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CoSiYamauchi, Hiroki; Sari, D. P.*; Yasui, Yukio*; Sakakura, Terutoshi*; Kimura, Hiroyuki*; Nakao, Akiko*; Ohara, Takashi; Honda, Takashi*; Kodama, Katsuaki; Igawa, Naoki; et al.
Physical Review Research (Internet), 6(1), p.013144_1 - 013144_9, 2024/02
Oikawa, Kenichi; Sato, Hirotaka*; Watanabe, Kenichi*; Su, Y. H.; Shinohara, Takenao; Kai, Tetsuya; Kiyanagi, Yoshiaki*; Hasemi, Hiroyuki
Journal of Physics; Conference Series, 2605, p.012013_1 - 012013_6, 2023/10
Tsuchikawa, Yusuke; Kai, Tetsuya; Abe, Yuta; Oikawa, Kenichi; Parker, J. D.*; Shinohara, Takenao; Sato, Ikken
Journal of Physics; Conference Series, 2605, p.012022_1 - 012022_6, 2023/10
We developed a method to obtain the areal density distribution of boron, which has a large neutron cross section, by means of an energy resolved neutron imaging. Commonly in a measurement of elements with very high neutron sensitivity, the quantitative measurement becomes more difficult with the amount of element due to the neutron self-shielding effect. To avoid this effect, an energy-resolved method using known cross section data was attempted, and a quantitative imaging of such elements was demonstrated at the MLF of J-PARC. This presentation introduces a measurement of melted simulated-fuel assemblies obtained in the research of the Fukushima Daiichi Nuclear Power Plant after the severe accident. Energy-dependent neutron transmission rates of the samples were measured by a neutron imaging detector, and were analyzed to obtained the areal density of boron at each position.
Nara, Fumiko*; Watanabe, Takahiro; Matsunaka, Tetsuya*; Yamasaki, Shinichi*; Tsuchiya, Noriyoshi*; Seto, Koji*; Yamada, Kazuyoshi*; Yasuda, Yoshinori*
Palaeogeography, Palaeoclimatology, Palaeoecology, 592, p.110907_1 - 110907_11, 2022/04
Times Cited Count：2 Percentile：28.09(Geography, Physical)Radiocarbon dating, tephrochronology, and geochemical signatures such as bromine (Br), iodine (I), total sulfur (TS), total organic carbon (TOC), and total nitrogen (TN) in a continuous sediment core (OG12-2) were applied to estimate past salinity change on the Lake Ogawara, Pacific coast of northeast Japan. Since the Lake Ogawara was the inner bay of the Pacific Ocean and became the brackish lake in the late Holocene, clarifying the past salinity change on the lake Ogawara could give us important insight into the past sea level changes of the Pacific Ocean. The core OG12-2 has two tephra layers, the Towada eruption and the Changbaishan eruption (B-Tm: AD 946). The age model for the core OG12-2 was established using the radiocarbon measurements of the plant residues in the core, also was constrained by the B-Tm tephra. Depletions of marine-derived elements (Br, I, and TS), from 88.4 to 64.2 mg/kg, 20.0 to 14.1 mg/kg, and 3.1 to 1.1 mass %, respectively, were observed in the layers with 2200-2000 cal BP. These results indicate paleosalinity changes from saline (inner bay) to brackish conditions within Lake Ogawara caused by sea level fluctuations during the late Holocene.
-violation studies on superheavy molecules; Theoretical and experimental perspectivesMitra, R.*; Prasannaa, V. S.*; Garcia Ruiz, R. F.*; Sato, Tetsuya; Abe, Minori*; Sakemi, Yasuhiro*; Das, B. P.*; Sahoo, B. K.*
Physical Review A, 104(6), p.062801_1 - 062801_9, 2021/12
Times Cited Count：2 Percentile：24.82(Optics)We provide detailed theoretical studies of quantities relevant to the electron electric dipole moment (eEDM) and nucleus-electron scalar-pseudoscalar interactions in diatomic molecules containing superheavy lawrencium nuclei. The sensitivity to parity and time (or, equivalently, ) reversal violating properties is studied for different neutral and ionic molecules. The effective electric fields in these systems are found to be about 3
4 times larger than other known molecules on which eEDM experiments are being performed. Similarly, these superheavy molecules exhibit an enhancement of more than 3 times for -violating scalar-pseudoscalar nucleus-electron interactions. Our preliminary analysis using the Woods-Saxon nuclear model also demonstrates that these results are sensitive to the diffuse surface interactions inside the Lr nucleus.
(001) surface using supersonic seeded oxygen molecular beamKatsube, Daiki*; Ono, Shinya*; Takayanagi, Shuhei*; Ojima, Shoki*; Maeda, Motoyasu*; Origuchi, Naoki*; Ogawa, Arata*; Ikeda, Natsuki*; Aoyagi, Yoshihide*; Kabutoya, Yuito*; et al.
Langmuir, 37(42), p.12313 - 12317, 2021/10
Times Cited Count：1 Percentile：6.77(Chemistry, Multidisciplinary)We investigated the oxidation of oxygen vacancies at the surface of anatase TiO(001) using supersonic seeded molecular beam (SSMB) of oxygen. The oxygen vacancies at the top-surface and sub-surface could be eliminated by the supply of oxygen using an SSMB. These results indicate that the interstitial vacancies can be mostly assigned to oxygen vacancies, which can be effectively eliminated by using an oxygen SSMB. Oxygen vacancies are present on the surface of anatase TiO(001) when it is untreated before transfer to a vacuum chamber. These vacancies, which are stable in the as-grown condition, could also be effectively eliminated using the oxygen SSMB.
Chiera, N. M.*; Sato, Tetsuya; Eichler, R.*; Tomitsuka, Tomohiro; Asai, Masato; Adachi, Sadia*; Dressler, R.*; Hirose, Kentaro; Inoue, Hiroki*; Ito, Yuta; et al.
Angewandte Chemie; International Edition, 60(33), p.17871 - 17874, 2021/08
Times Cited Count：2 Percentile：14.88(Chemistry, Multidisciplinary)The formation and the chemical characterization of single atoms of dubnium (Db, element 105), in the form of its volatile oxychloride, was investigated using the on-line gas phase chromatography technique, in the temperature range 350 - 600 
C. Under the exact same chemical conditions, comparative studies with the lighter homologs of group-5 in the Periodic Table clearly indicate the volatility sequence being NbOCl
TaOCl
DbOCl. From the obtained experimental results, thermochemical data for DbOCl were derived. The present study delivers reliable experimental information for theoretical calculations on the chemical properties of transactinides.
-P column by neutron resonance absorption imagingMiyazaki, Yasunori; Watanabe, So; Nakamura, Masahiro; Shibata, Atsuhiro; Nomura, Kazunori; Kai, Tetsuya; Parker, J. D.*
JPS Conference Proceedings (Internet), 33, p.011073_1 - 011073_7, 2021/03
Neutron resonance absorption imaging was adapted to observe the Eu band adsorbed in the CMPO/SiO-P column for minor actinide recovery by extraction chromatography. Several wet columns were prepared by either light water or heavy water and compared with the dry column to evaluate the neutron transmission. The neutron transmission spectra showed that 45% was transmitted through the dry column while 20% and 40% were transmitted through the wet columns of light water and heavy water, respectively. The results indicated that heavy water is more applicable than light water to observe the Eu adsorption band in the CMPO/SiO-P column.
Abe, Yuta; Tsuchikawa, Yusuke; Kai, Tetsuya; Matsumoto, Yoshihiro*; Parker, J. D.*; Shinohara, Takenao; Oishi, Yuji*; Kamiyama, Takashi*; Nagae, Yuji; Sato, Ikken
JPS Conference Proceedings (Internet), 33, p.011075_1 - 011075_6, 2021/03
Tsuchikawa, Yusuke; Abe, Yuta; Oishi, Yuji*; Kai, Tetsuya; Toh, Yosuke; Segawa, Mariko; Maeda, Makoto; Kimura, Atsushi; Nakamura, Shoji; Harada, Masahide; et al.
JPS Conference Proceedings (Internet), 33, p.011074_1 - 011074_6, 2021/03
In the decommissioning of the Fukushima-Daiichi (1F) Nuclear Power Plant, it is essential to understand characteristics of the melted core materials. The estimation of boride in the real debris is of great importance to develop safe debris removal plans. Hence, it is required to investigate the amount of boron in the melted core materials with nondestructive methods. Prompt gamma-ray activation analysis (PGAA) is one of the useful techniques to determine the amount of borides by means of the 478 keV prompt gamma-ray from neutron absorption reaction of boron. Moreover, it is well known that the width of the 478 keV gamma-ray peak is typically broadened due to the Doppler effect. The degree of the broadening is affected by coexisting materials, and can be recognized by the width of the prompt gamma-ray peak. As a feasibility study, the prompt gamma-ray from boride samples were measured using the ANNRI, NOBORU, and RADEN beamlines at the Materials and Life Science Experimental Facility (MLF) of Japan Proton Accelerator Complex (J-PARC).
Sakai, Kenji; Oi, Motoki; Haga, Katsuhiro; Kai, Tetsuya; Nakatani, Takeshi; Kobayashi, Yasuo*; Watanabe, Akihiko*
JPS Conference Proceedings (Internet), 33, p.011151_1 - 011151_6, 2021/03
For safely and efficiently operating a spallation neutron source and a muon target, a general control system (GCS) operates within Materials and Life Science Experimental Facility (MLF), GCS administers operation processes and interlocks of many instruments for various operation statuses. It consists of several subsystems such as an integral control system (ICS), interlock systems (ILS), shared servers, network system, and timing distribution system (TDS). Although GCS is an independent system that controls the target stations, it works closely with the control systems of other facilities in J-PARC. Since the first beam injection in 2008, GCS has operated stably without any serious troubles after modification based on commissioning for operation and control. Then, significant improvements in GCS such as upgrade of ICS by changing its framework software and function enhancement of ILS were proceeded until 2015, in considering sustainable long-term operation and maintenance. In recent years, many instruments in GCS have replaced due to end of production and support of them. In this way, many modifications have been proceeded in the entire GCS after start of beam operation. Under these situation, it is important to comprehend upgrade history and present status of GCS in order to decide its upgrade plan for the coming ten years. This report will mention upgrade history, present status and future agenda of GCS.
Tsuchikawa, Yusuke; Kai, Tetsuya; Abe, Yuta; Oishi, Yuji*; Sun, Y.*; Oikawa, Kenichi; Nakatani, Takeshi; Sato, Ikken
Nuclear Instruments and Methods in Physics Research A, 991, p.164964_1 - 164964_5, 2021/03
Times Cited Count：1 Percentile：18.91(Instruments & Instrumentation)Peak shape analysis was performed for the energy spectra of Doppler-broadened prompt 
-rays generated by neutron capture reactions with various boride or boron samples. Significant differences were observed between nonmetallic and metallic borides. Minor differences between the peak shapes of prompt -rays from zirconium- and ferro-borons were evaluated by a peak fitting method. The identification of zirconium- and ferro-borons and other types of borides was estimated.
) reaction at 12, 20, and 30 MeVPatwary, M. K. A*; Kin, Tadahiro*; Aoki, Katsumi*; Yoshinami, Kosuke*; Yamaguchi, Masaya*; Watanabe, Yukinobu*; Tsukada, Kazuaki; Sato, Nozomi*; Asai, Masato; Sato, Tetsuya; et al.
Journal of Nuclear Science and Technology, 58(2), p.252 - 258, 2021/02
Times Cited Count：0 Percentile：0.01(Nuclear Science & Technology)While designing deuteron accelerator neutron sources for radioisotopes production, nuclear data for light elements such as Li, Be, and C have been systematically measured in the deuteron energy range from a few MeV to around 50 MeV. Currently, the experimental data available on double-differential thick-target neutron yields (DDTTNYs) is insufficient, especially for deuteron energies between 18 and 33 MeV. In this study, we measured the DDTTNYs of () reactions on 
C target for incident deuteron energies of 12, 20, and 30 MeV using the multiple-foils activation method to improve nuclear data insufficiency. We applied the GRAVEL code for the unfolding process to derive the DDTTNYs. The results were compared with the calculation by DEURACS. The present data were also used to confirm the systematics of the differential neutron yields at 0
and total neutron yield per incident deuteron in the wide range of deuteron energy.
Watanabe, Takahiro; Ishii, Chikako; Ishizaka, Chika; Niwa, Masakazu; Shimada, Koji; Sawai, Yuki*; Tsuchiya, Noriyoshi*; Matsunaka, Tetsuya*; Ochiai, Shinya*; Nara, Fumiko*
Journal of Mineralogical and Petrological Sciences, 116(3), p.140 - 158, 2021/00
Times Cited Count：5 Percentile：51.59(Mineralogy)A portable energy dispersive X-ray fluorescence spectrometer (potable XRF) can be an effective tool for detecting chemical elements in various materials, such as geological, and environmental samples. In this study, working curves were confirmed using reference materials, such as igneous rocks and other geochemical standards, distributed by national and international organizations. Subsequently, quantification and semi-quantification analyses were performed by the portable XRF for inorganic elements in (A) fault rocks, (B) lake sediments from the middle Japan, and (C) soils with paleotsunami deposits from the Pacific coast of northeast Japan. Twenty-four elements (Mg-U) in these geological samples were measured by potable XRF using our working curves. Measured values by the portable XRF of the samples were good agreement with the reported values in almost cases.
Ishimaru, Tsuneari; Ogata, Nobuhisa; Kokubu, Yoko; Shimada, Koji; Hanamuro, Takahiro; Shimada, Akiomi; Niwa, Masakazu; Asamori, Koichi; Watanabe, Takahiro; Sueoka, Shigeru; et al.
JAEA-Research 2020-011, 67 Pages, 2020/10
JAEA-Research-2020-011.pdf:3.87MB
This annual report documents the progress of research and development (R&D) in the 5th fiscal year during the JAEA 3rd Mid- and Long-term Plan (fiscal years 2015-2021) to provide the scientific base for assessing geosphere stability for long-term isolation of the high-level radioactive waste. The planned framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques. The current status of R&D activities with previous scientific and technological progress is summarized.
AlGaO
scintillators by gamma-ray-induced positron annihilation lifetime spectroscopyFujimori, Kosuke*; Kitaura, Mamoru*; Taira, Yoshitaka*; Fujimoto, Masaki*; Zen, H.*; Watanabe, Shinta*; Kamada, Kei*; Okano, Yasuaki*; Kato, Masahiro*; Hosaka, Masahito*; et al.
Applied Physics Express, 13(8), p.085505_1 - 085505_4, 2020/08
Times Cited Count：5 Percentile：33.01(Physics, Applied)To clarify the existence of cation vacancies in Ce-doped GdAlGaO (Ce:GAGG) scintillators, we performed gamma-ray-induced positron annihilation lifetime spectroscopy (GiPALS). GiPAL spectra of GAGG and Ce:GAGG comprised two exponential decay components, which were assigned to positron annihilation at bulk and defect states. By an analogy with Ce:YAl
O, the defect-related component was attributed to Al/Ga-O divacancy complexes. This component was weaker for Ce, Mg:GAGG, which correlated with the suppression of shallow electron traps responsible for phosphorescence. Oxygen vacancies were charge compensators for Al/Ga vacancies. The lifetime of the defect-related component was significantly changed by Mg co-doping. This was understood by considering aggregates of Mg
ions at Al/Ga sites with oxygen vacancies, which resulted in the formation of vacancy clusters.
Abe, Yuta; Tsuchikawa, Yusuke; Kai, Tetsuya; Matsumoto, Yoshihiro*; Parker, J. D.*; Shinohara, Takenao; Oishi, Yuji*; Kamiyama, Takashi*; Nagae, Yuji; Sato, Ikken
Proceedings of 2020 International Conference on Nuclear Engineering (ICONE 2020) (Internet), 6 Pages, 2020/08
Ishimaru, Tsuneari; Ogata, Nobuhisa; Shimada, Koji; Kokubu, Yoko; Niwa, Masakazu; Asamori, Koichi; Watanabe, Takahiro; Sueoka, Shigeru; Komatsu, Tetsuya; Yokoyama, Tatsunori; et al.
JAEA-Review 2020-010, 46 Pages, 2020/07
JAEA-Review-2020-010.pdf:1.89MB
This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in Japan Atomic Energy Agency (JAEA), in fiscal year 2020. The objectives and contents in fiscal year 2020 are described in detail based on the JAEA 3rd Medium- and Long-term Plan (fiscal years 2015-2021). In addition, the background of this research is described from the necessity and the significance for site investigation and safety assessment, and the past progress. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques.
Oikawa, Kenichi; Kiyanagi, Yoshiaki*; Sato, Hirotaka*; Omae, Kazuma*; Pham, A.*; Watanabe, Kenichi*; Matsumoto, Yoshihiro*; Shinohara, Takenao; Kai, Tetsuya; Harjo, S.; et al.
Materials Research Proceedings, Vol.15, p.207 - 213, 2020/02
Ishimaru, Tsuneari; Ogata, Nobuhisa; Hanamuro, Takahiro; Shimada, Akiomi; Kokubu, Yoko; Asamori, Koichi; Niwa, Masakazu; Shimada, Koji; Watanabe, Takahiro; Saiga, Atsushi; et al.
JAEA-Research 2019-006, 66 Pages, 2019/11
JAEA-Research-2019-006.pdf:4.39MB
This annual report documents the progress of research and development (R&D) in the 4th fiscal year during the JAEA 3rd Mid- and Long-term Plan (fiscal years 2015-2021) to provide the scientific base for assessing geosphere stability for long-term isolation of the high-level radioactive waste. The planned framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques. In this report, the current status of R&D activities with previous scientific and technological progress is summarized.
