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JAEA Reports

Study on radionuclide analysis of rubble and plants for decommissioning of Fukushima Daiichi Nuclear Power Station

Seki, Kotaro; Sasaki, Takayuki*; Akimoto, Yuji*; Tokunaga, Takahito; Tanaka, Kiwamu; Haraga, Tomoko; Ueno, Takashi; Ishimori, Kenichiro; Hoshi, Akiko; Kameo, Yutaka

JAEA-Technology 2016-013, 37 Pages, 2016/07

JAEA-Technology-2016-013.pdf:2.09MB

In this study, based on the simple and rapid analytical method established from the wastes from research facilities, we created analytical schemes which is applicable to rubble and plants collected at Fukushima Daiichi, then transported to Nuclear Science Research Institute of JAEA. We examined the applicability, and confirmed quantifiability of radioactivity concentration with high recovery rate without being affected by fission products such as $$^{90}$$Sr and $$^{137}$$Cs.

Journal Articles

Anharmonic Pr guest modes in Pr(Os$$_{1-x}$$Ru$$_x$$)$$_4$$Sb$$_{12}$$ investigated by inelastic X-ray scattering

Tsutsui, Satoshi; Kaneko, Koji; Miyazaki, Ryoichi*; Higashinaka, Ryuji*; Aoki, Yuji*; Kobayashi, Riki*; Wakimoto, Shuichi; Baron, A. Q. R.*; Sugawara, Hitoshi*; Sato, Hideyuki*

JPS Conference Proceedings (Internet), 3, p.011060_1 - 011060_5, 2014/06

https://doi.org/10.7566/JPSCP.3.011060

Journal Articles

Emergent rank-5 nematic order in URu$$_2$$Si$$_2$$

Ikeda, Hiroaki*; Suzuki, Michito; Arita, Ryotaro*; Takimoto, Tetsuya*; Shibauchi, Takasada*; Matsuda, Yuji*

Nature Physics, 8(7), p.528 - 533, 2012/07

https://doi.org/10.1038/nphys2330
 Times Cited Count：132 Percentile：96.1(Physics, Multidisciplinary)

The origin of the hidden-order phase transition of URu$$_2$$Si$$_2$$ has been a long-standing mystery in condensed matter physics. We examine the complete set of multipole correlations allowed in URu$$_2$$Si$$_2$$ based on a first-principles theoretical approach. The results uncover that the hidden-order parameter is a rank-5 multipole (dotriacontapole) order with nematic $$E$$$$^{-}$$ symmetry. This naturally provides comprehensive explanations of all key features in the hidden-order phase including anisotropic magnetic excitations, nearly degenerate antiferromagnetic-ordered state, and spontaneous rotational symmetry breaking.

Journal Articles

AMATERAS; A Cold-neutron disk chopper spectrometer

Nakajima, Kenji; Kawamura, Seiko; Kikuchi, Tatsuya; Nakamura, Mitsutaka; Kajimoto, Ryoichi; Inamura, Yasuhiro; Takahashi, Nobuaki; Aizawa, Kazuya; Suzuya, Kentaro; Shibata, Kaoru; et al.

Journal of the Physical Society of Japan, 80(Suppl.B), p.SB028_1 - SB028_6, 2011/05

https://doi.org/10.1143/JPSJS.80SB.SB028
 Times Cited Count：125 Percentile：95.7(Physics, Multidisciplinary)

AMATERAS is a cold-neutron disk-chopper spectrometer in MLF, J-PARC. The construction of main part of the spectrometer has been completed in spring of 2009. Soon after that, we have started the commissioning work on AMATERAS. The performance of AMATERAS has been examined by test experiments in the course of commissioning. In parallel to these works, we have started the user program on AMATERAS from December 2009 and we are getting scientific results from our spectrometer. In this presentation, we will report the current status of AMATERAS including the results of performance tests and some of examples of scientific outputs.

Journal Articles

The Fermi chopper spectrometer 4SEASONS at J-PARC

Kajimoto, Ryoichi; Nakamura, Mitsutaka; Inamura, Yasuhiro; Mizuno, Fumio; Nakajima, Kenji; Kawamura, Seiko; Yokoo, Tetsuya*; Nakatani, Takeshi; Maruyama, Ryuji; Soyama, Kazuhiko; et al.

Journal of the Physical Society of Japan, 80(Suppl.B), p.SB025_1 - SB025_6, 2011/01

https://doi.org/10.1143/JPSJS.80SB.SB025
 Times Cited Count：102 Percentile：94.01(Physics, Multidisciplinary)

Oral presentation

Current status of the chopper spectrometer 4SEASONS at MLF, J-PARC

Kajimoto, Ryoichi; Yokoo, Tetsuya*; Nakamura, Mitsutaka; Nakajima, Kenji; Inamura, Yasuhiro; Takahashi, Nobuaki; Maruyama, Ryuji; Soyama, Kazuhiko; Mizuno, Fumio; Shibata, Kaoru; et al.

no journal, , 

no abstracts in English

Oral presentation

Chopper-type neutron inelastic spectrometer 4SEASONS at MLF, J-PARC

Kajimoto, Ryoichi; Yokoo, Tetsuya*; Nakamura, Mitsutaka; Nakajima, Kenji; Inamura, Yasuhiro; Takahashi, Nobuaki; Maruyama, Ryuji; Soyama, Kazuhiko; Mizuno, Fumio; Shibata, Kaoru; et al.

no journal, , 

no abstracts in English

Oral presentation

Starting-up of the chopper spectrometer 4SEASONS in J-PARC

Kajimoto, Ryoichi; Nakamura, Mitsutaka; Yokoo, Tetsuya*; Inamura, Yasuhiro; Mizuno, Fumio; Nakajima, Kenji; Takahashi, Nobuaki; Kawamura, Seiko; Maruyama, Ryuji; Soyama, Kazuhiko; et al.

no journal, , 

no abstracts in English

Oral presentation

Current status of the chopper spectrometer 4SEASONS at J-PARC

Kajimoto, Ryoichi; Nakamura, Mitsutaka; Yokoo, Tetsuya*; Inamura, Yasuhiro; Mizuno, Fumio; Nakajima, Kenji; Takahashi, Nobuaki; Kawamura, Seiko; Maruyama, Ryuji; Soyama, Kazuhiko; et al.

no journal, , 

no abstracts in English

Oral presentation

Starting-up of the chopper spectrometer 4SEASONS in J-PARC

Kajimoto, Ryoichi; Nakamura, Mitsutaka; Yokoo, Tetsuya*; Inamura, Yasuhiro; Mizuno, Fumio; Nakajima, Kenji; Takahashi, Nobuaki; Kawamura, Seiko; Maruyama, Ryuji; Soyama, Kazuhiko; et al.

no journal, , 

Oral presentation

The Fermi-chopper spectrometer 4SEASONS at J-PARC

Kajimoto, Ryoichi; Nakamura, Mitsutaka; Yokoo, Tetsuya*; Inamura, Yasuhiro; Mizuno, Fumio; Nakajima, Kenji; Takahashi, Nobuaki; Kawamura, Seiko; Maruyama, Ryuji; Soyama, Kazuhiko; et al.

no journal, , 

no abstracts in English

Oral presentation

Fermi-chopper neutron spectrometer 4SEASONS

Kajimoto, Ryoichi; Nakamura, Mitsutaka; Yokoo, Tetsuya*; Inamura, Yasuhiro; Mizuno, Fumio; Nakajima, Kenji; Takahashi, Nobuaki; Kawamura, Seiko; Maruyama, Ryuji; Soyama, Kazuhiko; et al.

no journal, , 

no abstracts in English

Oral presentation

The Fermi-chopper spectrometer 4SEASONS

Kajimoto, Ryoichi; Nakamura, Mitsutaka; Yokoo, Tetsuya*; Inamura, Yasuhiro; Mizuno, Fumio; Nakajima, Kenji; Takahashi, Nobuaki; Kawamura, Seiko; Maruyama, Ryuji; Soyama, Kazuhiko; et al.

no journal, , 

no abstracts in English

Oral presentation

Study on rapid analysis of the radioactive tritium in groundwater into the Fukushima-1 Nuclear Power Plant, 1; Applicability confirmation of the tritium column

Sasaki, Takayuki*; Akimoto, Yuji*; Seki, Kotaro; Nagano, Misato*; Ishimori, Kenichiro; Ueno, Takashi; Kameo, Yutaka

no journal, , 

no abstracts in English

Oral presentation

Development of analytical techniques of $$^{93}$$Zr and $$^{93}$$Mo in fuel debris by ICP-MS/MS

Horita, Takuma; Akimoto, Yuji*; Kikuchi, Hikaru*; Do, V. K.

no journal, , 

no abstracts in English

Oral presentation

Development of rational analytical technique of $$^{151}$$Sm by ICP-MS/MS

Horita, Takuma; Akimoto, Yuji*; Do, V. K.

no journal, , 

Samarium-151($$^{151}$$Sm) can be measured by liquid scintillation counting (LSC) or inductively coupled plasma mass spectrometry (ICP-MS). While the former method requires a complete radiochemical separation, the latter one must solve the isobaric interference from Europium-151 ($$^{151}$$Eu). In this study, we have been developing an analytical technique for $$^{151}$$Sm by ICP-tandem MS(ICP-MS/MS). The recent advances of MS/MS mode with a collision/reaction cell in mass spectrometry may enable sufficient removal of the mass spectroscopic interferences. Moreover, compared to LSC, ICP-MS is more rapid and more selective, and thus, it can simplify pretreatment process. As preliminary experiments, the selection of reaction gas for the separation of $$^{151}$$Sm from $$^{151}$$Eu were examined by checking the product ions of $$^{147}$$Sm and $$^{151}$$Eu produced by reactions with the various gases (H$$_{2}$$, O$$_{2}$$, NH$$_{3}$$, and N$$_{2}$$O). Our obtained data showed that in the reaction with NH$$_{3}$$, Sm formed a product ion at mass shift of 16, while the reaction tendency of Eu is different. Accordingly, the counts of $$^{147}$$Sm and $$^{151}$$Eu at the mass shift of 16 were 9842 [cps/$$mu$$g/L] and 162 [cps/$$mu$$g/L], respectively. The difference in reactivity of Sm and Eu to NH$$_{3}$$ gas can reduce interference of the $$^{151}$$Eu to the measurement of $$^{151}$$Sm.

Oral presentation

Development of simultaneous analytical method for $$^{93}$$Zr and $$^{93}$$Mo based on solid phase extraction combined with ICP-MS/MS, 2; Spectral interference removal for measurement of $$^{93}$$Zr and $$^{93}$$Mo by ICP-MS/MS

Do, V. K.; Furuse, Takahiro; Murakami, Erina; Aita, Rena; Ota, Yuki; Tomitsuka, Tomohiro; Sano, Yuichi; Akimoto, Yuji*; Endo, Tsubasa*; Katayama, Atsushi; et al.

no journal, , 

The paper presents removal of possible interferences including from an isobar ($$^{93}$$Nb) and tailings of adjacent peaks for the quantification of $$^{93}$$Zr and $$^{93}$$Mo using an ICP-MS/MS (Agilent 8900). By using ammonia gas (NH$$_{3}$$) as a reaction gas, $$^{93}$$Zr and $$^{93}$$Mo can be separated from each other and from $$^{93}$$Nb owing to the different reactions of those elements with the reaction gas. Based on the characterization results, we propose a measurement scheme aiming at quantification of $$^{93}$$Zr and $$^{93}$$Mo in environmental samples collected at adjacent location of Fukushima Daiichi Nuclear Power Station.

Oral presentation

Development of simultaneous analytical method for $$^{93}$$Zr and $$^{93}$$Mo based on solid phase extraction combined with ICP-MS/MS, 1; Sequential chemical separation of Zr and Mo from Nb

Furuse, Takahiro; Do, V. K.; Aita, Rena; Ota, Yuki; Murakami, Erina; Tomitsuka, Tomohiro; Sano, Yuichi; Akimoto, Yuji*; Endo, Tsubasa*; Katayama, Atsushi; et al.

no journal, , 

In order to simplify the analysis of $$^{93}$$Zr and $$^{93}$$Mo in radioactive waste from conventional radiation measurement, we have considered analysis method combining solid-phase extraction and ICP-MS/MS. In this presentation, we report the results of a study on sequential chemical separation of Zr and Mo from Nb and sample matrix using ZR resin as a solid-phase extraction resin.

18 (Records 1-18 displayed on this page)
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