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Journal Articles

Small dispersion limit of momentum conservation law

Sasa, Narimasa

JSIAM Letters, 16, p.37 - 40, 2024/06

Numerical properties of the momentum conservation law for Hamiltonian PDEs are investigated based on a symplectic time integration. In the nonlinear Klein-Gordon system, it is shown that the critical value of the coefficient of the dispersion term is nearly proportional to the inverse square of the total grid number. The result is consistent with the scaling law. On the other hand, in the nonlinear Schr$"o$dinger-type system, the critical value of the coefficient does not follow the scaling law.

Journal Articles

Field-induced insulator-metal transition in EuTe$$_2$$

Takeuchi, Tetsuya*; Honda, Fuminori*; Aoki, Dai*; Haga, Yoshinori; Kida, Takanori*; Narumi, Yasuo*; Hagiwara, Masayuki*; Kindo, Koichi*; Karube, Kosuke*; Harima, Hisatomo*; et al.

Journal of the Physical Society of Japan, 93(4), p.044708_1 - 044708_10, 2024/04

 Times Cited Count:0 Percentile:0.00(Physics, Multidisciplinary)

Journal Articles

Observation of high-pressure polymorphs in bulk silicon formed at relativistic laser intensities

Rapp, L.*; Matsuoka, Takeshi*; Firestein, K. L.*; Sagae, Daisuke*; Habara, Hideaki*; Mukai, Keiichiro*; Tanaka, Kazuo*; Gamaly, E. G.*; Kodama, Ryosuke*; Seto, Yusuke*; et al.

Physical Review Research (Internet), 6(2), p.023101_1 - 023101_18, 2024/04

It is generally known that irradiating a solid surface with a laser pulse of ultra-relativistic intensity generates a plasma on the surface, which in turn creates an ultrahigh pressure inside. In this study, the crystal structure analysis of high-pressure phases generated inside silicon single-crystals irradiated by this laser was performed using the diffraction system at the Stress and Imaging apparatus of BL22XU, which is a JAEA-BL. The results obtained confirm the existence of high-pressure phases that silicon is said to possess: body-centered, rhombohedral, hexagonal, and tetragonal phases in the interior. We can get the results that the crystal structure of silicon polymorphs of being include body-centered, rhombohedral, hexagonal-diamond, tetragonal exists. In the future, we will accumulate data and apply them to control the internal structure, strength, and functionality of materials.

Journal Articles

Flexible waste management system for the future application of MA P&T technology to the current high-level liquid waste

Fukasawa, Tetsuo*; Suzuki, Akihiro*; Endo, Yoichi*; Inagaki, Yaohiro*; Arima, Tatsumi*; Muroya, Yusa*; Endo, Keita*; Watanabe, Daisuke*; Matsumura, Tatsuro; Ishii, Katsunori; et al.

Journal of Nuclear Science and Technology, 61(3), p.307 - 317, 2024/03

 Times Cited Count:2 Percentile:27.70(Nuclear Science & Technology)

A flexible waste management system (FWM) is being developed to apply future MA partitioning and transmutation (P&T) technology to current HLLW. This FWM system will store high-level waste (HLLW) in granular form until MA partitioning and transmutation technology is realized. The feasibility of the main process was essentially confirmed by basic experiments and preliminary thermal analysis for granule production by rotary kiln from simulated HLLW and for temporary storage (50 years) of HLW granules at the HLW storage facility, respectively. The granule production experiments revealed that relatively large particles can be produced by the rotary kiln. The results of the thermal analysis showed that the small diameter canisters could be used to safely store the granules at a higher storage density than vitrified HLW. The effectiveness of the FWM system in terms of potential radiotoxicity and repository area was also evaluated, and it was shown that FWM can reduce these factors and has significant advantages in the disposal of HLW generated in current reprocessing plants. Since LWR fuel is stored for a long period of time in Japan and the operation of a reprocessing plant is expected to start soon, the FWM system is considered to be an effective system for reducing the environmental burden of HLW disposal.

Journal Articles

Uranium-plutonium-americium cation interdiffusion in polycrystalline (U,Pu,Am)O$$_{2 pm x}$$ mixed oxides

Vauchy, R.; Matsumoto, Taku; Hirooka, Shun; Uno, Hiroki*; Tamura, Tetsuya*; Arima, Tatsumi*; Inagaki, Yaohiro*; Idemitsu, Kazuya*; Nakamura, Hiroki; Machida, Masahiko; et al.

Journal of Nuclear Materials, 588, p.154786_1 - 154786_13, 2024/01

 Times Cited Count:6 Percentile:87.16(Materials Science, Multidisciplinary)

Journal Articles

Magnetic boson peak in classical spin glasses

Kofu, Maiko; Kawamura, Seiko; Murai, Naoki; Ishii, Rieko*; Hirai, Daigoro*; Arima, Hiroshi*; Funakoshi, Kenichi*

Physical Review Research (Internet), 6(1), p.013006_1 - 013006_9, 2024/01

Journal Articles

Structural changes of polystyrene particles in subcritical and supercritical water revealed by in situ small-angle neutron scattering

Shibata, Motoki*; Nakanishi, Yohei*; Abe, Jun*; Arima, Hiroshi*; Iwase, Hiroki*; Shibayama, Mitsuhiro*; Motokawa, Ryuhei; Kumada, Takayuki; Takata, Shinichi; Yamamoto, Katsuhiro*; et al.

Polymer Journal, 55(11), p.1165 - 1170, 2023/11

 Times Cited Count:2 Percentile:20.65(Polymer Science)

Journal Articles

Single crystal growths and magnetic properties of hexagonal polar semimetals $$R$$AuGe ($$R$$ = Y, Gd-Tm, and Lu)

Kurumaji, Takashi*; Gen, Masaki*; Kito, Shunsuke*; Ikeuchi, Kazuhiko*; Nakamura, Mitsutaka; Ikeda, Akihiko*; Arima, Takahisa*

Journal of Alloys and Compounds, 947, p.169475_1 - 169475_8, 2023/06

 Times Cited Count:4 Percentile:48.75(Chemistry, Physical)

Journal Articles

Crystallinity in periodic nanostructure surface on Si substrates induced by near- and mid-infrared femtosecond laser irradiation

Miyagawa, Reina*; Kamibayashi, Daisuke*; Nakamura, Hirotaka*; Hashida, Masaki*; Zen, H.*; Somekawa, Toshihiro*; Matsuoka, Takeshi*; Ogura, Hiroyuki*; Sagae, Daisuke*; Seto, Yusuke*; et al.

Scientific Reports (Internet), 12, p.20955_1 - 20955_8, 2022/12

 Times Cited Count:3 Percentile:26.55(Multidisciplinary Sciences)

We evaluated Laser-Induced Periodic Surface Structure (LIPSS) crystal structures using the stress imaging station at BL22XU of JAEA-BL on SPring-8. Crystallization of LIPPS was used different two types laser these are Ti:Sapphire laser (wavelength: 800 nm) and MIR-FEL (mid-infrared free electron laser, wavelength 11.4 $$mu$$m). These lasers are different in the laser pulse structure and the wavelength. We investigated on the effects of formed LIPSS crystallization using different kind of laser. Measured synchrotron X-ray energy is 30 keV and beam size is 20 $$mu$$m. Detector of diffracted X-ray is two-dimensional detector (PILATUS300K, DECTRIS). LIPSS formed using Ti:Sapphire laser has deformed structure with good crystallinity. LIPSS formed using MIR-FEL has dislocation or fault without structural stress. These results show depending on select of laser forming LIPPS structure. These information becomes important a point of the functional application of LIPSS.

Journal Articles

Liquid decontamination using acidic electrolyzed water for various uranium-contaminated steel surfaces in dismantled centrifuge

Sakasegawa, Hideo; Nomura, Mitsuo; Sawayama, Kengo; Nakayama, Takuya; Yaita, Yumi*; Yonekawa, Hitoshi*; Kobayashi, Noboru*; Arima, Tatsumi*; Hiyama, Toshiaki*; Murata, Eiichi*

Progress in Nuclear Energy, 153, p.104396_1 - 104396_9, 2022/11

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

When dismantling centrifuges in uranium-enrichment facilities, decontamination techniques must be developed to remove uranium-contaminated surfaces of dismantled parts selectively. Dismantled uranium-contaminated parts can be disposed of as nonradioactive wastes or recycled after decontamination appropriate for clearance. previously, we developed a liquid decontamination technique using acidic electrolyzed water to remove uranium-contaminated surfaces. However, further developments are still needed for its actual application. Dismantled parts have various uranium-contaminated surface features due to varied operational conditions, inhomogeneous decontamination using iodine heptafluoride gas, and changes in long-term storage conditions after dismantling. Here, we performed liquid decontamination on specimens with varying uranium-contaminated surfaces cut from a centrifuge made of low-carbon steel. From the results, the liquid decontamination can effectively remove the uranium-contaminated surfaces, and radioactive concentrations fell below the target value within twenty minutes. Although the required time should also depend on dismantled parts' sizes and shapes in their actual application, we demonstrated that it could be an effective decontamination technique for uranium-contaminated steels of dismantled centrifuges.

Journal Articles

Hydrogen vibration excitations of ZrH$$_{1.8}$$ and TiH$$_{1.84}$$ up to 21 GPa by incoherent inelastic neutron scattering

Hattori, Takanori; Nakamura, Mitsutaka; Iida, Kazuki*; Machida, Akihiko*; Sano, Asami; Machida, Shinichi*; Arima, Hiroshi*; Oshita, Hidetoshi*; Honda, Takashi*; Ikeda, Kazutaka*; et al.

Physical Review B, 106(13), p.134309_1 - 134309_9, 2022/10

 Times Cited Count:1 Percentile:0.00(Materials Science, Multidisciplinary)

Hydrogen vibration excitations of fluorite-type ZrH$$_{1.8}$$ and TiH$$_{1.84}$$ were investigated up to 21 GPa and 4 GPa, respectively, by incoherent inelastic neutron scattering experiments. The first excitation energies increased with pressure, as described by the equations $$E_1$$(meV) = 141.4(2) + 1.02(2)$$P$$(GPa) and $$E_1$$(meV) = 149.4(1) + 1.21(8)$$P$$(GPa) for ZrH$$_{1.8}$$ and TiH$$_{1.84}$$, respectively. Coupling with pressure dependence of lattice parameters, the relations between metal-hydrogen distance ($$d_{M-H}$$) and $$E_1$$ are found to be well described by the equations $$E_1$$(meV) = 1.62(9)$$times$$ 10$$^3$$ $$d_{M-H}^{-3.31(8)}$$($AA) and $E_1$$(meV) = 1.47(21)$$times$$ 10$$^3$$ $$d_{M-H}^{-3.5(2)}$$(AA), respectively. The slopes of these curves are much steep compared to the previously reported trend in various fluorite-type metal hydrides at ambient pressure. The hydrogen wave function spreading showed that the local potential field for a hydrogen atom shrinks more intensively than the tetrahedral site. These behavior is likely caused by the rigid metal ion core and the resulting confinement of the hydrogen atom in the narrower potential field at high pressures.

Journal Articles

First observation of the de Haas-van Alphen effect and Fermi surfaces in the unconventional superconductor UTe$$_2$$

Aoki, Dai*; Sakai, Hironori; Opletal, P.; Tokiwa, Yoshifumi; Ishizuka, Jun*; Yanase, Yoichi*; Harima, Hisatomo*; Nakamura, Ai*; Li, D.*; Homma, Yoshiya*; et al.

Journal of the Physical Society of Japan, 91(8), p.083704_1 - 083704_5, 2022/08

 Times Cited Count:54 Percentile:98.03(Physics, Multidisciplinary)

Journal Articles

Split Fermi surface properties of noncentrosymmetric compounds Fe$$_2$$P, Ni$$_2$$P, and Pd$$_2$$Si

Onuki, Yoshichika*; Nakamura, Ai*; Aoki, Dai*; Matsuda, Tatsuma*; Haga, Yoshinori; Harima, Hisatomo*; Takeuchi, Tetsuya*; Kaneko, Yoshio*

Journal of the Physical Society of Japan, 91(6), p.064712_1 - 064712_10, 2022/06

 Times Cited Count:2 Percentile:29.32(Physics, Multidisciplinary)

Journal Articles

Fourier interpolation method in phase space of Hamiltonian systems

Sasa, Narimasa

Journal of the Physical Society of Japan, 91(5), p.054001_1 - 054001_8, 2022/05

 Times Cited Count:1 Percentile:16.36(Physics, Multidisciplinary)

JAEA Reports

Development of high melting temperature measurement system by laser spot heating

Iwasa, Toma; Arima, Tatsumi*

JAEA-Technology 2021-036, 23 Pages, 2022/03

JAEA-Technology-2021-036.pdf:1.35MB

Knowledge on the liquefaction (thermal decomposition and melting) temperatures of MA-bearing nitride fuels for transmutation by accelerator-driven system is essential for elucidation of the fuel behaviors under abnormal condition and for the safety analysis. A melting temperature measurement system for refractory materials was developed based on a laser spot heating method, which is expected to measure in a very short time with a small amount of sample, and demonstration tests using refractory metals and zirconium nitride were performed. As the results, it was found that this melting temperature measurement system can be applicable up to the temperatures around 3000 K which is close to the thermal decomposition temperature of nitride fuels and we confirmed the technical feasibility of this system for future application to small specimens of transuranium nitrides.

Journal Articles

Square and rhombic lattices of magnetic skyrmions in a centrosymmetric binary compound

Takagi, Rina*; Matsuyama, Naofumi*; Ukleev, V.*; Yu, L.*; White, J. S.*; Francoual, S.*; Mardegan, J. R. L.*; Hayami, Satoru*; Saito, Hiraku*; Kaneko, Koji; et al.

Nature Communications (Internet), 13, p.1472_1 - 1472_7, 2022/03

 Times Cited Count:106 Percentile:99.56(Multidisciplinary Sciences)

JAEA Reports

Separation/removal of steel surface coating film by laser cleaning

Yamane, Ikumi; Takahashi, Nobuo; Sawayama, Kengo; Nishiwaki, Hiroki; Matsumoto, Takashi; Ogawa, Jumpei; Nomura, Mitsuo; Arima, Tatsumi*

JAEA-Technology 2021-038, 18 Pages, 2022/02

JAEA-Technology-2021-038.pdf:1.61MB

We have dismantled uranium enrichment facilities in Ningyo-toge Environmental Engineering Center since their operation finished in 2001, and the total amount of metallic wastes is estimated to be about 130 thousand tons. Eighty percent of them can be disposed as nonradioactive waste (NR), but there are some steel parts possibly uranium-contaminated. We need removing painted surface of such steels and radiologically surveying to dispose them as NRs. Though painted surfaces have been conventionally removed through hand working with grinders, this manual work requires installation of green house, protective clothing, and full-face mask, in order to prevent dispersion and inhalation of airborne dusts. We desire further developments of surface cleaning techniques to reduce time, cost, workload, and secondary waste generation caused by excessive grinding. Therefore, in this study, we focused on the laser cleaning technology used for the separation and removal of paint films at construction sites. In order to improve the coating separation and removal technology for NR objects, we evaluated the coating separation and removal performance of NR steel surface by laser cleaning system, observed the coating scattering behavior by high-speed camera and investigated the coating recovery method, evaluated the laser separation and removal performance of steel surface powder, and thermodynamically evaluated the uranium compounds on steel surface. We additionally evaluated the feasibility of laser cleaning techniques in our works basing on these results, and discussed future work plans for further developments of laser cleaning techniques.

Journal Articles

Journal Articles

Synchrotron analysis of simulated waste glasses different in boron isotope ingredient

Nagai, Takayuki; Okamoto, Yoshihiro; Baba, Yuji*; Akiyama, Daisuke*; Arima, Tatsumi*

Photon Factory Activity Report 2021 (Internet), 2 Pages, 2022/00

no abstracts in English

Journal Articles

Crystal structure of U$$_{1-y}$$Ln$$_{y}$$O$$_{2-x}$$ (Ln = Gd, Er) solid solution

Pham, V. M.*; Arima, Tatsumi*; Inagaki, Yaohiro*; Idemitsu, Kazuya*; Akiyama, Daisuke*; Nagai, Takayuki; Okamoto, Yoshihiro

Journal of Nuclear Materials, 556, p.153189_1 - 153189_9, 2021/12

 Times Cited Count:1 Percentile:10.40(Materials Science, Multidisciplinary)

The crystal structure change was evaluated for (1-x)UO$$_{2}$$-xLnO$$_{1.5}$$ (Ln=Gd or Er; x = 0 to 0.4) samples sintered at 1973 K for 8 h under Ar and Ar-10%H$$_{2}$$ atmospheres. The effect of LnO$$_{1.5}$$ doping on the crystal structure of UO$$_{2}$$ was investigated by X-ray diffraction (XRD) and X-ray absorption fine structure (XAFS). LnO$$_{1.5}$$ doping into UO$$_{2}$$ reduced the lattice parameter of UO$$_{2}$$-LnO$$_{1.5}$$ solid solutions up to 40mol% LnO$$_{1.5}$$. The lattice parameters of these samples were comparable to those of stoichiometric (U,Ln)O$$_{2.00}$$ solid solutions, that is, the O/M ratios were close to 2.00. The U L$$_{3}$$-edge XANES analysis showed that higher U oxidation states of +5 or +6 formed, in addition to + 4. The EXAFS analysis indicated that the interatomic distances of U-O and Gd-O decreased with increasing x, whereas those of Er-O may not decrease monotonically.

389 (Records 1-20 displayed on this page)