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論文

Distinct variation of electronic states due to annealing in $$T'$$-type La$$_{1.8}$$Eu$$_{0.2}$$CuO$$_{4}$$ and Nd$$_{2}$$CuO$$_{4}$$

浅野 駿*; 石井 賢司*; 松村 大樹; 辻 卓也; 工藤 康太*; 谷口 貴紀*; 齋藤 真*; 春原 稔樹*; 川股 隆行*; 小池 洋二*; et al.

Physical Review B, 104(21), p.214504_1 - 214504_7, 2021/12

 被引用回数:0 パーセンタイル:0(Materials Science, Multidisciplinary)

We performed Cu K-edge X-ray absorption fine-structure measurements on $$T'$$-type La$$_{1.8}$$Eu$$_{0.2}$$CuO$$_{4}$$ (LECO) and Nd$$_{2}$$CuO$$_{4}$$ (NCO) to investigate the variation in the electronic state associated with the emergence of superconductivity due to annealing. The X-ray absorption near-edge structure spectra of as-sintered (AS) LECO are quite similar to those of AS NCO, indicating that the ground state of AS LECO is a Mott insulator. The electron density after annealing $$n_{rm AN}$$ was evaluated for both superconducting LECO and nonsuperconducting NCO and was found to be 0.40 and 0.05 electron per Cu atom, respectively. In LECO but not in NCO, extended X-ray absorption fine-structure analysis revealed a reduction in the strength of the Cu-O bond in the CuO$$_{2}$$ plane due to annealing, which is consistent with the screening effect on phonons in the metallic state. The origin of the difference in doping processes due to annealing is discussed in relation to the size of the charge-transfer gap.

論文

One-dimensional spinon spin currents

廣部 大地*; 佐藤 正寛*; 川股 隆行*; 塩見 雄毅*; 内田 健一*; 井口 亮*; 小池 洋二*; 前川 禎通; 齊藤 英治

Nature Physics, 13(1), p.30 - 34, 2017/01

 被引用回数:91 パーセンタイル:96.69(Physics, Multidisciplinary)

Quantum spin fluctuation in a low-dimensional or frustrated magnet breaks magnetic ordering while keeping spin correlation. Such fluctuation has been a central topic in magnetism because of its relevance to high-Tc superconductivity and topological states. However, utilizing such spin states has been quite difficult. In a one-dimensional spin-1/2 chain, a particle-like excitation called a spinon is known to be responsible for spin fluctuation in a paramagnetic state. Spinons behave as a Tomonaga-Luttinger liquid at low energy, and the spin system is often called a quantum spin chain. Here we show that a quantum spin chain generates and carries spin current, which is attributed to spinon spin current. This is demonstrated by observing an anisotropic negative spin Seebeck effect along the spin chains in Sr$$_{2}$$CuO$$_{3}$$. The results show that spin current can flow even in an atomic channel owing to long-range spin fluctuation.

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