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Journal Articles

Visualisation and quantitative evaluation of chlorides in corroded crevice of stainless steel using radioisotope $$^{36}$$Cl$$^{-}$$

Aoki, So; Abe, Yosuke; Abe, Hiroshi*; Watanabe, Yutaka*; Yamamoto, Masahiro*

Corrosion Science, 255, p.113119_1 - 113119_10, 2025/10

 Times Cited Count:0 Percentile:0.00(Materials Science, Multidisciplinary)

This study aimed to visualise the distribution of chloride in the corroded crevice of stainless steel and to evaluate the chloride content quantitatively. Crevice corrosion tests were carried out using $$^{36}$$Cl$$^{-}$$, a radioactive isotope of chloride, as a tracer in NaCl test solutions. After crevice corrosion tests, stainless steel specimens were placed on an imaging plate. The imaging plate was sensitised by $$beta$$-ray emitted by $$^{36}$$Cl$$^{-}$$ adhering to the crevice. As a result, the chloride distribution in the corroded area inside the crevice was visualised. A calibration curve for the amount of $$^{36}$$Cl$$^{-}$$ was obtained from the relationship between the time of photosensitivity to $$beta$$-ray emitted by $$^{36}$$Cl$$^{-}$$ and the luminance of the imaging plate. The chloride content in the corroded crevice was quantitatively evaluated based on the calibration curve. These visualisation and quantitative evaluation methods were also applied to tests in which specimens were left in pure water after crevice corrosion tests, and the behaviour of chloride in crevice corrosion was discussed.

Journal Articles

Modeling the extraction of bound rubber from silica-filled styrene-butadiene rubber with toluene

Tamura, Yukiko*; Arakawa, Masato*; Takenaka, Mikihito*; Nakanishi, Yohei*; Fujinami, So*; Shibata, Motoki*; Yamamoto, Katsuhiro*; Miyata, Noboru*; Yamada, Masako*; Seto, Hideki*; et al.

Polymer, 333, p.128662_1 - 128662_8, 2025/08

 Times Cited Count:0 Percentile:0.00(Polymer Science)

Journal Articles

Incommensurate antiferromagnetism in UTe$$_2$$ under pressure

Knafo, W.*; Thebault, T.*; Raymond, S.*; Manuel, P.*; Khalyavin, D. D.*; Orlandi, F.*; Ressouche, E.*; Beauvois, K.*; Lapertot, G.*; Kaneko, Koji; et al.

Physical Review X, 15(2), p.021075_1 - 021075_16, 2025/05

 Times Cited Count:0 Percentile:0.00(Physics, Multidisciplinary)

Journal Articles

Adsorption isotherm and kinetics of diffusion of water accumulated between polypropylene thin film and Si substrate; Neutron reflectivity investigation

Miyazaki, Tsukasa*; Miyata, Noboru*; Arima-Osonoi, Hiroshi*; Shimokita, Keisuke*; Yamamoto, Katsuhiro*; Takenaka, Mikihito*; Nakanishi, Yohei*; Shibata, Motoki*; Aoki, Hiroyuki; Yamada, Norifumi*; et al.

Colloids and Surfaces A; Physicochemical and Engineering Aspects, 701, p.134928_1 - 134928_8, 2024/11

 Times Cited Count:0 Percentile:0.00(Chemistry, Physical)

Journal Articles

Characterization of mineral composition using PIXE and EXAFS analyses to elucidate the Barium adsorption mechanism

Oguri, Kaori; Hagura, Naoto*; Yamaguchi, Akiko; Okumura, Masahiko; Matsuura, Haruaki*; Tsunashima, Yasumichi; Aoki, Katsumi; Arai, Yoichi; Watanabe, So

Nuclear Instruments and Methods in Physics Research B, 556, p.165516_1 - 165516_8, 2024/11

 Times Cited Count:0 Percentile:0.00(Instruments & Instrumentation)

Ningyo-toge is the uranium mine that has been operated in Japan. Various radioactive elements such as Uranium (U), and Radium (Ra) are still present in the mine ground water with very small amount, and behavior of those elements is not fully understood. In this study, we investigated the composition of metal oxides and clay minerals in a soil of slag deposit at the mine, and systematics of adsorption structure of various ions were examined. Identifying the composition and chemical forms of minerals present in the soil of slag can provide useful information for the safety assessment and evaluation of influence on the surrounding environment.

Journal Articles

Introduction to dismantling and decommissioning chemistry

Sato, Nobuaki*; Kameo, Yutaka; Sato, Soichi; Kumagai, Yuta; Sato, Tomonori; Yamamoto, Masahiro*; Watanabe, Yutaka*; Nagai, Takayuki; Niibori, Yuichi*; Watanabe, Masayuki; et al.

Introduction to Dismantling and Decommissioning Chemistry, 251 Pages, 2024/09

This book focuses on the dismantling and decommissioning of nuclear facilities and reactors that have suffered severe accidents. In Part 1, we introduce basic aspects ranging from fuel chemistry, analytical chemistry, radiation chemistry, corrosion, and decontamination chemistry to waste treatment and disposal. Then, Part 2 covers the chemistry involved in the decommissioning of various nuclear facilities, and discusses what chemical approaches are necessary and possible for the decommissioning of TEPCO's Fukushima Daiichi Nuclear Power Plants, how decommissioning should be carried out, and what kind of research and development and also human resource development are required for this.

Journal Articles

Measuring unit for synchronously collecting air dose rate and measurement position

Kawabata, Kuniaki; Imabuchi, Takashi; Shirasaki, Norihito*; Suzuki, Soichiro; Ito, Rintaro; Aoki, Yuto; Omori, Takazumi

ROBOMECH Journal (Internet), 11, p.11_1 - 11_11, 2024/09

Journal Articles

Stability enhancement by hydrophobic anchoring and a cross-linked structure of a phospholipid copolymer film for medical devices

Uchida, Kazuto*; Masuda, Tsukuru*; Hara, Shintaro*; Matsuo, Yoichi*; Liu, Y.*; Aoki, Hiroyuki; Asano, Yoshihiko*; Miyata, Kazuki*; Fukuma, Takeshi*; Ono, Toshiya*; et al.

ACS Applied Materials & Interfaces, 16(30), p.39104 - 39116, 2024/07

 Times Cited Count:2 Percentile:22.47(Nanoscience & Nanotechnology)

Journal Articles

Influence of MC carbides on pitting corrosion resistance of weld metal in austenitic stainless steels

Kadoi, Kota*; Kanno, Yudai*; Aoki, So; Inoue, Hiroshige*

ISIJ International, 64(9), p.1450 - 1456, 2024/07

 Times Cited Count:1 Percentile:0.00(Metallurgy & Metallurgical Engineering)

The influence of the chemical composition on the pitting corrosion in the weld metal of austenitic stainless steel were investigated. The specimens containing higher content of chromium and molybdenum showed the lower the reactivation rate. The addition of titanium drastically deteriorated the pitting corrosion resistance. The chromium depleted region was formed near the carbide such as M$$_{23}$$C$$_{6}$$ and TiC. Besides, TiC phase which formed during solidification acted as nucleation sites for M$$_{23}$$C$$_{6}$$ precipitation. The depleted region caused by chromium diffusion because of the M$$_{23}$$C$$_{6}$$ precipitation, induced to deteriorate the pitting corrosion resistance.

Journal Articles

A Focusing supermirror for time-of-flight grazing-incidence small-angle neutron scattering measurement

Yamazaki, Dai; Maruyama, Ryuji; Aoki, Hiroyuki; Hanashima, Takayasu*; Akutsu-Suyama, Kazuhiro*; Miyata, Noboru*; Soyama, Kazuhiko

Quantum Beam Science (Internet), 9(2), p.20_1 - 20_12, 2024/06

Journal Articles

Generality assessment of a model considering heterogeneous cancer cells for predicting tumor control probability for stereotactic body radiation therapy against non-small cell lung cancer

Saga, Ryo*; Matsuya, Yusuke; Obara, Hideki*; Komai, Fumio*; Yoshino, Hironori*; Aoki, Masahiko*; Hosokawa, Yoichiro*

Advances in Radiation Oncology (Internet), 9(4), p.101437_1 - 101437_5, 2024/04

The curative effects after radiotherapy are evaluated by the index of tumor control probability (TCP), and the treatment regimen has been determined empirically based on clinical experiences. In recent years, in order to determine TCP for any treatment regimens based on cell experiments, it is necessary to consider the existence of radioresistant cancer stem cells, which are included in tumors at from a few to several tens of percent. Our previous study has proposed an integrated microdosimetric-kinetic (IMK) model that explicitly considers cancer stem cells, and successfully reproduced cancer cell death obtained from cell experiments and clinical TCP. However, the verification so far has been limited to comparison with the clinical data of Hirosaki University Hospital, and comparative verification with clinical data of other facilities has not been performed. In this study, we focused on the stereotactic radiotherapy against non-small cell lung cancer that prescribes a large dose at once, and compared the public data collected by meta-analysis with the IMK model. As a result, it was found that the IMK model considering cancer stem cells well reproduced the clinical TCP regardless of the observed facility type. This work would contribute to the development of technology for predicting curative effects of radiotherapy with high precision.

Journal Articles

Properties of duplex stainless steels

Aoki, So; Sakai, Junichi*

Zairyo To Kankyo, 73(3), p.49 - 56, 2024/03

This paper briefly reviews the history of the development of duplex stainless steels and summarises the grades that are currently standardised in JIS and used industrially. The chemical composition, phase equilibrium and phase transformation of duplex stainless steels are described, showing the basic data. The physical and mechanical properties of the duplex stainless steels are touched upon, and in particular the resistance to uniform corrosion and localised corrosion such as pitting corrosion, crevice corrosion and stress corrosion cracking are outlined, citing previously published data. Finally, the main environments in which duplex stainless steels are used and the results of their use are mentioned.

Journal Articles

Development of a D$$_2$$O/H$$_2$$O vapor generator for contrast-variation neutron scattering

Arima-Osonoi, Hiroshi*; Takata, Shinichi; Kasai, Satoshi*; Ouchi, Keiichi*; Morikawa, Toshiaki*; Miyata, Noboru*; Miyazaki, Tsukasa*; Aoki, Hiroyuki; Iwase, Hiroki*; Hiroi, Kosuke; et al.

Journal of Applied Crystallography, 56(6), p.1802 - 1812, 2023/12

 Times Cited Count:6 Percentile:78.07(Chemistry, Multidisciplinary)

Journal Articles

Transient analyses of hydraulic head in the fault slip experiments in fracture zones of Shionohira and Kuruma Faults

Wakahama, Hiroshi*; Nojo, Haruka*; Aoki, Kazuhiro; Imai, Hirotaro; Guglielmi, Y.*; Cook, P.*; Soom, F.*

Oyo Chishitsu, 64(5), p.236 - 254, 2023/12

Upon the Hamadori earthquake (Mw 6.7) of 11 April 2011, coseismic surface deformation of 14 km running NNW to SSE in southeast Fukushima Prefecture occurred and was newly named the Shionohira Fault. However, no surface deformation was observed along the Kuruma Fault which is a southern extension of the Shionohira Fault. Fault injection tests using SIMFIP method at the Shionohira site on the former active segment and the Minakamikita site on the latter inactive segment were conducted to evaluate the activity of the two faults. Based on hydraulic responses to water injection into the fault rupture zone in the monitoring boreholes at the two sites, hydraulic properties of the area across the fault zone were estimated using the GRF model (Barker, 1988). The results obtained on hydraulic conductivity, specific storage and flow dimension were consistent with those in the domestic and international literature. The hydraulic conductivity and specific storage were larger in Shionohira than in Minakamikita. The flow dimension of Shionohira was three-dimensional, while that of Minakamikita was found to be a two-dimensional fractional flow. In addition, it is understood that the volumetric expansion occurs in the former site in the triaxial direction and the latter in the uniaxial with the comparison between the uniaxial expansion coefficient calculated from the results of SIMFIP displacement measurements and the specific storage in the hydraulic analysis. The difference in the hydraulic parameters between the two sites corresponded to the difference in the spatial development of fractures considered to be the "water passway," indicating the possibility of a correlation between the parameters and the different possible causes for fault activity at the two sites.

Journal Articles

Time-lapse observation of crevice corrosion in grade 2205 duplex stainless steel

Aoki, So; Engelberg, D. L.*

Materials, 16(15), p.5300_1 - 5300_13, 2023/08

 Times Cited Count:4 Percentile:44.19(Chemistry, Physical)

The objective of this study was to investigate and visualize the initiation and propagation behaviour of crevice corrosion in grade 2205 duplex stainless steel by means of time-lapse, in-situ observations. All observed crevice corrosion initiated close to the edge of the washer, where the crevice gap was very tight. Crevice corrosion then expanded underneath the crevice forming disk into areas with wider gaps towards the crevice mouth. This was associated with a rise in anodic current, leading into hydrogen gas evolution within the crevice. Once crevice corrosion reached the crevice mouth, the corrosion propagated Circumferentially, but also in depth.

Journal Articles

Translational study for stereotactic body radiotherapy against non-small cell lung cancer, including oligometastases, considering cancer stem-like cells enable predicting clinical outcome from ${it in vitro}$ data

Saga, Ryo*; Matsuya, Yusuke; Sato, Hikari*; Hasegawa, Kazuki*; Obara, Hideki*; Komai, Fumio*; Yoshino, Hironori*; Aoki, Masahiko*; Hosokawa, Yoichiro*

Radiotherapy and Oncology, p.109444_1 - 109444_9, 2023/00

 Times Cited Count:3 Percentile:46.29(Oncology)

When treating non-small cell lung cancer (NSCLC), stereotactic body radiotherapy (SBRT) with high-dose irradiation is often utilized. The fractionation schemes and curative effects can be evaluated by mathematical models for predicting cell survival curve. Such model parameters can be determined from in vitro experiment, but they are empirically determined based on experiences in clinics. As such, there is a large gap between in vitro and clinical study. As such background, translational study between in vitro cell survival and clinical curative effects is necessary. In this study, explicitly considering existence of cancer stem-like cells (CSCs), we developed an all-in-one model for predicting both in vitro cell survival and clinical curative effects (integrated microdosimetric-kinetic (IMK) model) and performed retrospective evaluation of clinical outcomes following SBRT for NSCLC in Hirosaki University Hospital. As a result, the IMK model successfully reproduced both in vitro cell survival and the tumor control probability with various fractionation schemes (i.e., 6-10 Gy per fraction). The developed model would contribute on precisely understanding the impact of CSCs on curative effects after SBRT for NSCLC with high precision.

Journal Articles

Neutron reflectivity study on the suppression of interfacial water accumulation between a polypropylene thin film and Si substrate using a silane-coupling agent

Shimokita, Keisuke*; Yamamoto, Katsuhiro*; Miyata, Noboru*; Arima-Osonoi, Hiroshi*; Nakanishi, Yohei*; Takenaka, Mikihito*; Shibata, Motoki*; Yamada, Norifumi*; Seto, Hideki*; Aoki, Hiroyuki; et al.

Langmuir, 38(41), p.12457 - 12465, 2022/10

 Times Cited Count:3 Percentile:11.94(Chemistry, Multidisciplinary)

JAEA Reports

Fuel Unloading Operations -2019- in the decommissioning of prototype fast breeder reactor "Monju"

Yabe, Takanori; Murakami, Makio; Shiota, Yuki; Isobe, Yuta; Shiohama, Yasutaka; Hamano, Tomoharu; Takagi, Tsuyohiko; Nagaoki, Yoshihiro

JAEA-Technology 2022-002, 66 Pages, 2022/07

JAEA-Technology-2022-002.pdf:10.45MB

In the first stage of "Monju" decommissioning project, "Fuel Unloading Operations" have been carrying out. The operations consists of two processes. The first process is "Fuel Treatment and Storage" is that the fuel assemblies unloaded from the Ex-Vessel fuel Storage Tank are canned after sodium cleaning, and then transferred to the storage pool. The second process is "Fuel Unloading" that the fuel assemblies in the reactor core are replaced with dummy fuel assemblies and stored in the Ex-Vessel fuel Storage Tank. "Fuel Treatment and Storage" and "Fuel Unloading" are performed alternately until 370 fuel assemblies in the core and 160 fuel assemblies in the Ex-Vessel fuel Storage Tank are all transferred to the storage pool. In fiscal 2018, as "Fuel Treatment and Storage", 86 fuel assemblies were transferred to the storage pool. As "Fuel Unloading", 76 dummy fuel assemblies were stored in the Ex-Vessel fuel Storage Tank. In fiscal 2019, as "Fuel Unloading", 60 fuel assemblies and 40 blanket fuel assemblies were unloaded from the core. These assemblies were stored in the Ex-Vessel fuel Storage Tank, and dummy fuel assemblies were loaded into the core instead. During these operations, a total of 38 cases of alarming or equipment malfunctions classified into 24 types occurred. However, no significant events that menaces to safety have occurred. The operations were continued safely by removing the direct factors for the malfunctions in the equipment operation and performance.

JAEA Reports

Fuel unloading work in decommissioning of the prototype fast breeder reactor Monju; Fuel treatment and storage work in 2018 and 2019

Shiota, Yuki; Yabe, Takanori; Murakami, Makio; Isobe, Yuta; Sato, Masami; Hamano, Tomoharu; Takagi, Tsuyohiko; Nagaoki, Yoshihiro

JAEA-Technology 2022-001, 117 Pages, 2022/07

JAEA-Technology-2022-001.pdf:25.55MB

In the first stage of Monju decommissioning project, fuel unload work began to be carried out. There are two tasks in this work. One is fuel treatment and storage work that gets rid of sodium on the fuel assemblies unloaded from Ex-Vessel fuel Storage Tank (EVST) and carries it in the storage pool, and the other is fuel unloading that the fuel assemblies in the reactor core is replaced with dummy fuels and stored in EVST. Fuel treatment and storage work and fuel unloading work are performed alternately, and 370 bodies in the core and 160 pieces in EVST are all carried to the storage pool. 86 fuel assemblies was carried to the storage pool in fuel treatment and storage work in 2018 and 76 dummy fuels were stored in EVST for fuel unloading work. During the work, 86 types and 232 alarms / malfunctions occurred, but there was no impact on safety. There was one equipment's failure at gripper's claw open / close clutch of ex-vessel fuel transfer machine B, but it was repaired and restarted. Also it was eliminated the cause of problem or concession that the equipment failure due to the sticking of the sodium compound and continuous use of the equipment. Some problems related to system control occurred, but the work was done after checking the safety. With estimation of various troubles, reduction of frequency of trouble occurrence and minimization of impacts on schedule performed.

Journal Articles

Unconventional superconductivity in UTe$$_2$$

Aoki, Dai*; Brison, J.-P.*; Flouquet, J.*; Ishida, Kenji*; Knebel, G.*; Tokunaga, Yo; Yanase, Yoichi*

Journal of Physics; Condensed Matter, 34(24), p.243002_1 - 243002_41, 2022/06

 Times Cited Count:147 Percentile:89.95(Physics, Condensed Matter)

143 (Records 1-20 displayed on this page)