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論文

Deposition and dispersion of radio-cesium released due to the Fukushima Nuclear accident, 2; Sensitivity to aerosol microphysical properties of Cs-bearing microparticles (CsMPs)

梶野 瑞王*; 足立 光司*; 五十嵐 康人*; 佐藤 志彦; 澤田 壮弘*; 関山 剛*; 財前 祐二*; 佐谷 茜*; 鶴田 治雄*; 森口 祐一*

Journal of Geophysical Research; Atmospheres, 126(1), p.e2020JD033460_1 - e2020JD033460_23, 2021/01

 被引用回数:12 パーセンタイル:72.21(Meteorology & Atmospheric Sciences)

The dispersion and deposition of radio-cesium ($$^{137}$$Cs) carried by the two types (type A and type B) of water-insoluble Cs-bearing solid microparticles (CsMPs) released due to the Fukushima nuclear accident were simulated for the first time. The presence of type B CsMPs (70-400 $$mu$$m found in soil and 1-5 $$mu$$m found in air), associated with the hydrogen explosion of Unit 1 in the afternoon of March 12, could partly explain the simulated underestimation of total deposition over land by assuming that 100% of the Cs carriers were water-soluble submicron particles (WSPs). Type A CsMPs (0.1-10 $$mu$$m), released from Units 2 or 3 in the midnight between March 14 and 15, travelled over the Kanto Plain, the most populated plain in Japan. Differences in the size distribution of type A CsMPs altered the surface air concentration over Kanto substantially, by up to more than one order of magnitude. The major deposition mechanisms varied among dry, wet, and fog depositions depending on the size distribution. The simulated activity fractions due to the CsMPs in the total deposition were compared to those observed in surface soil for the first time. The observations could be explained by the simulations for the locations under the influence of type B CsMPs. However, the simulations were substantially underestimated for the locations influenced by type A CsMPs. There could be more fractions of type A CsMPs emission in the source term and/or the simulated deposition rates of type A CsMPs were underestimated.

口頭

Deposition and dispersion of radio-cesium; Sensitivity to meteorological models and aerosol properties

梶野 瑞王*; 関山 剛*; 五十嵐 康人*; 足立 光司*; 財前 祐二*; 澤田 壮弘*; 佐藤 志彦; 森口 祐一*

no journal, , 

A great number of atmospheric simulations have been conducted to understand the consequences of FDNPP accident. We came to know wet deposition is important but don't know to what extent. We know simulations vary but we don't know why. Meteorological model comparison with a single dispersion model was conducted to evaluate the magnitude of uncertainty in meteorological simulations. Among the deposition processes, rainout by liquid precipitation was the most important process. The fog deposition was the next, which was not considered in any other models but Katata et al., ACP (2015) and this study. Fog deposition is the main cause for the deposition in Gunma and Tochigi prefecture. All the simulation underestimated the airborne observation of Cs deposition, which amounted to 2.6 PBq. The underestimation is approximately 1.5 PBq (1 PBq in Hamadori and 0.4 PBq in Nakadori). It is due to underestimation of deposition process, which is the main finding of the meteorological model ensemble study: Some model overestimated while others underestimated both the precipitation and surface concentration, and therefore the precipitation and source term estimation should be reasonable and not be the cause of underestimation. By considering the A-type (Adachi et al., Sci. Rep., 2014) and S-type (Satou et al., Anthropocene, 2016) of Cs-ball particles, associated with the SRV opening of Unit 2 and Hydrogen explosion of Unit 1, respectively, the underestimation of simulated Cs deposition could be significantly improved. The maximum estimation of the additional deposition due to Cs-ball amounted approximately 1 PBq.

口頭

福島森林域における暖候期の放射性セシウム大気再浮遊は真菌胞子で説明できるか

北 和之*; 林 奈穂; 五十嵐 康人*; 濱 賢三*; 財前 祐二*; 関山 剛*; 足立 光司*; 吉田 尚弘*; 豊田 栄*; 保坂 健太郎*; et al.

no journal, , 

大気バイオエアロゾルは、東京電力福島第一原子力発電所事故で環境中に放出され土壌・植生に沈着した放射性セシウムが、大気中に再浮遊(再飛散,再放出)される現象に重要な役割を果たしていることが近年の研究で明らかになっている。しかし、どのようなバイオエアロゾルが再浮遊にどれだけ寄与しているかはまだ明らかになっていない。今回、セシウムを吸収・濃縮することが知られている真菌胞子に着目し、主な再浮遊担体となっているかを検討した。福島県浪江町で行ったエアロゾル粒径別サンプリングの結果、粒径2.1$$sim$$10.2$$mu$$mの範囲に大気放射性セシウムの約70%と大部分が存在していることが分かった。この粒径範囲は真菌胞子と一致する。大気セシウム放射能濃度とバイオエアロゾルの粒径別濃度は正相関を示し、特に粒径3$$sim$$15$$mu$$mの範囲で高い相関を示した。更に放射性セシウム沈着が多い林地において数種類のキノコ胞子のセシウム放射能を測定した。キノコ胞子の1個あたり放射能の中央値は、1.7$$times$$10$$^{-9}$$Bqであり、それを大気中の粒径3$$sim$$15$$mu$$mのバイオエアロゾル数濃度にかけ算して求めた大気セシウム放射能濃度は、実際の測定値を大きく上回る。他の地域から運ばれた胞子もあることを考えると、この胞子によって大気中の放射性セシウム濃度が充分説明できることが分かる。

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