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Takami, Kazusa*; Gomi, Yuibi*; Yasuda, Ryuichi*; Abe, Shinichiro; Ito, Masatoshi*; Kanda, Hiroki*; Fukuda, Mitsuhiro*; Hashimoto, Masanori*
IEEE Transactions on Nuclear Science, 72(8), p.2622 - 2628, 2025/08
Times Cited Count:1 Percentile:78.42Neutron-induced soft errors in the terrestrial environment pose reliability issues for semiconductor devices. We have developed the new method for estimating terrestrial SER based on simulation coupled with one-time irradiation using a conventional neutron source. This method has been validated using 65-nm planar SRAMs. However, with the ongoing progression of process shrinkage and the increasing adoption of devices fabricated with newer processes, there is a growing demand for further experimental validation of the terrestrial SER estimation method for these advanced processes. In this work, we validated the estimation method for 12-nm 1-fin FinFETs and 28-nm planer SRAMs. The SERs estimated by our method were consistent with the SERs measured using a white neutron beam at RCNP within 28% error.
Yokoyama, Keisuke; Watanabe, Masashi; Onishi, Takashi; Yano, Yasuhide; Tokoro, Daishiro*; Sugata, Hiromasa*; Kato, Masato*
JAEA-Research 2025-002, 18 Pages, 2025/05
It is advocated as a development target of fast reactors (FRs) to allow for the of use of mixed oxide (MOX) fuels containing minor actinide (MA) separated and recovered from spent fuels with the aim of reducing the volume and toxicity of high-level radioactive waste generated from nuclear reactors. In the development of MAMOX fuels, it is important behavior to understand the thermal properties such as thermal conductivity for fuel design and analysis of the irradiation. However, there are only a few reports on the thermal properties of MA-MOX fuels, and neither the effects of MA contents nor of oxygen non-stoichiometry in MOX fuels on their thermal conductivities have been fully understood. In this study, the thermal conductivities of MOX fuels with up to 15% Am content were measured at near-stoichiometric composition and the relationship between thermal conductivity and Am content was evaluated. Moreover, the thermal conductivities of Am-doped UO
fuels were also measured and evaluated by comparison with Am-MOX to evaluate the effect of Am content. The fuel samples used in this study were three types of MOX with a Pu content of 30% and different Am contents (5%, 10%, and 15%), and UO
containing 15% Am. The thermal conductivities of specimens were calculated from the thermal diffusivities measured by the laser flash method, the density of the specimens and, the heat capacity at constant pressure. The oxygen partial pressure during the measurement was controlled at that of the targeted near-stoichiometric composition. The thermal conductivities of all specimens exhibited a decline with increasing temperature and Am content, with a particularly pronounced reduction observed below 1,173 K. The results of the classical phonon scattering model analysis of the measured thermal conductivities showed that the effect of lattice strain due to the Am addition was significant on the thermal resistivity change, and the effect was comparable for both MOX and UO
.
Hirouchi, Jun; Takahara, Shogo; Watanabe, Masatoshi*
Journal of Radiological Protection, 45(2), p.021506_1 - 021506_13, 2025/05
Times Cited Count:0 Percentile:0.00(Environmental Sciences)Sheltering is a key countermeasure for mitigating radiation exposures during nuclear power plant accidents. The effectiveness of sheltering in minimizing inhalation exposure is commonly expressed using the reduction factor, which is the ratio of indoor to outdoor cumulative doses. The indoor dose is primarily influenced by the air exchange rate, penetration factor, and indoor deposition rate. Additionally, the air exchange rate is dependent on wind speed. In previous studies, the reduction factor was often treated as a constant value or calculated under constant wind speed conditions. However, wind speed varies in reality. This study investigated the effect of temporal variations in wind speed on the reduction factor and developed a simplified correction method to account for these variations. The results revealed that temporal variations in wind speed caused the reduction factor to differ by a factor of approximately two. Using the simplified correction method, the corrected reduction factors agreed, on average, within 10% of those calculated using a method that explicitly considers temporal variations in actual wind speed. Additionally, the computational cost was reduced by more than 20 times.
Hirouchi, Jun; Watanabe, Masatoshi*; Hayashi, Naho; Nagakubo, Azusa; Takahara, Shogo
JAEA-Research 2024-015, 114 Pages, 2025/03
The public living in areas contaminated by nuclear accidents is exposed to radiation in the early phase and over the long term. Even under the same accident scenario, the exposure doses and the effectiveness of sheltering, which is one of the protective measures, vary depending on the meteorological condition and the surrounding environment. The exposure doses and sheltering effectiveness in the early phase are important information for the public and the national and local governments planning a nuclear emergency preparedness. In this report, we evaluate the exposure doses and sheltering effectiveness at sites with nuclear facilities in Japan using OSCAAR, one of the probabilistic risk assessment codes, for five accident scenarios: three scenarios from past severe accident studies; a scenario defined by the Nuclear Regulatory Authority; and a scenario assuming the Fukushima Daiichi Nuclear Power Station accident. The sheltering effectiveness differed by approximately 20% among the sites. This was due to the differences in wind speed among the sites.
Hirouchi, Jun; Watanabe, Masatoshi*; Hayashi, Naho; Nagakubo, Azusa; Takahara, Shogo
Journal of Radiological Protection, 45(1), p.011506_1 - 011506_11, 2025/03
Times Cited Count:0 Percentile:0.00(Environmental Sciences)Public living in areas contaminated by nuclear accidents is exposed to radiation in the early phase and over the long term. Even under similar accident scenarios, radiation doses and sheltering effectiveness, which is one of the protective measures, depend on meteorological conditions and the surrounding environment. Radiation doses and sheltering effectiveness in the early phase of nuclear accidents are crucial information for the public as well as national and local governments planning a nuclear emergency preparedness. In this study, we assessed radiation doses and sheltering effectiveness at sites with nuclear facilities in Japan using the Off-Site Consequence Analysis code for Atmospheric Release accidents, which is one of the level-3 probabilistic risk assessment codes, for five accident scenarios: three scenarios from past severe accident studies, a scenario defined by the Nuclear Regulation Authority in Japan, and a scenario corresponding to the Fukushima-Daiichi Nuclear Power Station accident. The sheltering effectiveness differed by up to approximately 50% among the accident scenarios at the same sites and by approximately 20%
50% among sites under the same accident scenario. Differences in the radionuclide composition among the accident scenarios and the differences in wind speeds among the sites primarily caused these differences in sheltering effectiveness.
Pu
Am
)O
Yokoyama, Keisuke; Watanabe, Masashi; Usui, Akane; Seki, Takayuki*; Onishi, Takashi; Kato, Masato
Nuclear Materials and Energy (Internet), 42, p.101908_1 - 101908_6, 2025/03
Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)Oxygen potential of high Am content MOX, (U
Pu
Am
)O
, was measured at 1273 K, 1473 K, 1573 K, and 1623 K. by gas equilibrium method using thermogravimeter. Comparing the measured data with the literature data, it was found that the addition of 15% Am increases the oxygen potential of (U, Pu)O
by 100-150 kJ/mol for the same Pu content and O/M ratio. The proportion of cations in the stoichiometric composition was determined as (U
U
Pu
Am
)O
, assuming the presence of Am
and partial oxidation of U
to U
. The relationship between oxygen partial pressure and deviation x from stoichiometry in (U
Pu
Am
)O
was analyzed by defect chemistry model. The equation to represent the O/M ratio was derived as a function of temperature and oxygen partial pressure. A part of this study includes the results of MEXT Innovative Nuclear Research and Development Program Grant Number JPMXD0219214921.
Yamamoto, Keisuke; Nakagawa, Takuya; Shimojo, Hiroto; Kijima, Jun; Miura, Daiya; Onose, Yoshihiko*; Namba, Koji*; Uchida, Hiroaki*; Sakamoto, Kazuhiko*; Ono, Chika*; et al.
JAEA-Technology 2024-019, 211 Pages, 2025/02
The uranium enrichment facilities at the Nuclear Fuel Cycle Engineering Laboratories of Japan Atomic Energy Agency (JAEA) were constructed sequentially to develop uranium enrichment technology with centrifugal separation method. The developed technologies were transferred to Japan Nuclear Fuel Limited until 2001. And the original purpose has been achieved. Wastewater Treatment Facility, one of the uranium enrichment facilities, was constructed in 1976 to treat radioactive liquid waste generated at the facilities, and it finished the role in 2008. In accordance with the Medium/Long-Term Management Plan of JAEA Facilities, interior equipment installed in this facility had been dismantled and removed since November 2021 to August 2023. This report summarizes the findings obtained through the work related to the contamination inspection methods cancellation the controlled area of Wastewater Treatment Facility from September 2023 to March 2024.
Zheng, X.-G.*; Yamauchi, Ichihiro*; Hagihara, Masato; Nishibori, Eiji*; Kawae, Tatsuya*; Watanabe, Isao*; Uchiyama, Tomoki*; Chen, Y.*; Xu, C.-N.*
Nature Communications (Internet), 15, p.9989_1 - 9989_12, 2024/11
Times Cited Count:1 Percentile:15.90(Multidisciplinary Sciences)Miyabe, Masabumi; Iwata, Yoshihiro; Tomita, Hideki*; Morita, Masato*; Sakamoto, Tetsuo*
Spectrochimica Acta, Part B, 221, p.107036_1 - 107036_12, 2024/11
Two-color two-step resonance ionization spectroscopy of neodymium (Nd) was performed to identify more than 120 even-parity autoionizing levels and their candidate J-values. The analysis of the observed autoionizing Rydberg series yielded a value of 44560.11 (43)
(2)
cm
as a more accurate ionization potential of Nd. The saturation method was used to measure the transition cross-sections for some intense ionization transitions. From the measured cross-sections, the ionization efficiencies of some two-step ionization schemes were evaluated using the scheme cross-section formula to obtain several promising schemes.
Am
O
at 1473, 1573, and 1673 KWatanabe, Masashi; Yokoyama, Keisuke; Vauchy, R.; Kato, Masato; Sugata, Hiromasa*; Seki, Takayuki*; Hino, Tetsushi*
Journal of Nuclear Materials, 599, p.155232_1 - 155232_5, 2024/10
Times Cited Count:2 Percentile:59.21(Materials Science, Multidisciplinary)Oxygen potential data of U
Am
O
were measured at 1473, 1573, and 1673 K by thermogravimetry. In U
An
O
, where An stands for Pu or Am, and for a given value of y and Oxygen/Metal ratio, the oxygen potential of U
Am
O
is higher than that of U
Pu
O
. The valence of cations in the hypostoichiometric region is similar to that of Nd-doped UO
. At the stoichiometric composition, it is estimated to be Am
, U
, and U
(for charge compensation of Am
). The experimental data were analyzed using a defect chemistry model, and a relationship connecting the oxygen-to-metal ratio, the temperature, and the equilibrium oxygen partial pressure was proposed.
Sogabe, Joji; Ishida, Shinya; Tagami, Hirotaka; Okano, Yasushi; Kamiyama, Kenji; Onoda, Yuichi; Matsuba, Kenichi; Yamano, Hidemasa; Kubo, Shigenobu; Kubota, Ryuzaburo*; et al.
Proceedings of International Conference on Nuclear Fuel Cycle (GLOBAL2024) (Internet), 4 Pages, 2024/10
In the frame of France-Japan collaboration, the calculational methodologies were defined and assessed, and the phenomenology and the severe accident consequences were investigated in a pool-type sodium-cooled fast reactor.
Tanimura, Yoshihiko; Yoshitomi, Hiroshi; Nishino, Sho; Tsuji, Tomoya; Fukami, Tomoyo; Shinozuka, Tomoki; Oishi, Kohei; Ishii, Masato; Takamiya, Kei; Onuki, Takaya; et al.
Radiation Measurements, 176, p.107196_1 - 107196_6, 2024/08
Times Cited Count:1 Percentile:35.03(Nuclear Science & Technology)The ICRU has proposed to change the definitions of the operational quantities used for the area and individual monitoring for external exposure in the ICRU Report 95. As introducing the new operational quantities into the radiation monitoring may affect the dose assessment results using the present personal dosimeters, it is necessary to characterize the energy spectrum in the workplace and the energy dependency of the dosimeters to be used. In this work the photon spectra were measured using a NaI(Tl) scintillation detector or a LaBr
(Ce) scintillation detector at the workplaces in the Japanese Research Reactor No.3 (JRR-3) and the Japan Proton Accelerator Research Complex (J-PARC) at Japan Atomic Energy Agency (JAEA). Then the present and new operational quantities were evaluated using the above mention spectra at the workplaces and compared each other.
Watakabe, Tomoyoshi; Yamamoto, Tomohiko; Okamura, Shigeki; Miyazaki, Masashi; Miyagawa, Takayuki; Uchita, Masato*; Hirayama, Tomoyuki*; Somaki, Takahiro*; Yukawa, Masaki*; Fukasawa, Tsuyoshi*; et al.
Proceedings of ASME 2024 Pressure Vessels & Piping Conference (PVP 2024) (Internet), 10 Pages, 2024/07
To secure the seismic safety of the thin-walled mechanical components and piping under a severe design earthquake level, employing a three-dimensional (3D) seismic isolation system has been planned in a sodium-cooled fast reactor. The development results of the 3D isolation system have been reported in previous papers so far. Its update is reported in Part 7 to Part 9. Part 7 describes the overview of the development, the test plan of the isolation system in the assembled state of each element, and the performance of individual isolation elements. In part 8, the performance of the isolation device that each element was assembled into was investigated through loading tests. Part 9 reports analytical studies by an analysis model validated based on the insight of the test results.
Fukasawa, Tsuyoshi*; Somaki, Takahiro*; Yukawa, Masaki*; Hirayama, Tomoyuki*; Watakabe, Tomoyoshi; Yamamoto, Tomohiko; Okamura, Shigeki; Miyazaki, Masashi; Uchita, Masato*; Miyagawa, Takayuki; et al.
Proceedings of ASME 2024 Pressure Vessels & Piping Conference (PVP 2024) (Internet), 10 Pages, 2024/07
Somaki, Takahiro*; Yukawa, Masaki*; Fukasawa, Tsuyoshi*; Hirayama, Tomoyuki*; Uchita, Masato*; Miyagawa, Takayuki; Okamura, Shigeki; Yamamoto, Tomohiko; Watakabe, Tomoyoshi; Miyazaki, Masashi; et al.
Proceedings of ASME 2024 Pressure Vessels & Piping Conference (PVP 2024) (Internet), 9 Pages, 2024/07
Ishikado, Motoyuki*; Takahashi, Ryuta*; Yamauchi, Yasuhiro*; Nakamura, Masatoshi*; Ishimaru, Sora*; Yamauchi, Sara*; Kawamura, Seiko; Kira, Hiroshi*; Sakaguchi, Yoshifumi*; Watanabe, Masao; et al.
JPS Conference Proceedings (Internet), 41, p.011010_1 - 011010_7, 2024/05
Kato, Masato; Oki, Takumi; Watanabe, Masashi; Hirooka, Shun; Vauchy, R.; Ozawa, Takayuki; Uwaba, Tomoyuki; Ikusawa, Yoshihisa; Nakamura, Hiroki; Machida, Masahiko
Journal of the American Ceramic Society, 107(5), p.2998 - 3011, 2024/05
Times Cited Count:6 Percentile:46.63(Materials Science, Ceramics)Kaneko, Koji; Tabata, Chihiro; Hagihara, Masato; Yamauchi, Hiroki; Oba, Yojiro; Kumada, Takayuki; Kubota, Masato; Kojima, Yuki*; Nabatame, Nozomi; Sasaki, Miki; et al.
JPS Conference Proceedings (Internet), 41, p.011015_1 - 011015_6, 2024/03
10
W/cm
Skobelev, I. Yu.*; Ryazantsev, S. N.*; Kulikov, R. K.*; Sedov, M. V.*; Filippov, E. D.*; Pikuz, S. A.*; Asai, Takafumi*; Kanasaki, Masato*; Yamauchi, Tomoya*; Jinno, Satoshi; et al.
Photonics (Internet), 10(11), p.1250_1 - 1250_11, 2023/11
Times Cited Count:3 Percentile:37.32(Optics)It is challenging to clearly distinguish the impacts of the optical field and collisional ionization in the evolution of the charge state of a plasma produced when matter interacts with high-intensity laser pulses. In this work, time-dependent calculations of plasma kinetics are used to show that it is possible only when low-density gaseous targets with sufficiently small clusters are used. In the case of Ar plasma, the upper limit of the cluster radius was estimated to be
m.

Kaneko, Koji; Tabata, Chihiro; Hagihara, Masato; Yamauchi, Hiroki; Kubota, Masato; Osakabe, Toyotaka; Onuki, Yoshichika*
Journal of the Physical Society of Japan, 92(8), p.085001_1 - 085001_2, 2023/08
Times Cited Count:1 Percentile:17.82(Physics, Multidisciplinary)