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Journal Articles

Radiocarbon measurement of a small-scale sample with a cementite target at JAEA-AMS-TONO

Minamitani, Fumina; Nishio, Tomohiro; Fujita, Natsuko; Maeta, Yusuke; Miyake, Masayasu*; Matsubara, Akihiro*; Jinno, Satoshi; Ogita, Yasuhiro; Watanabe, Takahiro

Nuclear Instruments and Methods in Physics Research B, 579, p.166245_1 - 166245_7, 2026/10

The Tono Geoscience Centre has started to build up a small analysis of radiocarbon using cementite. It is characterised by homogeneous target synthesis and stable measurements with high accuracy and low background. In order to establish the optimum cementite preparation method at the centre, the type of iron, conditions of use, reaction yield, reproducibility of measurement and background were investigated. In sample preparation, target production in high yield was successfully achieved by devising the conditions for the use of iron catalysts. Although the measurement conditions are still under investigation, the beam intensity was found to be sufficient for the measurement and the prescisions were relatively high. This presentation will report on the characteristics of small-scale analysis with cementite at this centre.

Journal Articles

CIGMA experiments on integral phenomena related to thermal hydraulics in a reactor containment vessel and building during a severe accident

Abe, Satoshi; Hamdani, A.; Soma, Shu; Hangai, Ryosuke; Omori, Masashi; Owada, Akihiko; Omiya, Toshihito*; Shibamoto, Yasuteru

Nuclear Engineering and Design, 449, p.114787_1 - 114787_13, 2026/04

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

Present status of the JAEA-AMS-TONO (2024FY)

Fujita, Natsuko; Maeta, Yusuke; Miyake, Masayasu*; Matsubara, Akihiro*; Uno, Sadanori*; Omae, Akiomi*; Jinno, Satoshi; Minamitani, Fumina; Watanabe, Takahiro; Nishio, Tomohiro; et al.

Dai-37-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.22 - 25, 2026/03

no abstracts in English

Journal Articles

Temperature effect on radiolytically generated hydrogen yield from a plutonium nitric acid aqueous solution

Toigawa, Tomohiro; Hotoku, Shinobu; Kumagai, Yuta; Abe, Yuma*; Oyama, Kanichi*; Fukaya, Hiroyuki; Ban, Yasutoshi; Kida, Takashi; Hasegawa, Satoshi*; Nakano, Masanao*; et al.

Journal of Nuclear Science and Technology, 63(3), p.322 - 327, 2026/03

 Times Cited Count:1 Percentile:50.28(Nuclear Science & Technology)

The effect of temperature on hydrogen production generated from radiolysis was investigated to determine the associated implications for nuclear fuel reprocessing safety. The hydrogen yield from radiolysis of plutonium nitric acid solution was measured at temperatures up to the boiling temperature of the solution. The results showed no notable temperature dependence even under boiling conditions. The impact of solution agitation on hydrogen production was also assessed, which revealed minor differences in the hydrogen yield between static and agitated conditions at room temperature. These findings suggest that high temperatures or boiling the solution do not considerably enhance hydrogen generation, and provide crucial information for accurately modeling hydrogen risks under severe accidents.

Journal Articles

J-PARC LINAC 50 Hz operation verification study

Kondo, Yasuhiro; Chimura, Motoki; Cicek, E.*; Fukui, Yuji*; Futatsukawa, Kenta*; Fuwa, Yasuhiro; Goto, Rikuto*; Hirano, Koichiro; Ishikawa, Masaki*; Ito, Takashi; et al.

Proceedings of 22nd Annual Meeting of Particle Accelerator Society of Japan (Internet), p.124 - 129, 2026/03

Various upgrade plans of the J-PARC linac are underway, and repetition-rate doubling project is one of the most important part. Currently, the linac supplies a 400~MeV H$$^-$$ ion beam to the 3~GeV synchrotron (RCS) at a repetition rate of 25~Hz. However, to deliver the beam to both RCS and proton-beam irradiation facility under planning, it is necessary to raise the repetition rate from 25~Hz to 50~Hz. Prior to construction of the beamline to the irradiation facility, we conducted a verification of the 50~Hz operation of all the linac apparatus simultaneously within the current operational limits in May 2025. And also, the verification of the 50~Hz operation of the particle counter system, which is one of the most important safety device of the J-PARC accelerator, was conducted. As a result, any significant problems were not found out, and it is now ready for the upcoming 50~Hz-beam acceleration demonstration. This paper describes this details of the demonstration of the 50~Hz operation, without beam acceleration, of the J-PARC linac.

Journal Articles

Differences between radiation dose values under wearing and non-wearing geometries of personal dosimeters during sleep

Hirouchi, Jun; Takahara, Shogo; Watanabe, Masatoshi*

Health Physics, 130(1), p.87 - 93, 2026/01

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

With the return of residents after the Fukushima Daiichi Nuclear Power Station accident, some residents' radiation doses have been measured to ensure their safety. However, personal radiation doses vary depending on the behavior and residential environment of each subject even for a group of subjects living in the same region at the same time. In past studies, subjects were required to wear a personal dosimeter on their chest outdoors, while they were not required to wear the device indoors. This study investigated the difference between the dose values indicated for the wearing and nonwearing conditions of personal dosimeters during sleep. In particular, an adult human phantom was used to compare the indicated dose values when personal dosimeters were placed on the chest (reproducing the wearing condition) and near the head (reproducing the nonwearing condition) in two houses with a high radiation dose. Furthermore, to understand the reason for the difference in the indicated dose values, the radiation dose during sleep was calculated using a radiation transport calculation code. The dose values for the wearing condition were approximately 4% lower on the first floor and approximately 15% lower on the second floor than those for the nonwearing condition. In addition, the radiation doses and radiation dose ratios (head/chest) differed by approximately 30% and 20%, respectively, depending on the distance from the nearest window (1-3 m).

Journal Articles

Role of Alkyl Chain Branching in the Self-Assembly of Nitrilotriacetamide-Based Lanthanide Extractants

Ueda, Yuki; Kobayashi, Toru; Nakamura, Satoshi; Ban, Yasutoshi; Kaneta, Yui; Nabatame, Nozomi; Micheau, C.; Tokunaga, Kohei; Nakabe, Rintaro; Kaneko, Masashi*; et al.

Langmuir, 42(1), p.1613 - 1626, 2026/01

 Times Cited Count:0 Percentile:0.00(Chemistry, Multidisciplinary)

Understanding the structural factors governing the metal ions selectivity of solvent extraction systems is crucial for developing advanced processes for partitioning and transmutation of high-level radioactive waste. Here, we systematically investigated the effect of alkyl side-chain branching in nitrilotriacetamide (NTAamide) extractants on the extraction of lanthanum (La) and neodymium (Nd), chosen as representative lanthanides. Four extractants having each eight carbon atoms as one of the amide chains with identical molecular weights but different degrees of alkyl branching were examined. Distribution ratios were measured as a function of HNO$$_{3}$$ concentration, and the local coordination structures of La and Nd were analyzed by extended X-ray absorption fine structure (EXAFS), while supramolecular aggregation in the organic phase was characterized by small-angle neutron scattering (SANS). EXAFS analysis revealed that the inner-sphere coordination environment of La and Nd was essentially unaffected by the degree of alkyl branching. In contrast, SANS results showed that extractants with fewer branched alkyl groups formed larger aggregates at low HNO$$_{3}$$ concentrations, particularly in the case of Nd, where aggregation was found to facilitate extraction and prevent precipitation of poorly soluble complexes. These findings demonstrate that alkyl branching strongly influences supramolecular aggregation, which in turn governs extraction behavior. This work highlights the potential of nanoscale structural control as a new design concept for improving selectivity in lanthanide and actinide solvent extraction systems.

Journal Articles

Frustrated random-singlet state with ice-type structural fluctuation in spinel titanates

Hanasaki, Noriaki*; Hattori, Takayuki*; Komoda, Takumi*; Minamoto, Kakuei*; Torigoe, Shuhei*; Yamashita, Satoshi*; Nakazawa, Yasuhiro*; Nakano, Takehito*; Yoshimi, Kohei*; Yashima, Mitsuharu*; et al.

Proceedings of the National Academy of Sciences of the United States of America, 123(1), p.e2517926123_1 - e2517926123_6, 2026/01

 Times Cited Count:1 Percentile:82.83(Multidisciplinary Sciences)

Journal Articles

Effect of temperature on radiolytically generated hydrogen yield from actual nuclear fuel-derived solution

Toigawa, Tomohiro; Hotoku, Shinobu; Kumagai, Yuta; Abe, Yuma*; Oyama, Kanichi*; Fukaya, Hiroyuki; Tsubata, Yasuhiro; Ban, Yasutoshi; Kida, Takashi; Hasegawa, Satoshi*; et al.

Journal of Nuclear Science and Technology, 7 Pages, 2026/00

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

The effect of temperature on hydrogen generated from radiolysis was investigated to determine the safety implications in nuclear fuel reprocessing. Radiolytic hydrogen production poses a risk due to its flammability, especially when it accumulates in confined spaces without ventilation. Herein, generation of radiolytic hydrogen from an actual nuclear fuel-derived solution is investigated. Compared to previous studies using a plutonium nitric acid solution, this study evaluates radiolytic hydrogen yield under more realistic conditions, reflecting post-irradiation fuel composition. G-values of H$$_{2}$$ are determined at multiple temperatures, and the impact of alpha, beta, and gamma radiation doses is evaluated using PHITS-based simulations. Findings from this study confirmed a reduction in hydrogen yield due to scavenging effects of high-concentration nitric acid and metal ions dissolved in the solution, and temperature dependence appeared to be minor. A weak decreasing trend of G-values with temperature under agitated conditions might be related to hydrogen consumption by palladium species.

Journal Articles

Journal Articles

Progress in linac beam commissioning for high-intensity operations for J-PARC power upgrades

Liu, Y.*; Otani, Masashi*; Miyao, Tomoaki*; Nakazawa, Yuga*; Shibata, Takanori*; Nammo, Kesao*; Fang, Z.*; Futatsukawa, Kenta*; Fukui, Yuji*; Mizobata, Satoshi*; et al.

Proceedings of 16th International Particle Accelerator Conference (IPAC25) (Internet), p.855 - 857, 2025/11

JAEA Reports

Research plan on geosphere stability for long-term isolation of radioactive waste (Scientific program for fiscal year 2025)

Asamori, Koichi; Sueoka, Shigeru; Komatsu, Tetsuya; Ogata, Manabu; Uchida, Mao; Nishiyama, Nariaki; Tanaka, Kiriha; Kobayashi, Tomoharu; Mitsuguchi, Takehiro; Murakami, Osamu; et al.

JAEA-Review 2025-035, 29 Pages, 2025/10

JAEA-Review-2025-035.pdf:1.12MB

This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in Japan Atomic Energy Agency (JAEA), in fiscal year 2025. The objectives and contents of this research are described in detail based on the JAEA 4th Medium- and Long-term Plan (fiscal years 2022-2028). In addition, the background of this research is described from the necessity and the significance for site investigation and safety assessment, and the past progress. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques.

JAEA Reports

Annual report for research on geosphere stability for long-term isolation of radioactive waste in fiscal year 2024

Asamori, Koichi; Sueoka, Shigeru; Kobayashi, Tomoharu; Nishiyama, Nariaki; Tanaka, Kiriha; Murakami, Osamu; Fukuda, Shoma; Ogata, Manabu; Uchida, Mao; Komatsu, Tetsuya; et al.

JAEA-Research 2025-007, 99 Pages, 2025/10

JAEA-Research-2025-007.pdf:12.36MB

This annual report documents the progress of research and development (R&D) in the 3rd fiscal year of the JAEA 4th Medium- and Long-term Plan (fiscal years 2022-2028) to provide the scientific base for assessing geosphere stability for long-term isolation of high-level radioactive waste. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques. The current status of R&D activities with previous scientific and technological progress is summarized.

Journal Articles

On turbulence production in a jet passing through a grid-type obstacle; An LES approach

Abe, Satoshi; Hirose, Yoshiyasu; Shibamoto, Yasuteru

Results in Engineering (Internet), 27, p.106307_1 - 106307_16, 2025/09

The interaction of turbulent jets plays a critical role in heat and mass transfer across a variety of engineering applications. In particular, the merging phenomena of jets in nuclear reactors are important for validating the credibility of the core exit temperature (CET) as an indicator of core heat-up. CET serves as a key criterion for accident management and ensuring the safe operation of the reactor. Understanding the dynamics of these jet interactions is essential for improving reactor safety and efficiency. Furthermore, in the field of containment thermal hydraulics during severe accidents, the behavior of a jet interacting with a grid-type obstacle has attracted significant attention. This study utilized Large Eddy Simulation (LES) to gain a deeper understanding of the flow characteristics of a jet affected by such an obstacle, with particular focus on the turbulence production mechanism. To improve the accuracy of turbulence modeling, the Coherent Structure Smagorinsky Model (CSM) was employed. Validation against experimental data confirmed that LES is a valuable tool for investigating jet flow behavior. The vortex structure of the jet was visualized using the Q-criterion. Additionally, the impact of the grid-type obstacle on the turbulence kinetic energy production rate was analyzed through radial profiles at various locations and its cumulative production.

JAEA Reports

Compliance measures at the Radioactive Waste Treatment Facilities at the Nuclear Science Research Institute; Aseismic reinforcement of the Radioactive Waste Treatment Facility No. 3, Waste Size Reduction and Storage Facility, and Waste Volume Reduction Facility

Iketani, Shotaro; Suzuki, Takeshi; Yokobori, Tomohiko; Sugawara, Satoshi; Yokota, Akira; Kikuchi, Genta; Muraguchi, Yoshinori; Kitahara, Masaru; Seya, Manato; Kurosawa, Tsuyoshi; et al.

JAEA-Technology 2025-001, 169 Pages, 2025/08

JAEA-Technology-2025-001.pdf:14.22MB

The radioactive waste treatment facilities at the Nuclear Science Research Institute includes the Radioactive Waste Treatment Facility No. 3, Waste Size Reduction and Storage Facility, and Waste Volume Reduction Facility. These three facilities come under the purview of the Act on the Regulation of Nuclear Source Material, Nuclear Fuel Material and Reactors, and are included under Class C of the act based on the seismic requirements specified in the Act. We assessed the seismic capacity of these three radioactive waste treatment facilities based on the current Building Standards Act, to verify whether they comply with the new regulatory requirements enforced by the Nuclear Regulation Authority (NRA) in the aftermath of the 2011 nuclear accident at the Fukushima Daiichi Nuclear Power Station operated by the Tokyo Electric Power Company. We found that the allowable stress of a few structural members used in the construction of the facilities did not meet the regulatory requirements. After studying the approval granted by the NRA for the construction plans, including the design and construction methods (design and construction plans) of the three facilities on March 5, 2021, we made aseismic reinforcement at these facilities between 2021 and 2022. This report presents an overview of the seismic design of these facilities and an outline of the aseismic reinforcement conducted, management system existing, safety measures adopted, and the preoperational inspections conducted at these facilities.

Journal Articles

Validating terrestrial SER in 12-, 28-, and 65-nm SRAMs estimated by simulation coupled with one-time neutron irradiation

Takami, Kazusa*; Gomi, Yuibi*; Yasuda, Ryuichi*; Abe, Shinichiro; Ito, Masatoshi*; Kanda, Hiroki*; Fukuda, Mitsuhiro*; Hashimoto, Masanori*

IEEE Transactions on Nuclear Science, 72(8), p.2622 - 2628, 2025/08

 Times Cited Count:2 Percentile:73.73(Engineering, Electrical & Electronic)

Neutron-induced soft errors in the terrestrial environment pose reliability issues for semiconductor devices. We have developed the new method for estimating terrestrial SER based on simulation coupled with one-time irradiation using a conventional neutron source. This method has been validated using 65-nm planar SRAMs. However, with the ongoing progression of process shrinkage and the increasing adoption of devices fabricated with newer processes, there is a growing demand for further experimental validation of the terrestrial SER estimation method for these advanced processes. In this work, we validated the estimation method for 12-nm 1-fin FinFETs and 28-nm planer SRAMs. The SERs estimated by our method were consistent with the SERs measured using a white neutron beam at RCNP within 28% error.

Journal Articles

Revisiting hydrogen trapping in Mg$$_{32}$$(Al, Zn)$$_{49}$$ Approximant crystal; Influence of chemical disorder

Shimizu, Kazuyuki*; Yamaguchi, Masatake; Akamaru, Satoshi*; Nishimura, Katsuhiko*; Abe, Rion*; Sasaki, Taisuke*; Wang, Y.*; Toda, Hiroyuki*

Scripta Materialia, 265, p.116730_1 - 116730_7, 2025/08

 Times Cited Count:5 Percentile:73.85(Nanoscience & Nanotechnology)

Journal Articles

Seismic fragility evaluation of a thin-walled vessel in a sodium-cooled fast reactor

Watakabe, Tomoyoshi; Yamano, Hidemasa; Futagami, Satoshi

Transactions of the 28th International Conference on Structural Mechanics in Reactor Technology (SMiRT28) (Internet), 10 Pages, 2025/08

The fragility evaluation method of the RV in the SFR has been developed for both failure mode buckling and fatigue. The past studies showed the fragility using the RV of a loop-type SFR: radius R / thickness t is about 100. Recently, Japan Atomic Energy Agency together with Japanese industrial partners has been conducting a pool-type SFR design. The fragility of the pool-type RV has never been evaluated by the proposed method, which is based on the fatigue failure mode instead of the buckling. To investigate the basic behaviour of the pool-type RV under excessive seismic loading, this report investigated the fragility by using a simple cylindrical model with a wall thickness close to the design of the pool-type RV: R/t is 200, as the first trial.

Journal Articles

Non-condensable gas accumulation and distribution due to condensation in the CIGMA Facility; Implications for Fukushima Daiichi Unit 3 (1F3)

Hamdani, A.; Soma, Shu; Abe, Satoshi; Shibamoto, Yasuteru

Progress in Nuclear Energy, 185, p.105771_1 - 105771_13, 2025/07

 Times Cited Count:3 Percentile:85.00(Nuclear Science & Technology)

Journal Articles

Effects of inert gas addition on the characteristics of spherically expanding hydrogen-methane-air premixed flames in closed combustion vessels

Katsumi, Toshiyuki*; Zemba, Atsushi*; Kogishi, Makoto*; Iwanaga, Kohei*; Abe, Satoshi; Di$'e$vart, P.*; Chaumeix, N.*; Kadowaki, Satoshi*

Journal of Thermal Science and Technology (Internet), 20(1), p.25-00103_1 - 25-00103_13, 2025/06

 Times Cited Count:0 Percentile:0.00(Thermodynamics)

In the serious accident at Fukushima Daiichi Nuclear Power Station, the presence of steam together with flammable organic compounds affected the hydrogen explosion. To investigate the effects of addition of inert gas, i.e. steam or nitrogen, on the explosion characteristics, we conducted the experiments of spherically expanding hydrogen-methane-air premixed flames in closed combustion vessels. Two types of vessels were used, and expanding flames were caught by Schlieren method. The flame propagation velocity depending on the flame radius was obtained by analyzing Schlieren images. When the flame radius was sufficiently small, smooth surface was found. The addition of inert gas to hydrogen-methane-air premixtures caused the decrease of propagation velocity of unstretched flame. When the flame radius was large, on the other hand, cellular surface generated by intrinsic instability was found. In this range, the flame acceleration was confirmed, which was induced by the evolution of cellular surface. We obtained the parameters of flame acceleration model and predicted the flame propagation velocity depending on the flame radius. The increment coefficient normalized by the propagation velocity of unstretched flame became larger at low equivalence ratios, which was due to stronger diffusive-thermal instability. Under the same equivalence ratio, the inert gas addition caused the increase of normalized increment coefficient. This denoted that the inert gas addition promoted the instability of premixed flames, which was due to the reduction of the effective Lewis number. The maximum pressure in a combustion vessel became lower in the case of inert gas addition. Moreover, the maximum pressure of experiments was lower than that of calculations under the adiabatic conditions, because of heat loss during premixed combustion. The obtained results were valuable knowledge to elucidate the hydrogen explosion at Fukushima Daiichi Nuclear Power Station.

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