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渡邊 正理*; 栗田 伸之*; 田中 秀数*; 植野 航*; 松井 一樹*; 後藤 貴行*; 萩原 雅人
Physical Review B, 105(5), p.054414_1 - 054414_12, 2022/02
被引用回数:4 パーセンタイル:59.24(Materials Science, Multidisciplinary)We report the magnetic properties of the double perovskites SrLaCuSbO (SLCSO) and SrLaCuNbO (SLCNO). The temperature dependence of the magnetic susceptibilities of both com-pounds shows a broad maximum characteristic of an = 1/2 square lattice Heisenberg antiferromagnet. Magnetic ordering occurs at = 13.6 and 15.7 K for SLCSO and SLCNO, respectively. Neutron powder diffraction measurements reveal contrasting spin structures in both compounds. The spin structures of SLCSO and SLCNO below are Nel antiferromagnetic and collinear antiferromagnetic, respectively. This result demonstrates that the nearest-neighbor interaction is dominant in SLCSO, whereas the next-nearest-neighbor interaction is dominant in SLCNO. The magnitude of the ordered moment was evaluated at 3.5 K to be = 0.39(3) for SLCSO and 0.29(2) for SLCNO, which are significantly smaller than those calculated using linear spin wave theory. We infer that the small ordered moment is caused by the effect of exchange bond randomness arising from the site disorder of Sr and La ions.
酒井 宏典; 比嘉 野乃花; 服部 泰佑; 徳永 陽; 芳賀 芳範; 神戸 振作; 後藤 貴行*; 平田 倫啓*; 淡路 智*; 佐々木 孝彦*
no journal, ,
強相関電子系のウラン化合物URuSiの単結晶を用いて、軸方向に外部磁場を約24Tをかけて、Si核磁気共鳴(NMR)観測を行った。常磁性状態におけるNMRシフトの温度依存性は、外部磁場依存することがわかった。この磁場依存性は、パルス磁場で測定された帯磁率の磁場依存性に似ている。