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Cl
Aoki, So; Abe, Yosuke; Abe, Hiroshi*; Watanabe, Yutaka*; Yamamoto, Masahiro*
Corrosion Science, 255, p.113119_1 - 113119_10, 2025/10
This study aimed to visualise the distribution of chloride in the corroded crevice of stainless steel and to evaluate the chloride content quantitatively. Crevice corrosion tests were carried out using Cl, a radioactive isotope of chloride, as a tracer in NaCl test solutions. After crevice corrosion tests, stainless steel specimens were placed on an imaging plate. The imaging plate was sensitised by 
-ray emitted by Cl adhering to the crevice. As a result, the chloride distribution in the corroded area inside the crevice was visualised. A calibration curve for the amount of Cl was obtained from the relationship between the time of photosensitivity to -ray emitted by Cl and the luminance of the imaging plate. The chloride content in the corroded crevice was quantitatively evaluated based on the calibration curve. These visualisation and quantitative evaluation methods were also applied to tests in which specimens were left in pure water after crevice corrosion tests, and the behaviour of chloride in crevice corrosion was discussed.
Watanabe, Taku*; Maejima, Yui*; Ueda, Yuki; Motokawa, Ryuhei; Takabatake, Ai*; Takeda, Shinichi*; Fudoji, Hiroshi*; Kishikawa, Keiki*; Koori, Michinari*
Langmuir, 41(34), p.22762 - 22773, 2025/09
The assembled structures of melanin particles, i.e., colloidal particles coated with a melanin-like polydopamine (PDA) layer, create vivid structural colors. While the thickness of the PDA layer influences the particle arrangement and optical properties, the underlying mechanism has remained controversial. We demonstrate that the waterswelling characteristics of PDA are crucial factors governing the dispersion and aggregation of these particles in solution. Detailed comparisons between dry and wet conditions revealed that the PDA layer readily absorbs water molecules, which leads to significant swelling in the thicker layers. The swelling of the PDA layers determined whether the particles remained dispersed or partially aggregated in the water, ultimately controlling the particle arrangement in the dry state once the water evaporated. These findings provide insights into the self-assembly of colloidal particles and offer a strategy for tuning the periodic particle order. This feature is pivotal for various applications in optical and sensing technologies.
Ogawa, Tatsuhiko; Hirata, Yuho; Matsuya, Yusuke; Kai, Takeshi; Sato, Tatsuhiko; Iwamoto, Yosuke; Hashimoto, Shintaro; Furuta, Takuya; Abe, Shinichiro; Matsuda, Norihiro; et al.
EPJ Nuclear Sciences & Technologies (Internet), 10, p.13_1 - 13_8, 2024/11
The latest updates on PHITS, a versatile radiation transport code, focusing specifically on track-structure models are presented. Track structure calculations are methods used to simulate the movement of charged particles while explicitly considering each atomic reaction. Initially developed for radiation biology, these calculation methods aimed to analyze the radiation-induced damage to DNA and chromosomes. Several track-structure calculation models, including PHITS-ETS, PHITS-ETS for Si, PHITS-KURBUC, ETSART, and ITSART, have been developed and implemented to PHITS. These models allow users to study the behavior of various particles at the nano-scale across a wide range of materials. Furthermore, potential applications of track-structure calculations have also been proposed so far. This collection of track-structure calculation models, which encompasses diverse conditions, opens up new avenues for research in the field of radiation effects.
Ishii, Junya*; Shimizu, Morihito*; Kato, Masahiro*; Kurosawa, Tadahiro*; Tsuji, Tomoya; Yoshitomi, Hiroshi; Tanimura, Yoshihiko; Watabe, Hiroshi*
Journal of Radiological Protection, 44(3), p.031516_1 - 031516_8, 2024/09
Times Cited Count：0 Percentile：0.00(Environmental Sciences)Kawai, Kiyoshi*; Sogabe, Tomochika*; Nakagawa, Hiroshi; Yamada, Takeshi*; Koseki, Shigenobu*
Journal of Food Engineering, 375, p.112066_1 - 112066_9, 2024/08
Times Cited Count：1 Percentile：23.31(Engineering, Chemical)The purpose of this study was to clarify effect of glycerol and glucose on the mechanical glass transition and dynamical transition of freeze-dried bacteria at various water activity (aw)-conditions. From the water sorption isotherm, it was noted that the water content at each aw and monolayer water content were higher in the order of glycerol, glucose, non-added samples. Effect of temperature on the mean square displacement (MSD) of atoms in the samples was investigated by incoherent elastic neutron scattering. The MSD increased gradually with an increase in temperature depending on the aw and added solute. From the linear fitting, three dynamical transition temperatures (low-, middle- and high-Tds) were determined. The Couchman-Karasz model suggested that the added solute and bacteria were not completely miscible.
Tanimura, Yoshihiko; Yoshitomi, Hiroshi; Nishino, Sho; Tsuji, Tomoya; Fukami, Tomoyo; Shinozuka, Tomoki; Oishi, Kohei; Ishii, Masato; Takamiya, Kei; Onuki, Takaya; et al.
Radiation Measurements, 176, p.107196_1 - 107196_6, 2024/08
Times Cited Count：1 Percentile：43.12(Nuclear Science & Technology)The ICRU has proposed to change the definitions of the operational quantities used for the area and individual monitoring for external exposure in the ICRU Report 95. As introducing the new operational quantities into the radiation monitoring may affect the dose assessment results using the present personal dosimeters, it is necessary to characterize the energy spectrum in the workplace and the energy dependency of the dosimeters to be used. In this work the photon spectra were measured using a NaI(Tl) scintillation detector or a LaBr
(Ce) scintillation detector at the workplaces in the Japanese Research Reactor No.3 (JRR-3) and the Japan Proton Accelerator Research Complex (J-PARC) at Japan Atomic Energy Agency (JAEA). Then the present and new operational quantities were evaluated using the above mention spectra at the workplaces and compared each other.
Cf rotation method with a water Cherenkov neutron detectorTanabe, Kosuke*; Komeda, Masao; Toh, Yosuke; Kitamura, Yasunori*; Misawa, Tsuyoshi*; Tsuchiya, Kenichi*; Sagara, Hiroshi*
Scientific Reports (Internet), 14, p.18828_1 - 18828_10, 2024/08
Times Cited Count：0 Percentile：0.00(Multidisciplinary Sciences)Ichikawa, Tsubasa*; Hakoshima, Hideaki*; Inui, Koji*; Ito, Kosuke*; Matsuda, Ryo*; Mitarai, Kosuke*; Miyamoto, Koichi*; Mizukami, Wataru*; Mizuta, Kaoru*; Mori, Toshio*; et al.
Nature Reviews Physics (Internet), 6(6), p.345 - 347, 2024/06
Times Cited Count：8 Percentile：98.87(Physics, Applied)Ishikado, Motoyuki*; Takahashi, Ryuta*; Yamauchi, Yasuhiro*; Nakamura, Masatoshi*; Ishimaru, Sora*; Yamauchi, Sara*; Kawamura, Seiko; Kira, Hiroshi*; Sakaguchi, Yoshifumi*; Watanabe, Masao; et al.
JPS Conference Proceedings (Internet), 41, p.011010_1 - 011010_7, 2024/05
Sanada, Yukihisa; Abe, Tomohisa; Sasaki, Miyuki; Kanno, Marina*; Yamada, Tsutomu*; Nakasone, Takamasa*; Miyazaki, Nobuyuki*; Oshikiri, Keisuke*; Watabe, Hiroshi*
Journal of Nuclear Science and Technology, 61(5), p.693 - 702, 2024/05
Times Cited Count：7 Percentile：86.26(Nuclear Science & Technology)The "treated water" from which the main radioactive materials were removed contains tritium, and stakeholders in Japan have been debating how to treat it. The amount of treated water stored in the facility has reached its limit, and the Japanese government has decided that the treatment method will be to discharge the water into the ocean by FY 2023 (FY: Fiscal Year). The present research developed a simple and practical tritium monitor for the Fukushima Daiichi Nuclear Power Station (FDNPS) tritiated water release. A simple and practical tritium monitor was developed for FDNPS tritiated water release based on thin plastic scintillator sheets. The developed devices were calibrated using standard tritium solutions and a method for calculating the minimum detectable activity. Fifteen 0.25 mm-thick scintillators can be placed in the 0.26 L flow cell where the sample water is fed, yielding an active surface area of 3,200 mm
. The efficiency of tritiated water with full water is 0.000035 cps Bq
. The minimum detectable activity under simple shielding conditions was 7,800 Bq L (Measurement time was 3,600 s).
Watabe, Hiroshi*; Sato, Tatsuhiko; Yu, K. N.*; Zivkovic, M.*; Krstic, D.*; Nikezic, D.*; Kim, K. M.*; Yamaya, Taiga*; Kawachi, Naoki*; Tanaka, Hiroki*; et al.
Radiation Protection Dosimetry, 200(2), p.130 - 142, 2024/02
Times Cited Count：2 Percentile：40.17(Environmental Sciences)Previously, we have developed DynamicMC for modelling relative movement of ORNL phantom in a radiation field for MCNP. Using this software, 3-dimensional dose distributions in a phantom irradiated by a certain mono-energetic source can be deduced through its graphical user interface (GUI). In this study, we extended DynamicMC to be used in combination with the PHITS by providing it with a higher flexibility for dynamic movement for a less sophisticated anthropomorphic phantom. We anticipate that the present work and the developed open-source tools will be in the interest of nuclear radiation physics community for research and teaching purposes.
Sato, Tatsuhiko; Iwamoto, Yosuke; Hashimoto, Shintaro; Ogawa, Tatsuhiko; Furuta, Takuya; Abe, Shinichiro; Kai, Takeshi; Matsuya, Yusuke; Matsuda, Norihiro; Hirata, Yuho; et al.
Journal of Nuclear Science and Technology, 61(1), p.127 - 135, 2024/01
Times Cited Count：144 Percentile：99.97(Nuclear Science & Technology)The Particle and Heavy Ion Transport code System (PHITS) is a general-purpose Monte Carlo radiation transport code that can simulate the behavior of most particle species with energies up to 1 TeV (per nucleon for ions). Its new version, PHITS3.31, was recently developed and released to the public. In the new version, the compatibility with high-energy nuclear data libraries and the algorithm of the track-structure modes have been improved. In this paper, we summarize the upgraded features of PHITS3.31 with respect to the physics models, utility functions, and application software introduced since the release of PHITS3.02 in 2017.
Okuno, Hiroshi; Kawakami, Takeshi; Watanabe, Fumitaka; Horikoshi, Hidehiko*
Journal of Disaster Research, 18(8), p.911 - 917, 2023/12
In response to residents' concerns about the radiation health effects following the nuclear accidents at the Fukushima Daiichi Nuclear Power Station of the Tokyo Electric Power Company in March 2011, the Japan Atomic Energy Agency (JAEA) established a telephone consultation system. Eight toll-free telephone lines were prepared, and employees with knowledge of radiation health effects were assigned for consultation. Approximately 35,000 consultations were conducted from March 17, 2011, to September 18, 2012. The results of the text mining analysis revealed that the greatest source of anxiety was the impact on children's health from radiation. The JAEA's system for telephone consultation was improved following this telephone consultation experience. The description of telephone hotlines in the International Atomic Energy Agency (IAEA) guide, GSG-14, was discussed for further improvements of the JAEA's telephone consultation system.
states in the electronic structure of the intermediate-valence superconductor CeIrFujimori, Shinichi; Kawasaki, Ikuto; Takeda, Yukiharu; Yamagami, Hiroshi; Sasabe, Norimasa*; Sato, Yoshiki*; Shimizu, Yusei*; Nakamura, Ai*; Maruya, A.*; Homma, Yoshiya*; et al.
Electronic Structure (Internet), 5(4), p.045009_1 - 045009_7, 2023/11
Shibata, Motoki*; Nakanishi, Yohei*; Abe, Jun*; Arima, Hiroshi*; Iwase, Hiroki*; Shibayama, Mitsuhiro*; Motokawa, Ryuhei; Kumada, Takayuki; Takata, Shinichi; Yamamoto, Katsuhiro*; et al.
Polymer Journal, 55(11), p.1165 - 1170, 2023/11
Times Cited Count：2 Percentile：24.51(Polymer Science)Kutsukake, Kenichi; Matsuda, Makoto; Nakamura, Masahiko; Ishizaki, Nobuhiro; Kabumoto, Hiroshi; Otokawa, Yoshinori; Asozu, Takuhiro; Matsui, Yutaka; Nakagawa, Sohei; Abe, Shinichi
Proceedings of 20th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1080 - 1084, 2023/11
no abstracts in English
Yoshitomi, Hiroshi; Manabe, Kentaro; Ochi, Kotaro; Kono, Takahiko; Sasaki, Michiya*; Yoshida, Hiroko*
Hoken Butsuri (Internet), 58(2), p.105 - 111, 2023/08
This article gives the report on participation in the 6th Asian and Oceanic Congress on Radiation Protection (AOCRP6), which was held in Mumbai, India on between February 7th and 11th, 2023.
Abe, Takeyasu; Iida, Yoshihisa; Sasamoto, Hiroshi; Ishii, Eiichi
Proceedings of Water-Rock Interaction (WRI-17)/ Applied Isotope Geochemistry (AIG-14) (Internet), 6 Pages, 2023/08
Cation exchange is one of important elementary reactions among water-rock interactions in sedimentary rocks. In order to model non-constant Na-K-Ca-Mg-H exchange selectivity of sedimentary rocks, exchange isotherms and pH dependence on cation exchange capacity of smectite were analyzed following active fraction model. As the result of comparison of exchangeable cationic composition between measured and calculated, selectivity coefficients determined in this study were preferred to those presented by previous studies. Using the coefficients and groundwater hydrochemistry reported previously, expected compositions of exchangeable cations were calculated. The results suggested that pH and total Na-K-Ca-Mg-H concentration of groundwater are important factors to interpret observed compositional variation in exchangeable base cations.
Watanabe, Yukinobu*; Sadamatsu, Hiroki*; Araki, Shohei; Nakano, Keita; Kawase, Shoichiro*; Kin, Tadahiro*; Iwamoto, Yosuke; Satoh, Daiki; Hagiwara, Masayuki*; Yashima, Hiroshi*; et al.
EPJ Web of Conferences, 284, p.01041_1 - 01041_4, 2023/05
Times Cited Count：0 Percentile：0.00(Nuclear Science & Technology)Intensive fast neutron sources using deuteron accelerators have been proposed for the study of medical RI production, radiation damage for fusion reactor materials, nuclear transmutation of radioactive waste, and so on. Neutron production data from various materials bombarded by deuterons are required for the design of such neutron sources. In the present work, we have conducted a systematic measurement of double-differential neutron production cross sections (DDXs) for a wide atomic number range of targets (Li, Be, C, Al, Cu, Nb, In, Ta, and Au) at an incident energy of 200 MeV in the Research Center for Nuclear Physics (RCNP), Osaka University. A deuteron beam accelerated to 200 MeV was transported to the neutron experimental hall and focused on a thin target foil. Emitted neutrons from the target were detected by two different-size EJ301 liquid organic scintillators located at two distances of 7 m and 20 m, respectively. The neutron DDXs were measured at six angles from 0
to 25). The neutron energy was determined by a conventional time-of-flight (TOF) method. The measured DDXs were compared with theoretical model calculations by the DEUteron-induced Reaction Analysis Code System (DEURACS) and PHITS. The result indicated that the DEURACS calculation provides better agreement with the measured DDXs than the PHITS calculation.
Iwamoto, Hiroki; Nakano, Keita; Meigo, Shinichiro; Satoh, Daiki; Iwamoto, Yosuke; Sugihara, Kenta*; Nishio, Katsuhisa; Ishi, Yoshihiro*; Uesugi, Tomonori*; Kuriyama, Yasutoshi*; et al.
EPJ Web of Conferences, 284, p.01023_1 - 01023_4, 2023/05
Times Cited Count：0 Percentile：0.00(Nuclear Science & Technology)For accurate prediction of neutronic characteristics for accelerator-driven systems (ADS) and a source term of spallation neutrons for reactor physics experiments for the ADS at Kyoto University Critical Assembly (KUCA), we have launched an experimental program to measure nuclear data on ADS using the Fixed Field Alternating Gradient (FFAG) accelerator at Kyoto University. As part of this program, the proton-induced double-differential thick-target neutron-yields (TTNYs) and cross-sections (DDXs) for iron, lead, and bismuth have been measured with the time-of-flight (TOF) method. For each measurement, the target was installed in a vacuum chamber on the beamline and bombarded with 107-MeV proton beams accelerated from the FFAG accelerator. Neutrons produced from the targets were detected with stacked, small-sized neutron detectors for several angles from the incident beam direction. The TOF spectra were obtained from the detected signals and the FFAG kicker magnet's logic signals, where gamma-ray events were eliminated by pulse shape discrimination. Finally, the TTNYs and DDXs were obtained from the TOF spectra by relativistic kinematics. The measured TTNYs and DDXs were compared with calculations by the Monte Carlo transport code PHITS with its default physics model of INCL version 4.6 combined with GEM and those with the JENDL-4.0/HE nuclear data library.
