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JAEA Reports

Development of hydrogen behavior integrated analysis system

Terada, Atsuhiko; Thwe Thwe, A.; Hino, Ryutaro*; Harai, Yasutaka*; Sasaki, Gaku*; Shingeya, Hideshi*; Yamashita, Toshiyuki*; Yoneda, Jiro*; Okabayashi, Kazuki*; Sakamoto, Hiroyuki*; et al.

JAEA-Data/Code 2025-012, 151 Pages, 2025/12

JAEA-Data-Code-2025-012.pdf:9.69MB

Based on the lessons learned from the Fukushima Daiichi Nuclear Power Station accident, we have highly paid attention to the advancement of the fundamental technologies which are indispensable in timely response to hydrogen safety measures and assessments especially in both nuclear reactors and decommissioning. Focusing on this attention, we developed an analysis system that predicts the behavior of hydrogen from generation to diffusion, combustion and explosion. The system utilizes the commercial computational fluid dynamics software (FLUENT, AUTODYN), and incorporates new modules and pre/post-processors in order to withstand the general practical use. We also developed a system by utilizing open-source code (OpenFOAM) that can be used in hydrogen disaster prevention plans for nuclear facilities. So far, we have expanded the system to deal with the phenomena that should be considered from the practical point of view for PWR (Pressurized Water Reactor) in nuclear power plants. This report summarizes the overview of the integrated analysis system for hydrogen behavior, the handling method, and real scale analysis examples.

Journal Articles

Development of dose estimation method using wild animal teeth for low dose exposure

Mitsuyasu, Yusuke*; Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; et al.

KEK Proceedings 2021-2, p.91 - 96, 2021/12

We examined whether the ESR dose estimation method could be applied to wild Japanese macaque. In this work, we investigated the enamel preparation protocol and the analytical method of the ESR spectra.

Journal Articles

Rapid analysis of $$^{90}$$Sr in cattle bone and tooth samples by inductively coupled plasma mass spectrometry

Koarai, Kazuma; Matsueda, Makoto; Aoki, Jo; Yanagisawa, Kayo*; Terashima, Motoki; Fujiwara, Kenso; Kino, Yasushi*; Oka, Toshitaka; Takahashi, Atsushi*; Suzuki, Toshihiko*; et al.

Journal of Analytical Atomic Spectrometry, 36(8), p.1678 - 1682, 2021/08

 Times Cited Count:10 Percentile:52.81(Chemistry, Analytical)

Rapid analysis of $$^{90}$$Sr in bone and tooth samples of cattle were achieved by an inductively coupled plasma mass spectrometry (ICP-MS) coupled with mass shift and solid phase extraction techniques. Limit of detection (LOD) in the ICP-MS measurement of 0.1 g samples was lower than that of the radioactivity measurement. Analytical time of the ICP-MS method was reduced from 20 days to 11 hours, compared with the radiometric method. Therefore, the ICP-MS method can be rapid and useful procedure of $$^{90}$$Sr in small bone and tooth samples derived from terrestrial animals.

Journal Articles

Thermally altered subsurface material of asteroid (162173) Ryugu

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.

Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03

 Times Cited Count:66 Percentile:94.57(Astronomy & Astrophysics)

Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 $$^{circ}$$C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200 $$^{circ}$$C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.

Journal Articles

External exposure dose estimation by electron spin resonance technique for wild Japanese macaque captured in Fukushima Prefecture

Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Mitsuyasu, Yusuke*; Kino, Yasushi*; Sekine, Tsutomu*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; Osaka, Ken*; et al.

Radiation Measurements, 134, p.106315_1 - 106315_4, 2020/06

 Times Cited Count:10 Percentile:60.65(Nuclear Science & Technology)

The relationship between the CO$$_{2}$$ radical intensity and the absorbed dose (dose response curve) of tooth enamel of Japanese macaque was observed by electron spin resonance and the detection limit of our system was estimated to be 33.5 mGy, which is comparable to the detection limit for human molar teeth. Using the dose response curve, external exposure dose for seven wild Japanese macaques captured in Fukushima prefecture were examined. The results suggest that the external exposure dose for the wild Japanese macaques were ranged between 45 mGy to 300 mGy.

Journal Articles

The Surface composition of asteroid 162173 Ryugu from Hayabusa2 near-infrared spectroscopy

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Arai, Takehiko*; Nakauchi, Yusuke*; Nakamura, Tomoki*; Matsuoka, Moe*; et al.

Science, 364(6437), p.272 - 275, 2019/04

 Times Cited Count:342 Percentile:99.61(Multidisciplinary Sciences)

The near-Earth asteroid 162173 Ryugu, the target of Hayabusa2 sample return mission, is believed to be a primitive carbonaceous object. The Near Infrared Spectrometer (NIRS3) on Hayabusa2 acquired reflectance spectra of Ryugu's surface to provide direct measurements of the surface composition and geological context for the returned samples. A weak, narrow absorption feature centered at 2.72 micron was detected across the entire observed surface, indicating that hydroxyl (OH)-bearing minerals are ubiquitous there. The intensity of the OH feature and low albedo are similar to thermally- and/or shock-metamorphosed carbonaceous chondrite meteorites. There are few variations in the OH-band position, consistent with Ryugu being a compositionally homogeneous rubble-pile object generated from impact fragments of an undifferentiated aqueously altered parent body.

Journal Articles

Development status of the NMR system for the polarized $$^{3}$$He Neutron Spin Filter (NSF) in the MLF at J-PARC

Sakai, Kenji; Oku, Takayuki; Hayashida, Hirotoshi*; Kira, Hiroshi*; Hiroi, Kosuke; Ino, Takashi*; Oyama, Kenji*; Okawara, Manabu*; Kakurai, Kazuhisa; Shinohara, Takenao; et al.

JPS Conference Proceedings (Internet), 8, p.036015_1 - 036015_6, 2015/09

The polarized $$^{3}$$He filter, which polarizes neutrons due to a large neutron absorption cross section of $$^{3}$$He with strong spin selectivity, becomes a convenient neutron spin filter (NSF) because it is operated immediately after its installation in beam lines without any neutron beam adjustments. For realizing such the NSF, a nuclear magnetic resonance (NMR) system is indispensable for monitoring $$^{3}$$He nuclear spin polarization ${it P}$ of the NSF. We have developed the flexible NMR system based on adiabatic fast passage (AFP) and pulse NMR methods by using their complementary features. In comparing with the values of ${it P}$ obtained by neutron transmission measurement at the beam line 10 of the J-PARC, we measured the correlations between the AFP and pulse NMR signals as changing condition of temperature, amplitude and applying period of the radio frequency field for the pulse NMR, and so on. As the results, we confirmed that our system would function enough as the ${it P}$ monitor.

Journal Articles

Radiation response of silicon carbide diodes and transistors

Oshima, Takeshi; Onoda, Shinobu; Iwamoto, Naoya; Makino, Takahiro; Arai, Manabu*; Tanaka, Yasunori*

Physics and Technology of Silicon Carbide Devices, p.379 - 402, 2012/10

SiC is regarded as a promising candidate for electronic devices used in harsh radiation environments because of its high radiation tolerance. Radiation effects on SiC devices are reviewed. Firstly, the Total Ionizing Dose (TID) effect in Metal-Oxide-Semiconductor (MOS) Field Effect Transistors (FETs) is introduced. Then, the radiation hardness of SiC based transistors such as MOSFETs, Metal-Semiconductor (MES) FETs, Static Induction Transistors (SITs) is discussed from the point of view of $$gamma$$-ray irradiation effects. Transient current induced in SiC pn diodes by heavy ions incidence, which is important information on the single event effects (SEEs), is also expressed.

Journal Articles

Spatial, LET and range dependence of enhanced charge collection by single ion strike in 4H-SiC MESFETs

Onoda, Shinobu; Makino, Takahiro; Ono, Shuichi*; Katakami, Shuji*; Arai, Manabu*; Oshima, Takeshi

IEEE Transactions on Nuclear Science, 59(4), p.742 - 748, 2012/08

 Times Cited Count:4 Percentile:28.59(Engineering, Electrical & Electronic)

no abstracts in English

Journal Articles

Development of silicon carbide devices with high radiation resistance

Oshima, Takeshi; Onoda, Shinobu; Tanaka, Yasunori*; Arai, Manabu*

Isotope News, (686), p.8 - 12, 2011/06

no abstracts in English

Journal Articles

Transient response of charge collection by single ion strike in 4H-SiC MESFETs

Onoda, Shinobu; Iwamoto, Naoya; Ono, Shuichi*; Katakami, Shuji*; Arai, Manabu*; Kawano, Katsuyasu*; Oshima, Takeshi

IEEE Transactions on Nuclear Science, 56(6), p.3218 - 3222, 2009/12

 Times Cited Count:19 Percentile:73.46(Engineering, Electrical & Electronic)

no abstracts in English

Oral presentation

Development status of NMR monitor for polarized $$^{3}$$He spin filter at J-PARC/MLF

Sakai, Kenji; Oku, Takayuki; Hayashida, Hirotoshi; Kira, Hiroshi*; Okawara, Manabu*; Shinohara, Takenao; Oikawa, Kenichi; Harada, Masahide; Kakurai, Kazuhisa; Aizawa, Kazuya; et al.

no journal, , 

A polarized $$^{3}$$He spin filter, which polarizes neutrons due to a large neutron absorption cross section of $$^{3}$$He with strong spin selectivity, works as a simple and convenient neutron spin polarizer. For realizing this filter, a device which monitors a polarization of $$^{3}$$He spin filter is indispensable. We developed the $$^{3}$$He polarization monitor based on a nuclear magnetic resonance method by an adiabatic fast passage (AFP NMR) at the MLF of J-PARC. The monitor based on the AFP NMR realizes the polarized $$^{3}$$He spin flipper functioning as the neutron spin polarizer and flipper. However it has disadvantages on the size of $$^{3}$$He cell limited by a RF coil and its complicated device structure. So we have developed the monitor based on a pulse NMR which uses only a pick up coil and enables the simple device structure of its own, and realized the more flexible monitor system by utilizing the both of pulse NMR and AFP NMR.

Oral presentation

FET characteristics of photo-polymerized C$$_{60}$$ thin films on graphene electrodes

Arai, Daijiro; Tanimoto, Hisanori*; Otomo, Manabu; Entani, Shiro; Matsumoto, Yoshihiro*; Sakai, Seiji

no journal, , 

no abstracts in English

Oral presentation

Incorporation record of radionuclides in teeth and otoliths

Koarai, Kazuma; Matsueda, Makoto; Fujiwara, Kenso; Ono, Takumi*; Kino, Yasushi*; Oka, Toshitaka; Okutsu, Kenichi*; Takahashi, Atsushi*; Suzuki, Toshihiko*; Shimizu, Yoshinaka*; et al.

no journal, , 

We have investigated incorporation of $$^{90}$$Sr and $$^{137}$$Cs in teeth of cattle and otoliths of fish. Specific activity of $$^{90}$$Sr in the dentin tissue was higher than that in the enamel tissue. The result shows change of $$^{90}$$Sr incorporation in cattle even within a tooth. Concentrations of stable Sr and Cs were 94 ppm and 3 ppb. Distributions of stable Sr and Cs were uniform in the otolith of fish. If distribution of $$^{90}$$Sr and $$^{137}$$Cs in the otolith was measured, change of $$^{90}$$Sr and $$^{137}$$Cs incorporation into the fish would be found. These findings suggest that distribution patterns of $$^{90}$$Sr and $$^{137}$$Cs in the environment could be estimated from distribution of the radionuclides in the tooth and otolith.

Oral presentation

$$gamma$$-ray irradiation effects on the I-V characteristics of 4H-SiC MESFET

Onoda, Shinobu; Iwamoto, Naoya; Ono, Shuichi*; Katakami, Shuji*; Arai, Manabu*; Kawano, Katsuyasu*; Oshima, Takeshi

no journal, , 

no abstracts in English

Oral presentation

Dose estimation for animals exposed low dose using their teeth

Mitsuyasu, Yusuke*; Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; et al.

no journal, , 

The improvement of the ESR dosimetry is required to apply that for the low-dose exposure of wild animals. We will report our progress of the improvement, and compare the external exposure dose estimated by the ESR dosimetry technique and the calculated result based on the external exposure dose rate of the captured point.

Oral presentation

Rapid analysis of $$^{90}$$Sr in trace amount of bone; Application of inductively coupled plasma mass spectrometry

Koarai, Kazuma; Matsueda, Makoto; Aoki, Jo; Yanagisawa, Kayo*; Terashima, Motoki; Fujiwara, Kenso; Kino, Yasushi*; Oka, Toshitaka; Takahashi, Atsushi*; Suzuki, Toshihiko*; et al.

no journal, , 

Rapid analysis of $$^{90}$$Sr in bone and tooth samples of cattle were achieved by an inductively coupled plasma mass spectrometry (ICP-MS) coupled with mass shift and solid phase extraction techniques. Limit of detection (LOD) in the ICP-MS measurement of 0.1 g samples was lower than that of the radioactivity measurement. Analytical time of the ICP-MS method was reduced from 20 days to 11 hours, compared with the radiometric method. Therefore, the ICP-MS method can be rapid and useful procedure of $$^{90}$$Sr in small bone and tooth samples derived from terrestrial animals.

Oral presentation

Development of analytical method for Sr-90 using ICP-MS; Aim for Sr-90 measurement for otolith

Koarai, Kazuma; Matsueda, Makoto; Aoki, Jo; Yanagisawa, Kayo*; Terashima, Motoki; Fujiwara, Kenso; Kino, Yasushi*; Oka, Toshitaka; Takahashi, Atsushi*; Suzuki, Toshihiko*; et al.

no journal, , 

Rapid analysis of $$^{90}$$Sr in bone and tooth samples of cattle were achieved by an inductively coupled plasma mass spectrometry (ICP-MS) coupled with mass shift and solid phase extraction techniques. Limit of detection (LOD) in the ICP-MS measurement of 0.1 g samples was lower than that of the radioactivity measurement. Analytical time of the ICP-MS method was reduced from 20 days to 11 hours, compared with the radiometric method. The ICP-MS method was improved by ICP-MS/MS and oxygen-ammonia mixed gas reaction.

Oral presentation

Spectral characteristics of asteroid (162173) Ryugu with Hayabusa2 NIRS3

Takir, D.*; Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Arai, Takehiko*; Nakauchi, Yusuke*; Nakamura, Tomoki*; et al.

no journal, , 

JAXA spacecraft and sample return mission Hayabusa2 has arrived at the near-Earth asteroid 162173 Ryugu, which is classified a primitive carbonaceous object. Here we report recent results of near-infrared spectrometer (NIRS3) on the Hayabusa2 spacecraft. The observations provide direct measurements of the surface composition of Ryugu and context for the returned samples. NIRS3 has detected a weak and narrow absorption feature centered at 2.72 micrometer across entire observed surface. This absorption feature is attributed to the presence of OH-bearing minerals. The NIRS3 observations also revealed that Ryugu is the darkest object to be observed up-close by a visiting spacecraft. The intensity of the OH feature and low albedo are consistent with thermally-and/or shock-metamorphosed, and/or carbon-rich space-weathered primitive and hydrated carbonaceous chondrites.

Oral presentation

Strontium-90 measurement in trace amount of hard tissues for distribution analysis

Koarai, Kazuma; Matsueda, Makoto; Aoki, Jo; Yanagisawa, Kayo*; Fujiwara, Kenso; Terashima, Motoki; Kino, Yasushi*; Oka, Toshitaka; Okutsu, Kenichi*; Yamashita, Takuma*; et al.

no journal, , 

We demonstrated a method of $$^{90}$$Sr measurement in small pieces of hard tissues with radioactivity measurement or ICP-MS measurement. Interference elements of the measurements were removed by chemical separation. We could determine $$^{90}$$Sr in 0.1 g of hard tissues by radioactivity measurement method and ICP-MS method. Limit of detection of the ICP-MS method was lower than that of the radioactivity measurement. The ICP-MS method is adequate method for distribution analysis of $$^{90}$$Sr in the hard tissues.

33 (Records 1-20 displayed on this page)