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Journal Articles

Atomic distribution and local structure in ice VII from in situ neutron diffraction

Yamashita, Keishiro*; Komatsu, Kazuki*; Klotz, S.*; Fabelo, O.*; Fern$'a$ndez-D$'i$az, M. T.*; Abe, Jun*; Machida, Shinichi*; Hattori, Takanori; Irifune, Tetsuo*; Shimmei, Toru*; et al.

Proceedings of the National Academy of Sciences of the United States of America, 119(40), p.e2208717119_1 - e2208717119_6, 2022/10

 Times Cited Count:2 Percentile:22.35(Multidisciplinary Sciences)

Here we present the first elucidation of the disordered structure of ice VII, the dominant high-pressure form of water, at 2.2 GPa and 298 K from both single-crystal and powder neutron diffraction techniques. We reveal the three-dimensional atomic distributions from the maximum entropy method and unexpectedly find a ring-like distribution of hydrogen in contrast to the commonly-accepted discrete sites. In addition, total scattering analysis at 274 K clarified the difference in the intermolecular structure from ice VIII, the ordered counterpart of ice VII, despite an identical molecular geometry. Our complementary structure analyses robustly demonstrate the unique disordered structure of ice VII. Furthermore, these noble findings are related to the proton dynamics which drastically vary with pressure, and will contribute to an understanding of the structural origin of anomalous physical properties of ice VII under pressures.

Journal Articles

Odd-parity autoionizing levels of uranium observed by two-color two-step photoionization optogalvanic spectroscopy

Miyabe, Masabumi; Satou, Yukihiko; Wakaida, Ikuo; Terabayashi, Ryohei*; Sonnenschein, V.*; Tomita, Hideki*; Zhao, Y.*; Sakamoto, Tetsuo*

Journal of Physics B; Atomic, Molecular and Optical Physics, 54(14), p.145003_1 - 145003_8, 2021/07

 Times Cited Count:0 Percentile:0.01(Optics)

Two-color two-step photoionization optogalvanic spectroscopy was performed using high-repetition-rate titanium sapphire lasers and a uranium hollow cathode lamp to find the two-step resonance ionization schemes of uranium. Many ionization transitions were observed by exciting uranium atoms in a ground state into five, even parity, excited levels with the first-step laser and by scanning the second-step laser wavelengths. By blocking the first-step laser, single-color, two-photon ionization transitions were also identified. From these results, we have found more than 50 odd-parity autoionizing levels of uranium in the energy, ranging from the ionization potential (49958.4 cm$$^{-1}$$) to 51150 cm$$^{-1}$$. The determined energy levels are within 1 cm$$^{-1}$$ of previously reported values.

Journal Articles

How different is the core of $$^{25}$$F from $$^{24}$$O$$_{g.s.}$$ ?

Tang, T. L.*; Uesaka, Tomohiro*; Kawase, Shoichiro; Beaumel, D.*; Dozono, Masanori*; Fujii, Toshihiko*; Fukuda, Naoki*; Fukunaga, Taku*; Galindo-Uribarri, A.*; Hwang, S. H.*; et al.

Physical Review Letters, 124(21), p.212502_1 - 212502_6, 2020/05

 Times Cited Count:14 Percentile:74.18(Physics, Multidisciplinary)

The structure of a neutron-rich $$^{25}$$F nucleus is investigated by a quasifree ($$p,2p$$) knockout reaction. The sum of spectroscopic factors of $$pi 0d_{5/2}$$ orbital is found to be 1.0 $$pm$$ 0.3. The result shows that the $$^{24}$$O core of $$^{25}$$F nucleus significantly differs from a free $$^{24}$$O nucleus, and the core consists of $$sim$$35% $$^{24}$$O$$_{rm g.s.}$$, and $$sim$$65% excited $$^{24}$$O. The result shows that the $$^{24}$$O core of $$^{25}$$F nucleus significantly differs from a free $$^{24}$$O nucleus. The result may infer that the addition of the $$0d_{5/2}$$ proton considerably changes the neutron structure in $$^{25}$$F from that in $$^{24}$$O, which could be a possible mechanism responsible for the oxygen dripline anomaly.

JAEA Reports

A Study for a fire gas behavior by using a vertical shaft model (Contract research)

Abe, Hironobu; Hatakeyama, Nobuya; Yamazaki, Masanao; Okuzono, Akihiko*; Sakai, Tetsuo*; Inoue, Masahiro*

JAEA-Research 2009-019, 192 Pages, 2020/02

JAEA-Research-2009-019.pdf:8.07MB

Construction of the underground facility is on going at the Horonobe Underground Research Center, a division of the Japan Atomic Energy Agency. The facility is consisted of three shafts and horizontal drifts at the completion of construction and it is excavated in geological environment with methane gas, so it is important to secure the workers and visitors security in case of fire in the underground. However, it is known that the fire gas such as methane shows a complicated behavior by drift effect and so on and very difficult to predict its behavior, even if under enforced ventilation. In order to construct new prediction method of the fire gas behavior, the model scaled experiments were conducted by using the basic model which consists of shafts and drifts. As a results, fundamental data of the fire gas behavior was grasped and complicated behavior of the fire gas such as three-dimensional backflow and main flow inversion phenomena at the underground structure were ascertained. A new fire gas behavior analysis system has been designed and a prototype system has been programmed which is able to simulate the phenomena noted above. Coupling analysis method is adapted to the system, which consists of mainly one-dimensional ventilation network analysis and simplified computational fluid dynamics program named M-CFD. To minimize calculation time, M-CFD was designed as two-dimensional calculation with simulators multi area analysis system. Using the prototype system, several experimented models representing typical behavior of fire gas have been simulated for model scaled experiments. The system qualitatively reappeared the phenomena such as back flow or main flow inversion, and most of calculations completed in expected time. This indicates appropriateness of the prototype system, but some upgrade such as heat conductivity analysis in the wall rock mass transfer calculation, user friendly interface system and others will be required.

Journal Articles

In situ X-ray diffraction study of the oxide formed on alloy 600 in borated and lithiated high-temperature water

Watanabe, Masashi*; Yonezawa, Toshio*; Shobu, Takahisa; Shiro, Ayumi; Shoji, Tetsuo*

Corrosion, 72(9), p.1155 - 1169, 2016/09

 Times Cited Count:1 Percentile:6.28(Materials Science, Multidisciplinary)

Journal Articles

In situ X-ray diffraction measurement method for investigating the oxides films on austenitic stainless steel in simulated pressurized water reactor primary water

Watanabe, Masashi*; Yonezawa, Toshio*; Shobu, Takahisa; Shoji, Tetsuo*

Corrosion, 71(10), p.1224 - 1236, 2015/10

 Times Cited Count:3 Percentile:17.9(Materials Science, Multidisciplinary)

Journal Articles

Carbon transport and fuel retention in JT-60U with higher temperature operation based on postmortem analysis

Yoshida, Masafumi; Tanabe, Tetsuo*; Adachi, Ayumu*; Hayashi, Takao; Nakano, Tomohide; Fukumoto, Masakatsu; Yagyu, Junichi; Miyo, Yasuhiko; Masaki, Kei; Itami, Kiyoshi

Journal of Nuclear Materials, 438, p.S1261 - S1265, 2013/07

 Times Cited Count:6 Percentile:44.02(Materials Science, Multidisciplinary)

Fuel retention rates and carbon re-deposition rates in the plasma shadowed areas in JT-60U were measured. Distributions of the fuel retention as well as the carbon re-deposition in the whole in-vessel of a large tokamak were clarified for the first time in the world. The fuel retention in the plasma shadowed areas was about two times larger than that in the carbon re-deposited layers on the plasma facing surface, although the amount of the carbon re-deposited on the plasma shadowed areas were about a half of that on the plasma facing surface, because of relatively lower temperature in the shadow areas causing higher hydrogen saturation concentration in the carbon re-deposited layers. The total fuel retention rate in JT-60U, including previously measured for all plasma facing areas, was evaluated to be 1.3$$times$$10$$^{20}$$ H+Ds$$^{-1}$$, which was lower than that in other devices, due to probably to higher temperature operation in JT-60U.

Journal Articles

Hydrogen isotopes retention in gaps at the JT-60U first wall tiles

Yoshida, Masafumi; Tanabe, Tetsuo*; Hayashi, Takao; Nakano, Tomohide; Fukumoto, Masakatsu; Yagyu, Junichi; Miyo, Yasuhiko; Masaki, Kei; Itami, Kiyoshi

Fusion Science and Technology, 63(1T), p.367 - 370, 2013/05

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

In this study, the retentions of hydrogen isotopes (H and D) in the gaps in JT-60U are clarified. Carbon tiles used in 1992-2004 were poloidally and toroidally taken out from outboard first wall in JT-60U to measure the retentions. The H and D retentions in the samples were measured by thermal desorption spectrometry (TDS). The H+D retention in the top side was higher than that of the bottom side, which might be due to thicker re-deposited carbon layers on the surface of the top side. The retentions in the surface of the side surfaces were slightly lower than that in the plasma facing surface where the retention was saturated to be 3-4e22 atoms/m$$^{2}$$. The retention rate was evaluated to be 3e17 H+D atoms/m$$^{2}$$/s from the measured retentions in two different discharge times by assuming the retention to increase linearly with the discharge time.

Journal Articles

In-vessel tritium

Ueda, Yoshio*; Oya, Kaoru*; Ashikawa, Naoko*; Ito, Atsushi*; Ono, Tadayoshi*; Kato, Daiji*; Kawashima, Hisato; Kawamura, Gakushi*; Kenmotsu, Takahiro*; Saito, Seiki*; et al.

Purazuma, Kaku Yugo Gakkai-Shi, 88(9), p.484 - 502, 2012/09

no abstracts in English

Journal Articles

Application of tritium tracer techniques to observation of hydrogen on surface and in bulk of F82H

Otsuka, Teppei*; Tanabe, Tetsuo*; Tokunaga, Kazutoshi*; Yoshida, Naoaki*; Ezato, Koichiro; Suzuki, Satoshi; Akiba, Masato

Journal of Nuclear Materials, 417(1-3), p.1135 - 1138, 2011/10

 Times Cited Count:2 Percentile:18.29(Materials Science, Multidisciplinary)

Journal Articles

Effects of carbon impurity on deuterium retention in VPS-tungsten coatings exposed to JT-60U divertor plasmas

Fukumoto, Masakatsu; Nakano, Tomohide; Itami, Kiyoshi; Wada, Takaaki*; Ueda, Yoshio*; Tanabe, Tetsuo*

Journal of Nuclear Materials, 415(Suppl.1), p.S705 - S708, 2011/08

 Times Cited Count:5 Percentile:38.65(Materials Science, Multidisciplinary)

Tungsten coating on the first wall in ITER is proposed to reduce in-vessel tritium retention. However, it is possibility that carbon based materials would be used at high heat load components such as limiter. To predict the tritium retention in tungsten coating, it is essential to investigate the effects of carbon impurity on deuterium retention in tungsten coating. In this study, effects of carbon impurity on deuterium retention in the tungsten coating exposed to JT-60U divertor plasmas were investigated. Deuterium was trapped by carbon which was implanted and accumulated in the tungsten coating during the plasma discharge. D/C ration of 0.04-0.08 in the tungsten coating was reached to 1/2-1/4 compared to T/C ration in carbon co-deposition layer. Therefore, simultaneous use of carbon armor materials and tungsten coating would enhance tritium retention in tungsten coating.

Journal Articles

Study on effectiveness assessment of proliferation resistance

Kuno, Yusuke; Oda, Takuji*; Tanaka, Satoru*; Fukasawa, Tetsuo*; Tanabe, Tomoyuki*; Tamai, Hiroshi; Horio, Kenta*; Hamasaki, Manabu*; Shinohara, Nobuo*; Ikeda, Yuta*

Proceedings of INMM 52nd Annual Meeting (CD-ROM), 10 Pages, 2011/07

The substance and implication of PR from the viewpoints of risk evaluation on nuclear proliferation was studied in this paper. As an example, ten next-generation reprocessing technology candidates were evaluated with GIF PR and PP methodology to find degree of relative difference in PR from the presently available technology - PUREX. PR effectiveness in proliferation risk was also assessed and it was found that the effectiveness of PR measures is subject to the status of each nation.

Journal Articles

Report on ITPA meeting, 33

Asakura, Nobuyuki; Ashikawa, Naoko*; Ueda, Yoshio*; Ono, Noriyasu*; Tanabe, Tetsuo*; Nakano, Tomohide; Masuzaki, Suguru*; Itami, Kiyoshi; Kawano, Yasunori; Kawahata, Kazuo*; et al.

Purazuma, Kaku Yugo Gakkai-Shi, 87(7), p.485 - 486, 2011/07

no abstracts in English

Journal Articles

Deuterium retention in tungsten coating on the CFC tiles exposed to JT-60U divertor plasmas

Fukumoto, Masakatsu; Nakano, Tomohide; Masaki, Kei; Itami, Kiyoshi; Ueda, Yoshio*; Tanabe, Tetsuo*

Journal of Plasma and Fusion Research SERIES, Vol.9, p.369 - 374, 2010/08

no abstracts in English

Journal Articles

Recent progress in the energy recovery linac project in Japan

Sakanaka, Shogo*; Akemoto, Mitsuo*; Aoto, Tomohiro*; Arakawa, Dai*; Asaoka, Seiji*; Enomoto, Atsushi*; Fukuda, Shigeki*; Furukawa, Kazuro*; Furuya, Takaaki*; Haga, Kaiichi*; et al.

Proceedings of 1st International Particle Accelerator Conference (IPAC '10) (Internet), p.2338 - 2340, 2010/05

Future synchrotron light source using a 5-GeV energy recovery linac (ERL) is under proposal by our Japanese collaboration team, and we are conducting R&D efforts for that. We are developing high-brightness DC photocathode guns, two types of cryomodules for both injector and main superconducting (SC) linacs, and 1.3 GHz high CW-power RF sources. We are also constructing the Compact ERL (cERL) for demonstrating the recirculation of low-emittance, high-current beams using above-mentioned critical technologies.

Journal Articles

28th report on the ITPA (International Tokamak Physics Activity) meeting

Asakura, Nobuyuki; Nakano, Tomohide; Masuzaki, Takashi*; Ashikawa, Naoko*; Ueda, Yoshio*; Tanabe, Tetsuo*; Ono, Noriyasu*

Purazuma, Kaku Yugo Gakkai-Shi, 86(2), P. 124, 2010/02

no abstracts in English

Journal Articles

Experimental studies on in-vessel tritium inventory in complicated environment of fusion reactors

Ueda, Yoshio*; Hino, Tomoaki*; Ono, Noriyasu*; Takagi, Ikuji*; Nakano, Tomohide; Tanabe, Tetsuo*; Kajita, Shin*; Fukumoto, Masakatsu

Purazuma, Kaku Yugo Gakkai-Shi, 85(10), p.684 - 694, 2009/10

Relation between deuterium retention, wall temperature and hydrocarbon generation in 30-s H-mode discharges of JT-60U was described. In discharges with a density below 50% of the Greenwald density, the trend of the deuterium retention against pulse number depended on the wall temperature: with increasing pulse number, the deuterium retention decreased at a wall temperature of 300 $$^{circ}$$C, decreased gradually at 150 $$^{circ}$$C, and remained constant at 80 $$^{circ}$$C. In contrast, in discharges with high densities above 70% of the Greenwald density, the deuterium retention increased with increasing pulse number at the above three wall temperatures. In the high density discharges, the deuterium retention flux increased with increasing hydrocarbon generation flux, suggesting that the deuterium is retained in co-deposition layers of carbon, which originated from the hydrocarbons.

Journal Articles

Transport of heavy hydrocarbon and its redeposition on plasma facing walls

Oya, Kaoru*; Inai, Kensuke*; Kikuhara, Yasuyuki*; Nakano, Tomohide; Kawata, Jun*; Kawazome, Hayato*; Ueda, Yoshio*; Tanabe, Tetsuo*

Journal of Plasma and Fusion Research SERIES, Vol.8, p.419 - 424, 2009/09

Redeposition of C$$_{2}$$H$$_{4}$$ and C$$_{2}$$H$$_{6}$$ chemically eroded from carbon walls is simulated by EDDY code incorporated with the reflection on a hydrogenated and amorphized carbon surface. The redeposition rate for heavy hydrocarbons is drastically decreased by introduction of the reflection. The redeposition patterns on the surface are enlarged by the reflection, but it is narrower for the heavy hydrocarbons than for CH$$_{4}$$. The photon emissions of C$$_{2}$$ from C$$_{2}$$H$$_{4}$$ (C$$_{2}$$H$$_{6}$$) decay faster than that of CH from CH$$_{4}$$ in high-temperature ($$>$$10 eV) plasmas, which reproduces the difference of the decay of the CD and C$$_{2}$$ light intensities observed in the vicinity of the outer diverter plates of JT-60U. For such temperatures, the inverse photon-efficiency, which is defined as the ratio of the number of the launching hydrocarbons to the photoemission events of CH and C$$_{2}$$, is in good agreement with the values observed in JT-60U experiments.

JAEA Reports

Activity report for feasibility study on PKI authentication method with IC card in Authentication System Sub Group of J-PARC Information System Group

Teshima, Naoya; Aoyagi, Tetsuo; Hashimoto, Kiyoharu*; Manabe, Atsushi*; Yuasa, Fukuko*; Nakajima, Norihiro

JAEA-Data/Code 2009-004, 24 Pages, 2009/06

JAEA-Data-Code-2009-004.pdf:1.65MB

The authentication System Group of J-PARC Information System Group carried out the feasibility study about PKI authentication method that used IC card. Its purpose was that we validated its practical utility to choose an authentication method to adjust a security level desired at the information system of J-PARC. As a target of the feasibility studies, we chose following four validation items. (1) "The EAP-TLS wireless LAN authentication method" (2) "The Web-SSL client authentication method when accessed via SSL-VPN device" (3) "The PKI authentication method that used IC card stored the certificate which issued by NAREGI-CA software. (4) "The PKI authentication method that used Dual card type FeliCa". We established validation point for each validation item, and carried out it. So, we got the results and useful information. This report is that we organized a validation procedure, result and knowledge that we got by feasibility studies.

Journal Articles

Hydrogen isotope retention in the outboard first wall tiles of JT-60U

Yoshida, Masafumi; Tanabe, Tetsuo*; Nobuta, Yuji*; Hayashi, Takao; Masaki, Kei; Sato, Masayasu

Journal of Nuclear Materials, 390-391, p.635 - 638, 2009/06

 Times Cited Count:9 Percentile:53.3(Materials Science, Multidisciplinary)

We have investigated hydrogen isotopes retention in the outboard first wall tiles of JT-60U by means of TDS, SIMS and SEM. The outboard first wall tiles of JT-60U are mostly eroded. The total retention (H+D) normalized by a unit area and integrated NBI time in the eroded first wall tiles and the eroded divertor tiles were nearly the same, in spite of the lower temperature of the first wall. Differently from divertor tiles, in which H retention was dominated owing to HH discharges preformed after DD discharges, deuterium is dominated in hydrogen isotopes retention and penetrates deeper from the surface. This is attributed to injection of high energy D and difficulty of isotopic replacement owing to their lower temperature. The integrated amount over the whole surface could be appreciably large. This type of hydrogen retention could be also possible for the metallic wall.

186 (Records 1-20 displayed on this page)