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筋田 涼太*; 今井 彩帆里*; 大内 誠*; 青木 裕之; 寺島 崇矢*
Macromolecules, 56(23), p.9738 - 9749, 2023/12
被引用回数：0 パーセンタイル：0(Polymer Science)Constructing ordered ionic nanostructures into bulk polymers and thin films is an important technique to create functional materials, such as polyelectrolytes and proton- and ion-conducting materials, for various applications. Herein, we report microphase separation of cationic homopolymers bearing alkyl ammonium bromides to create sub-4 nm lamellar materials, where an ionic phase is alternatingly layered with a hydrophobic alkyl phase and serves as a channel for water intercalation. We prepared cationic homopolymers with linear or branched alkyl pendants (octyl or 2-ethylhexyl group: C8-eicosyl or 2-octyldodecyl group: C20) via the free radical polymerization of 2-(dimethylamino)ethyl acrylate (DMAEA), followed by the quaternization of the polyDMAEA with corresponding alkyl bromides. The homopolymers carrying linear hexadecyl, octadecyl, and eicosyl groups were crystalline at room temperature, whereas the others were amorphous. The homopolymers bearing linear alkyl pendants longer than the decyl group or branched alkyl pendants larger than the 2-butyloctyl group formed lamellar structures by the self-assembly of the side chains. The domain spacing can be controlled between 2.5 and 3.7 nm by tuning the pendant structures and are smaller than that formed by the corresponding random copolymers. A cationic homopolymer bearing crystalline octadecyl groups maintained lamellar structures up to 
210 
C far beyond the melting temperature (50 C). The cationic homopolymer further formed a multilayered lamellar thin film on a silicon substrate, in which the cationic layers absorbed water under humid conditions and reversibly released the water therefrom in a N
gas atmosphere.
真野 晃宏; 今井 隆太*; 宮本 裕平*; Lu, K.; 勝山 仁哉; Li, Y.
International Journal of Pressure Vessels and Piping, 199, p.104700_1 - 104700_13, 2022/10
被引用回数：1 パーセンタイル：28.33(Engineering, Multidisciplinary)有限要素法に基づく弾塑性解析は、金属材料の非線形挙動の再現に広く用いられる。この弾塑性解析を陰解法により実施する場合、応力値は通常リターンマッピングアルゴリズムを通じて時間増分ごとに更新される。一方、延性破壊等の複雑な挙動の解析では、リターンマッピングアルゴリズムに係る連立方程式の数が多くなり、収束解を得ることが困難となる場合がある。そのため、本論文では、連立方程式の数の削減を通じて陰解法による安定的な非線形解析を実現することを目的として、陰関数定理に基づき連立方程式の数を削減する一般的な手法を提案した。また、提案手法を、延性破壊解析に用いられるGurson-Tvergaard-Needleman(GTN)モデルに適用し、弾塑性解析を実施した。その結果、解析により、延性破壊に係る実験結果が再現できることを確認した。以上を踏まえ、提案手法は、金属材料の延性破壊解析に有用であると結論付けた。
今井 彩帆里*; 荒川 勝利*; 中西 洋平*; 竹中 幹人*; 青木 裕之; 大内 誠*; 寺島 崇矢*
Macromolecules, 55(20), p.9113 - 9125, 2022/10
被引用回数：2 パーセンタイル：27.19(Polymer Science)Microphase separation of copolymers is a key technique to produce polymer bulk materials or thin films with ordered nanostructures for applications in various research fields including nanotechnologies, electronic devices, among many others. Herein, we report water-assisted microphase separation of amphiphilic random copolymers bearing quaternary ammonium cations and hydrophobic alkyl or oleyl groups in the solid state and the thin films. We investigated the effects of sample preparation protocols and the hydrophobic pendants (a butyl group: C4 - octadecyl or oleyl group: C18), composition, and molecular weight of the copolymers on the microphase separation behavior. By annealing under humid conditions, the copolymers bearing alkyl groups longer than an octyl group (C8) formed sub-5 nm lamellar structures comprising cationic layers and hydrophobic layers. Water hardly remained in the resulting lamellar materials under ambient conditions. The domain spacing was controlled between 3.7 and 5.3 nm by tuning the length of the hydrophobic pendants and composition and was independent of the molecular weight and molecular weight distribution. The cationic random copolymers carrying amorphous hydrophobic pendants provided transparent or translucent polymer materials containing small lamellar structures. The random copolymers further formed multilayered lamellar thin films on silicon substrates by spin-coating the copolymer solutions, followed by a humid annealing process. The layered lamellae were directly observed as terrace structures with about 4-5 nm steps by atomic force microscopy.
elastic scattering in the momentum range 0.44-0.80 GeV/c七村 拓野; 藤田 真奈美; 長谷川 勝一; 市川 真也; 市川 裕大; 今井 憲一*; 成木 恵; 佐藤 進; 佐甲 博之; 田村 裕和; et al.
Progress of Theoretical and Experimental Physics (Internet), 2022(9), p.093D01_1 - 093D01_35, 2022/09
被引用回数：5 パーセンタイル：67.44(Physics, Multidisciplinary)We performed a novel 
scattering experiment at the J-PARC Hadron Experimental Facility. Approximately 2400 elastic scattering events were identified from 
tagged 
particles in the momentum range 0.44 - 0.80 GeV/c. The differential cross sections of the elastic scattering were derived with much better precision than in previous experiments. The obtained differential cross sections were approximately 2 mb/sr or less, which were not as large as those predicted by the fss2 and FSS models based on the quark cluster model in the short-range region. By performing phase-shift analyses for the obtained differential cross sections, we experimentally derived the phase shifts of the 
and 
channels for the first time. The phase shift of the 3S1 channel, where a large repulsive core was predicted owing to the Pauli effect between quarks, was evaluated to be 
. If the sign of 
is assumed to be negative, the interaction in this channel is moderately repulsive, as the Nijmegen extended-sort-core models predicted.
elastic scattering in momentum range 470 to 850 MeV/
三輪 浩司*; 藤田 真奈美; 長谷川 勝一; 細見 健二; 市川 裕大; 今井 憲一*; 七村 拓野; 成木 恵; 佐甲 博之; 佐藤 進; et al.
Physical Review C, 104(4), p.045204_1 - 045204_20, 2021/10
被引用回数：12 パーセンタイル：89.15(Physics, Nuclear)A high statistics 
scattering experiment is performed at the J-PARC Hadron Experimental Facility. Momentum-tagged 
s running in a liquid hydrogen target are accumulated by detecting the reaction with a high intensity 
beam of 20 M/spill. The differential cross sections of the elastic scattering were derived with a drastically improved accuracy by identifying approximately 4,500 events from 1.72 
10
. The derived differential cross section shows a clear forward-peaking angular distribution for a momentum range from 470 to 850 MeV/. The accurate data will impose a strong constraint on the theoretical models of the baryon-baryon interactions.
-state of a 
hypernucleus, 
吉本 雅浩*; 藤田 真奈美; 橋本 直; 早川 修平; 市川 裕大; 市川 真也; 今井 憲一*; 七村 拓野; 成木 恵; 佐甲 博之; et al.
Progress of Theoretical and Experimental Physics (Internet), 2021(7), p.073D02_1 - 073D02_19, 2021/07
被引用回数：13 パーセンタイル：81.3(Physics, Multidisciplinary)Bound-systems of 
-
are studied via capture at rest followed by emission of a twin single-
hypernucleus in the emulsion detectors. Two events forming extremely deep bound states were obtained by analysis of a hybrid method in the E07 experiment at J-PARC and reanalysis of the E373 experiment at KEK-PS. The decay mode of one event was assigned as 
+
+
+
. Since there are no excited states for daughter particles, the binding energy of the hyperon, 
, in nucleus was uniquely determined to be 6.27 
0.27 MeV. Another - system via the decay 
+ + brings a value, 8.00 0.77 MeV or 4.96 0.77 MeV, where the two possible values of correspond to the ground and the excited states of the daughter nucleus, respectively. Because the values are larger than those of the previously reported events (KISO and IBUKI), which are both interpreted as the nuclear 
state of the - system, these new events give the first indication of the nuclear 
state of the hypernucleus, .
吉田 純也; 赤石 貴也; 藤田 真奈美; 長谷川 勝一; 橋本 直; 細見 健二; 市川 真也; 市川 裕大; 今井 憲一*; Kim, S.; et al.
JPS Conference Proceedings (Internet), 33, p.011112_1 - 011112_8, 2021/03
J-PARC E07 is the most ambitious and complex emulsion experiment to date investigating double hypernuclei with Hybrid emulsion method. The physics run at the K1.8 beam line in the J-PARC hadron experimental facility have been completed in 2017. The emulsion sheets are presently being analyzed with dedicated optical microscopes. Current statistics are estimated to be more 3 times than that of previous experiments. Quantitative data on the 
and 
interaction are being accumulated successfully via analysis of double and hypernuclei. Multiple hypernucleus candidates suggests several features about hypernucleus that the identification efficiency of 
C is significantly higher than other mode, many daughters of C are identified as He or Be, and multiple bound states of exist in the 
N nucleus. An analysis of X-ray spectroscopy of hyperatoms are ongoing.
identification method by the 
reaction for a 
scattering experiment at J-PARC坂尾 珠和*; 藤田 真奈美; 長谷川 勝一; 細見 健二; 市川 真也; 市川 裕大; 今井 憲一*; 七村 拓野; 成木 恵; 佐甲 博之; et al.
JPS Conference Proceedings (Internet), 33, p.011133_1 - 011133_6, 2021/03
The reaction is an important elementary process to produce from a proton target and is a key for a scattering experiment where the momentum of should be tagged from the missing momentum of the 
reaction. However, the spectroscopy method has not been established yet due to the difficulty of the 
detection. Therefore, we have proposed a new detection method where 
and from the decay are measured by a forward magnetic spectrometer and a detector cluster surrounding the target, respectively. The feasibility of the detection method was confirmed by analyzing the J-PARC E40 data taken with such a detector system. In the analysis, 's were successfully identified in the missing mass spectrum of the 
reaction.
武田 哲明*; 稲垣 嘉之; 相原 純; 青木 健; 藤原 佑輔; 深谷 裕司; 後藤 実; Ho, H. Q.; 飯垣 和彦; 今井 良行; et al.
High Temperature Gas-Cooled Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.5, 464 Pages, 2021/02
本書は、原子力機構における今までの高温ガス炉の研究開発の総括として、HTTRの設計、燃料、炉内構造物や中間熱交換器などの要素技術の開発、出力上昇試験、950
Cの高温運転、安全性実証試験などの運転経験及び成果についてまとめたものである。また、HTTRでの知見をもとに、商用炉の設計、高性能燃料、ヘリウムガスタービン、ISプロセスによる水素製造などの要素技術開発の現状について記述しており、今後の高温ガス炉の開発に非常に有用である。本書は、日本機械学会の動力エネルギーシステム部門による化石燃料及び原子力によるエネルギーシステムの技術書のシリーズの一冊として刊行されるものである。
-N system早川 修平; 藤田 真奈美; 長谷川 勝一; 橋本 直; 細見 健二; 市川 裕大; 今井 憲一*; 七村 拓野; 成木 恵; 佐甲 博之; et al.
Physical Review Letters, 126(6), p.062501_1 - 062501_6, 2021/02
被引用回数：34 パーセンタイル：95.34(Physics, Multidisciplinary)In an emulsion-counter hybrid experiment performed at J-PARC, a absorption event was observed which decayed into twin single- hypernuclei. Kinematic calculations enabled a unique identification of the reaction process as 
N
Be + 
He. For the binding energy of the 
hyperon in the -N system a value of 
MeV was deduced. The energy level of is likely a nuclear state which indicates a weak 
-
coupling.
hypernuclear spectroscopy with the 
reaction後神 利志*; 藤田 真奈美; 長谷川 勝一; 細見 健二; 今井 憲一*; 市川 裕大; 七村 拓野; 成木 恵; 佐甲 博之; 佐藤 進; et al.
Journal of Physics; Conference Series, 1643, p.012133_1 - 012133_6, 2020/12
被引用回数：2 パーセンタイル：84.57(Astronomy & Astrophysics)We performed hypernuclear spectroscopy with the reaction at J-PARC to investigate the interaction (J-PARC E05). A new experiment (J-PARC E70) in which a better energy resolution could be achieved is now being prepared. In this article, an analysis status of J-PARC E05 and a preparation status of J-PARC E70 are described.
interaction from the scattering experiment at J-PARC三輪 浩司*; 藤田 真奈美; 長谷川 勝一; 細見 健二; 市川 真也; 市川 裕大; 今井 憲一*; 七村 拓野; 成木 恵; 佐甲 博之; et al.
Journal of Physics; Conference Series, 1643, p.012174_1 - 012174_6, 2020/12
被引用回数：2 パーセンタイル：84.57(Astronomy & Astrophysics)A high statistics scattering experiment has been performed at the K1.8 beamline in the J-PARC Hadron Experimental Facility. Data for momentum-tagged beam running in a liquid hydrogen target were accumulated by detecting the 
reaction with a high intensity beam of 20 M/spill. The number of the beam was about 
in total. The elastic scattering and the 
inelastic scattering events were successfully observed with about 100 times larger statistics than that in past experiments.
scattering experiment at J-PARC and the analysis status中田 祥之*; 長谷川 勝一; 早川 修平*; 細見 健二; 市川 裕大; 今井 憲一; 七村 拓野*; 成木 恵*; 佐甲 博之; 佐藤 進; et al.
JPS Conference Proceedings (Internet), 26, p.023024_1 - 023024_5, 2019/11
J-PARC E40 aims to measure the differential cross sections of the 
elastic scatterings and the 
conversion. A clear peak of was observed in a missing mass spectrum of the 
reaction and recoil protons from the 
elastic scattering were successfully observed in the data taken in the summer 2018. The rest of data taking is coming in the spring 2019.
-ray spectroscopy of an 
-shell hypernucleus, 
FYang, S. B.*; 長谷川 勝一; 早川 修平*; 細見 健二; 市川 裕大; 今井 憲一; 佐甲 博之; 佐藤 進; 田村 裕和*; 谷田 聖; et al.
JPS Conference Proceedings (Internet), 26, p.023015_1 - 023015_5, 2019/11
We performed a gamma-ray spectroscopy of 
at J-PARC Hadron Experimental Facility in 2015. It is the first measurement of rays emitted from -shell hypernuclei. In this experiment, we determined the energy spacing between the ground state spin doublet, 
and 
states, as 316 keV. The excitation energies of 
and states are also determined to be 895 and 1266 keV, respectively. The energy spacing is found to be well reproduced by shell-model calculations which describe - and 
-shell hypernuclei well. The results show that the present theories of the 
interaction describe not only the light hypernuclei but also a heavier hypernucleus.
in nuclei through C
spectrum at 1.8 GeV/ in the J-PARC E05 experiment本多 良太郎*; 長谷川 勝一; 早川 修平; 細見 健二; 今井 憲一; 市川 裕大; 七村 拓野; 成木 恵; 佐甲 博之; 佐藤 進; et al.
JPS Conference Proceedings (Internet), 26, p.023014_1 - 023014_4, 2019/11
We measured the 
reaction spectra at 1.8 GeV/ for the graphite and the polyethylene targets in the J-PARC E05 pilot experiment. By comparing the spectra for these two targets, it was found that 
in the 
B nucleus is quite broadened. Furthermore, we also compared broadness of with 
obtained in the 
spectrum. seems to be much more broadened in nuclei than . We gave a possible interpretation, which is related to compositeness of decuplet baryons, for this situation.
hypernucleus in the J-PARC E13 experiment中川 真菜美*; 長谷川 勝一; 早川 修平; 細見 健二; 市川 裕大; 今井 憲一; 佐甲 博之; 佐藤 進; 田村 裕和; 谷田 聖; et al.
JPS Conference Proceedings (Internet), 26, p.023005_1 - 023005_3, 2019/11
The interaction is not much studied than the interaction. To understand the interaction, we study 
hypernuclei. As for the hypernucleus, only the ground state of has been observed. To obtain more information about the interaction, the excited state should be studied. Therefore, we measure the missing-mass of the 
He
reaction at 
GeV/ and 
2-14 at the J-PARC K1.8 beam line. The ground state of is observed whereas a peak of the excited states is not observed. We also observe suppression of the quasi-free process at smaller angles.
-hypernuclei at J-PARC; Results and perspective小池 武志*; 長谷川 勝一; 早川 修平*; 細見 健二; 市川 裕大; 今井 憲一; 佐甲 博之; 佐藤 進; 杉村 仁志; 田村 裕和; et al.
AIP Conference Proceedings 2130, p.020011_1 - 020011_9, 2019/07
被引用回数：2 パーセンタイル：73.22(Physics, Nuclear)Experimental results from the J-PARC E13 experiments are summarized. A new experimental set up of E13 has established a platform for the future -ray hypernuclear spectroscopy at J-PARC using kaon beams. New rays are identified in 
He and F. The energy of 1.406 MeV for the He
transition confirmed a sizable effect of Charge Symmetry Breaking (CSB) in interaction in the 
hypernuclear system. The identification of four rays in F is made for the first time in shell hypernuclei. Especially, energy spacing of the ground state doublet is found to be 315.5 keV. A good agreement with two theoretical calculations suggests that the theoretical formalism used in shell hypernuclei is also applicable to heavier hypernuclei. Lastly, an overview of the future J-PARC E63 experiment is given.
bound state in the 
C reaction at 1.8 GeV/永江 知文*; 江川 弘行; 長谷川 勝一; 早川 修平; 細見 健二; 市川 裕大; 今井 憲一; 金原 慎二; 七村 拓野*; 成木 恵; et al.
AIP Conference Proceedings 2130, p.020015_1 - 020015_9, 2019/07
被引用回数：12 パーセンタイル：98.33(Physics, Nuclear)For the full understanding of baryon-baryon interactions in flavor 
, the interaction is the last missing piece of information. So far, we have revealed the interaction to be attractive (
MeV), and interaction to be repulsive in the medium to heavy mass-number region. The bonding energy is weakly attractive. While we have a few experimental observations suggesting the interaction would be attractive, there still exist large theoretical ambiguities weather it is attractive or not. Experimental determinations on the existence of bound states of hypernuclei by observing bound-state peaks are strongly awaited. In this report, a new preliminary result on the missing-mass spectrum of a C reaction, which strongly suggests the existence of -hypernuclear bound states, is presented.
江川 弘行; 足利 沙希子; 長谷川 勝一; 橋本 直; 早川 修平; 細見 健二; 市川 裕大; 今井 憲一; 金原 慎二*; 七村 拓野; et al.
Progress of Theoretical and Experimental Physics (Internet), 2019(2), p.021D02_1 - 021D02_11, 2019/02
被引用回数：25 パーセンタイル：83.76(Physics, Multidisciplinary)A double- hypernucleus, 
, was observed by the J-PARC E07 collaborationin nuclear emulsions tagged by the 
reaction. This event was interpreted as a production and decay of 
,
, or 
via capture in 
.By assuming the capture in the atomic 3D state, the binding energy of two hyperons
(
)of these double- hypernuclei are obtained to be
, 
, and 
, respectively. Based on the kinematic fitting, is the most likely explanation for the observed event.
今井 正樹; 緒方 裕大*; 中堂 博之; 小野 正雄; 針井 一哉; 松尾 衛*; 大沼 悠一*; 前川 禎通; 齊藤 英治
Applied Physics Letters, 113(5), p.052402_1 - 052402_3, 2018/07
被引用回数：18 パーセンタイル：65.6(Physics, Applied)We report direct observation of gyromagnetic reversal, which is the sign change of gyromagnetic ratio in a ferrimagnet Ho
Fe
O
, by using the Barnett effect measurement technique at low temperatures. The Barnett effect is a phenomenon in which magnetization is induced by mechanical rotation through the coupling between rotation and total angular momentum 
of electrons. The magnetization of HoFeO induced by mechanical rotation disappears at 135 K and 240 K. The temperatures correspond to the magnetization compensation temperature 
and the angular momentum compensation temperature 
, respectively. Between and , the magnetization flips over to be parallel against the angular momentum due to the sign change of gyromagnetic ratio. This study provides an unprecedented technique to explore the gyromagnetic properties.
