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JAEA Reports

Sampling of radioactive materials remaining in JMTR Reactor Facility

Ouchi, Takuya; Nagata, Hiroshi; Shinoda, Yuya; Yoshida, Hayato; Inoue, Shuichi; Chinone, Marina; Abe, Kazuyuki; Ide, Hiroshi; Watahiki, Shunsuke

JAEA-Technology 2025-006, 25 Pages, 2025/10

JAEA-Technology-2025-006.pdf:1.59MB

In the future, radioactive waste which generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried for the near surface disposal. It is necessary to establish the method to evaluate the radioactivity concentrations of the radioactive wastes. Therefore, at the Oarai Nuclear Engineering Institute, in order to contribute to the study of methods for evaluating radioactivity concentrations of the radioactive wastes from nuclear research facilities, samples were taken from radioactive waste that are expected to be buried in the future and radiochemical analysis is used to obtain data on the radioactivity concentration of each nuclide contained in the radioactive waste. This report presents the concept of selecting sample collection targets and summarizes the sampling of radioactive materials conducted at the JMTR reactor facility in fiscal years 2023 and 2024 to obtain data on radioactivity concentrations.

Journal Articles

Visualisation and quantitative evaluation of chlorides in corroded crevice of stainless steel using radioisotope $$^{36}$$Cl$$^{-}$$

Aoki, So; Abe, Yosuke; Abe, Hiroshi*; Watanabe, Yutaka*; Yamamoto, Masahiro*

Corrosion Science, 255, p.113119_1 - 113119_10, 2025/10

 Times Cited Count:0 Percentile:0.00(Materials Science, Multidisciplinary)

This study aimed to visualise the distribution of chloride in the corroded crevice of stainless steel and to evaluate the chloride content quantitatively. Crevice corrosion tests were carried out using $$^{36}$$Cl$$^{-}$$, a radioactive isotope of chloride, as a tracer in NaCl test solutions. After crevice corrosion tests, stainless steel specimens were placed on an imaging plate. The imaging plate was sensitised by $$beta$$-ray emitted by $$^{36}$$Cl$$^{-}$$ adhering to the crevice. As a result, the chloride distribution in the corroded area inside the crevice was visualised. A calibration curve for the amount of $$^{36}$$Cl$$^{-}$$ was obtained from the relationship between the time of photosensitivity to $$beta$$-ray emitted by $$^{36}$$Cl$$^{-}$$ and the luminance of the imaging plate. The chloride content in the corroded crevice was quantitatively evaluated based on the calibration curve. These visualisation and quantitative evaluation methods were also applied to tests in which specimens were left in pure water after crevice corrosion tests, and the behaviour of chloride in crevice corrosion was discussed.

Journal Articles

Particle arrangements and optical changes induced by the water swelling of melanin-like polydopamine layers

Watanabe, Taku*; Maejima, Yui*; Ueda, Yuki; Motokawa, Ryuhei; Takabatake, Ai*; Takeda, Shinichi*; Fudoji, Hiroshi*; Kishikawa, Keiki*; Koori, Michinari*

Langmuir, 41(34), p.22762 - 22773, 2025/09

 Times Cited Count:0

The assembled structures of melanin particles, i.e., colloidal particles coated with a melanin-like polydopamine (PDA) layer, create vivid structural colors. While the thickness of the PDA layer influences the particle arrangement and optical properties, the underlying mechanism has remained controversial. We demonstrate that the water swelling characteristics of PDA are crucial factors governing the dispersion and aggregation of these particles in solution. Detailed comparisons between dry and wet conditions revealed that the PDA layer readily absorbs water molecules, which leads to significant swelling in the thicker layers. The swelling of the PDA layers determined whether the particles remained dispersed or partially aggregated in the water, ultimately controlling the particle arrangement in the dry state once the water evaporated. These findings provide insights into the self-assembly of colloidal particles and offer a strategy for tuning the periodic particle order. This feature is pivotal for various applications in optical and sensing technologies.

Journal Articles

Meeting report on the EPRBioDose2024, Hirosaki

Fujishima, Yohei*; Anderson, D.*; Abe, Yu*; Alkebsi, L.*; Oka, Toshitaka; Tani, Atsushi*; Kranrod, C.*; Toyoda, Shin*; Hamasaki, Kanya*; Hirota, Seiko*; et al.

Nihon Hoshasen Jiko, Saigai Igakkai Zasshi, 7(1), p.21 - 26, 2024/12

no abstracts in English

Journal Articles

Overview of PHITS Ver.3.34 with particular focus on track-structure calculation

Ogawa, Tatsuhiko; Hirata, Yuho; Matsuya, Yusuke; Kai, Takeshi; Sato, Tatsuhiko; Iwamoto, Yosuke; Hashimoto, Shintaro; Furuta, Takuya; Abe, Shinichiro; Matsuda, Norihiro; et al.

EPJ Nuclear Sciences & Technologies (Internet), 10, p.13_1 - 13_8, 2024/11

The latest updates on PHITS, a versatile radiation transport code, focusing specifically on track-structure models are presented. Track structure calculations are methods used to simulate the movement of charged particles while explicitly considering each atomic reaction. Initially developed for radiation biology, these calculation methods aimed to analyze the radiation-induced damage to DNA and chromosomes. Several track-structure calculation models, including PHITS-ETS, PHITS-ETS for Si, PHITS-KURBUC, ETSART, and ITSART, have been developed and implemented to PHITS. These models allow users to study the behavior of various particles at the nano-scale across a wide range of materials. Furthermore, potential applications of track-structure calculations have also been proposed so far. This collection of track-structure calculation models, which encompasses diverse conditions, opens up new avenues for research in the field of radiation effects.

Journal Articles

Cavity ionization chamber responses in the JAEA and the NMIJ high-energy photon reference fields for radiation protection

Ishii, Junya*; Shimizu, Morihito*; Kato, Masahiro*; Kurosawa, Tadahiro*; Tsuji, Tomoya; Yoshitomi, Hiroshi; Tanimura, Yoshihiko; Watabe, Hiroshi*

Journal of Radiological Protection, 44(3), p.031516_1 - 031516_8, 2024/09

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

Journal Articles

Effect of water activity on the mechanical glass transition and dynamical transition of bacteria-solute systems

Kawai, Kiyoshi*; Sogabe, Tomochika*; Nakagawa, Hiroshi; Yamada, Takeshi*; Koseki, Shigenobu*

Journal of Food Engineering, 375, p.112066_1 - 112066_9, 2024/08

 Times Cited Count:1 Percentile:23.31(Engineering, Chemical)

The purpose of this study was to clarify effect of glycerol and glucose on the mechanical glass transition and dynamical transition of freeze-dried bacteria at various water activity (aw)-conditions. From the water sorption isotherm, it was noted that the water content at each aw and monolayer water content were higher in the order of glycerol, glucose, non-added samples. Effect of temperature on the mean square displacement (MSD) of atoms in the samples was investigated by incoherent elastic neutron scattering. The MSD increased gradually with an increase in temperature depending on the aw and added solute. From the linear fitting, three dynamical transition temperatures (low-, middle- and high-Tds) were determined. The Couchman-Karasz model suggested that the added solute and bacteria were not completely miscible.

Journal Articles

Present and new operational quantities evaluated from photon spectrum measurements at workplaces in the research reactor and accelerator facility at the JAEA

Tanimura, Yoshihiko; Yoshitomi, Hiroshi; Nishino, Sho; Tsuji, Tomoya; Fukami, Tomoyo; Shinozuka, Tomoki; Oishi, Kohei; Ishii, Masato; Takamiya, Kei; Onuki, Takaya; et al.

Radiation Measurements, 176, p.107196_1 - 107196_6, 2024/08

 Times Cited Count:1 Percentile:43.12(Nuclear Science & Technology)

The ICRU has proposed to change the definitions of the operational quantities used for the area and individual monitoring for external exposure in the ICRU Report 95. As introducing the new operational quantities into the radiation monitoring may affect the dose assessment results using the present personal dosimeters, it is necessary to characterize the energy spectrum in the workplace and the energy dependency of the dosimeters to be used. In this work the photon spectra were measured using a NaI(Tl) scintillation detector or a LaBr$$_3$$(Ce) scintillation detector at the workplaces in the Japanese Research Reactor No.3 (JRR-3) and the Japan Proton Accelerator Research Complex (J-PARC) at Japan Atomic Energy Agency (JAEA). Then the present and new operational quantities were evaluated using the above mention spectra at the workplaces and compared each other.

Journal Articles

Compact and transportable system for detecting lead-shielded highly enriched uranium using $$^{252}$$Cf rotation method with a water Cherenkov neutron detector

Tanabe, Kosuke*; Komeda, Masao; Toh, Yosuke; Kitamura, Yasunori*; Misawa, Tsuyoshi*; Tsuchiya, Kenichi*; Sagara, Hiroshi*

Scientific Reports (Internet), 14, p.18828_1 - 18828_10, 2024/08

 Times Cited Count:0 Percentile:0.00(Multidisciplinary Sciences)

Journal Articles

Probing water-driven nanostructures in an ionic liquid using small- and wide-angle neutron scattering; 1-Dodecyl-3-methylimidazolium iodide

Abe, Hiroshi*; Maruyama, Shusei*; Hiroi, Kosuke; Takata, Shinichi

Journal of Molecular Liquids, 404, p.124952_1 - 124952_8, 2024/06

Journal Articles

Current numbers of qubits and their uses

Ichikawa, Tsubasa*; Hakoshima, Hideaki*; Inui, Koji*; Ito, Kosuke*; Matsuda, Ryo*; Mitarai, Kosuke*; Miyamoto, Koichi*; Mizukami, Wataru*; Mizuta, Kaoru*; Mori, Toshio*; et al.

Nature Reviews Physics (Internet), 6(6), p.345 - 347, 2024/06

 Times Cited Count:10 Percentile:98.87(Physics, Applied)

Journal Articles

Recent status of the cryogenic sample environment at the MLF, J-PARC

Ishikado, Motoyuki*; Takahashi, Ryuta*; Yamauchi, Yasuhiro*; Nakamura, Masatoshi*; Ishimaru, Sora*; Yamauchi, Sara*; Kawamura, Seiko; Kira, Hiroshi*; Sakaguchi, Yoshifumi*; Watanabe, Masao; et al.

JPS Conference Proceedings (Internet), 41, p.011010_1 - 011010_7, 2024/05

Journal Articles

Basic study on tritium monitor using plastic scintillator for treated water discharge at Fukushima Daiichi Nuclear Power Plant

Sanada, Yukihisa; Abe, Tomohisa; Sasaki, Miyuki; Kanno, Marina*; Yamada, Tsutomu*; Nakasone, Takamasa*; Miyazaki, Nobuyuki*; Oshikiri, Keisuke*; Watabe, Hiroshi*

Journal of Nuclear Science and Technology, 61(5), p.693 - 702, 2024/05

 Times Cited Count:7 Percentile:86.26(Nuclear Science & Technology)

The "treated water" from which the main radioactive materials were removed contains tritium, and stakeholders in Japan have been debating how to treat it. The amount of treated water stored in the facility has reached its limit, and the Japanese government has decided that the treatment method will be to discharge the water into the ocean by FY 2023 (FY: Fiscal Year). The present research developed a simple and practical tritium monitor for the Fukushima Daiichi Nuclear Power Station (FDNPS) tritiated water release. A simple and practical tritium monitor was developed for FDNPS tritiated water release based on thin plastic scintillator sheets. The developed devices were calibrated using standard tritium solutions and a method for calculating the minimum detectable activity. Fifteen 0.25 mm-thick scintillators can be placed in the 0.26 L flow cell where the sample water is fed, yielding an active surface area of 3,200 mm$$^{2}$$. The efficiency of tritiated water with full water is 0.000035 cps Bq$$^{-1}$$. The minimum detectable activity under simple shielding conditions was 7,800 Bq L$$^{-1}$$ (Measurement time was 3,600 s).

Journal Articles

Development of DynamicMC for PHITS Monte Carlo package

Watabe, Hiroshi*; Sato, Tatsuhiko; Yu, K. N.*; Zivkovic, M.*; Krstic, D.*; Nikezic, D.*; Kim, K. M.*; Yamaya, Taiga*; Kawachi, Naoki*; Tanaka, Hiroki*; et al.

Radiation Protection Dosimetry, 200(2), p.130 - 142, 2024/02

 Times Cited Count:2 Percentile:40.17(Environmental Sciences)

Previously, we have developed DynamicMC for modelling relative movement of ORNL phantom in a radiation field for MCNP. Using this software, 3-dimensional dose distributions in a phantom irradiated by a certain mono-energetic source can be deduced through its graphical user interface (GUI). In this study, we extended DynamicMC to be used in combination with the PHITS by providing it with a higher flexibility for dynamic movement for a less sophisticated anthropomorphic phantom. We anticipate that the present work and the developed open-source tools will be in the interest of nuclear radiation physics community for research and teaching purposes.

Journal Articles

Recent improvements of the Particle and Heavy Ion Transport code System; PHITS version 3.33

Sato, Tatsuhiko; Iwamoto, Yosuke; Hashimoto, Shintaro; Ogawa, Tatsuhiko; Furuta, Takuya; Abe, Shinichiro; Kai, Takeshi; Matsuya, Yusuke; Matsuda, Norihiro; Hirata, Yuho; et al.

Journal of Nuclear Science and Technology, 61(1), p.127 - 135, 2024/01

 Times Cited Count:183 Percentile:99.97(Nuclear Science & Technology)

The Particle and Heavy Ion Transport code System (PHITS) is a general-purpose Monte Carlo radiation transport code that can simulate the behavior of most particle species with energies up to 1 TeV (per nucleon for ions). Its new version, PHITS3.31, was recently developed and released to the public. In the new version, the compatibility with high-energy nuclear data libraries and the algorithm of the track-structure modes have been improved. In this paper, we summarize the upgraded features of PHITS3.31 with respect to the physics models, utility functions, and application software introduced since the release of PHITS3.02 in 2017.

Journal Articles

Arrangements for telephone consultation on radiation health effects in a nuclear emergency in Japan; Lessons learned from the nuclear accident in Fukushima, Japan, 2011

Okuno, Hiroshi; Kawakami, Takeshi; Watanabe, Fumitaka; Horikoshi, Hidehiko*

Journal of Disaster Research, 18(8), p.911 - 917, 2023/12

In response to residents' concerns about the radiation health effects following the nuclear accidents at the Fukushima Daiichi Nuclear Power Station of the Tokyo Electric Power Company in March 2011, the Japan Atomic Energy Agency (JAEA) established a telephone consultation system. Eight toll-free telephone lines were prepared, and employees with knowledge of radiation health effects were assigned for consultation. Approximately 35,000 consultations were conducted from March 17, 2011, to September 18, 2012. The results of the text mining analysis revealed that the greatest source of anxiety was the impact on children's health from radiation. The JAEA's system for telephone consultation was improved following this telephone consultation experience. The description of telephone hotlines in the International Atomic Energy Agency (IAEA) guide, GSG-14, was discussed for further improvements of the JAEA's telephone consultation system.

Journal Articles

Impact of the Ce$$4f$$ states in the electronic structure of the intermediate-valence superconductor CeIr$$_3$$

Fujimori, Shinichi; Kawasaki, Ikuto; Takeda, Yukiharu; Yamagami, Hiroshi; Sasabe, Norimasa*; Sato, Yoshiki*; Shimizu, Yusei*; Nakamura, Ai*; Maruya, A.*; Homma, Yoshiya*; et al.

Electronic Structure (Internet), 5(4), p.045009_1 - 045009_7, 2023/11

Journal Articles

Structural changes of polystyrene particles in subcritical and supercritical water revealed by in situ small-angle neutron scattering

Shibata, Motoki*; Nakanishi, Yohei*; Abe, Jun*; Arima, Hiroshi*; Iwase, Hiroki*; Shibayama, Mitsuhiro*; Motokawa, Ryuhei; Kumada, Takayuki; Takata, Shinichi; Yamamoto, Katsuhiro*; et al.

Polymer Journal, 55(11), p.1165 - 1170, 2023/11

 Times Cited Count:3 Percentile:24.51(Polymer Science)

Journal Articles

Present status of JAEA-Tokai tandem accelerator

Kutsukake, Kenichi; Matsuda, Makoto; Nakamura, Masahiko; Ishizaki, Nobuhiro; Kabumoto, Hiroshi; Otokawa, Yoshinori; Asozu, Takuhiro; Matsui, Yutaka; Nakagawa, Sohei; Abe, Shinichi

Proceedings of 20th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1080 - 1084, 2023/11

no abstracts in English

Journal Articles

Nanoconfined water in ionic liquid and lyotropic ionic liquid crystals by small- and wide-angle X-ray and neutron scattering; 1-Decyl-3-methylimidazolium nitrate

Abe, Hiroshi*; Nemoto, Fumiya*; Hiroi, Kosuke; Takata, Shinichi

Journal of Molecular Liquids, 386, p.122551_1 - 122551_7, 2023/09

850 (Records 1-20 displayed on this page)