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論文

$$beta$$-delayed fission of isomers in $$^{188}$$Bi

Andel, B.*; Andreyev, A. N.; Antalic, S.*; Al Monthery, M.*; Barzakh, A.*; Bissell, M. L.*; Chrysalidis, K.*; 他29名*

Physical Review C, 102(1), p.014319_1 - 014319_12, 2020/07

$$beta$$-delayed fission ($$beta$$DF) decay of a low-spin (ls) and a high-spin (hs) isomer in $$^{188}$$Bi was studied at the ISOLDE facility at CERN. Their $$beta$$DF partial half-lives were determined: $$T_{rm 1/2p}$$, $$beta$$DF($$^{188}$$Bi$$^{hs}$$)= 5.6(8) $$times$$ 10$$^{3}$$ s and $$T_{rm 1/2p}$$, $$beta$$DF($$^{188}$$Bi$$^{ls}$$)=1.7(6) $$times$$ 10$$^{3}$$ s. This work is the first $$beta$$DF study of two states in one isotope and allows the spin dependence of low-energy fission to be explored. The fission fragment mass distribution of a daughter nuclide $$^{188}$$Pb, following the $$beta$$ decay of the high-spin isomer, was deduced and indicates a mixture of symmetric and asymmetric fission modes.

論文

Shape coexistence in $$^{187}$$Au studied by laser spectroscopy

Barzakh, A. E.*; Atanasov, D.*; Andreyev, A. N.; Al Monthery, M.*; Althubiti, N. A.*; Andel, B.*; Antalic, S.*; Blaum, K.*; 他34名*

Physical Review C, 101(6), p.064321_1 - 064321_7, 2020/06

Hyperfine-structure parameters and isotope shift of the $$9/2^{-}$$ isomeric state in $$^{187}$$Au relative to $$^{197}$$Au for the 267.6-nm atomic transition have been measured for the first time using the in-source resonance-ionization spectroscopy technique. The magnetic dipole moment and change in the mean-square charge radius for this $$9/2^{-}$$ isomer have been deduced. The observed large isomer shift relative to the $$1/2^{+}$$ ground state in $$^{187}$$Au confirms the occurrence of the shape coexistence in $$^{187}$$Au proposed earlier from the analysis of the nuclear spectroscopic data and particle plus triaxial rotor calculations. The analysis of the magnetic moment supports the previously proposed $$9/2^{-}$$, $$1/2^{-}$$[541] assignment at moderate prolate deformation for $$^{187}$$Au$$^{m}$$.

論文

Hyperfine anomaly in gold and magnetic moments of $$I^{pi}$$ = 11/2$$^{-}$$ gold isomers

Barzakh, A. E.*; Atanasov, D.*; Andreyev, A. N.; Al Monthery, M.*; Althubiti, N. A.*; Andel, B.*; Antalic, S.*; Blaum, K.*; 他39名*

Physical Review C, 101(3), p.034308_1 - 034308_9, 2020/03

Hyperfine-structure constants for the $$I^{pi}$$ = 11/2$$^{-}$$ gold isomers $$^{177,191,193,195}$$Au$$^{m}$$ have been measured at CERN-ISOLDE, using the in-source laser resonance-ionization spectroscopy technique. From the measured hyperfine constants the differences between hyperfine anomalies have been deduced. These differential hyperfine anomaly values have been used to determine the hyperfine anomaly relative to the stable $$^{197}$$Au with advanced atomic calculations. Magnetic dipole moments for the gold isomers in question have been deduced, taking into account the corresponding relative hyperfine-anomaly values. It has been shown that the commonly used prescription for the extraction of the magnetic moment values for the gold isotopes should be reconsidered. The magnetic moments calculated by this prescription have been reevaluated by properly accounting for the hyperfine anomaly, which is as large as 10% for several gold isotopes.

論文

$$alpha$$-decay branching ratio of $$^{180}$$Pt

Cubiss, J. G.*; Harding, R. D.*; Andreyev, A. N.; Althubiti, N.*; Andel, B.*; Antalic, S.*; Barzakh, A. E.*; Cocolios, T. E.*; Day Goodacre, T.*; Farooq-Smith, G. J.*; et al.

Physical Review C, 101(1), p.014314_1 - 014314_4, 2020/01

 被引用回数:2 パーセンタイル:25.8(Physics, Nuclear)

$$^{180}$$Ptの基底状態から娘核$$^{176}$$Osの基底状態への$$alpha$$崩壊分岐比を0.52(5)%と、過去の値と比較してより高精度で再決定した。$$^{180}$$PtはCERN-ISOLDE実験施設において$$^{180}$$Hgを単離し、その$$beta$$崩壊孫核種として生成した。今回の結果を用いて導出した$$alpha$$崩壊の換算崩壊幅は、中性子欠損Pt同位体の$$alpha$$崩壊幅の系統性について新しい描像を与えることとなった。

論文

$$alpha$$-decay properties of $$^{200,202}$$Fr

Ghys, L.*; Andreyev, A. N.; Huyse, M.*; Van Duppen, P.*; Antalic, S.*; Barzakh, A.*; Capponi, L.*; Cocolios, T. E.*; Cubiss, J.*; Derkx, X.*; et al.

Physical Review C, 100(5), p.054310_1 - 054310_13, 2019/11

 被引用回数:4 パーセンタイル:22.15(Physics, Nuclear)

The aim of this work was to investigate the $$alpha$$-decay properties of $$^{200,202}$$Fr and daughter products. Neutron-deficient francium nuclei are produced at ISOLDE-CERN bombarding a UCx target with 1.4 GeV protons. Due to the very high statistics and the high beam purity, improved decay data for $$^{202}$$Fr and its daughters were obtained. The observation of crossover transitions positioned the isomeric high-spin level of $$^{198}$$At at an excitation energy of 265(3) keV. Half-life values of 4.47(5) s and 1.28(10) s were extracted for the ground state and isomeric state of $$^{198}$$At and 52(3) ms for the ground-state decay of $$^{200}$$Fr.

論文

Identification of a 6.6$$mu$$s isomeric state in $$^{175}$$Ir

Gillespie, S. A.*; Andreyev, A. N.; Al Monthery, M.*; Barton, C. J.*; Antalic, S.*; Auranen, K.*; Badran, H.*; Cox, D.*; Cubiss, J. G.*; O'Donnell, D.*; et al.

Physical Review C, 99(6), p.064310_1 - 064310_6, 2019/06

 被引用回数:0 パーセンタイル:100(Physics, Nuclear)

An experiment has been performed to study excited states in the neutron-deficient nucleus $$^{175}$$Ir via the use of the JUROGAM II high-purity germanium detector array and the RITU gas-filled separator at JYFL, Jyv$"a$skyl$"a$. By using isomer tagging, an isomeric state with a half-life of 6.58(15) $$mu$$s has been observed in $$^{175}$$Ir for the first time. It has been established that the isomer decays via a 45.2 ($$E1$$) - 26.1 ($$M1$$) keV cascade to new states below the previously reported ground state in $$^{175}$$Ir with $$I^{pi} = (5/2^{-})$$. We now reassign this $$(5/2^{-})$$ state to the isomeric state discovered in this study.

論文

Fine structure in the $$alpha$$ decay of $$^{218}$$At

Cubiss, J. G.*; Andreyev, A. N.; Barzakh, A. E.*; Andel, B.*; Antalic, S.*; Cocolios, T. E.*; Day Goodacre, T.*; Fedorov, D. V.*; Fedosseev, V. N.*; Ferrer, R.*; et al.

Physical Review C, 99(6), p.064317_1 - 064317_6, 2019/06

 被引用回数:3 パーセンタイル:22.15(Physics, Nuclear)

$$^{218}$$Atの$$alpha$$崩壊について、CERN-ISOLDE施設においてレーザーイオン化法を使うことで研究した。$$alpha$$-$$gamma$$同時計数データを初めて取得し、より精度の良い半減期の値として1.27(6)秒を得た。$$alpha$$崩壊の微細構造を基に新しい$$alpha$$崩壊図式を構築した。それらの結果から、$$^{218}$$Atの基底状態のスピン・パリティは(3$$^{-}$$)がより確からしいことが解ったが、(2)$$^{-}$$の可能性も完全には否定しきれない。

論文

Inverse odd-even staggering in nuclear charge radii and possible octupole collectivity in $$^{217,218,219}$$At revealed by in-source laser spectroscopy

Barzakh, A. E.*; Cubiss, J. G.*; Andreyev, A. N.; Seliverstov, M. D.*; Andel, B.*; Antalic, S.*; Ascher, P.*; Atanasov, D.*; Beck, D.*; Biero$'n$, J.*; et al.

Physical Review C, 99(5), p.054317_1 - 054317_9, 2019/05

 被引用回数:3 パーセンタイル:22.15(Physics, Nuclear)

Hyperfine-structure parameters and isotope shifts for the 795-nm atomic transitions in $$^{217,218,219}$$At have been measured at CERN-ISOLDE, using the in-source resonance-ionization spectroscopy technique. Magnetic dipole and electric quadrupole moments, and changes in the nuclear mean-square charge radii, have been deduced. A large inverse odd-even staggering in radii, which may be associated with the presence of octupole collectivity, has been observed. Namely, the radius of the odd-odd isotope $$^{218}$$At has been found to be larger than the average.

論文

Detailed $$alpha$$-decay study of $$^{180}$$Tl

Andel, B.*; Andreyev, A.; Antalic, S.*; Barzakh, A.*; Bree, N.*; Cocolios, T. E.*; Comas, V. F.*; Diriken, J.*; Elseviers, J.*; Fedorov, D. V.*; et al.

Physical Review C, 96(5), p.054327_1 - 054327_11, 2017/12

 被引用回数:0 パーセンタイル:100(Physics, Nuclear)

A detailed $$alpha$$-decay spectroscopy study of $$^{180}$$Tl has been performed at ISOLDE (CERN). Z-selective ionization by the Resonance Ionization Laser Ion Source (RILIS) coupled to mass separation provided a high-purity beam of $$^{180}$$Tl. Fine-structure $$alpha$$ decays to excited levels in the daughter $$^{176}$$Au were identified and an $$alpha$$-decay scheme of $$^{180}$$Tl was constructed based on an analysis of $$alpha$$-$$gamma$$ and $$alpha$$-$$gamma$$ -$$gamma$$ coincidences. Multipolarities of several $$gamma$$-ray transitions deexciting levels in $$^{176}$$Au were determined. Based on the analysis of reduced $$alpha$$-decay widths, it was found that all $$alpha$$ decays are hindered, which signifies a change of configuration between the parent and all daughter states.

論文

$$beta$$-delayed fission of $$^{230}$$Am

Wilson, G. L.*; 武山 美麗*; Andreyev, A.; Andel, B.*; Antalic, S.*; Catford, W. N.*; Ghys, L.*; 羽場 宏光*; He${ss}$berger, F. P.*; Huang, M.*; et al.

Physical Review C, 96(4), p.044315_1 - 044315_7, 2017/10

 被引用回数:3 パーセンタイル:55.66(Physics, Nuclear)

The exotic decay process of $$beta$$-delayed fission has been studied in the neutron-deficient isotope $$^{230}$$Am at RIKEN, Japan. The $$^{230}$$Am nuclei were produced in the complete fusion reaction $$^{207}$$Pb($$^{27}$$Al,4n)$$^{230}$$Am and separated by using the GARIS gas-filled recoil ion separator. A lower limit for the $$beta$$-delayed fission probability larger than 0.30 was deduced, which so far is the highest value among all known nuclei exhibiting this decay mode.

論文

$$beta$$-delayed fission and $$alpha$$ decay of $$^{196}$$At

Truesdale, V. L.*; Andreyev, A.; Ghys, L.*; Huyse, M.*; Van Duppen, P.*; Sels, S.*; Andel, B.*; Antalic, S.*; Barzakh, A.*; Capponi, L.*; et al.

Physical Review C, 94(3), p.034308_1 - 034308_11, 2016/09

 被引用回数:7 パーセンタイル:36.29(Physics, Nuclear)

A nuclear-decay spectroscopy study of the neutron-deficient isotope $$^{196}$$At is reported where an isotopically pure beam was produced using the selective Resonance Ionization Laser Ion Source and On-Line Isotope Mass Separator (CERN). The fine-structure $$alpha$$ decay of $$^{196}$$At allowed the low-energy excited states in the daughter nucleus $$^{192}$$Bi to be investigated. A $$beta$$-delayed fission study of $$^{196}$$At was also performed. A mixture of symmetric and asymmetric fission-fragment mass distributions of the daughter isotope $$^{196}$$Po (populated by $$beta$$ decay of $$^{196}$$At) was deduced based on the measured fission-fragment energies. A $$beta$$DF probability $$P_{rm beta DF}$$($$^{196}$$At) = 9(1)$$times$$10$$^{-5}$$ was determined.

論文

Review of even element super-heavy nuclei and search for element 120

Hofmann, S.*; Heinz, S.*; Mann, R.*; Maurer, J.*; M$"u$nzenberg, G.*; Antalic, S.*; Barth, W.*; Burkhard, K. G.*; Dahl, L.*; Eberhardt, K.*; et al.

European Physical Journal A, 52(6), p.180_1 - 180_34, 2016/06

 被引用回数:82 パーセンタイル:9.09(Physics, Nuclear)

The reaction $$^{54}$$Cr+$$^{248}$$Cm was investigated at the velocity filter SHIP at GSI with the intention to study production and decay properties of isotopes of element 120. Three correlated signals were measured, which occurred within a period of 279 ms. The heights of the signals correspond with the expectations for a decay sequence starting with an isotope of element 120. However, a complete decay chain cannot be established, since a signal from the implantation of the evaporation residue cannot be identified unambiguously. Measured properties of the event chain are discussed in detail. The result is compared with theoretical predictions. Previously measured decay properties of even element super-heavy nuclei were compiled in order to find arguments for an assignment from the systematics of experimental data. In the course of this review, a few tentatively assigned data could be corrected. New interpretations are given for results which could not be assigned definitely in previous studies. The discussion revealed that the cross-section for production of element 120 could be high enough so that a successful experiment seems possible with presently available techniques. However, a continuation of the experiment at SHIP for a necessary confirmation of the results obtained in a relatively short irradiation of five weeks is not possible at GSI presently. In the summary and outlook section we also present concepts for the continuation of research in the field of super-heavy nuclei.

論文

Short-lived isomers in $$^{192}$$Po and $$^{194}$$Po

Andel, B.*; Andreyev, A.; Antalic, S.*; He${ss}$berger, F. P.*; Ackermann, D.*; Hofmann, S.*; Huyse, M.*; Kalaninov$'a$, Z.*; Kindler, B.*; Kojouharov, I.*; et al.

Physical Review C, 93(6), p.064316_1 - 064316_12, 2016/06

 被引用回数:0 パーセンタイル:100(Physics, Nuclear)

Isomeric states in $$^{194}$$Po and $$^{192}$$Po were studied at the velocity filter SHIP. The isotopes were produced in the fusion-evaporation reactions $$^{141}$$Pr($$^{56}$$Fe, $$p2n$$)$$^{194}$$Po and $$^{144}$$Sm($$^{51}$$V, $$p2n$$)$$^{192}$$Po. Several new $$gamma$$-ray transitions were attributed to the isomers and $$gamma$$-$$gamma$$ coincidences for both isomers were studied for the first time. The 459-keV transition earlier, tentatively proposed as de-exciting the isomeric level in $$^{194}$$Po, was replaced by a new 248-keV transition, and the spin of this isomer was reassigned from (11$$^{-}$$) to (10$$^{-}$$). The de-excitation of the (11$$^{-}$$) isomeric level in $$^{192}$$Po by the 154-keV transition was confirmed and a parallel de-excitation by a 733-keV (E3) transition to (8$$^{+}$$) level of the ground-state band was suggested. Moreover, side feeding to the (4$$^{+}$$) level of the ground-state band was proposed. The paper also discusses strengths of transitions de-exciting 11$$^{-}$$ isomers in neighboring Po and Pb isotopes.

論文

Remarks on the fission barriers of super-heavy nuclei

Hofmann, S.*; Heinz, S.*; Mann, R.*; Maurer, J.*; M$"u$nzenberg, G.*; Antalic, S.*; Barth, W.*; Dahl, L.*; Eberhardt, K.*; Grzywacz, R.*; et al.

European Physical Journal A, 52(4), p.116_1 - 116_12, 2016/04

 被引用回数:20 パーセンタイル:10.37(Physics, Nuclear)

Shell-correction energies of super-heavy nuclei are approximated by using Q$$_{alpha}$$ values of measured decay chains. Five decay chains were analyzed, which start at the isotopes $$^{285}$$Fl, $$^{294}$$118, $$^{291}$$Lv, $$^{292}$$Lv and $$^{293}$$Lv. The data are compared with predictions of macroscopic-microscopic models. Fission barriers are estimated that can be used to eliminate uncertainties in partial fission half-lives and in calculations of evaporation-residue cross-sections. In that calculations, fission probability of the compound nucleus is a major factor contributing to the total cross-section. The data also provide constraints on the cross-sections of capture and quasi-fission in the entrance channel of the fusion reaction. Arguments are presented that fusion reactions for synthesis of isotopes of elements 118 and 120 may have higher cross-sections than assumed so far.

論文

Experimental study of the $$^{66}$$Ni($$d$$,$$p$$)$$^{67}$$Ni one-neutron transfer reaction

Diriken, J.*; Patronis, N.*; Andreyev, A.; Antalic, S.*; Bildstein, V.*; Blazhev, A.*; Darby, I. G.*; De Witte, H.*; Eberth, J.*; Elseviers, J.*; et al.

Physical Review C, 91(5), p.054321_1 - 054321_15, 2015/05

 被引用回数:8 パーセンタイル:37.23(Physics, Nuclear)

Excited states up to an excitation energy of 5.8 MeV were populated in the neutron-rich isotope $$^{67}$$Ni via the $$^{66}$$Ni(d,p) transfer reaction at REX-Isolde, CERN. In particular, single-neutron states above the N=40 sub-shell gap were populated, and the relative spectroscopic factors were extracted using distorted-wave Born approximation analysis. The positive parity g$$_{9/2}$$, d$$_{5/2}$$ and s$$_{1/2}$$ neutron orbits above the shell closure are assumed to induce strong quadrupole collectivity in neutron-rich Fe and Cr isotopes. The extracted relative spectroscopic factors show that the strength of the d$$_{5/2}$$ orbit is mostly split over two states, hinting to substantial mixing of the neutron d$$_{5/2}$$ configuration with collective modes of the core. The size of the N=50 shell gap was also estimated, and found to be 2.6 MeV near $$^{68}$$Ni, as also determined in lighter Ni isotopes.

論文

Empirical description of $$beta$$-delayed fission partial half-lives

Ghys, L.*; Andreyev, A.; Antalic, S.*; Huyse, M.*; Van Duppen, P.*

Physical Review C, 91(4), p.044314_1 - 044314_7, 2015/04

 被引用回数:6 パーセンタイル:46.64(Physics, Nuclear)

The process of $$beta$$-delayed fission ($$beta$$DF) provides a versatile tool to study low-energy fission in nuclei far away from the $$beta$$-stability line, especially for nuclei which do not fission spontaneously. The aim of this paper is to investigate systematic trends in $$beta$$DF partial half-lives. A semi-phenomenological framework was developed to systematically account for the behavior of $$beta$$DF partial half-lives. The $$beta$$DF partial half-life appears to exponentially depend on the difference between the Q value for $$beta$$ decay of the parent nucleus and the fission-barrier energy of the daughter (after $$beta$$ decay) product. Such dependence was found to arise naturally from some simple theoretical considerations. This systematic trend was confirmed for experimental $$beta$$DF partial half-lives spanning over seven orders of magnitude when using fission barriers calculated from either the Thomas-Fermi or the liquid-drop fission model. The same dependence was also observed, although less pronounced, when comparing to fission barriers from the finite-range liquid-drop model or the Thomas-Fermi plus Strutinsky integral method.

論文

In-source laser spectroscopy with the laser ion source and trap; First direct study of the ground-state properties of $$^{217,219}$$Po

Fink, D. A.*; Cocolios, T. E.*; Andreyev, A.; Antalic, S.*; Barzakh, A. E.*; Bastin, B.*; Fedorov, D. V.*; Fedosseev, V. N.*; Flanagan, K. T.*; Ghys, L.*; et al.

Physical Review X, 5(1), p.011018_1 - 011018_15, 2015/01

 被引用回数:17 パーセンタイル:21.7(Physics, Multidisciplinary)

A Laser Ion Source and Trap (LIST) for a thick-target, isotope-separation on-line facility has been implemented at CERN ISOLDE for the production of pure, laser-ionized, radioactive ion beams. The first physics application of the LIST enables the suppression of francium contamination in ion beams of neutron-rich polonium isotopes at ISOLDE by more than 1000 with a reduction in laser-ionization efficiency of only 20. Resonance ionization spectroscopy is performed directly inside the LIST device, allowing the study of the hyperfine structure and isotope shift of $$^{217}$$Po for the first time. Nuclear decay spectroscopy of $$^{219}$$Po is performed for the first time, revealing its half-life, $$alpha$$-to-$$beta$$-decay branching ratio, and $$alpha$$-particle energy. This experiment demonstrates the applicability of the LIST at radioactive ion-beam facilities for the production and study of pure beams of exotic isotopes.

論文

Study of the deformation-driving $$nu$$d$$_{5/2}$$ orbital in $$_{28}^{67}$$Ni$$_{39}$$ using one-neutron transfer reactions

Diriken, J.*; Patronis, N.*; Andreyev, A. N.*; Antalic, S.*; Bildstein, V.*; Blazhev, A.*; Darby, I. G.*; De Witte, H.*; Eberth, J.*; Elseviers, J.*; et al.

Physics Letters B, 736, p.533 - 538, 2014/09

 被引用回数:12 パーセンタイル:28.45(Astronomy & Astrophysics)

The neutron orbits $$g_{9/2}$$, d$$_{5/2}$$ and s$$_{1/2}$$ are assumed to be responsible for the swift onset of collectivity observed in the region below $$^{68}$$Ni. In order to gather information on the single-particle energies and spectroscopic factors of these orbitals, single-particle states in the nucleus $$^{67}$$Ni were populated using the reaction $$^{66}$$Ni(d,p), in inverse kinematics, at REX-ISOLDE, CERN. The new isotope was studied using combined particle-$$gamma$$ spectroscopy. Comparison with DWBA calculations, permitted the identification of positive parity states with a substantial amount of $$nu$$d$$_{9/2}$$ (1007 keV) and $$nu$$d$$_{5/2}$$ (2207 and 3277 keV) single-particle strength. Comparisons with extended Shell-Model calculations was also performed to confirm the single-particle nature of these states, and to deduce general properties around $$^{68}$$Ni.

論文

$$beta$$-delayed fission of $$^{180}$$Tl

Elseviers, J.*; Andreyev, A. N.*; Huyse, M.*; Van Duppen, P.*; Antalic, S.*; Barzakh, A.*; Bree, N.*; Cocolios, T. E.*; Comas, V. F.*; Diriken, J.*; et al.

Physical Review C, 88(4), p.044321_1 - 044321_13, 2013/10

 被引用回数:29 パーセンタイル:10.63(Physics, Nuclear)

The detailed analysis of the $$beta$$-delayed fission data of $$^{180}$$Tl is presented. The experiment was performed by producing a pure beam of $$^{180}$$Tl by means of highly selective resonance laser ionization followed by mass separation with the ISOLDE isotope separator. A surprising asymmetric mass distribution of fission fragments from $$^{180}$$Hg, the daughter of $$^{180}$$Tl $$beta$$ decays, was obtained. Here, the energy calibration of the silicon detectors, which is crucial for a proper determination of the fission fragments' energy and mass split, is presented and the total kinetic energy and its dependence on the mass split ratio is discussed. A more precise $$beta$$-delayed fission probability of 3.2(2)$$times$$10$$^{-3}$$$$%$$ was deduced.

論文

Signature of the Z=82 shell closure in $$alpha$$-decay process

Andreyev, A. N.*; Huyse, M.*; Van Duppen, P.*; Qi, C.*; Liotta, R. J.*; Antalic, S.*; Ackermann, D.*; Franchoo, S.*; He${ss}$berger, F. P.*; Hofmann, S.*; et al.

Physical Review Letters, 110(24), p.242502_1 - 242502_5, 2013/06

 被引用回数:53 パーセンタイル:7.94(Physics, Multidisciplinary)

$$alpha$$-decay data for more than 20 nuclei of the most neutron-deificient isotopes in the region from lead to thorium was obtained. The combined analysis allowed us for the first time to clearly show that crossing the Z=82 shell to higher proton numbers strongly accelerates the $$alpha$$ decay. The analysis support the conjecture that both the N=126 and Z=82 shell closures stongly influence the $$alpha$$-formation probability.

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