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JAEA Reports

Suppression of electrolytic corrosion at accelerator cooling-water facility by changing of rust inhibitors; Reduction of rust and cost

Dei, Tatsumi; Suganuma, Kazuaki; Fujirai, Kosuke; Suzuki, Katsuo; Suzuki, Hiroshi*; Nakata, Morihiro*; Hosokawa, Hideaki*; Onose, Yuichiro*; Watanabe, Yasuhiro; Shinozaki, Shinichi; et al.

JAEA-Technology 2026-003, 27 Pages, 2026/03

JAEA-Technology-2026-003.pdf:1.3MB

Accelerator cooling-water facility cannot prevent electrolytic corrosion because the systems consist of several different kinds of metals. We have confirmed that the electrolytic corrosion certainly occurs between oxygen-free copper and carbon steel, and cannot be suppressed by the rust inhibitor used so far. We have chosen a new rust inhibitor and confirmed that the new rust inhibitor can prevent the corrosion progression of carbon steel as well as oxygen-free copper. Moreover, using the new rust inhibitor brings about saving water and the cost reduction of the inhibitors.

Journal Articles

Cooling capability of remaining core fuel after core degradation in SFRs

Imaizumi, Yuya; Sogabe, Joji*; Onoda, Yuichi; Yamano, Hidemasa

Proceedings of 2025 International Congress on Advances in Nuclear Power Plants (ICAPP 2025) (Internet), 9 Pages, 2025/09

Journal Articles

Development of a quantitative, radiation-resistant feeding pump for use in extraction chromatography techniques for MA(III) recovery

Hasegawa, Kenta; Ambai, Hiromu; Takahatake, Yoko; Watanabe, So; Nakamura, Masahiro; Sano, Yuichi; Takeuchi, Masayuki

Progress in Nuclear Science and Technology (Internet), 8, p.248 - 251, 2025/09

Journal Articles

Validating terrestrial SER in 12-, 28-, and 65-nm SRAMs estimated by simulation coupled with one-time neutron irradiation

Takami, Kazusa*; Gomi, Yuibi*; Yasuda, Ryuichi*; Abe, Shinichiro; Ito, Masatoshi*; Kanda, Hiroki*; Fukuda, Mitsuhiro*; Hashimoto, Masanori*

IEEE Transactions on Nuclear Science, 72(8), p.2622 - 2628, 2025/08

 Times Cited Count:2 Percentile:83.88(Engineering, Electrical & Electronic)

Neutron-induced soft errors in the terrestrial environment pose reliability issues for semiconductor devices. We have developed the new method for estimating terrestrial SER based on simulation coupled with one-time irradiation using a conventional neutron source. This method has been validated using 65-nm planar SRAMs. However, with the ongoing progression of process shrinkage and the increasing adoption of devices fabricated with newer processes, there is a growing demand for further experimental validation of the terrestrial SER estimation method for these advanced processes. In this work, we validated the estimation method for 12-nm 1-fin FinFETs and 28-nm planer SRAMs. The SERs estimated by our method were consistent with the SERs measured using a white neutron beam at RCNP within 28% error.

JAEA Reports

Background aerial monitoring and UAV radiation monitoring technology development for emergency response and preparedness in fiscal year 2023 (Contract research)

Futemma, Akira; Sanada, Yukihisa; Nakama, Shigeo; Sasaki, Miyuki; Ochi, Kotaro; Sawahata, Yoshiro*; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Haginoya, Masashi*; et al.

JAEA-Technology 2024-022, 170 Pages, 2025/03

JAEA-Technology-2024-022.pdf:15.09MB

On March 11, 2011, the 2011 off the Pacific coast of Tohoku Earthquake caused a tsunami that led to the Fukushima Daiichi Nuclear Power Station accident, releasing radioactive material into the environment. Since then, Aerial Radiation Monitoring (ARM) using manned helicopters has been employed to measure radiation distribution. As a commissioned project from the Nuclear Regulation Authority, the Japan Atomic Energy Agency (JAEA) utilizes this technology for emergency monitoring during nuclear facility accidents, aiming to provide prompt results by pre-arranging information on background radiation, topography, and control airspaces around nuclear power plants nationwide. In fiscal year 2023, the commissioned project included conducting ARM around the Sendai Nuclear Power Station and preparing related information. To enhance effectiveness during emergencies, ARM and the first domestic training flight of Unmanned Aerial Vehicles (UAVs) were conducted during the FY2023 Nuclear Energy Disaster Prevention Drill. Furthermore, UAVs radiation monitoring technology was advanced by selecting UAVs and investigating their performance. This report summarizes the results and technical issues identified providing insights to improve emergency preparedness.

JAEA Reports

Aerial monitoring around TEPCO's Fukushima Daiichi Nuclear Power Station and development of radiation monitoring technology for unmanned airplanes in fiscal year 2023 (Contract research)

Futemma, Akira; Sanada, Yukihisa; Nakama, Shigeo; Sasaki, Miyuki; Ochi, Kotaro; Nagakubo, Azusa; Sawahata, Yoshiro*; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; et al.

JAEA-Technology 2024-021, 232 Pages, 2025/03

JAEA-Technology-2024-021.pdf:25.79MB

The 2011 off the Pacific coast of Tohoku Earthquake on March 11, 2011, caused a tsunami that led to the TEPCO's Fukushima Daiichi Nuclear Power Station (FDNPS) accident, releasing a large amount of radioactive material into the surrounding environment. Since the accident, Aerial Radiation Monitoring (ARM) has been used to quickly and widely measure radiation distribution. As a commissioned project from the Nuclear Regulation Authority, the Japan Atomic Energy Agency (JAEA) has continuously conducted ARM around FDNPS using manned and unmanned helicopters. This report summarizes the monitoring results for fiscal year 2023, evaluates changes in dose rate from past results, and discusses the factors contributing to these changes. Additionally, an analysis considering terrain undulation was conducted to improve accuracy for converting ARM data into dose rate. Furthermore, a method to discriminate airborne radon progeny was applied for ARM results to evaluate its impact. Moreover, to perform wide-area monitoring more efficiently, we advanced the development of unmanned airplane monitoring technology.

Journal Articles

Combustion properties of glove-box panel resins under fire accidents

Tashiro, Shinsuke; Uchiyama, Gunzo; Ono, Takuya; Amano, Yuki; Yoshida, Ryoichiro; Watanabe, Koji*; Abe, Hitoshi; Yamane, Yuichi

Nuclear Technology, 211(3), p.429 - 438, 2025/03

 Times Cited Count:1 Percentile:25.34(Nuclear Science & Technology)

Contributing to the confinement safety evaluation of glove-box (GB) connected with high efficiency particle air (HEPA) filters for radioactive materials under fire accidents, combustion tests of a flammable polymer, Polymethyl methacrylate (PMMA), and a flame retardant polymer, Polycarbonate (PC), as typical GB panel resins have been conducted with an engineering-scale combustion apparatus. The combustion properties such as the mass loss rate (MLR) and the heat release rate (HRR) of PMMA and PC were investigated in the combustion tests. In the tests with the same shapes, it was found the followings; MLRs and HRRs of PMMA were larger than those of PC under the same supply flow rate into the combustion cell (Fv); MLRs and HRRs of PMMA and PC were constant under different Fv. Moreover, in the tests of PMMA with different cross section areas (S), MLRs and HRRs were found to be proportional to S. Using these results, the relationships of MLR and HRR to S of PMMA and PC were deduced.

Journal Articles

Development of treatment method for analytical waste solutions in STRAD project; Role of trace chloride ion in ammonium ion oxidation with the presence of Co(II) ion

Aihara, Haruka; Watanabe, So; Kitawaki, Shinichi; Kamiya, Yuichi*

Progress in Nuclear Science and Technology (Internet), 7, p.175 - 181, 2025/03

Journal Articles

New filter concept for removal of fine particle generated in high level radioactive solution

Takahatake, Yoko; Watanabe, So; Watanabe, Masayuki; Sano, Yuichi; Takeuchi, Masayuki

Progress in Nuclear Science and Technology (Internet), 7, p.195 - 198, 2025/03

Extraction chromatgraphy technology for trivalent minor actinide (MA(III) ; Am(III) and Cm(III)) recovery from the solution generated by an extraction process in reprocessing of spent nuclear fuel has been developed. A fine particle is generated in the solution. The fine particle must be removed before MA recovery operation, because that leads clogging of the extraction chlomatography column. In order to prevent clogging the column, filtration system utilizing porous silica beads packed column has been designed. In this study, a fine particle trapping system was developed and particle removal performance of the system was experimentally evaluated using alumina particles as simulated fine particle. Column experiments revealed that the fine particle with the particle size from 0.12 to 15 $$mu$$m is cause of clogging of the filtration column. Since simulated fine particles were trapped on filtration experiments, a filtration system using the porous silica beads column is practical,

Journal Articles

Development of analysis methods for SFR severe accidents in JAEA and assessment of applicability to safety analysis

Tobita, Yoshiharu; Tagami, Hirotaka; Ishida, Shinya; Onoda, Yuichi; Sogabe, Joji; Okano, Yasushi

IAEA-TECDOC-2079, p.72 - 84, 2025/01

Since the fast reactor core is not in the maximum reactivity configuration, a hypothetical core disruptive accident could lead to the prompt criticality due to a change in the core material configuration, and the resulting energy generation has been one of the issues in fast reactor safety, and therefore appropriate measures are needed to mitigate and contain the effect of energy generated in the accident. In order to assess the effectiveness of these mitigative measures, a set of computer codes to analyze the event progressions and energy generation behavior in the ATWS of fast reactors have been developed, maintained, and improved under international collaboration in JAEA. Since the important physical phenomena, which govern the event progression, vary along with the progression of the accident, the whole accident process is divided into several phases in the analysis of accident, and dedicated analysis methods for each phase are provided to analyze the event progression in each phase. The organization and overview of these analysis methods are described in this paper. As a representative example of the validation approaches in applying these analysis methods to the reactor safety assessment in licensing procedure in Japan, the validation studies to confirm the applicability to reactor analysis of the SIMMER code for analyzing core material movement and reactor power, which is important to analyze the energy generation in the accident, are presented in the paper. The validation studies of the SIMMER code confirmed the applicability of SIMMER to the reactor analysis, while the critical phenomena that the effect of their uncertainty in the reactor analysis should be checked were also recognized.

Journal Articles

Release behavior of gaseous ruthenium tetroxide during heating of high-level liquid waste simulant during simulated accident conditions

Yoshida, Naoki; Ono, Takuya; Amano, Yuki; Yoshida, Ryoichiro; Abe, Hitoshi; Yamane, Yuichi

Nuclear Technology, 210(10), p.1999 - 2007, 2024/10

 Times Cited Count:1 Percentile:25.34(Nuclear Science & Technology)

A malfunction of the cooling system of high-level liquid waste (HLLW) and failure of countermeasures may lead to the "evaporation to dryness due to the loss of cooling functions" (EDLCF) of HLLW. In the EDLCF, ruthenium (Ru) can be released at a greater fraction to initial amount than other elements in HLLW by forming gaseous Ru. It is important to identify the chemical form of the released gaseous Ru to achieve a comprehensive understanding of the events impacting the source term assessment of Ru in this accident, such as particle formation, gas absorption and deposition on migration pathways. In this study, we observed the ultraviolet/visible spectroscopy of the off-gas generated during the heating of an HLLW simulant. Employing a program that allows the separation and quantification of known components within the spectrum (ruthenium tetroxide (RuO$$_{4}$$), nitrogen dioxide, and nitric acid), we attempted to analyze the composition of gaseous Ru within the generated off-gas. Our findings reveal RuO$$_{4}$$ as the main component of the gaseous Ru in off-gas after comparing the total amount of released Ru and the RuO$$_{4}$$ released amount obtained via spectroscopic analysis.

Journal Articles

France-Japan collaboration on severe accident studies in sodium-cooled fast reactors, 2; Methodologies and calculations of severe accident phases

Sogabe, Joji; Ishida, Shinya; Tagami, Hirotaka; Okano, Yasushi; Kamiyama, Kenji; Onoda, Yuichi; Matsuba, Kenichi; Yamano, Hidemasa; Kubo, Shigenobu; Kubota, Ryuzaburo*; et al.

Proceedings of International Conference on Nuclear Fuel Cycle (GLOBAL2024) (Internet), 4 Pages, 2024/10

In the frame of France-Japan collaboration, the calculational methodologies were defined and assessed, and the phenomenology and the severe accident consequences were investigated in a pool-type sodium-cooled fast reactor.

Journal Articles

Introduction to dismantling and decommissioning chemistry

Sato, Nobuaki*; Kameo, Yutaka; Sato, Soichi; Kumagai, Yuta; Sato, Tomonori; Yamamoto, Masahiro*; Watanabe, Yutaka*; Nagai, Takayuki; Niibori, Yuichi*; Watanabe, Masayuki; et al.

Introduction to Dismantling and Decommissioning Chemistry, 251 Pages, 2024/09

This book focuses on the dismantling and decommissioning of nuclear facilities and reactors that have suffered severe accidents. In Part 1, we introduce basic aspects ranging from fuel chemistry, analytical chemistry, radiation chemistry, corrosion, and decontamination chemistry to waste treatment and disposal. Then, Part 2 covers the chemistry involved in the decommissioning of various nuclear facilities, and discusses what chemical approaches are necessary and possible for the decommissioning of TEPCO's Fukushima Daiichi Nuclear Power Plants, how decommissioning should be carried out, and what kind of research and development and also human resource development are required for this.

Journal Articles

Power profile analysis of criticality accidents involving fissile solution boiling with considering evaporation

Watanabe, Tomoaki; Yamane, Yuichi

Journal of Nuclear Science and Technology, 61(7), p.958 - 966, 2024/07

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

The total fission energy released in a criticality accident involving fissile solution boiling tends to be high because the relatively high fission power continues during boiling. Simulating fission power change correctly during boiling seems essential to estimate the total fission energy. Fission power during boiling changes depending on fissile concentration and volume as the solution evaporates. In this study, we investigated the effect of concentration and volume change on estimated total fission energy for a long time of boiling. We introduced a model calculating the evaporation of fissile solution into the modified quasi-steady-state method to simulate power change during boiling. Three CRAC experiments and the Idaho Chemical Processing Plant (ICPP) criticality accident in 1959 were analyzed. As a result, the calculated energy considering concentration and volume change during boiling reproduced the measured energy well.

Journal Articles

Current numbers of qubits and their uses

Ichikawa, Tsubasa*; Hakoshima, Hideaki*; Inui, Koji*; Ito, Kosuke*; Matsuda, Ryo*; Mitarai, Kosuke*; Miyamoto, Koichi*; Mizukami, Wataru*; Mizuta, Kaoru*; Mori, Toshio*; et al.

Nature Reviews Physics (Internet), 6(6), p.345 - 347, 2024/06

 Times Cited Count:13 Percentile:98.48(Physics, Applied)

Journal Articles

Development of a process for the separation of MA(III) from Ln(III) fission products using HONTA impregnated adsorbent

Kubota, Masahiko*; Kim, S.-Y.*; Wu, H.*; Watanabe, So; Sano, Yuichi; Takeuchi, Masayuki; Arai, Tsuyoshi*

Journal of Radioanalytical and Nuclear Chemistry, 333(5), p.2413 - 2420, 2024/05

 Times Cited Count:2 Percentile:25.34(Chemistry, Analytical)

Journal Articles

Overview of development program for engineering scale extraction chromatography MA(III) recovery system

Watanabe, So; Takahatake, Yoko; Hasegawa, Kenta; Goto, Ichiro*; Miyazaki, Yasunori; Watanabe, Masayuki; Sano, Yuichi; Takeuchi, Masayuki

Mechanical Engineering Journal (Internet), 11(2), p.23-00461_1 - 23-00461_10, 2024/04

Journal Articles

Optimization in granulation conditions for adsorbent of extraction chromatography

Hasegawa, Kenta; Goto, Ichiro*; Miyazaki, Yasunori; Ambai, Hiromu; Watanabe, So; Watanabe, Masayuki; Sano, Yuichi; Takeuchi, Masayuki

Mechanical Engineering Journal (Internet), 11(2), p.23-00407_1 - 23-00407_8, 2024/04

JAEA Reports

Utilization of gamma ray irradiation at the WASTEF Facility

Sano, Naruto; Yamashita, Naoki; Watanabe, Masaya; Tsukada, Manabu*; Hoshino, Kazutoyo*; Hirai, Koki; Ikegami, Yuta*; Tashiro, Shinsuke; Yoshida, Ryoichiro; Hatakeyama, Yuichi; et al.

JAEA-Technology 2023-029, 36 Pages, 2024/03

JAEA-Technology-2023-029.pdf:2.47MB

At the Waste Safety Testing Facility (WASTEF), the gamma ray irradiation device "Gamma Cell 220" was relocated from the 4th Research Building of the Nuclear Science Research Institute in FY2019, and the use of gamma ray irradiation has begun. Initially, Fuel Cycle Safety Research Group, Fuel Cycle Safety Research Division, Nuclear Safety Research Center, Sector of Nuclear Safety Research and Emergency Preparedness, the owner of this device, conducted the tests as the main user, but since 2022, other users, including those outside the organization, have started using it. The gamma ray irradiation device "Gamma Cell 220" is manufactured by Nordion International Inc. in Canada. Since it was purchased in 1989, the built-in $$^{60}$$Co radiation source has been updated once, and safety research related to nuclear fuel cycles, etc. It is still used for this purpose to this day. This report summarizes the equipment overview of the gamma ray irradiation device "Gamma Cell 220", its permits and licenses at WASTEF, usage status, maintenance and inspection, and future prospects.

JAEA Reports

Radiation monitoring via manned helicopter around the nuclear power station in the fiscal year 2022 (Contract research)

Futemma, Akira; Sanada, Yukihisa; Nagakubo, Azusa; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Haginoya, Masashi*; Matsunaga, Yuki*; Akutsu, Yuichiro*; Arai, Yoshinori*; et al.

JAEA-Technology 2023-027, 146 Pages, 2024/03

JAEA-Technology-2023-027.pdf:18.12MB

By the accident at Tokyo Electric Power Company's (TEPCO's) Fukushima Daiichi Nuclear Power Station (FDNPS), caused by tsunami triggered by the 2011 off the Pacific coast of Tohoku Earthquake, a large amount of radioactive material was released into the surrounding environment. After the accident, Airborne Radiation Monitoring (ARM) via manned helicopter has been applied as a method to quickly and extensively measure the distribution of radiation. Japan Atomic Energy Agency (JAEA) has continuously conducted ARM via manned helicopter around FDNPS. In this report, we summarize the results of the ARM around FDNPS in the fiscal year 2022, evaluate the changes of ambient dose rates and other parameters based on the comparison to the past ARM results, and discuss the causes of such changes. In order to contribute to improve the accuracy of ambient dose rate conversion, we analyzed the ARM data taking into account undulating topography, and evaluated the effect of this method. Furthermore, the effect of radon progenies in the air on the ARM was evaluated by applying the discrimination method to the measurement results.

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