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Journal Articles

Modernization of the DCHAIN-PHITS activation code with new features and updated data libraries

Ratliff, H.; Matsuda, Norihiro; Abe, Shinichiro; Miura, Takamitsu*; Furuta, Takuya; Iwamoto, Yosuke; Sato, Tatsuhiko

Nuclear Instruments and Methods in Physics Research B, 484, p.29 - 41, 2020/12

Journal Articles

Study of the Li($$d,xn$$) reaction for the development of accelerator-based neutron sources

Watanabe, Yukinobu*; Sadamatsu, Hiroki*; Araki, Shohei*; Nakano, Keita*; Kawase, Shoichiro*; Kin, Tadahiro*; Iwamoto, Yosuke; Satoh, Daiki; Hagiwara, Masayuki*; Yashima, Hiroshi*; et al.

EPJ Web of Conferences, 239, p.20012_1 - 20012_4, 2020/09

Accelerator-based neutron sources induced by deuteron beams are attractive for study of nuclear transmutation of radioactive waste as well as radiation damage for fusion reactor materials. In the present work, we have carried out a Double Differential cross section (DDX) measurement for Li at 200 MeV in the Research Center for Nuclear Physics (RCNP), Osaka University. A deuteron beam accelerated to 200 MeV was transported to the neutron experimental hall and focused on a thin Li target. Emitted neutrons from the target were detected by two different-size EJ301 liquid organic scintillators located at two distances of 7 m and 20 m, respectively. The neutron DDXs were measured at six angles from 0$$^{circ}$$ to 25$$^{circ}$$). The neutron detection efficiencies of the detectors were calculated by SCINFUL-QMD code. We will present the results of the present DDX measurement and compare them with theoretical model calculations with DEURACS and PHITS.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2018

Nakano, Masanao; Fujii, Tomoko; Nemoto, Masashi; Tobita, Keiji; Kono, Takahiko; Hosomi, Kenji; Nishimura, Shusaku; Matsubara, Natsumi; Maehara, Yushi; Narita, Ryosuke; et al.

JAEA-Review 2019-048, 165 Pages, 2020/03

JAEA-Review-2019-048.pdf:2.69MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2018 to March 2019. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Co., Inc. (the trade name was changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016) in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and exceeded the normal range of fluctuation in the monitoring, were evaluated.

Journal Articles

Effects of one-dimensional migration of self-interstitial atom clusters on the decreasing behaviour of their number density in electron-irradiated $$alpha$$-iron

Abe, Yosuke; Sato, Yuki*; Hashimoto, Naoyuki*; Onuki, Somei*

Philosophical Magazine, 100(1), p.110 - 125, 2020/00

 Times Cited Count:0 Percentile:100(Materials Science, Multidisciplinary)

We derive analytical models associated with the experimentally revealed one-dimensional (1D) migration mechanisms to examine the decreasing behavior of the cluster number density. The model calculation indicates that the detrapping of the stationary SIA clusters causes the surface annihilation of the liberated SIA clusters, leading to the decrease in their number density. The decreasing behavior is in closer accordance with the experimental data when setting the impurity concentration in the same order as the estimation from the previous in situ HVEM experiment. This result suggests that the trapping and detrapping of the SIA clusters are the possible underlying processes for the decreasing behavior.

Journal Articles

Enhancement of element production by incomplete fusion reaction with weakly bound deuteron

Wang, H.*; Otsu, Hideaki*; Chiga, Nobuyuki*; Kawase, Shoichiro*; Takeuchi, Satoshi*; Sumikama, Toshiyuki*; Koyama, Shumpei*; Sakurai, Hiroyoshi*; Watanabe, Yukinobu*; Nakayama, Shinsuke; et al.

Communications Physics (Internet), 2(1), p.78_1 - 78_6, 2019/07

 Times Cited Count:4 Percentile:25.43(Physics, Multidisciplinary)

Searching for effective pathways for the production of proton- and neutron-rich isotopes through an optimal combination of reaction mechanism and energy is one of the main driving forces behind experimental and theoretical nuclear reaction studies as well as for practical applications in nuclear transmutation of radioactive waste. We report on a study on incomplete fusion induced by deuteron, which contains one proton and one neutron with a weak binding energy and is easily broken up. This reaction study was achieved by measuring directly the cross sections for both proton and deuteron for $$^{107}$$Pd at 50 MeV/u via inverse kinematics technique. The results provide direct experimental evidence for the onset of a cross-section enhancement at high energy, indicating the potential of incomplete fusion induced by loosely-bound nuclei for creating proton-rich isotopes and nuclear transmutation of radioactive waste.

Journal Articles

Micro-PIXE analysis study of ferrite products synthesized from simulated radioactive liquid waste containing chemical hazardous elements

Abe, Tomohisa; Shimazaki, Takejiro; Osugi, Takeshi; Nakazawa, Osamu; Yamada, Naoto*; Yuri, Yosuke*; Sato, Takahiro*

QST-M-16; QST Takasaki Annual Report 2017, P. 140, 2019/03

no abstracts in English

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2017

Nakano, Masanao; Fujita, Hiroki; Mizutani, Tomoko; Nemoto, Masashi; Tobita, Keiji; Kono, Takahiko; Hosomi, Kenji; Hokama, Tomonori; Nishimura, Tomohiro; Matsubara, Natsumi; et al.

JAEA-Review 2018-025, 171 Pages, 2019/02

JAEA-Review-2018-025.pdf:3.81MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2016 to March 2017. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Electric Power Company Holdings, Inc. in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and were exceeded the normal range of fluctuation in the monitoring, were evaluated.

Journal Articles

Quantum magnetisms in uniform triangular lattices Li$$_{2}$$$$A$$Mo$$_{3}$$O$$_{8}$$ ($$A$$ = In, Sc)

Iida, Kazuki*; Yoshida, Hiroyuki*; Okabe, Hirotaka*; Katayama, Naoyuki*; Ishii, Yuto*; Koda, Akihiro*; Inamura, Yasuhiro; Murai, Naoki; Ishikado, Motoyuki*; Kadono, Ryosuke*; et al.

Scientific Reports (Internet), 9(1), p.1826_1 - 1826_9, 2019/02

 Times Cited Count:1 Percentile:65.14(Multidisciplinary Sciences)

Journal Articles

Establishment of a novel detection system for measuring primary knock-on atoms

Tsai, P.-E.; Iwamoto, Yosuke; Hagiwara, Masayuki*; Sato, Tatsuhiko; Ogawa, Tatsuhiko; Satoh, Daiki; Abe, Shinichiro; Ito, Masatoshi*; Watabe, Hiroshi*

Proceedings of 2017 IEEE Nuclear Science Symposium and Medical Imaging Conference (NSS/MIC 2017) (Internet), 3 Pages, 2018/11

The energy spectra of primary knock-on atoms (PKAs) are essential for radiation damage assessment in design of accelerator facilities. However up to date the experimental data are still limited, due to the poor mass resolution and the high measurement threshold energies in the conventional setup of nuclear physics experiments using solid state detectors, which are typically above a few MeV/nucleon. In this study, a novel detection system consisting of two time detectors and one dE-E energy detector is proposed and being constructed to measure the PKA spectra. The system and detector design was based on Monte Carlo simulations by using the PHITS code. The PHITS simulations show that the system is able to distinguish the PKA isotopes above $$sim$$0.2-0.3 MeV/nucleon for A=20$$sim$$30 amu; the PKA mass identification thresholds decrease to $$<$$0.1 MeV/nucleon for PKAs lighter than 20 amu. The detection system will be tested in the summer of 2017, and the test results will be presented at the conference.

Journal Articles

Effect of the headgroup structure on counterion binding in adsorbed surfactant films investigated by total reflection X-ray absorption fine structure spectroscopy

Imai, Yosuke*; Tokiwa, Yuhei*; Ueno, Shusaku*; Tanida, Hajime; Watanabe, Iwao*; Matsubara, Hiroki*; Takiue, Takanori*; Aratono, Makoto*

Bulletin of the Chemical Society of Japan, 91(10), p.1487 - 1494, 2018/10

 Times Cited Count:0 Percentile:100(Chemistry, Multidisciplinary)

Competitive binding of binary mixed counterions to the headgroups of adsorbed surfactant films has been investigated at solution surfaces by total reflection X-ray absorption fine structure (XAFS) spectroscopy. The obtained extended XAFS $$chi$$ spectra for bromide counterions are linear combinations of the spectra of fully hydrated bromide ions (free Br) and partially dehydrated bromide ions bound to the headgroups of the surfactant ions (bound Br). From the fraction of bound Br in counterion mixed systems, two series of the relative strengths of counterion binding are proposed for the trimethylammonium (TA$$^{+}$$) and 3-methylimidazolium (MIM$$^{+}$$) headgroups: (a) TA-SO$$_{4}$$ $$<$$ TA-Cl $$<$$ TA-Br $$<$$ TA-BF$$_{4}$$ and (b) MIM-Br $$<$$ TA-Br $$<$$ TA-BF$$_{4}$$ $$<$$ MIM-BF$$_{4}$$. For the TA headgroup, matching the hydration of the headgroups and counterions gives series (a) according to Collins' law, which states that the tendency of contact ion pair formation becomes larger when the absolute values of the hydration enthalpies of the ions match. For the MIM headgroup, the number of binding sites of hydrogen bonds between the MIM headgroup and counterion is essential, which leads to series (b) because of competition between the counterion and water for interaction with the MIM headgroup.

Journal Articles

Features of particle and heavy ion transport code system (PHITS) version 3.02

Sato, Tatsuhiko; Iwamoto, Yosuke; Hashimoto, Shintaro; Ogawa, Tatsuhiko; Furuta, Takuya; Abe, Shinichiro; Kai, Takeshi; Tsai, P.-E.; Matsuda, Norihiro; Iwase, Hiroshi*; et al.

Journal of Nuclear Science and Technology, 55(6), p.684 - 690, 2018/06

 Times Cited Count:200 Percentile:0.01(Nuclear Science & Technology)

We have upgraded many features of the Particle and Heavy Ion Transport code System (PHITS) and released the new version as PHITS3.02. The accuracy and the applicable energy ranges of the code were greatly improved and extended, respectively, owing to the revisions to the nuclear reaction models and the incorporation of new atomic interaction models. In addition, several user-supportive functions were developed, such as new tallies to efficiently obtain statistically better results, radioisotope source-generation function, and software tools useful for applying PHITS to medical physics. In this paper, we summarize the basic features of PHITS3.02, especially those of the physics models and the functions implemented after the release of PHITS2.52 in 2013.

Journal Articles

2018 Annual Meeting of Japan Atomic Energy Society, Joint Session of Nuclear Data Subcommittee and Sigma Special Advisory Committee; Present status and future of nuclear data evaluation code in Japan, 4; Role and improvement of nuclear reaction models in the PHITS code

Hashimoto, Shintaro; Sato, Tatsuhiko; Iwamoto, Yosuke; Ogawa, Tatsuhiko; Furuta, Takuya; Abe, Shinichiro; Niita, Koji*

Kaku Deta Nyusu (Internet), (120), p.26 - 34, 2018/06

Particle and heavy-ion transport code system PHITS has been used for calculations of radiation shielding in accelerator facilities. PHITS describes physical phenomena induced by radiation as combination of transport and collision processes. The collision process including nuclear reactions is simulated by the three-step calculation: a generation of a reaction, pre-equilibrium, and compound processes. In the simulation, many physics models are used. This report explains roles of the models in PHITS and shows their developments we recently performed.

Journal Articles

Recontamination prevention technologies to prevent radioactive cesium from its runoff from not decontaminated forests to living areas

Nagasu, Ryosuke*; Tanabe, Daijiro*; Yokotsuka, Satoshi*; Kumazawa, Noriyuki*; Ajiki, Takaya*; Aizawa, Yusuke*; Naganawa, Hirochika; Nagano, Tetsushi; Yanase, Nobuyuki*; Mitamura, Hisayoshi*; et al.

Kankyo Joka Gijutsu, 17(2), p.58 - 61, 2018/03

A new technology to suppress cesium migration from forests has been developed collaboratively by Ibaraki University, Kumagai-gumi Co., Ltd. and its group company, Technos, and JAEA. The new technology utilizes polyelectrolytes (polymers with electric charges) and clay minerals to control Cs migration with the aid of natural forces such as rainfall and rainwater runoff. In Imitate-mura, Fukushima, verification tests of the new technology have been performed and its effect on controlling Cs migration from forests to grass farm adjoining the forests has been proven.

Journal Articles

Application of ferrite process to radioactive waste; Study of ferrite product stability by micro-PIXE analysis

Abe, Tomohisa; Shimazaki, Takejiro; Osugi, Takeshi; Yamada, Naoto*; Yuri, Yosuke*; Sato, Takahiro*

QST-M-8; QST Takasaki Annual Report 2016, P. 61, 2018/03

no abstracts in English

Journal Articles

Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex, 2; Neutron scattering instruments

Nakajima, Kenji; Kawakita, Yukinobu; Ito, Shinichi*; Abe, Jun*; Aizawa, Kazuya; Aoki, Hiroyuki; Endo, Hitoshi*; Fujita, Masaki*; Funakoshi, Kenichi*; Gong, W.*; et al.

Quantum Beam Science (Internet), 1(3), p.9_1 - 9_59, 2017/12

The neutron instruments suite, installed at the spallation neutron source of the Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex (J-PARC), is reviewed. MLF has 23 neutron beam ports and 21 instruments are in operation for user programs or are under commissioning. A unique and challenging instrumental suite in MLF has been realized via combination of a high-performance neutron source, optimized for neutron scattering, and unique instruments using cutting-edge technologies. All instruments are/will serve in world-leading investigations in a broad range of fields, from fundamental physics to industrial applications. In this review, overviews, characteristic features, and typical applications of the individual instruments are mentioned.

Journal Articles

Neutron production in deuteron-induced reactions on Li, Be, and C at an incident energy of 102 MeV

Araki, Shohei*; Watanabe, Yukinobu*; Kitajima, Mizuki*; Sadamatsu, Hiroki*; Nakano, Keita*; Kin, Tadahiro*; Iwamoto, Yosuke; Satoh, Daiki; Hagiwara, Masayuki*; Yashima, Hiroshi*; et al.

EPJ Web of Conferences, 146, p.11027_1 - 11027_4, 2017/09

 Times Cited Count:0 Percentile:100

In recently years, deuteron-induced reaction is considered to produce the neutron source for application fields such as radiation damage fusion materials and boron neutron capture therapy. However, as the experimental data are not sufficient at incident energies above 60 MeV, the theoretical models are not validated. Therefore, we measured the double differential cross sections (DDXs) for Li, Be and C at 100 MeV at the Research Center for Nuclear Physics in Osaka University. The DDXs were measured at 6 angles (0$$^{circ}$$$$sim$$25$$^{circ}$$ and neutron energy was determined by a time of flight method. Three different-size NE213 liquid organic scintillators located at a distance of 7 m, 24 m and 74 m respectively were adopted as neutron detectors. In the measured DDXs, a broad peak due to deuteron breakup process was observed at approximately half of the deuteron incident energy. The DDXs calculated by PHITS did not reproduce the experimental ones due to lack of theoretical model.

Journal Articles

Recent improvements of particle and heavy ion transport code system: PHITS

Sato, Tatsuhiko; Niita, Koji*; Iwamoto, Yosuke; Hashimoto, Shintaro; Ogawa, Tatsuhiko; Furuta, Takuya; Abe, Shinichiro; Kai, Takeshi; Matsuda, Norihiro; Okumura, Keisuke; et al.

EPJ Web of Conferences, 153, p.06008_1 - 06008_6, 2017/09

 Times Cited Count:2 Percentile:10.14

Particle and Heavy Ion Transport code System, PHITS, has been developed under the collaboration of several institutes in Japan and Europe. It can deal with the transport of nearly all particles up to 1 TeV (per nucleon for ion) using various nuclear reaction models and data libraries. More than 2,500 researchers and technicians have used the code for a variety of applications such as accelerator design, radiation shielding and protection, medical physics, and space and geosciences. This paper briefly summarizes physics models and functions newly implemented in PHITS between versions 2.52 and 2.82.

Journal Articles

Features of PHITS version 2.88

Sato, Tatsuhiko; Iwamoto, Yosuke; Hashimoto, Shintaro; Ogawa, Tatsuhiko; Furuta, Takuya; Abe, Shinichiro; Kai, Takeshi; Matsuda, Norihiro; Iwase, Hiroshi*; Niita, Koji*

Hoshasen, 43(2), p.55 - 58, 2017/05

Particle and Heavy Ion Transport code System, PHITS, has been developed under the collaboration of several institutes in Japan and Europe. It can deal with the transport of nearly all particles up to 1 TeV (per nucleon for ion) using various nuclear reaction models and data libraries. More than 2,500 registered researchers and technicians have used this system for various applications such as accelerator design, radiation shielding and protection, medical physics, and space- and geo-sciences. This paper summarizes the physics models and functions recently implemented in PHITS, between versions 2.52 and 2.88.

Journal Articles

Benchmark study of the recent version of the PHITS code

Iwamoto, Yosuke; Sato, Tatsuhiko; Hashimoto, Shintaro; Ogawa, Tatsuhiko; Furuta, Takuya; Abe, Shinichiro; Kai, Takeshi; Matsuda, Norihiro; Hosoyamada, Ryuji*; Niita, Koji*

Journal of Nuclear Science and Technology, 54(5), p.617 - 635, 2017/05

 Times Cited Count:24 Percentile:1.13(Nuclear Science & Technology)

We performed a benchmark study for 58 cases using the recent version 2.88 of the Particle and Heavy Ion Transport code System (PHITS) in the following fields: particle production cross-sections for nuclear reactions, neutron transport calculations, and electro-magnetic cascade. This paper reports details for 22 cases. In cases of nuclear reactions with energies above 100 MeV and electro-magnetic cascade, overall agreements were found to be satisfactory. On the other hand, PHITS did not reproduce the experimental data for an incident proton energy below 100 MeV, because the intranuclear cascade model INCL4.6 in PHITS is not suitable for the low-energy region. For proton incident reactions over 100 MeV, PHITS did not reproduce fission product yields due to the problem of high-energy fission process in the evaporation model GEM. To overcome these inaccuracies, we are planning to incorporate a high-energy version of the evaluated nuclear data library JENDL-4.0/HE, and so on.

Journal Articles

Element distribution measurement in incineration ash using micro-PIXE analysis

Abe, Tomohisa; Shimazaki, Takejiro; Nakayama, Takuya; Osone, Osamu; Osugi, Takeshi; Nakazawa, Osamu; Yuri, Yosuke*; Yamada, Naoto*; Sato, Takahiro*

QST-M-2; QST Takasaki Annual Report 2015, P. 83, 2017/03

no abstracts in English

147 (Records 1-20 displayed on this page)