Production cross-sections of residual nuclides from Zr + at 27 MeV/nucleon

Hwang, J.*; Chillery, T.*; Dozono, Masanori*; Imai, Nobuaki*; Michimasa, Shinichiro*; Sumikama, Toshiyuki*; Chiga, Nobuyuki*; Ota, Shinsuke*; Nakayama, Shinsuke; 49 of others*

Progress of Theoretical and Experimental Physics (Internet), 2024(9), p.093D03_1 - 093D03_12, 2024/09

https://doi.org/10.1093/ptep/ptae139

Nuclear transmutation emerges as a promising approach for reprocessing high-level waste, specifically treating long-lived nuclides like Zr from spent fuel. It is essential to accumulate reaction data for these nuclei to advance this prominent treatment and to build a comprehensive understanding of reaction mechanisms. In this study, the residual production cross-sections resulting from proton-induced reactions on Zr were measured at 27 MeV/nucleon in inverse kinematics. At the RIKEN-RIBF facility the OEDO beamline was used to deduce production cross-sections for isotopes, Nb, Zr, and Y. Comparing the results from this study and prior research with calculated excitation functions, a moderate agreement is found with theoretical predictions derived from TALYS and CCONE. Despite the potential limitations of low-energy proton-induced reactions for Zr transmutation, the measured cross-sections offer valuable insights for future considerations in nuclear-waste treatment facilities. This is particularly relevant for facilities exploring innovative methods, such as accelerator-driven systems.

Studying the impact of deuteron non-elastic breakup on Zr + d reaction cross sections measured at 28 MeV/nucleon

Chillery, T.*; Hwang, J.*; Dozono, Masanori*; Imai, Nobuaki*; Michimasa, Shinichiro*; Sumikama, Toshiyuki*; Chiga, Nobuyuki*; Ota, Shinsuke*; Nakayama, Shinsuke; 49 of others*

Progress of Theoretical and Experimental Physics (Internet), 2023(12), p.121D01_1 - 121D01_11, 2023/12

https://doi.org/10.1093/ptep/ptad139

The deuteron is a loosely bound system which can easily break up into its constituent proton and neutron whilst in the presence of Coulomb and nuclear fields. Previous experimental studies have shown that this breakup process has a significant impact on residual nucleus production from deuteron bombardment in the high energy range of 50 - 210 MeV/nucleon. However, there remains a lack of cross-section data at energies below 50 MeV/nucleon. The current study determined Zr + d reaction cross sections under inverse kinematics at approximately 28 MeV/nucleon using the BigRIPS separator, OEDO beamline, and SHARAQ spectrometer. Cross sections from this research were compared with previous measurements and theoretical calculations. The experimental results show a large enhancement of the production cross sections of residual nuclei, especially those produced from a small number of particle emissions, compared to the proton-induced reaction data at similar bombarding energy. The DEURACS calculation, which quantitatively takes deuteron-breakup effects into account, reproduces the data well. As a long-lived fission product, Zr remains a challenge for nuclear waste disposal and treatment. This study's low-energy data may assist future consideration of nuclear-waste treatment facilities, where Zr + d may feasibly transmute the waste into short-lived/stable nuclei.

Accelerator design for 1.3-MW beam power operation of the J-PARC Main Ring

Igarashi, Susumu*; Nomura, Masahiro; Tamura, Fumihiko; Yamamoto, Masanobu; Shimada, Taihei; 49 of others*

Progress of Theoretical and Experimental Physics (Internet), 2021(3), p.033G01_1 - 033G01_28, 2021/03

https://doi.org/10.1093/ptep/ptab011

Beamline test of a transition-edge-sensor spectrometer in preparation for kaonic-atom measurements

Hashimoto, Tadashi*; Tanida, Kiyoshi; 49 of others*

IEEE Transactions on Applied Superconductivity, 27(4), p.2100905_1 - 2100905_5, 2017/06

https://doi.org/10.1109/TASC.2016.2646374

TES application to kaonic atom X-ray spectroscopy in a charged-particle beamline

Hashimoto, Tadashi*; Tanida, Kiyoshi; 49 of others*

no journal, ,