Pressure-modulated magnetism and negative thermal expansion in the HoFe intermetallic compound

Cao, Y.*; Zhou, H.*; Khmelevskyi, S.*; Lin, K.*; Avdeev, M.*; Wang, C.-W.*; Wang, B.*; Hu, F.*; Kato, Kenichi*; Hattori, Takanori; et al.

Chemistry of Materials, 35(8), p.3249 - 3255, 2023/04

https://doi.org/10.1021/acs.chemmater.3c00158

Hydrostatic and chemical pressure are efficient stimuli to alter the crystal structure and are commonly used for tuning electronic and magnetic properties in materials science. However, chemical pressure is difficult to quantify and a clear correspondence between these two types of pressure is still lacking. Here, we study intermetallic candidates for a permanent magnet with a negative thermal expansion (NTE). Based on in situ synchrotron X-ray diffraction, negative chemical pressure is revealed in HoFe on Al doping and quantitatively evaluated by using temperature and pressure dependence of unit cell volume. A combination of magnetization and neutron diffraction measurements also allowed one to compare the effect of chemical pressure on magnetic ordering with that of hydrostatic pressure. Intriguingly, pressure can be used to control suppression and enhancement of NTE. Electronic structure calculations indicate that pressure affected the top of the majority band with respect to the Fermi level, which has implications for the magnetic stability, which in turn plays a critical role in modulating magnetism and NTE. This work presents a good example of understanding the effect of pressure and utilizing it to control properties of functional materials.

Deexcitation dynamics of muonic atoms revealed by high-precision spectroscopy of electronic X rays

Okumura, Takuma*; Azuma, Toshiyuki*; Bennet, D. A.*; Caradonna, P.*; Chiu, I. H.*; Doriese, W. B.*; Durkin, M. S.*; Fowler, J. W.*; Gard, J. D.*; Hashimoto, Tadashi; et al.

Physical Review Letters, 127(5), p.053001_1 - 053001_7, 2021/07

https://doi.org/10.1103/PhysRevLett.127.053001

We observed electronic X rays emitted from muonic iron atoms using a superconducting transition-edge-type sensor microcalorimeter. The energy resolution of 5.2 eV in FWHM allowed us to observe the asymmetric broad profile of the electronic characteristic and X rays together with the hypersatellite X rays around 6 keV. This signature reflects the time-dependent screening of the nuclear charge by the negative muon and the -shell electrons, accompanied by electron side-feeding. Assisted by a simulation, this data clearly reveals the electronic - and -shell hole production and their temporal evolution during the muon cascade process.

Closed-form stress intensity factor solutions for deep surface cracks in plates

Azuma, Kisaburo*; Li, Y.; Hasegawa, Kunio; Xu, S.*

Proceedings of 2017 ASME Pressure Vessels and Piping Conference (PVP 2017) (CD-ROM), 9 Pages, 2017/07

Superconductivity in noncentrosymmetric iridium silicide LiIrSi

Pyon, S.*; Kudo, Kazutaka*; Matsumura, Junichi*; Ishii, Hiroyuki*; Matsuo, Genta*; Nohara, Minoru*; Hojo, Hajime*; Oka, Kengo*; Azuma, Masaki*; Garlea, V. O.*; et al.

Journal of the Physical Society of Japan, 83(9), p.093706_1 - 093706_5, 2014/09

https://doi.org/10.7566/JPSJ.83.093706

Efficient production of a collimated MeV proton beam from a Polyimide target driven by an intense femtosecond laser pulse

Nishiuchi, Mamiko; Daido, Hiroyuki; Yogo, Akifumi; Orimo, Satoshi; Ogura, Koichi; Ma, J.-L.; Sagisaka, Akito; Mori, Michiaki; Pirozhkov, A. S.; Kiriyama, Hiromitsu; et al.

Physics of Plasmas, 15(5), p.053104_1 - 053104_10, 2008/05

https://doi.org/10.1063/1.2928161

High-flux energetic protons whose maximum energies are up to 4 MeV are generated by an intense femtosecond Titanium Sapphire laser pulse interacting with a 7.5, 12.5, and 25m thick Polyimide tape targets. The laser pulse energy is 1.7 J, duration is 34 fs, and intensity is 310Wcm. The amplified spontaneous emission (ASE) has the intensity contrast ratio of 410. The conversion efficiency from laser energy into proton kinetic energies of 3% is achieved, which is comparable or even higher than those achieved in the previous works with nanometer-thick targets and the ultrahigh contrast laser pulses (10).

Efficient production of MeV proton beam from a Polyimide target driven by an intense femto-second laser

Nishiuchi, Mamiko; Daido, Hiroyuki; Yogo, Akifumi; Orimo, Satoshi; Ogura, Koichi; Ma, J.-L.; Sagisaka, Akito; Mori, Michiaki; Pirozhkov, A. S.; Kiriyama, Hiromitsu; et al.

no journal, , 

The efficient proton beam whose maximum energy of up to 4 MeV was produced by the 50TW short pulse intensity Ti:Sap laser irradiated on the polyimide target [(CHON)n] with the thicknesses of 7.5m, 12.5m, 25m, which is transparent to the 800 nm laser. The laser parameters are energy of 1.7J, pulse width of 35fs and the intensity of 310 Wcm. The contrast of the ASE component is 410. The conversion efficiency from laser energy into the proton kinetic energy is up to 3%. This conversion efficiency is comparable or even higher than the results obtained with the same level laser ( J energy) interacts with the nano-meter level ultra thin target. In this paper we discuss on the comparison between our results and other experimental results obtained in other facilities.