like thermal conduction' picture. Rather, a striking thermal broadening of low-energy phonons, starting even below 50 K, reveals extreme phonon anharmonicity and weak bonding as underlying features of the potential energy surface responsible for the ultralow thermal conductivity ($$<$$ 0.5 Wm$$^{-1}$$K$$^{-1}$$) and fast diffusion. Our results provide fundamental insights into the complex atomic dynamics in superionic materials for energy conversion and storage.

論文

$$beta^-$$ decay of exotic P and S isotopes with neutron number near 28

Tripathi, V.*; Bhattacharya, S.*; Rubino, E.*; Benetti, C.*; Perello, J. F.*; Tabor, S. L.*; Liddick, S. N.*; Bender, P. C.*; Carpenter, M. P.*; Carroll, J. J.*; et al.

Physical Review C, 106(6), p.064314_1 - 064314_14, 2022/12

https://doi.org/10.1103/PhysRevC.106.064314
 被引用回数：4 パーセンタイル：54.93(Physics, Nuclear)

ミシガン州立大学の国立超伝導サイクロトロン研究所にて、中性子過剰なリン、硫黄同位体を生成し、そこからのベータ崩壊半減期および娘核の励起準位を測定した。$$^{42}$$Pの崩壊によって得られるエネルギー準位から、この原子核の基底状態は$$2^-$$あるいは$$3^-$$であることが示唆された。中性子数が偶数の硫黄同位体からの崩壊様式を系統的に調べた結果、中性子数が増えるにつれてガモフテラー遷移強度の大きな準位の励起エネルギーが高くなることがわかった。これは、大規模殻模型計算によって予言されている現象に一致する。

論文

Solving the puzzles of the decay of the heaviest known proton-emitting nucleus $$^{185}$$Bi

Doherty, D. T.*; Andreyev, A. N.; Seweryniak, D.*; Woods, P. J.*; Carpenter, M. P.*; Auranen, K.*; Ayangeakaa, A. D.*; Back, B. B.*; Bottoni, S.*; Canete, L.*; et al.

Physical Review Letters, 127(20), p.202501_1 - 202501_6, 2021/11

https://doi.org/10.1103/PhysRevLett.127.202501
 被引用回数：10 パーセンタイル：65.49(Physics, Multidisciplinary)

$$^{185}$$Bi is the heaviest known proton emitting isotope. Its decay had been observed, but the assumed ground-state lifetime ($$sim$$$$60~mu$$s) was incorrect, leading to unexplained hindrance. With two new experiments at Argonne National Laboratory, two states were clearly identified. One is the proton-emitting ground-state (spin 1/2$$^+$$, half-life: 2.8$$^{+2.3}_{-1.0}$$ $$mu$$s), the second is a 58(2) $$mu$$s $$gamma$$-decaying isomer. The new data show the inversion of the ground and isomeric states compared to neighboring Bi isotopes. This is the only known example of a ground-state proton decay to a daughter nucleus ($$^{184}$$Pb) with a major shell closure.

論文

Martensitic transformation in CrCoNi medium-entropy alloy at cryogenic temperature

Naeem, M.*; Zhou, H.*; He, H.*; Harjo, S.; 川崎 卓郎; Lan, S.*; Wu, Z.*; Zhu, Y.*; Wang, X.-L.*

Applied Physics Letters, 119(13), p.131901_1 - 131901_7, 2021/09

https://doi.org/10.1063/5.0067268
 被引用回数：20 パーセンタイル：77.22(Physics, Applied)

We investigated the in situ deformation behavior of the CrCoNi medium-entropy alloy at a cryogenic temperature of 140 K and compared it with deformation at room temperature. The sample exhibited higher strength and larger ductility at the cryogenic temperature. The CrCoNi alloy remained single-phase face-centered cubic at room temperature, while deformation at 140 K resulted in a martensitic transformation to the hexagonal close-packed structure. The phase transformation, an additional deformation mechanism to stacking faults, twinning, and dis- location slip, resulted in a higher work hardening at cryogenic temperature. The study addresses the structure metastability in the CrCoNi alloy, which led to the formation of epsilon-martensite from the intrinsic stacking faults.

論文

Manipulation of saturation magnetization and perpendicular magnetic anisotropy in epitaxial Co$$_{x}$$Mn$$_{4-x}$$N films with ferrimagnetic compensation

伊藤 啓太*; 安富 陽子*; Zhu, S.*; Nurmamat, M.*; 田原 昌樹*; 都甲 薫*; 秋山 了太*; 竹田 幸治; 斎藤 祐児; 小口 多美夫*; et al.

Physical Review B, 101(10), p.104401_1 - 104401_8, 2020/03

https://doi.org/10.1103/PhysRevB.101.104401
 被引用回数：22 パーセンタイル：74.23(Materials Science, Multidisciplinary)

Spintronics devices utilizing a magnetic domain wall motion have attracted increasing attention, and ferrimagentic materials with almost compensated magnetic moments are highly required to realize the fast magnetic domain wall motion. Here, we report a key function for this purpose in anti-perovskite Co$$_{x}$$Mn$$_{4-x}$$N films. Perpendicular magnetization emerges for $$0.8 leq x$$, and the saturation magnetization reaches a minimum value at $$x = 0.8$$.

論文

Negative Te spin polarization responsible for ferromagnetic order in the doped topological insulator V$$_{0.04}$$(Sb$$_{1-x}$$Bi$$_{x}$$)$$_{1.96}$$Te$$_{3}$$

Ye, M.*; Xu, T.*; Li, G.*; Qiao, S.*; 竹田 幸治; 斎藤 祐児; Zhu, S.-Y.*; Nurmamat, M.*; 角田 一樹*; 石田 行章*; et al.

Physical Review B, 99(14), p.144413_1 - 144413_7, 2019/04

AA2018-0697.pdf:1.89MB

https://doi.org/10.1103/PhysRevB.99.144413
 被引用回数：15 パーセンタイル：57.22(Materials Science, Multidisciplinary)

We investigate the microscopic origin of ferromagnetism coupled with topological insulators in V-doped (Sb,Bi)$$_{2}$$Te$$_{3}$$ employing X-ray magnetic circular dichroism and angle-resolved two-photon photoemission spectroscopies, combined with first-principles calculations. We found an magnetic moment at the Te site anti-parallel to that of the V and Sb sites, which plays a key role in the ferromagnetic order. We ascribe it to the hybridization between Te 5${it p}$ and V 3${it d}$ majority spin states at the Fermi energy, consistent with the Zener-type ${it p}$-${it d}$ exchange interaction scenario. The substitution of Bi for Sb suppresses the bulk ferromagnetism by introducing extra electron carriers in the majority spin channel of the Te ${it p}$ states that compensates the antiparallel magnetic moment on the Te site. Our findings reveal important clues to designing magnetic topological insulators with higher Curie temperature that work under ambient conditions.

論文

$$^{239}$$Pu nuclear magnetic resonance in the candidate topological insulator PuB$$_4$$

Dioguardi, A. P.*; 安岡 弘志*; Thomas, S. M.*; 酒井 宏典; Cary, S. K.*; Kozimor, S. A.*; Albrecht-Schmitt, T. E.*; Choi, H. C.*; Zhu, J.-X.*; Thompson, J. D.*; et al.

Physical Review B, 99(3), p.035104_1 - 035104_6, 2019/01

https://doi.org/10.1103/PhysRevB.99.035104
 被引用回数：10 パーセンタイル：43.10(Materials Science, Multidisciplinary)

正方晶プルトニウムボロン化合物PuB$$_{4}$$の単結晶、および粉末試料を用いて、$$^{239}$$Pu核核磁気共鳴(NMR)実験を行なった。この化合物は、最近になって強相関電子系のトポロジカル絶縁体候補物質と考えられている。$$^{239}$$Pu核NMRスペクトルは、結晶内Pu位置の局所対称性を反映したものとなっており、NMRシフトとNMR緩和率の温度依存性は、エネルギーギャップをもつ非磁性状態にあることが示唆された。これは、密度汎関数理論計算結果とも矛盾しない。実際に観測された巨視的なギャップ状態は、本化合物がトポロジカル絶縁体候補であることを支持している。

論文

Stability and synthesis of superheavy elements; Fighting the battle against fission - Example of $$^{254}$$No

Lopez-Martens, A.*; Henning, G.*; Khoo, T. L.*; Seweryniak, D.*; Alcorta, M.*; 浅井 雅人; Back, B. B.*; Bertone, P. F.*; Boilley, D.*; Carpenter, M. P.*; et al.

EPJ Web of Conferences, 131, p.03001_1 - 03001_6, 2016/12

https://doi.org/10.1051/epjconf/201613103001
 被引用回数：1 パーセンタイル：42.24(Chemistry, Inorganic & Nuclear)

原子番号が100を超える原子核の核分裂障壁の高さとその角運動量依存性を初めて測定した。核分裂による崩壊が優勢となり始める励起エネルギーを決定できる初期分布法という方法を$$^{254}$$Noの測定に適用した。$$^{254}$$Noの核分裂障壁はスピンゼロにおいて6.6MeVと決定された。このことは、$$^{254}$$Noが原子核の殻効果によって強く安定化されていることを示している。

論文

Population and decay of a $$K^{pi}$$ = 8$$^{-}$$ two-quasineutron isomer in $$^{244}$$Pu

Hota, S.*; Tandel, S.*; Chowdhury, P.*; Ahmad, I.*; Carpenter, M. P.*; Chiara, C. J.*; Greene, J. P.*; Hoffman, C. R.*; Jackson, E. G.*; Janssens, R. V. F.*; et al.

Physical Review C, 94(2), p.021303_1 - 021303_5, 2016/08

https://doi.org/10.1103/PhysRevC.94.021303
 被引用回数：9 パーセンタイル：50.87(Physics, Nuclear)

$$^{244}$$Puにおける$$K^{pi}$$ = 8$$^{-}$$アイソマーからの崩壊と集団的バンド構造が$$^{47}$$Tiと$$^{208}$$Pbのビームによる深部非弾性散乱実験によって調べられた。バンド内の正確な$$M1/E2$$分岐比の測定によって、偶$$Z$$, $$N$$=150アイソトーンにおける$$K^{pi}$$ = 8$$^{-}$$二準中性子アイソマーが9/2$$^-$$[734]$$_{nu}$$$$otimes$$7/2$$^+$$[624]$$_{nu}$$の配位であることを確かめた。$$N$$=152における変形シェルギャップ近傍のこれらのアイソマーは、超重核の一粒子エネルギーの理論的な予言において重要なベンチマークとなる。

論文

Carrier-mediated ferromagnetism in the magnetic topological insulator Cr-doped (Sb,Bi)$$_{2}$$Te$$_{3}$$

Ye, M.*; Li, W.*; Zhu, S.-Y.*; 竹田 幸治; 斎藤 祐児; Wang, J.*; Pan, H.*; Nurmamat, M.*; 角田 一樹*; Ji, F.*; et al.

Nature Communications (Internet), 6, p.8913_1 - 8913_7, 2015/11

AA2015-0647.pdf:0.64MB

https://doi.org/10.1038/ncomms9913
 被引用回数：60 パーセンタイル：90.42(Multidisciplinary Sciences)

磁性元素を添加したトポロジカル絶縁体は、量子異常ホール効果や無散逸伝導などの魅力的な現象の発現が予言され、低消費電力スピンデバイスの開発につながっていくものと期待されている。既に、いくつかの磁性添加トポロジカル絶縁体で長距離磁気秩序が確認されている。しかし、量子異常ホール効果の発現は、極低温におけるCrを添加した(Sb,Bi)$$_{2}$$Te$$_{3}$$系に限られており、強磁性の微視的な起源はほとんど分かっていない。そこで、今回、X線磁気円二色性実験による元素選択的研究を行うことにより、本物質系の強磁性は、母体の正孔キャリアーを媒介としたものであり、Crの3d電子とSbやTeのp電子の相互作用が極めて重要であることを明らかにした。この結果は、異常量子ホール素子の実現に向けても重要である。

論文

Spectroscopic evidence of band Jahn-Teller distortion upon martensitic phase transition in Heusler-type Ni-Fe(Co)-Ga ferromagnetic shape-memory alloy films

角田 一樹*; 白井 開渡*; Zhu, S.-Y.*; 谷口 雅樹*; Ye, M.*; 上田 茂典*; 竹田 幸治; 斎藤 祐児; Aseguinolaza, I. R.*; Barandiar$'a$n, J. M.*; et al.

Physical Review B, 91(13), p.134417_1 - 134417_6, 2015/04

https://doi.org/10.1103/PhysRevB.91.134417
 被引用回数：6 パーセンタイル：26.30(Materials Science, Multidisciplinary)

The temperature evolution of the electronic structure of a Ni-Fe(Co)-Ga/MgO(100), Heusler-type, ferromagnetic shape-memory alloy thin film has been followed by a bulk-sensitive hard X-ray photoelectron spectroscopy, element-selective soft X-ray magnetic circular dichroism, and first-principles calculation. The reversible changes of the electronic states near the Fermi energy show a hysteresis associated with the martensitic phase transition (MPT), where the pseudogap opens on cooling and closes again on warming. In addition, the Ni 3d spin magnetic moment increases by approximately two times across the MPT, whereas the change of Fe 3d moment is moderate. By comparing the experimental results with the calculated spin-resolved density of states, we conclude that the band Jahn-Teller effect of Ni 3d and Fe 3d orbitals is responsible for MPT.

論文

Identification of deformed intruder states in semi-magic $$^{70}$$Ni

Chiara, C. J.*; Weisshaar, D.*; Janssens, R. V. F.*; 角田 佑介*; 大塚 孝治*; Harker, J. L.*; Walters, W. B.*; Recchia, F.*; Albers, M.*; Alcorta, M.*; et al.

Physical Review C, 91(4), p.044309_1 - 044309_10, 2015/04

https://doi.org/10.1103/PhysRevC.91.044309
 被引用回数：40 パーセンタイル：90.88(Physics, Nuclear)

アルゴンヌ国立研究所にて中性子過剰核$$^{70}$$Niを$$^{70}$$Znの多核子移行反応によって生成し、$$gamma$$線検出器GRETINAを用いて$$gamma$$線分光を行った。その結果、$$2^+_2$$, $$4^+_2$$準位を初めて観測した。これらの準位は小さな模型空間を採用した殻模型計算では再現されないため、陽子の$$f_{7/2}$$軌道からの励起を伴った大きな変形状態であると考えられる。本論文の理論グループが2014年に発表した大規模殻模型計算によって$$^{70}$$Niの励起状態を解析した結果、これらの状態は大きなプロレート変形を持つ状態とよく対応することがわかった。この結果は、中性子過剰ニッケル同位体における変形共存が$$^{68}$$Ni以外にも存在することを実証するとともに、中性子過剰核における大規模殻模型計算の予言能力を確かめるものである。

論文

Fission barrier of superheavy nuclei and persistence of shell effects at high spin; Cases of $$^{254}$$No and $$^{220}$$Th

Henning, G.*; Khoo, T. L.*; Lopez-Martens, A.*; Seweryniak, D.*; Alcorta, M.*; 浅井 雅人; Back, B. B.*; Bertone, P. F.*; Boilley, D.*; Carpenter, M. P.*; et al.

Physical Review Letters, 113(26), p.262505_1 - 262505_6, 2014/12

https://doi.org/10.1103/PhysRevLett.113.262505
 被引用回数：34 パーセンタイル：81.88(Physics, Multidisciplinary)

殻効果によって安定に存在する超重核である$$^{254}$$Noの核分裂障壁の高さを実験的に決定した。核反応で生成した$$^{254}$$Noからの脱励起$$gamma$$線の本数と全エネルギーを測定することで$$gamma$$崩壊の開始点の励起エネルギーとスピン値を導出し、その分布から核分裂障壁の高さをスピンの関数として19$$hbar$$まで決定した。$$^{254}$$Noの核分裂障壁の高さは、スピン15$$hbar$$において6.0MeV、スピン0$$hbar$$における外挿値として6.6MeVと決定された。この結果は、殻効果が、このような重い原子核の核分裂障壁を高くしていることを明確に示し、またその高さが高スピン状態まで保持されていることを証明するものである。

論文

Exploring the stability of super heavy elements; First measurement of the fission barrier of $$^{254}$$No

Henning, G.*; Lopez-Martens, A.*; Khoo, T. L.*; Seweryniak, D.*; Alcorta, M.*; 浅井 雅人; Back, B. B.*; Bertone, P. F.*; Boilley, D.*; Carpenter, M. P.*; et al.

EPJ Web of Conferences, 66, p.02046_1 - 02046_8, 2014/03

https://doi.org/10.1051/epjconf/20146602046
 被引用回数：3 パーセンタイル：68.10(Physics, Nuclear)

初期状態分布法により$$^{254}$$Noの核分裂障壁の高さを決定した。初期状態分布とは、核融合-粒子蒸発反応によって励起された原子核が$$gamma$$線放出による脱励起を開始する励起エネルギーとスピンの状態を二次元で表示したものであり、$$gamma$$線多重度と全$$gamma$$線エネルギーの測定から求めることができる。本論文では、初期状態分布法の詳細を詳しく記述し、$$^{254}$$Noの核分裂障壁の高さを初めて決定した実験結果について報告する。なお、$$^{254}$$Noは核分裂障壁が測定された最も重い原子核である。

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