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Tomiyasu, Keisuke*; Ito, Naoko*; Okazaki, Ryuji*; Takahashi, Yuki*; Onodera, Mitsugi*; Iwasa, Kazuaki*; Nojima, Tsutomu*; Aoyama, Takuya*; Ogushi, Kenya*; Ishikawa, Yoshihisa*; et al.
Advanced Quantum Technologies (Internet), 1(3), p.1800057_1 - 1800057_7, 2018/12
Spin-state transition, also known as spin crossover, plays a key role in diverse systems. In theory, the boundary range between the low- and high-spin states is expected to enrich the transition and give rise to unusual physical states. However, no compound that realizes a nearly degenerate critical range as the ground state without requiring special external conditions has yet been experimentally identified. This study reports that the Sc substitution in LaCoO3 destabilizes its nonmagnetic low-spin state and generates an anomalous paramagnetic state accompanied by the enhancement of transport gap and magneto-lattice-expansion as well as the contraction of Co-O distance with the increase of electron site transfer. These phenomena are not well described by the mixture of conventional low- and high-spin states, but by their quantum superposition occurring on the verge of a spin-state transition.
Tomizawa, Hiromitsu*; Sato, Takahiro*; Ogawa, Kanade*; Togawa, Kazuaki*; Tanaka, Takatsugu*; Hara, Toru*; Yabashi, Makina*; Tanaka, Hitoshi*; Ishikawa, Tetsuya*; Togashi, Tadashi*; et al.
High Power Laser Science and Engineering, 3, p.e14_1 - e14_10, 2015/04
Times Cited Count:8 Percentile:39.66(Optics)no abstracts in English
Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Yamanouchi, Kaoru*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Togashi, Tadashi*; Fukami, Kenji*; et al.
Journal of Physics B; Atomic, Molecular and Optical Physics, 46(16), p.164006_1 - 164006_6, 2013/08
Times Cited Count:3 Percentile:17.90(Optics)By introducing 13th- (61.7 nm) and 15th-order harmonics (53.4 nm) of femtosecond laser pulses at 800 nm into an undulator of SCSS (SPring-8 Compact SASE Source) test accelerator at RIKEN, these harmonic pulses were amplified by a factor of more than 10
with a high contrast ratio through the interaction between accelerated electron bunches and the harmonic pulses. From numerical simulations of the amplification processes of high-order harmonic pulses in the undulator, optimum conditions of the electron bunch duration interacting with the high-order harmonic pulses were investigated for generating full-coherent and intense pulses in the extreme ultraviolet wavelength region.
Togashi, Tadashi*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Okino, Tomoya*; Yamanouchi, Kaoru*; et al.
Optics Express (Internet), 19(1), p.317 - 324, 2011/01
Times Cited Count:97 Percentile:95.90(Optics)The 13th harmonic of a Ti:sapphire (Ti:S) laser in the plateau region was injected as a seeding source to a 250-MeV free-electron-laser (FEL) amplifier. When the amplification conditions were fulfilled, strong enhancement of the radiation intensity by a factor of 650 was observed. The random and uncontrollable spikes, which appeared in the spectra of the Self-Amplified Spontaneous Emission (SASE) based FEL radiation without the seeding source, were found to be suppressed drastically to form to a narrow-band, single peak profile at 61.2 nm. The properties of the seeded FEL radiation were well reproduced by numerical simulations. We discuss the future precept of the seeded FEL scheme to the shorter wavelength region.
Tsutagi, Koichi; Yoshino, Yasuyuki; Aoyama, Kazuaki; Tomiyama, Masahiro; Uchida, Toyomi; Nakamura, Yoshinobu
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Tomizawa, Hiromitsu*; Hara, Toru*; Ishikawa, Tetsuya*; Ogawa, Kanade*; Tanaka, Hitoshi*; Tanaka, Takatsugu*; Togashi, Tadashi*; Togawa, Kazuaki*; Yabashi, Makina*; Aoyama, Makoto; et al.
no journal, ,
no abstracts in English
Matsubara, Shinichi*; Aoyama, Makoto; Iwasaki, Atsushi*; Okayasu, Yuichi*; Ogawa, Kanade*; Owada, Shigeki*; Sato, Takahiro*; Takahashi, Eiji*; Tanaka, Takashi*; Togashi, Tadashi*; et al.
no journal, ,
no abstracts in English
Watanabe, Takahiro*; Aoyama, Makoto; Iwasaki, Atsushi*; Otake, Yuji*; Oshima, Takashi*; Okayasu, Yuichi*; Ogawa, Kanade*; Owada, Shigeki*; Sato, Takahiro*; Togashi, Tadashi*; et al.
no journal, ,
no abstracts in English