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mixed oxidesVauchy, R.; 松本 卓; 廣岡 瞬; 宇野 弘樹*; 田村 哲也*; 有馬 立身*; 稲垣 八穂広*; 出光 一哉*; 中村 博樹; 町田 昌彦; et al.
Journal of Nuclear Materials, 588, p.154786_1 - 154786_13, 2024/01
被引用回数：1 パーセンタイル：72.91(Materials Science, Multidisciplinary)Diffusion couples made of dense polycrystalline (U,Pu,Am)O oxides were annealed in various thermodynamic conditions (temperature, oxygen partial pressure), and for different durations. The associated actinide redistribution was quantified using Electron Probe Micro-Analysis (EPMA). Average diffusion profiles were obtained from elemental U, Pu, and Am X-ray maps and the resulting interdiffusion coefficients were calculated, then analyzed at the light of our model of point defect chemistry.
阿部 雄太; 土川 雄介; 甲斐 哲也; 松本 吉弘*; Parker, J. D.*; 篠原 武尚; 大石 佑治*; 加美山 隆*; 永江 勇二; 佐藤 一憲
JPS Conference Proceedings (Internet), 33, p.011075_1 - 011075_6, 2021/03
Since the hardness of fuel debris containing boride from B
C pellet in control rod is estimated to be two times higher as that of oxide, such as UO
and ZrO, distribution of such boride in the fuel debris formed in the Fukushima-Daiichi Nuclear Power Plants may affect the process of debris cutting and removal. The high neutron absorption of boron may affect the possibility of re-criticality during the process of debris removal. Therefore, boride distribution in fuel debris is regarded as an important issue to be addressed. However, boron tends to have difficult in quantification with conventionally applied methods like EPMA and XPS. In this study, accelerator-driven neutron-imaging system was applied. Since boron is the material for neutron absorption, its sensitivity in terms of neutron penetration through specimens is concerned. To adjust neutron attenuation of a specimen to suit a particular measurement by selecting the neutron energy range, we focused on the energy resolved neutron imaging system RADEN, which utilizes wide energy range from meV to keV. Development of a method to visualize boron distribution using energy-resolved neutrons has been started. In this presentation the authors show the status of the development of a method utilizing energy-resolved neutrons and provide some outcome from its application to the Core Material Melting and Relocation (CMMR)-0 and -2 specimens.
土川 雄介; 阿部 雄太; 大石 佑治*; 甲斐 哲也; 藤 暢輔; 瀬川 麻里子; 前田 亮; 木村 敦; 中村 詔司; 原田 正英; et al.
JPS Conference Proceedings (Internet), 33, p.011074_1 - 011074_6, 2021/03
福島原子力発電所の解体作業では、溶融した燃料棒に含まれるホウ素分布を事前に把握することが重要である。溶融燃料棒の模擬試験体を用意し、ホウ素やホウ化物の含有量を調査する研究が行われてきた。本研究では、その一環として中性子を用いたホウ素並びにホウ化物分布の測定技術開発を行った。ホウ素の中性子吸収に伴う即発ガンマ線を測定し、ホウ素量や二次元分布を測定した。また、n(B,
)反応における478keV線は、ホウ素の化合状態により、線ピークの幅が変化することが知られている。このことを用い、特に溶融燃料棒周辺に存在することが予測されているZrBやFeBといったホウ化物の識別可能性について調査した。測定はJ-PARC/MLFのANNRI, NOBORU, RADENにて行った。これらの解析結果について報告する。
阿部 雄太; 土川 雄介; 甲斐 哲也; 松本 吉弘*; Parker, J. D.*; 篠原 武尚; 大石 佑治*; 加美山 隆*; 永江 勇二; 佐藤 一憲
Proceedings of 2020 International Conference on Nuclear Engineering (ICONE 2020) (Internet), 6 Pages, 2020/08
Boron carbide is used as a neutron-absorbing material in Fukushima-Daiichi Nuclear Power Station (1F), producing borides that are twice as hard as oxides (such as UO and ZrO). The high neutron absorption of boron affects the evaluation of re-criticality during the process of debris retrieval. Therefore, it is important not only to determine the presence of boron but also to investigate the distribution of boron inside the material in a non-destructive manner during decommissioning. To address the uncertainties in the core material relocation behavior of boiling water reactor (BWR) during a severe accident (SA), solidified melt specimens of a simulated fuel assembly were prepared by plasma heating. If core material melting and relocation (CMMR) specimens can be used to estimate the B distribution in 1F Unit-3, that will provide valuable information in the decommissioning of 1F. To address this, the authors focused on the energy-resolved neutron imaging system, RADEN, which utilizes a wide energy range, from meV to keV. This is an innovative three-dimensional analysis technology for boride distribution that affects the evaluation of hardness and re-criticality. In the calibration standard samples (Zr
B
and FeB), there was a good correlation between boron concentration and the energy-dependence of the cross sections of cold and epi-thermal neutrons. In the CMMR specimens, boron distribution was confirmed from the contrast difference between cold and epi-thermal neutrons. In the future, the results of calibration standard samples will be applied to the results of CMMR specimens. With this method, three-dimensional boron distribution will be measured, and the understanding of boride distribution 1F Unit-3 will be improved, which may be reflected in an improved SA code.
Parker, J. D.*; 原田 正英; 林田 洋寿*; 廣井 孝介; 甲斐 哲也; 松本 吉弘*; 中谷 健; 及川 健一; 瀬川 麻里子; 篠原 武尚; et al.
Materials Research Proceedings, Vol.15, p.102 - 107, 2020/05
At the RADEN instrument, we take advantage of the accurate measurement of neutron energy by time-of-flight to perform energy-resolved neutron imaging using event-type neutron imaging detectors. We are continually working to improve these detectors for better spatial resolution and shorter measurement times and, as a user facility, to improve the ease-of-use of their control and analysis software. In particular, we are actively developing a 
He-based gaseous micropattern detector known as the Micro-pixel chamber based Neutron Imaging Detector (
NID). We have recently redesigned the NID control software to allow full integration into the automated experiment control system at RADEN, and we are carrying out optimization of the analysis algorithms for improved image quality and rate performance.
篠原 武尚; 甲斐 哲也; 及川 健一; 中谷 健; 瀬川 麻里子; 廣井 孝介; Su, Y. H.; 大井 元貴; 原田 正英; 飯倉 寛; et al.
Review of Scientific Instruments, 91(4), p.043302_1 - 043302_20, 2020/04
被引用回数：51 パーセンタイル：96.48(Instruments & Instrumentation)The energy-resolved neutron imaging system, RADEN, has been installed at the pulsed neutron source in the Materials and Life Science Experimental Facility of the Japan Proton Accelerator Research Complex. In addition to conventional neutron radiography and tomography, RADEN, the world's first imaging beam-line at a pulsed neutron source, provides three main options for new, quantitative neutron imaging techniques: Bragg-edge imaging to visualize the spatial distribution of crystallographic information, resonance absorption imaging for elemental composition and temperature information, and polarized neutron imaging for magnetic field information. This paper describes the results of characterization studies of the neutronic performance and installed devices at RADEN and shows the results of several demonstration studies for pulsed neutron imaging.
甲斐 哲也; 篠原 武尚; 松本 吉弘*
検査技術, 25(2), p.1 - 5, 2020/02
J-PARC物質・生命科学実験施設に設置されたエネルギー分析型中性子イメージング装置RADENは、エネルギー分析を行わない中性子ラジオグラフィ/トモグラフィの利用でも相応の役割を果たしている。本稿では、検査技術の一つとしての検討材料を提供するため、これまでにRADENで中性子ラジオグラフィ/トモグラフィの利用で得られた成果について紹介する。
及川 健一; 鬼柳 善明*; 佐藤 博隆*; 大前 良磨*; Pham, A.*; 渡辺 賢一*; 松本 吉弘*; 篠原 武尚; 甲斐 哲也; Harjo, S.; et al.
Materials Research Proceedings, Vol.15, p.207 - 213, 2020/02
Japanese swords are very attractive not only as a work of art but also a metallurgical point of view. Since Japanese vintage swords became valuable, it is indispensable to establish non-destructive analysis method to identify some peculiar characteristics. Bragg edge imaging gives real-space distributions of bulk information in a crystalline material as well as neutron tomography. In this work, we investigated crystallographic information of a Japanese sword made by Sukemasa in Izumi province in the first quarter of the 16th century. The experiments have been performed at RADEN at J-PARC. The Sukemasa sword was measured with a counting-type 2D detector and with a CCD camera. We are now analyzing the measured 2D-transmission spectra using RITS code to obtain spatial distribution of the crystallite size, the texture variation, the d110 shift and its broadening. Complementary data analysis using white beam tomography is also on going. Detailed analysis results will be presented.
甲斐 哲也; 廣井 孝介; Su, Y. H.; 瀬川 麻里子; 篠原 武尚; 松本 吉弘*; Parker, J. D.*; 林田 洋寿*; 及川 健一
Materials Research Proceedings, Vol.15, p.149 - 153, 2020/02
A two-dimensional thermometry technique based on neutron resonance reactions derives the temperature of specified elements in an object by analyzing the Doppler broadening of a neutron resonance measured by a time-analyzing neutron imaging-detector. This technique is expected to be one of the important applications of the energy-resolved neutron imaging system, RADEN, at J-PARC. The authors focused on molybdenum contained in 316 stainless-steel (with a weight fraction of 2-3 wt%). Energy-dependent transmitted neutrons were measured through a 3 mm thick 316 stainless-steel plate placed in a heater at temperatures between 23 and 500 degrees Celsius at RADEN using a gas-electron multiplier (GEM) detector. Thermal and cold neutrons were eliminated from the incident beam by a cadmium filter. The sample area within the neutron beam was 30 by 50 mm
. The feasibility is discussed in the presentation.
庄司 衛太*; 磯谷 祥世*; 鈴木 陸人*; 久保 正樹*; 塚田 隆夫*; 甲斐 哲也; 篠原 武尚; 松本 吉弘*; 福山 博之*
Scripta Materialia, 175, p.29 - 32, 2020/01
被引用回数：19 パーセンタイル：78.21(Nanoscience & Nanotechnology)The effect of melt convection on the phase separation structures in undercooled Cu- Co alloys was investigated using the electromagnetic levitation technique, where the melt convection was controlled by applying a static magnetic field. The three-dimensional phase separation structures of the solidified Cu-Co alloys were first observed using neutron computed tomography. A large number of small spherical Co-rich phases were dispersed in the Cu-rich phase matrix when the static magnetic field was relatively small. In contrast, several coalesced Co-rich phases, which were elongated along the direction of the static magnetic field, appeared in the higher strength of static magnetic field.
清水 一行*; 林田 洋寿*; 戸田 裕之*; 甲斐 哲也; 松本 吉弘*; 松本 佳久*
日本金属学会誌, 83(11), p.434 - 440, 2019/11
被引用回数：1 パーセンタイル：6.23(Metallurgy & Metallurgical Engineering)Neutron imaging experiment was performed to visualize the distribution of solute hydrogen in an Al-10.1%Zn-1.2%Mg alloy and a pure palladium after hydrogen charging. Changes in the contrast of neutron transmission images caused by hydrogen were clearly observed in a palladium. In the wavelength range of 2-3 AA and 5-13.5 AA, the mean neutron transmission around the center of a hydrogen-charged palladium were 0.692 and 0.511, respectively. The hydrogen content in a palladium was estimated to be 10.8 mol% from the measured neutron transmission. This study has demonstrated that hydrogen content can be analyzed by considering the wavelength dependence of neutron intensity. On the other hand, hydrogen could not be observed from the neutron transmission image in Al-Zn-Mg alloys. This was due to the low hydrogen content, which was mass ppm level even after hydrogen charging, and statistical precision was not sufficient to discuss the amount of hydrogen of the mass ppm order.
及川 健一; Su, Y. H.; 鬼柳 亮嗣; 川崎 卓郎; 篠原 武尚; 甲斐 哲也; 廣井 孝介; Harjo, S.; Parker, J. D.*; 松本 吉弘*; et al.
Physica B; Condensed Matter, 551, p.436 - 442, 2018/12
被引用回数：8 パーセンタイル：30.3(Physics, Condensed Matter)We are promoting for practical product observation by the energy-resolved neutron imaging method using high-intensity pulsed neutrons at J-PARC, under the Photon and Quantum Basic Research Coordinated Development Program from the Ministry of Education, Culture, Sports, Science and Technology, Japan. Bragg edge imaging, one of the energy-resolved neutron imaging methods for visualizing material properties, was applied to feasibility study of the temperature distribution of copper rod, complementary study of the texture and strain distribution of bent steel plates using neutron diffraction and EBSD, and so on. Outline of results obtained by these imaging experiments will be presented.
甲斐 哲也; 佐藤 節夫*; 廣井 孝介; Su, Y. H.; 瀬川 麻里子; Parker, J. D.*; 松本 吉弘*; 林田 洋寿*; 篠原 武尚; 及川 健一; et al.
Physica B; Condensed Matter, 551, p.496 - 500, 2018/12
被引用回数：2 パーセンタイル：10.36(Physics, Condensed Matter)The 2012 model lithium-6 time-analyzer neutron detector (LiTA12) system, based on a lithium glass scintillator and multi-anode photomultiplier tube, has the highest neutron efficiency among the detectors for pulsed neutron imaging together with a flexibility of the efficiency by changing the thickness of the lithium glass. The authors expect this detector system could become a main detector system for the energy-resolved neutron imaging system, RADEN, at J-PARC, and have started evaluation of the LiTA12 system. For example, spatial resolution for resonance absorption imaging was evaluated by using a line-pair pattern made by 3 micro meter thick gold on a quartz plate. Less than 1 mm width line pairs were resolved at an 8 Mcps neutron counting rate and around 5 eV neutron energy.
瀬川 麻里子; 及川 健一; 甲斐 哲也; 篠原 武尚; 林田 洋寿*; 松本 吉弘*; Parker, J. D.*; 中谷 健; 廣井 孝介; Su, Y. H.; et al.
JPS Conference Proceedings (Internet), 22, p.011028_1 - 011028_8, 2018/11
We have fabricated and utilized spatial resolution test targets made of gadolinium and gold for conventional and resonance neutron imaging performed at RADEN, located at beam line BL22 of the J-PARC Materials and Life Science Experimental Facility (MLF). RADEN covers a broad energy range from cold neutrons to high-energy neutrons with energy of several tens keV and was designed to perform energy-resolved neutron imaging utilizing two-dimensional detectors combined with the accurate measurement of neutron energy by the time-of-flight method. The test targets were designed to verify the spatial resolution and image uniformity of two kinds of neutron detectors, counting-type detectors and camera-type detectors. In this presentation, we report the details of these two-dimensional test targets, and the results of demonstrations using the test targets with our neutron imaging detectors. This work was supported in part by the Photon and Quantum Basic Research Coordinated Development Program from the Ministry of Education, Culture, Sports, Science and Technology, Japan.
小山 拓*; 上野 一貴*; 関根 麻里子*; 松本 吉弘*; 甲斐 哲也; 篠原 武尚; 飯倉 寛; 鈴木 裕士; 兼松 学*
Materials Research Proceedings, Vol.4, p.155 - 160, 2018/05
被引用回数：0 パーセンタイル：0.18(Materials Science, Characterization & Testing)We developed, in this study, a novel method to observe internal deformation of concrete by the neutron transmission imaging technique. In order to visualize the internal deformation of concrete, the cement paste markers containing GdO
powder were two-dimensionally dispersed around the ferritic deformed rebar in the reinforced concrete. This experiment was conducted using BL22, RADEN, in the Material and Life Science Experimental Facility of the Japan Proton Accelerator Research Complex. The transmission images of the reinforced concrete sample were taken at several positions on the vertical sample stage, and the displacement of the marker from the initial position was successfully evaluated within approximately 
0.1 mm accuracy by image analysis for selected markers with higher contrast and circularity. Furthermore, concrete deformation under pull-out loading to the embedded rebar was evaluated by the same way, and its reaction compressive deformation was successfully observed by analyzing the displacement of the markers. The results obtained in this study bring beneficial knowledge that the measurement accuracy of the marker displacement can be improved more by choosing a spherical shape of the marker and by increasing the contrast of the marker.
甲斐 哲也; 廣井 孝介; Su, Y. H.; 篠原 武尚; Parker, J. D.*; 松本 吉弘*; 林田 洋寿*; 瀬川 麻里子; 中谷 健; 及川 健一; et al.
Physics Procedia, 88, p.306 - 313, 2017/06
被引用回数：4 パーセンタイル：85.09(Instruments & Instrumentation)Neutron resonance thermometry, which measures material temperature by analyzing the Doppler broadening of a neutron resonance peak, is one of the applications of energy-resolved neutron imaging at RADEN of J-PARC. Although this technique is promising, advantages and disadvantages have not been discussed in practical applications. The authors measured neutron transmission rates of tantalum and tungsten foils in a heater chamber up to 300 degrees Celsius at RADEN. The energy-dependent neutron transmission rates with different statistics were obtained after the measurements by selecting arbitrary measuring intervals from one measurement, and the temperatures of the foils were estimated from those transmission rates with different statistics. The reliability of the neutron resonance thermometry with statistical accuracy, irradiation time and spatial resolution are discussed.
-orbital symmetry of the ground state in Yb compounds by linear dichroism in core-level photoemission森 健雄*; 北山 賢*; 金井 惟奈*; 内免 翔*; 藤原 秀紀*; 東谷 篤志*; 玉作 賢治*; 田中 新*; 寺嶋 健成*; 今田 真*; et al.
Journal of the Physical Society of Japan, 83(12), p.123702_1 - 123702_5, 2014/12
被引用回数：16 パーセンタイル：68.53(Physics, Multidisciplinary)正方晶YbRhSi及びYbCuSiに対して、角度分解内殻光電子分光における直線偏光線二色性を発見し、それにより、基底状態の強相関4軌道の対称性を明らかにした。理論計算から、この線二色性は結晶場効果に由来する異方的な電荷分布を反映することが示された。結晶場の第一励起エネルギーよりもはるかに低温での測定により、両物質の基底状態の4波動関数の決定に成功した。更に、温度依存性測定により、励起状態の対称性についても調べた。
伊藤 賢志*; 岡 壽崇*; 小林 慶規*; 白井 泰治*; 和田 健一郎*; 松本 昌高*; 藤浪 真紀*; 平出 哲也; 誉田 義英*; 細見 博之*; et al.
Materials Science Forum, 607, p.248 - 250, 2009/00
現在までに陽電子消滅寿命測定(PAL)の標準化が行われたことはない。標準がないと各々の研究室データの比較における信頼性の欠如に繋がる。そこで標準化への第一歩として、金属,高分子,シリカガラスの3種類の試料において合意した測定、及び解析手法で測定を行い、研究室間において比較を行った。金属試料では1寿命成分、それ以外では3寿命成分で解析を行った。陽電子寿命、及びオルソーポジトロニウム寿命に関して、研究室間における測定結果の違いが起こる原因について考察した。その結果、研究室ごとに使用している検出器の形状,配置などが異なり、コンプトン散乱された低エネルギーの線がもう一方の検出器に入ることで寿命スペクトル上にゆがみができるためと考えられた。検出器間に薄い金属板を挿入することで、各研究室間の違いが低減されることを確認した。
伊藤 賢志*; 岡 壽崇*; 小林 慶規*; 白井 泰治*; 和田 健一郎*; 松本 昌高*; 藤浪 真紀*; 平出 哲也; 誉田 義英*; 細見 博之*; et al.
Journal of Applied Physics, 104(2), p.026102_1 - 026102_3, 2008/07
被引用回数：48 パーセンタイル：83.5(Physics, Applied)同一の溶融石英とポリカーボネートを試料に用い、陽電子消滅寿命測定及び解析を12の研究室において実施し、その比較を行った。各研究室で得られた陽電子寿命のばらつきは、測定方法と解析方法を統一することで、過去に報告されている、何も制約を与えずに行われた試験結果に比較して、小さくできることがわかった。
米田 安宏; 松本 徳真; 古川 行人*; 石川 哲也*
Physica Scripta, T115, p.995 - 997, 2005/00
サジタルフォーカスは放射光X線の集光技術の中でも最も効率的な方法の一つで、サンプル位置におけるX線強度を増大させるために用いられる。この結晶ベンダーとして、シリコン(311)結晶を用いた場合についての結果を報告する。ベンダーはSPring-8標準2結晶分光器の第2結晶としてインストールされるもので、4ポイントメカニズムにより、定位置出射を実現している。このベンダーにリブなし結晶を用いたところ、35-60keVのエネルギー領域において0.5mmの集光サイズを達成した。このようなエネルギー領域においては、全反射ミラーなどはまだ使うことができないため、多くの実験に結晶ベンダーが用いられることになる。
