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Journal Articles

Electrochemical studies of uranium (IV) in an ionic liquid-DMF mixture to build a redox flow battery using uranium as an electrode active material

Ouchi, Kazuki; Komatsu, Atsushi; Takao, Koichiro*; Kitatsuji, Yoshihiro; Watanabe, Masayuki

Chemistry Letters, 50(6), p.1169 - 1172, 2021/06

 Times Cited Count:1 Percentile:6.77(Chemistry, Multidisciplinary)

The electrochemical behavior of uranium (IV) tetrachloride in ionic liquid-DMF mixture was studied for first time in order to build a redox flow battery (RFB) using U as an electrode active material. We found a quasi-reversible U$$^{III}$$/U$$^{IV}$$ couple that could be applied to the anode reaction of the RFB.

Journal Articles

Role of advection in atmospheric ammonia; A Case study at a Japanese lake basin influenced by agricultural ammonia sources

Kubota, Tomohiro; Kuroda, Hisao*; Watanabe, Mirai*; Takahashi, Akiko*; Nakazato, Ryoji*; Tarui, Mika*; Matsumoto, Shunichi*; Nakagawa, Keita*; Numata, Yasuko*; Ouchi, Takao*; et al.

Atmospheric Environment, 243, p.117856_1 - 117856_9, 2020/12

 Times Cited Count:3 Percentile:15.82(Environmental Sciences)

The dry and wet depositions of atmospheric ammonia (NH$$_{3}$$) is one of the important pathways of nitrogen loads to aquatic ecosystems. Crop and livestock agriculture, one of the largest emitters of NH$$_{3}$$ in Asian countries, are known to cause high spatial and seasonal variation of NH$$_{3}$$ and influence the surrounding lake basin areas via its dry and wet deposition. However, the spatial characteristics of the NH$$_{3}$$ concentration in basin scale are not completely understood for regulation in NH$$_{3}$$ emission. Here we aim to clarify dominant factors of spatial and seasonal variations of the NH$$_{3}$$ concentration in a eutrophic lake basin surrounded by agricultural areas in Japan. Passive sampling over various land use categories in the basin was conducted at 36 sites in total from October 2018 to January 2020. Interestingly, the observed NH$$_{3}$$ concentration near the livestock houses were higher in winter than summer, which was inconsistent with knowledge of seasonal changes of current NH$$_{3}$$ emission inventory based on temperature-driven volatilization process. Comparing monthly NH$$_{3}$$ concentrations with various meteorological factors, we suggested the importance of seasonal advection of NH$$_{3}$$ from high emission sources to which has been rarely paid attention by the previous past studies. As for this, should be considered for lake ecosystem management since deposition of NH$$_{3}$$ is known to be closely related to the ecological processes such as phytoplankton blooming.

Journal Articles

Investigation of removal factors of various materials inside houses after Nuclear Power Station Accident

Mori, Airi; Ishizaki, Azusa; Futemma, Akira; Tanabe, Tsutomu; Wada, Takao; Kato, Mitsugu; Munakata, Masahiro

Hoken Butsuri (Internet), 54(1), p.45 - 54, 2019/04

Journal Articles

Technical basis of accident tolerant fuel updated under a Japanese R&D project

Yamashita, Shinichiro; Nagase, Fumihisa; Kurata, Masaki; Nozawa, Takashi; Watanabe, Seiichi*; Kirimura, Kazuki*; Kakiuchi, Kazuo*; Kondo, Takao*; Sakamoto, Kan*; Kusagaya, Kazuyuki*; et al.

Proceedings of 2017 Water Reactor Fuel Performance Meeting (WRFPM 2017) (USB Flash Drive), 10 Pages, 2017/09

In Japan, the research and development (R&D) project on accident tolerant fuel and other components (ATFs) of light water reactors (LWRs) has been initiated in 2015 for establishing technical basis of ATFs. The Japan Atomic Energy Agency (JAEA) has coordinated and carried out this ATF R&D project in cooperation with power plant providers, fuel venders and universities for making the best use of the experiences, knowledges in commercial uses of zirconium-base alloys (Zircaloy) in LWRs. ATF candidate materials under consideration in the project are FeCrAl steel strengthened by dispersion of fine oxide particles(FeCrAl-ODS) and silicon carbide (SiC) composite, and are expecting to endure severe accident conditions in the reactor core for a longer period of time than the Zircaloy while maintaining or improving fuel performance during normal operations. In this paper, the progresses of the R&D project are reported.

Journal Articles

Improving the corrosion resistance of silicon carbide for fuel in BWR environments by using a metal coating

Ishibashi, Ryo*; Tanabe, Shigetada*; Kondo, Takao*; Yamashita, Shinichiro; Nagase, Fumihisa

Proceedings of 2017 Water Reactor Fuel Performance Meeting (WRFPM 2017) (USB Flash Drive), 10 Pages, 2017/09

For improving the corrosion resistance of silicon carbide (SiC) in boiling-water-reactor environments, corrosion-resistant coatings on SiC were evaluated. Due to its hydrogen-generation rate and reaction heat being lower than those of conventional Zircaloy, SiC is expected to be an appropriate material for accident-tolerant fuels. However, there are still many critical issues with the practical application of SiC fuel cladding and fuel channel boxes, one of which is hydrothermal corrosion. Silicon carbide is chemically stable, but silicon oxide formed by oxidation of SiC dissolves in high temperature water. Although the rate of SiC dissolution is very small, the dissolution must be suppressed to comply with regulations for dissolved silica concentration in reactor coolant. In this study, the corrosion behavior of candidate coatings for SiC substrates were evaluated before and after exposure to unirradiated high-purity-water environments.

Journal Articles

Probabilistic risk assessment method development for high temperature gas-cooled reactors, 1; Project overviews

Sato, Hiroyuki; Nishida, Akemi; Ohashi, Hirofumi; Muramatsu, Ken*; Muta, Hitoshi*; Itoi, Tatsuya*; Takada, Tsuyoshi*; Hida, Takenori*; Tanabe, Masayuki*; Yamamoto, Tsuyoshi*; et al.

Proceedings of 2017 International Congress on Advances in Nuclear Power Plants (ICAPP 2017) (CD-ROM), 7 Pages, 2017/04

JAEA, in conjunction with Tokyo City University, The University of Tokyo and JGC Corporation, have started development of a PRA method considering the safety and design features of HTGR. The primary objective of the project is to develop a seismic PRA method which enables to provide a reasonably complete identification of accident scenario including a loss of safety function in passive system, structure and components. In addition, we aim to develop a basis for guidance to implement the PRA. This paper provides the overview of the activities including development of a system analysis method for multiple failures, a component failure data using the operation and maintenance experience in the HTTR, seismic fragility evaluation method, and mechanistic source term evaluation method considering failures in core graphite components and reactor building.

Journal Articles

Probabilistic risk assessment method development for high temperature gas-cooled reactors, 2; Development of accident sequence analysis methodology

Matsuda, Kosuke*; Muramatsu, Ken*; Muta, Hitoshi*; Sato, Hiroyuki; Nishida, Akemi; Ohashi, Hirofumi; Itoi, Tatsuya*; Takada, Tsuyoshi*; Hida, Takenori*; Tanabe, Masayuki*; et al.

Proceedings of 2017 International Congress on Advances in Nuclear Power Plants (ICAPP 2017) (CD-ROM), 7 Pages, 2017/04

This paper proposes a set of procedures for accident sequence analysis in seismic PRAs of HTGRs that can consider the unique accident progression characteristics of HTGRs. Main features of our proposed procedure are as follows: (1) Systematic analysis techniques including Master Logic Diagrams are used to ensure reasonable completeness in identification of initiating events and classification of accident sequences, (2) Information on factors that govern the accident progression and source terms are effectively reflected to the construction of event trees for delineation of accident sequences, and (3) Frequency quantification of seismically-initiated accident sequence frequencies that involve multiplepipe ruptures are made with the use of the Direct Quantification of Fault Trees by Monte Carlo (DQFM) method by a computer code SECOM-DQFM.

JAEA Reports

Examination of decontamination of various materials at houses in difficult-to-return zone

Mori, Airi; Tanabe, Tsutomu; Wada, Takao; Kato, Mitsugu

JAEA-Technology 2017-006, 38 Pages, 2017/03

JAEA-Technology-2017-006.pdf:2.98MB

Large quantities of radioactive materials were released into the environment as a result of the Fukushima Daiichi Nuclear Power Station accident. Residential areas and forest areas near the power station were contaminated with the radioactive materials. Outside of the houses, schools and the other buildings are being decontaminated by national authority and local government. On the other hand, the materials (such as walls, floors, or windows) which constitute the houses are not decontaminated officially. In order to prepare decontamination methods that can be applied easily, we conducted examinations of decontamination for various materials in houses. Fibrous materials, woods, glasses, concretes, plastics, vinyl chloride materials, metals and synthetic leathers were used in our examinations. These materials were collected from houses in difficult-to-return zone, and were contaminated by radioactive materials released by the accident. Dry methods (suction, wiping, adsorption and peelable coating), wet methods (wiping, brushing, polishing and washing) and physical method (peeling of materials) were used for decontamination. As a result of our examinations, materials with low water permeability, such as glasses, concretes, vinyl chloride materials and metals, were able to be decontaminated efficiently (about 90% reduction) by using wet methods. Materials with high water permeability like woods were relatively well decontaminated by peelable coating (about 60%-70% reduction). In addition to the examination described above, the difference of contamination reduction effect between chemical properties of detergents and the effect of rubbing of peelable coating were also examined. Finally, the most effective method was summarized based on these examinations.

Journal Articles

Analysis on ex-vessel loss of coolant accident for a water-cooled fusion DEMO reactor

Watanabe, Kazuhito; Nakamura, Makoto; Tobita, Kenji; Someya, Yoji; Tanigawa, Hisashi; Uto, Hiroyasu; Sakamoto, Yoshiteru; Araki, Takao*; Asano, Shiro*; Asano, Kazuhito*

Proceedings of 26th IEEE Symposium on Fusion Engineering (SOFE 2015), 6 Pages, 2016/06

Safety studies of a water-cooled fusion DEMO reactor have been performed. In the event of the blanket cooling pipe break outside the vacuum vessel, i.e. ex-vacuum vessel loss of coolant accident (ex-VV LOCA), the pressurized steam and air may lead to damage reactor building walls which have confinement function, and to release the radioactive materials to the environment. In response to this accident, we proposed three cases of confinement strategies. In each case, the pressure and thermal loads to the confinement boundaries and total mass of tritium released to outside the boundaries were analyzed by accident analysis code MELCOR modified for fusion reactor. These analyses developed design parameters to maintain the integrity of the confinement boundaries.

JAEA Reports

Decontamination test of gravel; Establishment of effective decontamination methods about paving gravel and ballast

Kato, Mitsugu; Tanabe, Tsutomu; Umezawa, Katsuhiro; Wada, Takao

JAEA-Technology 2016-004, 129 Pages, 2016/03

JAEA-Technology-2016-004.pdf:20.42MB

After the Fukushima-Daiichi Nuclear Power Station accident, widespread contamination by radioactive materials occurred. Thus, decontamination work have been developed because of reducing air dose rate. Of this, in order to examine decontamination effect about gravel which cover sites of houses, communal facilities and cemeteries, and about ballast laid on a track, JAEA examined a decontamination test by physical plural methods. The objective of this testing is to establish rational and high effective decontamination methods to decontaminate each different gravel of materials and the shape, using the equipment which have possibility of the decontamination effect by trituration or blast. From the test results, applicability of the decontamination method depending on a characteristic of the gravel and the decontamination effect (reduction rate) are confirmed. There are various characteristics with the thing said to be gravel. It is confirmed that one decontamination method cannot be applied to all types of gravel. Furthermore, it is confirmed that there is great variability among individual polluted condition in the gravel gathered from the same place. Therefore, it is important to measure the degree of pollution so that a measurement error becomes as little as possible. For example, to measure plural points of the measurement side and keeping the height of measurement constant.

Journal Articles

Study of safety features and accident scenarios in a fusion DEMO reactor

Nakamura, Makoto; Tobita, Kenji; Gulden, W.*; Watanabe, Kazuhito*; Someya, Yoji; Tanigawa, Hisashi; Sakamoto, Yoshiteru; Araki, Takao*; Matsumiya, Hisato*; Ishii, Kyoko*; et al.

Fusion Engineering and Design, 89(9-10), p.2028 - 2032, 2014/10

 Times Cited Count:13 Percentile:70.2(Nuclear Science & Technology)

After the Fukushima Dai-ichi nuclear accident, a social need for assuring safety of fusion energy has grown gradually in the Japanese (JA) fusion research community. DEMO safety research has been launched as a part of BA DEMO Design Activities (BA-DDA). This paper reports progress in the fusion DEMO safety research conducted under BA-DDA. Safety requirements and evaluation guidelines have been, first of all, established based on those established in the Japanese ITER site invitation activities. The amounts of radioactive source terms and energies that can mobilize such source terms have been assessed for a reference DEMO, in which the blanket technology is based on the Japanese fusion technology R&D programme. Reference event sequences expected in DEMO have been analyzed based on the master logic diagram and functional FMEA techniques. Accident initiators of particular importance in DEMO have been selected based on the event sequence analysis.

Journal Articles

Key aspects of the safety study of a water-cooled fusion DEMO reactor

Nakamura, Makoto; Tobita, Kenji; Someya, Yoji; Tanigawa, Hisashi; Gulden, W.*; Sakamoto, Yoshiteru; Araki, Takao*; Watanabe, Kazuhito*; Matsumiya, Hisato*; Ishii, Kyoko*; et al.

Plasma and Fusion Research (Internet), 9, p.1405139_1 - 1405139_11, 2014/10

Key aspects of the safety study of a water-cooled fusion DEMO reactor is reported. Safety requirements, dose target, DEMO plant model and confinement strategy of the safety study are briefly introduced. The internal hazard of a water-cooled DEMO, i.e. radioactive inventories, stored energies that can mobilize these inventories and accident initiators and scenarios, are evaluated. It is pointed out that the enthalpy in the first wall/blanket cooling loops, the decay heat and the energy potentially released by the Be-steam chemical reaction are of special concern for the water-cooled DEMO. An ex-vessel loss-of-coolant of the first wall/blanket cooling loop is also quantitatively analyzed. The integrity of the building against the ex-VV LOCA is discussed.

Journal Articles

Carbon transport and fuel retention in JT-60U with higher temperature operation based on postmortem analysis

Yoshida, Masafumi; Tanabe, Tetsuo*; Adachi, Ayumu*; Hayashi, Takao; Nakano, Tomohide; Fukumoto, Masakatsu; Yagyu, Junichi; Miyo, Yasuhiko; Masaki, Kei; Itami, Kiyoshi

Journal of Nuclear Materials, 438, p.S1261 - S1265, 2013/07

 Times Cited Count:6 Percentile:44.02(Materials Science, Multidisciplinary)

Fuel retention rates and carbon re-deposition rates in the plasma shadowed areas in JT-60U were measured. Distributions of the fuel retention as well as the carbon re-deposition in the whole in-vessel of a large tokamak were clarified for the first time in the world. The fuel retention in the plasma shadowed areas was about two times larger than that in the carbon re-deposited layers on the plasma facing surface, although the amount of the carbon re-deposited on the plasma shadowed areas were about a half of that on the plasma facing surface, because of relatively lower temperature in the shadow areas causing higher hydrogen saturation concentration in the carbon re-deposited layers. The total fuel retention rate in JT-60U, including previously measured for all plasma facing areas, was evaluated to be 1.3$$times$$10$$^{20}$$ H+Ds$$^{-1}$$, which was lower than that in other devices, due to probably to higher temperature operation in JT-60U.

Journal Articles

Hydrogen isotopes retention in gaps at the JT-60U first wall tiles

Yoshida, Masafumi; Tanabe, Tetsuo*; Hayashi, Takao; Nakano, Tomohide; Fukumoto, Masakatsu; Yagyu, Junichi; Miyo, Yasuhiko; Masaki, Kei; Itami, Kiyoshi

Fusion Science and Technology, 63(1T), p.367 - 370, 2013/05

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

In this study, the retentions of hydrogen isotopes (H and D) in the gaps in JT-60U are clarified. Carbon tiles used in 1992-2004 were poloidally and toroidally taken out from outboard first wall in JT-60U to measure the retentions. The H and D retentions in the samples were measured by thermal desorption spectrometry (TDS). The H+D retention in the top side was higher than that of the bottom side, which might be due to thicker re-deposited carbon layers on the surface of the top side. The retentions in the surface of the side surfaces were slightly lower than that in the plasma facing surface where the retention was saturated to be 3-4e22 atoms/m$$^{2}$$. The retention rate was evaluated to be 3e17 H+D atoms/m$$^{2}$$/s from the measured retentions in two different discharge times by assuming the retention to increase linearly with the discharge time.

JAEA Reports

Experiment on evaluation of confinement capability of fuel cycle facility under combustion of glove-box and cable sheath materials (Contract research)

Abe, Hitoshi; Kashima, Takao; Uchiyama, Gunzo

JAEA-Research 2011-015, 27 Pages, 2011/06

JAEA-Research-2011-015.pdf:1.81MB

To contribute on confirmation of safety of fuel cycle facilities, evaluation method for soundness of confinement capability of the facilities under fire has been investigated. Panel materials of glove-box and cable sheath materials were considered to be an examination object as the representative organic materials in the facilities. Combustion property data, such as mass loss rate and soot generation ratio of the materials, and clogging property data of HEPA filter with combustion of the materials were measured as a parameter with radiation heat given to the materials, supply flow rate to the materials and oxygen concentration in the supply flow. Furthermore, progress of rising differential pressure of HEPA filter under hypothetical scenario of fire accident was evaluated quantitatively by applying these data mutually.

Journal Articles

Identified charged hadron production in $$p + p$$ collisions at $$sqrt{s}$$ = 200 and 62.4 GeV

Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Yasuyuki*; Al-Bataineh, H.*; Alexander, J.*; Aoki, Kazuya*; Aphecetche, L.*; Armendariz, R.*; et al.

Physical Review C, 83(6), p.064903_1 - 064903_29, 2011/06

 Times Cited Count:184 Percentile:99.44(Physics, Nuclear)

Transverse momentum distributions and yields for $$pi^{pm}, K^{pm}, p$$, and $$bar{p}$$ in $$p + p$$ collisions at $$sqrt{s}$$ = 200 and 62.4 GeV at midrapidity are measured by the PHENIX experiment at the RHIC. We present the inverse slope parameter, mean transverse momentum, and yield per unit rapidity at each energy, and compare them to other measurements at different $$sqrt{s}$$ collisions. We also present the scaling properties such as $$m_T$$ and $$x_T$$ scaling and discuss the mechanism of the particle production in $$p + p$$ collisions. The measured spectra are compared to next-to-leading order perturbative QCD calculations.

Journal Articles

Azimuthal correlations of electrons from heavy-flavor decay with hadrons in $$p+p$$ and Au+Au collisions at $$sqrt{s_{NN}}$$ = 200 GeV

Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Yasuyuki*; Al-Bataineh, H.*; Alexander, J.*; Aoki, Kazuya*; Aphecetche, L.*; Aramaki, Y.*; et al.

Physical Review C, 83(4), p.044912_1 - 044912_16, 2011/04

 Times Cited Count:8 Percentile:49.7(Physics, Nuclear)

Measurements of electrons from the decay of open-heavy-flavor mesons have shown that the yields are suppressed in Au+Au collisions compared to expectations from binary-scaled $$p+p$$ collisions. Here we extend these studies to two particle correlations where one particle is an electron from the decay of a heavy flavor meson and the other is a charged hadron from either the decay of the heavy meson or from jet fragmentation. These measurements provide more detailed information about the interaction between heavy quarks and the quark-gluon matter. We find the away-side-jet shape and yield to be modified in Au+Au collisions compared to $$p+p$$ collisions.

Journal Articles

Development and basic study for lesion size measuring system on an endoscopic image

Oka, Kiyoshi; Seki, Takeshi*; Naito, Takehito*; Watanabe, Shinya*; Wakabayashi, Takao*; Naganawa, Akihiro*; Inui, Kazuo*; Yoshino, Junji*

Nihon Gazo Igaku Zasshi, 28(1), p.12 - 24, 2010/05

Focusing on the measurement function loaded on our rigid-typed endoscope for the fetal surgery treatment, we proposed that its combination with a generally used digestive endoscope enabled calibration of lesion size in stomach. While adding the function, with which the target size is to be easily measured, on the endoscope, we simplified the system structure as much as possible. We also tried to minimize the total cost by using the generally used endoscope, instead of making it from scratch. Combining another development, the composite-type optical fiberscope with diameter of 1.1mm, with a generally used endoscope, we proposed the following as the features: (1)acquisition of fiberscope image, (2)laser irradiation for treatments, (3)applying the real time measurement function of distance and blood flow by semiconductor laser to the generally used endoscope. We have operated the clinical study to the gastric wall of person with no health problem, using this system and confirmed it was available for practical use.

Journal Articles

Development of an instrument system for measuring the internal pressure of the small intestine using an ileus tube

Ishikawa, Noriko; Oka, Kiyoshi; Naganawa, Akihiro*; Yoshino, Junji*; Wakabayashi, Takao*; Watanabe, Shinya*; Naito, Takehito*

Nihon Kikai Gakkai Rombunshu, C, 75(756), p.2359 - 2361, 2009/08

Instruments for measuring the internal pressure of digestive organs are used for diagnosing functional diseases, judging how critical the condition is, and deciding the treatment method or determining the degree of alleviation. However, the technique wherein the internal pressure of the small intestine is measured is highly invasive and painful for patients, and the insertion of the catheter via transducers is not preferred because it involves the insertion of an electric instrument in the body. In this study, we developed a system that measures the pressure of the small intestine with an ileus tube, which is generally used for the treatment of ileus. The main feature of our system is that can be used to measure internal pressure without the insertion of electric instruments such as transducers into the body, allowing the assessment of ileus without causing pain to the patient being treated. In this note, we present a brief description of the structure and function of this instrument used to measure the internal pressure of the small intestine.

Journal Articles

Hydrogen isotope retention in the outboard first wall tiles of JT-60U

Yoshida, Masafumi; Tanabe, Tetsuo*; Nobuta, Yuji*; Hayashi, Takao; Masaki, Kei; Sato, Masayasu

Journal of Nuclear Materials, 390-391, p.635 - 638, 2009/06

 Times Cited Count:9 Percentile:53.3(Materials Science, Multidisciplinary)

We have investigated hydrogen isotopes retention in the outboard first wall tiles of JT-60U by means of TDS, SIMS and SEM. The outboard first wall tiles of JT-60U are mostly eroded. The total retention (H+D) normalized by a unit area and integrated NBI time in the eroded first wall tiles and the eroded divertor tiles were nearly the same, in spite of the lower temperature of the first wall. Differently from divertor tiles, in which H retention was dominated owing to HH discharges preformed after DD discharges, deuterium is dominated in hydrogen isotopes retention and penetrates deeper from the surface. This is attributed to injection of high energy D and difficulty of isotopic replacement owing to their lower temperature. The integrated amount over the whole surface could be appreciably large. This type of hydrogen retention could be also possible for the metallic wall.

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