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Journal Articles

Implementation of ideal cascade model for uranium enrichment to nuclear fuel cycle simulator

Abe, Takumi; Suzuki, Taiga*; Okamura, Tomohiro*; Nakase, Masahiko*

Annals of Nuclear Energy, 232, p.112224_1 - 112224_7, 2026/07

 Times Cited Count:0

Journal Articles

Quantitative analysis of ionization quenching in CaF$$_2$$:Ce using PHITS track-structure simulations

Hirata, Yuho; Kai, Takeshi; Ogawa, Tatsuhiko; Matsuya, Yusuke; Sato, Tatsuhiko; Watanabe, Kenichi*; Kato, Takumi*; Kawaguchi, Noriaki*; Yanagida, Takayuki*

Radiation Measurements, 193, p.107651_1 - 107651_8, 2026/04

 Times Cited Count:0

CaF$$_2$$:Ce has a high potential to be used as a dosimeter due to its high optically stimulated luminescence (OSL) intensity. However, when phosphors such as CaF$$_2$$:Ce are irradiated with swift ions, the OSL intensity per dose decreases due to quenching effects. Traditionally, quenching effects in phosphors have been evaluated based on energy deposition density, using linear energy transfer (LET) as a metric. However, the relationship between quenching effects and LET varies with ion type, complicating unified evaluations. The track structure in PHITS can precisely simulate the radiation interactions. In this study, we simulated the detector response of CaF$$_2$$:Ce irradiated with swift-ions and compared these results with experimental data. The comparison suggests that the quantum yield of OSL is a critical parameter influencing the quenching effect in CaF$$_2$$:Ce. These findings are expected to contribute to the development of improved phosphor detectors.

JAEA Reports

Conceptual design of pilot ADS

Nishihara, Kenji; Fukushima, Masahiro; Abe, Takumi; Katano, Ryota; Yee-Rendon, B.; Iwamoto, Hiroki; Sugawara, Takanori; Obayashi, Hironari; Saito, Shigeru

JAEA-Research 2025-013, 125 Pages, 2026/03

JAEA-Research-2025-013.pdf:4.68MB

A conceptual design for a pilot Accelerator Driven subcritical System (ADS) was developed as a precursor to a commercial ADS aimed at partitioning and transmutation of minor actinides. The output of the pilot ADS was set at 200 MW. Based on safety assessment results, the design incorporates deep subcriticality and safety rods. Core design, accelerator design, target design, and in-vessel equipment design were performed, clarifying the specific concept.

Journal Articles

Frustrated random-singlet state with ice-type structural fluctuation in spinel titanates

Hanasaki, Noriaki*; Hattori, Takayuki*; Komoda, Takumi*; Minamoto, Kakuei*; Torigoe, Shuhei*; Yamashita, Satoshi*; Nakazawa, Yasuhiro*; Nakano, Takehito*; Yoshimi, Kohei*; Yashima, Mitsuharu*; et al.

Proceedings of the National Academy of Sciences of the United States of America, 123(1), p.e2517926123_1 - e2517926123_6, 2026/01

 Times Cited Count:1 Percentile:0.00(Multidisciplinary Sciences)

Journal Articles

Evaluation of Aluminum Hexacyanoferrate utilization for PGM and Mo removal from simulated high-level-raffinates in reprocessing for repository area minimization

Nakase, Masahiko*; Mishima, Ria; Abe, Takumi; Okamura, Tomohiro*; Asano, Hidekazu*

Annals of Nuclear Energy, 224, p.111569_1 - 111569_14, 2025/12

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

Impact of nuclear fuel cycle operation factor uncertainty on nuclear power plant operation

Abe, Takumi; Nishihara, Kenji

Progress in Nuclear Science and Technology (Internet), 8, p.47 - 51, 2025/09

Journal Articles

Impact of fast reactor fuel type on backend processes in the nuclear fuel cycle

Takeshita, Kenji*; Okamura, Tomohiro*; Nakase, Masahiko*; Abe, Takumi; Nishihara, Kenji

Progress in Nuclear Science and Technology (Internet), 8, p.52 - 57, 2025/09

Journal Articles

Initial benchmark comparison of the open-source Cyclus and NMB fuel cycle simulators

Bachmann, A. M.*; Nishihara, Kenji; Richards, S.*; Abe, Takumi; Feng, B.*

Progress in Nuclear Science and Technology (Internet), 8, p.11 - 16, 2025/09

JAEA Reports

Investigation of measurement accuracy of burnup reactivity of accelerator-driven system during normal operation

Katano, Ryota; Abe, Takumi; Cibert, H.*

JAEA-Research 2024-019, 22 Pages, 2025/05

JAEA-Research-2024-019.pdf:1.03MB

An accelerator-driven system (ADS) dedicated to transmutation of minor actinides (MAs) is driven in subcritical states. It is important for establishment of the subcriticality control of ADS to predict the burnup reactivity. To validate the prediction accuracy, the burnup reactivity, especially at the first cycle, must be measured with sufficient accuracy. In this study, we focus on Current-To-Flux (CTF) method. We have simulated the burnup reactivity monitoring during the ADS normal operation with the CTF method by performing fixed-source-burnup calculations using a continuous energy Monte Carlo code SERPENT2 with some tallies that models in-core fission chambers and have estimated its measurement uncertainty. We have clarified that the 10% biases of measure burnup reactivities appear independently of the burnup duration and their detector position dependence is particularly small in the outer region of the system.

Journal Articles

Achievements and status of the STRAD project for radioactive liquid waste management

Arai, Yoichi; Watanabe, So; Nakahara, Masaumi; Funakoshi, Tomomasa; Hoshino, Takanori; Takahatake, Yoko; Sakamoto, Atsushi; Aihara, Haruka; Hasegawa, Kenta; Yoshida, Toshiki; et al.

Progress in Nuclear Science and Technology (Internet), 7, p.168 - 174, 2025/03

The Japan Atomic Energy Agency (JAEA) has been conducting a project named "Systematic Treatment of RAdioactive liquid waste for Decommissioning (STRAD)" project since 2018 for fundamental and practical studies for treating radioactive liquid wastes with complicated compositions. Fundamental studies have been conducted using genuine liquid wastes accumulated in a hot laboratory of the JAEA called the Chemical Processing Facility (CPF), and treatment procedures for all liquid wastes in CPF were successfully designed on the results obtained. As the next phase of the project, new fundamental and practical studies on primarily organic liquid wastes accumulated in different facilities of JAEA are in progress. This paper reviews the representative achievements of the STRAD project and introduces an overview of ongoing studies.

Journal Articles

Scenario analysis of future nuclear energy use in Japan, 1; Methodology of nuclear fuel cycle simulator: NMB4.0

Abe, Takumi; Oizumi, Akito; Nishihara, Kenji; Nakase, Masahiko*; Asano, Hidekazu*; Takeshita, Kenji*

Progress in Nuclear Science and Technology (Internet), 7, p.299 - 304, 2025/03

Currently, much research continues on stable energy sources that do not emit CO$$_{2}$$ in order to achieve a carbon-neutral and sustainable society. Nuclear energy is one of the such sources, and various new reactors and reprocessing technologies are being developed. In order to implement the nuclear fuel cycle with these technologies, a nuclear fuel cycle simulator is required to quantitatively evaluate various quantities, such as the distribution of nuclear fuel materials and the scale of waste loading. For this purpose, NMB4.0 was developed in collaboration with Tokyo Institute of Technology and Japan Atomic Energy Agency. This code calculates the material balance of 179 nuclides including actinides and fission products (FPs) from the front-end to the back-end and simulates the nuclear fuel cycle in an integrated manner. Unlike other nuclear fuel cycle simulators, the code is capable of performing precise back-end analyses such as the number of radioactive wastes and the scale of the geological repository considering heat generation of waste package under diverse nuclear energy scenario, and is an open source code that runs on Microsoft Excel. By these features, it is possible to quantitatively study nuclear energy utilization strategies with various stakeholders. The presentation will detail the numerical model used in NMB4.0.

Journal Articles

Impact of metal fuel fast reactor cycle implementation on back-end system including final disposal

Takeshita, Kenji*; Okamura, Tomohiro*; Nakase, Masahiko*; Nishihara, Kenji; Abe, Takumi

Proceedings of International Conference on Nuclear Fuel Cycle (GLOBAL2024) (Internet), 2 Pages, 2024/10

Using the dynamic nuclear fuel cycle simulator NMB4.0, the mass balance analysis of the nuclear fuel cycle assuming the introduction of the metal fuel fast reactor in the second half of this century was evaluated. The impact of the introduction of the fast reactor cycle on the back-end including final disposal was discussed.

Journal Articles

The Impact of nuclear fuel cycle operation factor uncertainty on nuclear power plant operation

Abe, Takumi; Nishihara, Kenji

Proceedings of International Conference on Nuclear Fuel Cycle (GLOBAL2024) (Internet), 4 Pages, 2024/10

The robustness of whole of a nuclear fuel cycle (NFC) can be evaluated by a simulation of future operation factors (OFs) of the NFC facilities and mass flow analysis coupled with the simulated OF. In this study, the impact of a reprocessing plant OF on a fast reactor OF was quantified.

Journal Articles

Design policy of pilot plant for accelerator-driven system

Nishihara, Kenji; Sugawara, Takanori; Fukushima, Masahiro; Iwamoto, Hiroki; Katano, Ryota; Abe, Takumi

Proceedings of International Conference on Nuclear Fuel Cycle (GLOBAL2024) (Internet), 4 Pages, 2024/10

A pilot plant for the accelerator-driven system is proposed as a scaled-down version of a lead-bismuth cooled ADS with 800 MW thermal output for transmutation of minor actinides. In this presentation, the design policy of the pilot plant is presented.

Journal Articles

Initial verification of Cyclus and NMB fuel cycle simulators

Bachmann, A. M.*; Richards, S.*; Feng, B.*; Nishihara, Kenji; Abe, Takumi

Proceedings of International Conference on Nuclear Fuel Cycle (GLOBAL2024) (Internet), 4 Pages, 2024/10

This work demonstrates the value of code verification as an initial step in utilizing fuel cycle simulation. Cyclus and NMB are open-source fuel cycle simulators that provide computational modeling of nuclear fuel cycle alternatives and were chosen by Argonne National Laboratory and Japan Atomic Energy Agency (JAEA), respectively, for a multi-year collaboration on fuel cycle benchmarks. Both are relatively new and can be improved after conducting a rigorous code-to-code comparison. Initial verification of these simulators was performed using a set of hypothetical scenarios for once-through and multi-recycle fuel cycles. The results of this work identify how differences in scenario definitions and the modeling methodologies of the two simulators lead to differences in results in material inventories, mass flows, and other important metrics for fuel cycle assessments.

Journal Articles

Direct disposal concepts of spent mixed oxide fuel from light water reactors based on heat transfer calculations

Abe, Takumi; Nishihara, Kenji

Journal of Nuclear Science and Technology, 61(8), p.1048 - 1060, 2024/08

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Methods of direct disposal of mixed oxide spent fuel (MOXSF) consumed in light water reactors were investigated via heat transfer calculation. The temperature of the buffer material surrounding the waste is the most stringent limitation on the direct disposal of MOXSF. Therefore, the effects on the maximum temperature of the buffer material were examined by changing the occupied area, cooling term of MOXSF, and other parameters considering the direct disposal of uranium spent fuel. The results showed that it is necessary to change the cooling term and disposal depth in addition to the change of the occupied area. Accordingly, some disposal concepts that satisfy the limitation of the maximum buffer material temperature were derived, and estimates revealed that the occupied area per unit waste of the MOXSF is three to five times that of uranium spent fuel.

Journal Articles

A Science-based mixed oxide property model for developing advanced oxide nuclear fuels

Kato, Masato; Oki, Takumi; Watanabe, Masashi; Hirooka, Shun; Vauchy, R.; Ozawa, Takayuki; Uwaba, Tomoyuki; Ikusawa, Yoshihisa; Nakamura, Hiroki; Machida, Masahiko

Journal of the American Ceramic Society, 107(5), p.2998 - 3011, 2024/05

 Times Cited Count:8 Percentile:51.19(Materials Science, Ceramics)

Journal Articles

Magnetic structure and magnetoelectric properties of the spin-flop phase in LiFePO$$_{4}$$

Holm-Janas, S.*; Akaki, Mitsuru*; Fogh, E.*; Kihara, Takumi*; Le, M. D.*; Forino, P. C.*; Nikitin, S. E.*; Fennell, T.*; Painganoor, A.*; Vaknin, D.*; et al.

Physical Review B, 109(17), p.174413_1 - 174413_11, 2024/05

 Times Cited Count:6 Percentile:65.40(Materials Science, Multidisciplinary)

Journal Articles

Development of irradiation capsules with adjusting neutron spectrum

Fuyushima, Takumi; Takabe, Yugo; Sayato, Natsuki; Kimura, Akihiro; Takemoto, Noriyuki

The IV International Scientific Forum "Nuclear Science and Technologies"; AIP Conference Proceedings 3020, p.040007_1 - 040007_6, 2024/01

We studied irradiation tests of structural materials simulating fast reactor conditions in JMTR. We fabricated capsules that can simulate fast reactor irradiation in JMTR by using He/dpa ratio as index. To simulate fast reactor, cadmium, which shield thermal neutrons, was placed inside the capsule to adjust the neutron spectrum. According to the result of irradiation tests by neutron spectrum adjusting capsule, we confirmed that it can simulate the He/dpa ratio of fast reactor. Currently, since it is impossible to conduct irradiation tests in Japan, a plan is underway to partly replace the irradiation function of JMTR with overseas reactors. The alternative irradiation will be carried out by succeeding and developing the irradiation technology accumulated in the JMTR, and as a part of this, a trial of such irradiation in which the neutron spectrum is adjusted is under consideration.

Journal Articles

Eu(III) transfer in single $$N,N,N',N'$$-tetraoctyldiglycolamide-impregnated polymer-coated silica particle using fluorescence microspectroscopy; Transfer mechanism and effect of polymer crosslinking degree

Miyagawa, Akihisa*; Takahashi, Takumi*; Kuzure, Yoshiaki*; Iwamoto, Hibiki*; Arai, Tsuyoshi*; Nagatomo, Shigenori*; Watanabe, So; Sano, Yuichi; Nakatani, Kiyoharu*

Analytical Sciences, 39(11), p.1929 - 1936, 2023/11

 Times Cited Count:2 Percentile:5.68(Chemistry, Analytical)

In this study, we revealed the Eu(III) distribution in a single diglycolamide-derivative extractant (TODGA)-impregnated polymer-coated silica particle. The reaction of Eu(III) with two TODGA molecules in the polymer layer was the rate-limiting process, as evidenced by the absence of any correlation between the rate constants (k$$_{1}$$ and k$$_{-1}$$) and concentrations of Eu(III) and HNO$$_{3}$$.

106 (Records 1-20 displayed on this page)