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論文

Quantum critical behavior of the hyperkagome magnet Mn$$_3$$CoSi

山内 宏樹; Sari, D. P.*; 安井 幸夫*; 坂倉 輝俊*; 木村 宏之*; 中尾 朗子*; 大原 高志; 本田 孝志*; 樹神 克明; 井川 直樹; et al.

Physical Review Research (Internet), 6(1), p.013144_1 - 013144_9, 2024/02

$$beta$$-Mn-type family alloys Mn$$_3$$$$TX$$ have three-dimensional antiferromagnetic (AFM) corner-shared triangular network. The antiferromagnet Mn$$_3$$RhSi shows magnetic short-range order (SRO) over a wide temperature range of approximately 500 K above the N$'{e}$el temperature $$T_{rm N}$$ = 190 K. Mn$$_3$$CoSi has the smallest lattice parameter and the lowest $$T_{rm N}$$ in the family compounds. The quantum critical point (QCP) from AFM to the quantum paramagnetic state is expected near a cubic lattice parameter of 6.15 $AA. Although $T_N$$ of Mn$$_3$$CoSi is only 140 K, quantum critical behavior is observed in Mn$$_3$$CoSi as the enhancement of the electronic specific heat coefficient $$gamma$$. We study how the magnetic SRO appears in Mn$$_3$$CoSi by using neutron scattering, $$mu$$SR, and physical property measurements. The experimental results show that the neutron scattering intensity of the magnetic SRO does not change much regardless of the suppressed magnetic moment in the long-range magnetic ordered state compared to those of Mn$$_3$$RhSi. The initial asymmetry drop ratio of $$mu$$SR above $$T_{rm N}$$ becomes small, and the magnetic SRO temperature $$T_{SRO}$$ is suppressed to 240 K. The results suggest that the Mn$$_3$$CoSi is close to the QCP in the Mn$$_3$$$$TX$$ system.

論文

Spiral spin cluster in the hyperkagome antiferromagnet Mn$$_{3}$$RhSi

社本 真一; 山内 宏樹; 飯田 一樹*; 池内 和彦*; Hall, A. E.*; Chen, Y.-S.*; Lee, M. K.*; Balakrishnan, G.*; Chang, L.-J.*

Communications Physics (Internet), 6, p.248_1 - 248_6, 2023/09

 被引用回数:1 パーセンタイル:0(Physics, Multidisciplinary)

Mn$$_{3}$$RhSi単結晶の中性子散乱測定により、局所スピン相関秩序がらせん構造を持つことがわかった。磁気クラスター形成の起源の可能性を、リフシッツ不変量とグリフィス相の観点から議論し、Co$$_{7}$$Zn$$_{7}$$Mn$$_{6}$$の室温スキルミオン相とMnの非フェルミ液体挙動と比較した。

論文

The Temperature evolution of the magnetic correlations in pure and diluted spin ice Ho$$_{2-x}$$Y$$_{x}$$Ti$$_{2}$$O$$_{7}$$

Chang, L.-J.; Su, Y.*; Kao, Y.-J.*; Chou, Y. Z.*; 加倉井 和久; Mittal, R.*; Schneider, H.*; Br$"u$ckel, T.*; Balakrishnan, G.*; Lees, M. R.*

Physica B; Condensed Matter, 406(12), p.2393 - 2396, 2011/06

 被引用回数:1 パーセンタイル:5.4(Physics, Condensed Matter)

Diffuse polarized neutron scattering studies have been carried out on single crystals of pyrochlore spin ice Ho$$_{2-x}$$Y$$_{x}$$Ti$$_{2}$$O$$_{7}$$ (x = 0, 0.3, and 1) to investigate the effects of doping and anisotropy on spin correlations in the system. For all the samples studied the spin flip (SF) diffuse scattering (i.e. the in-plane component) reveals that the spin correlations can be described using a nearest-neighbour spin ice model (NNSM) at higher temperatures ($$T$$ = 3.6 K) and a dipolar spin ice model (DSM) as the temperature is reduced ($$T$$ = 30 mK). In this paper, we focus on the experimental results of the highly doped spin ice HoYTi$$_{2}$$O$$_{7}$$ and compare our results with pure spin ice Ho$$_{2}$$Ti$$_{2}$$O$$_{7}$$.

口頭

Observations of the novel magnetic correlations in the Y doping dipolar spin ice Ho$$_{2-x}$$Y$$_{x}$$Ti$$_{2}$$O$$_{7}$$

Chang, L.-J.; Su, Y.*; Kao, Y.-J.*; Chou, Y. Z.*; Mittal, R.*; Schneider, H.*; Brueckel, T.*; Balakrishnan, G.*; Lees, M. R.*

no journal, , 

Diffuse polarized neutron scatterings have been carried out on the pyrochlore spin ice Ho$$_{2-x}$$Y$$_{x}$$Ti$$_{2}$$O$$_{7}$$ (x = 0, 0.3 and 1) single crystals to investigate the doping effects and anisotropy of spin correlations in the system. The crystals were aligned in the (1-10) orientation to coincide with the direction of neutron polarization. The spin flip diffuse scattering (i.e. the in-plane component) reveals an anomalous crossover in the spin correlations from the nearest-neighbor spin ice correlation to a typical dipolar spin ice correlation as the temperature is reduced for all the samples. A signature of strong antiferromagnetic correlation is observed in the non-spin flip channel (i.e. the out-of-plane component), at the same temperatures where the dipolar spin ice correlation appears in the spin flip channel.

口頭

ハイパーカゴメ格子Mn$$_{3}$$RhSiで共存する異なる短距離と長距離の磁気秩序

社本 真一; 池内 和彦*; 梶本 亮一; 山内 宏樹; Balakrishnan, G.*; Chang, L.-J.*

no journal, , 

ハイパーカゴメ格子Mn$$_{3}$$RhSi単結晶を用いた中性子非弾性散乱で、共存する異なる短距離と長距離の磁気秩序を観測したので報告する。

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