Release behavior of gaseous ruthenium tetroxide during heating of high-level liquid waste simulant during simulated accident conditions

Yoshida, Naoki; Ono, Takuya; Amano, Yuki; Yoshida, Ryoichiro; Abe, Hitoshi; Yamane, Yuichi

Nuclear Technology, 210(10), p.1999 - 2007, 2024/10

https://doi.org/10.1080/00295450.2024.2306688

A malfunction of the cooling system of high-level liquid waste (HLLW) and failure of countermeasures may lead to the "evaporation to dryness due to the loss of cooling functions" (EDLCF) of HLLW. In the EDLCF, ruthenium (Ru) can be released at a greater fraction to initial amount than other elements in HLLW by forming gaseous Ru. It is important to identify the chemical form of the released gaseous Ru to achieve a comprehensive understanding of the events impacting the source term assessment of Ru in this accident, such as particle formation, gas absorption and deposition on migration pathways. In this study, we observed the ultraviolet/visible spectroscopy of the off-gas generated during the heating of an HLLW simulant. Employing a program that allows the separation and quantification of known components within the spectrum (ruthenium tetroxide (RuO), nitrogen dioxide, and nitric acid), we attempted to analyze the composition of gaseous Ru within the generated off-gas. Our findings reveal RuO as the main component of the gaseous Ru in off-gas after comparing the total amount of released Ru and the RuO released amount obtained via spectroscopic analysis.

Suggestions for energy storage best mix to achieve carbon neutrality, 1; Development of energy storage best mix

Kato, Yukitaka*; Yamano, Hidemasa

Dai-28-Kai Doryoku, Enerugi Gijutsu Shimpojiumu Koen Rombunshu (Internet), 5 Pages, 2024/06

The research committee of energy storage technologies toward carbon neutrality developed four suggestions: 1) Development of energy storage best mix, 2) Transformation to green society, 3) utilization of heat storage technologies, and 4) Development of energy storage strategy beyond 2050. This paper describes suggestion 1) Development of energy storage best mix in response to large-scale deployments of variable renewable energy.

Development of failure mitigation technologies for improving resilience of nuclear structures, 1; Failure mitigation by passive safety structures without catastrophic failure

Kasahara, Naoto*; Yamano, Hidemasa; Nakamura, Izumi*; Demachi, Kazuyuki*; Sato, Takuya*; Ichimiya, Masakazu*

Transactions of the 27th International Conference on Structural Mechanics in Reactor Technology (SMiRT 27) (Internet), 8 Pages, 2024/03

In this study, we propose failure mitigation methods by application of passive safety structures. The idea of the passive safety structures was applied to next generation fast reactors under high temperature conditions and excessive earthquake conditions.

Physical protection corrective action program activities in JAEA

Shibata, Ryodai; Amano, Tsukasa; Yamada, Hiroyuki; Miyaji, Noriko; Nakamura, Hironobu

Dai-44-Kai Nihon Kaku Busshitsu Kanri Gakkai Nenji Taikai Kaigi Rombunshu (Internet), 4 Pages, 2023/11

In April 2020, JAEA has been introduced Physical Protection Corrective Action Program (PPCAP) with full-scale. It was needed to introduce unified operation for six sites with different business scales, and headquarters developed the common guideline. There was an impression that physical protection activities were carried out by a limited number of employees. Therefore, a problem was to root and activate PPCAP activities among all employees in order to make them effective. Five activities were implemented to solve this problem. As a result, more than 3,700 condition reports (CR) have been collected for 4 years. This paper reports on the activities related to the PPCAP that have been implemented at JAEA.

A Predicted CRISPR-mediated symbiosis between uncultivated archaea

Esser, S. P.*; Rahlff, J.*; Zhao, W.*; Predl, M.*; Plewka, J.*; Sures, K.*; Wimmer, F.*; Lee, J.*; Adam, P. S.*; McGonigle, J.*; et al.

Nature Microbiology (Internet), 8(9), p.1619 - 1633, 2023/09

https://doi.org/10.1038/s41564-023-01439-2

Development of probabilistic risk assessment methodology against strong wind for sodium-cooled fast reactors

Nishino, Hiroyuki; Yamano, Hidemasa; Kurisaka, Kenichi

Mechanical Engineering Journal (Internet), 10(4), p.22-00387_1 - 22-00387_20, 2023/08

https://doi.org/10.1299/mej.22-00387

For nuclear power plants, probabilistic risk assessment (PRA) should be performed not only against earthquake and tsunami, which are critical events especially in Japan, but also other external hazards such as strong wind. The aim of the present study is to develop a practical PRA methodology for sodium-cooled fast reactors (SFRs) against strong wind, paying attention to the final heat sink, ambient air, that removes decay heat under accident conditions. First, this study used Gumbel distributions to estimate hazard curves of the strong wind based on weather data recorded in Japan. Second, it identified important structures, systems and components (SSCs) for decay heat removal, and developed an event tree that results in core damage, focusing on the impacts of missiles (e.g., steel pipes) caused by strong wind. It also identified missiles that can reach SSCs at elevated places, and calculated the fragility of the SSCs against the missiles as a product of two probabilities. One is a probability of the missiles that would enter an inlet or outlet of the decay heat removal system, and another is a probability of failure caused by missile impacts. Finally, it quantified conditional decay heat removal failure probabilities by introducing the fragilities into the event tree. The core damage frequency (CDF) was estimated at about 5x10-10/y. The dominant sequence is that strong wind causes offsite power loss and missiles, the missiles penetrate the diesel fuel tank, cause a fire, and the fire increases air temperature around the reactor building where air cooler inlets of decay heat removal systems are installed, leads to loss of power for the diesel generator for forced circulation cooling, resulting in loss of decay heat removal. Through the above, this study has developed the practical PRA methodology for SFRs against strong wind.

Anaerobic methane-oxidizing activity in a deep underground borehole dominantly colonized by Methanoperedenaceae

Nishimura, Hiroki*; Kozuka, Mariko*; Fukuda, Akari*; Ishimura, Toyoho*; Amano, Yuki; Beppu, Hikari*; Miyakawa, Kazuya; Suzuki, Yohei*

Environmental Microbiology Reports (Internet), 15(3), p.197 - 205, 2023/06

https://doi.org/10.1111/1758-2229.13146

The family Methanoperedenaceae archaea mediate anaerobic oxidation of methane (AOM). We newly developed a high-pressure laboratory incubation system and investigated groundwater from 214- and 249-m deep boreholes at Horonobe Underground Research Laboratory, Japan, where the high and low abundances of Methanoperedenaceae archaea have been revealed, respectively. We incubated the samples amended with or without amorphous Fe(III) and C-labelled methane at an in-situ pressure of 1.6 MPa. After three to seven-day incubation, AOM activities were not detected from the 249-m sample but from the 214-m sample. The AOM rates were 93.740.6 and 27.737.5 nM/day with and without Fe(III) amendment. Suspended particulates were not visible in the 249-m sample on the filter, while they were abundant and contained amorphous Fe(III) and Fe(III)-bearing phyllosilicates in the 214-m sample. This supports the in-situ activity of Fe(III)-dependent AOM in the deep subsurface borehole.

Case study activities for nuclear security culture development in JAEA

Amano, Tsukasa; Shibata, Ryodai; Sato, Yoshiharu; Yamazaki, Katsuyuki; Shiromo, Hideo; Nakamura, Hironobu

Proceedings of INMM & ESARDA Joint Annual Meeting 2023 (Internet), 6 Pages, 2023/05

In Japan, about 10 years have passed since the law obligated nuclear operators to develop and maintain a nuclear security culture. During this period, the global nuclear situation has changed significantly, and it is becoming important to maintain a stance that emphasizes compliance with regulations and nuclear security culture. In JAEA, the policy of legal compliance and developing nuclear security culture is determined by the president of JAEA. For legal compliance and developing nuclear security culture, many activities are carried out based on that policy. Finally, these activities are evaluated and improved it every year. Case study is the one of activities that can obtain skills for legal compliance and developing nuclear security culture, such as sensitivity of nuclear security risks, correct understanding of the laws. The procedure for the case study was created with reference to a method called KY-Training which is often applied to safety training program in Japan. KY-Training is a training that participants (groups) can reach the conclusion how to respond to cases through four questions. Firstly, participants are given illustrations and descriptions which has potential of nuclear security risks. Then, participants make discussion according to four questions. Consequently, participants can effectively become aware of nuclear security risks. In the 2022 case study, we prepared 23 cases so that they can select choose freely according to role of participants such as in charge of nuclear security, guards, general employees. Finally, participants are asked to fill a questionnaire to evaluate effectiveness of case study. The result of questionnaires indicated that the case study was able to lead to improvement sensitivity of nuclear security risks and correct understanding of the laws. Overall, case study results suggested that JAEA's efforts were implying sufficiently to develop and maintain a nuclear security culture.

Verification of fuel assembly bowing analysis model for core deformation reactivity evaluation

Doda, Norihiro; Uwaba, Tomoyuki; Ohgama, Kazuya; Yoshimura, Kazuo; Nemoto, Toshiyuki*; Tanaka, Masaaki; Yamano, Hidemasa

Nihon Kikai Gakkai Kanto Shibu Dai-29-Ki Sokai, Koenkai Koen Rombunshu (Internet), 5 Pages, 2023/03

An evaluation method for reactivity feedback due to core deformation during reactor power increase in sodium-cooled fast reactors is being developed for realistic core design evaluation. In this evaluation method, fuel assembly bowing was modeled with a beam element of the finite element method, and the assembly's pad contact between adjacent assemblies was modeled with a dedicated element which could consider the wrapper tube cross-sectional distortion and the pad stiffness depending on pad contact conditions. This fuel assembly bowing analysis model was verified for thermal bowing of a single assembly and assembly pad contact between adjacent assemblies in a core as past benchmark problems. The calculation results by this model showed good agreement with those of reference solutions of theoretical solutions or results by participating institutions in the benchmark. This study confirmed that the analysis model was able to calculate thermal assembly bowing appropriately.

Legal compliance activities and nuclear security culture development activities in JAEA

Amano, Tsukasa; Sato, Yoshiharu; Shibata, Ryodai; Yamazaki, Katsuyuki; Shiromo, Hideo; Nakamura, Hironobu

Dai-43-Kai Nihon Kaku Busshitsu Kanri Gakkai Nenji Taikai Kaigi Rombunshu (Internet), 4 Pages, 2022/11

About ten years have passed since the introduction of nuclear security compliance and security culture development activities. While there have been changes in domestic and international situations, it is essential for nuclear security that the entire organization maintains an attitude that emphasizes compliance with laws and regulations and nuclear security. JAEA has been effectively implementing various activities with evaluation and improvement. Especially, e-learning which combines education and awareness, case studies, and internal audits are considered effective in maintaining nuclear security compliance and security culture development activities.