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Lee, O.*; Yamamoto, Kei; Umeda, Maki; Zollitsch, C. W.*; Elyasi, M.*; Kikkawa, Takashi*; Saito, Eiji; Bauer, G. E. W.*; Kurebayashi, Hidekazu*
Physical Review Letters, 130(4), p.046703_1 - 046703_6, 2023/01
Times Cited Count:5 Percentile:80.44(Physics, Multidisciplinary)Elyasi, M.*; Saito, Eiji; Bauer, G. E. W.*
Physical Review B, 105(5), p.054403_1 - 054403_12, 2022/02
Times Cited Count:7 Percentile:77.62(Materials Science, Multidisciplinary)Nambu, Yusuke*; Barker, J.*; Okino, Yuki*; Kikkawa, Takashi*; Shiomi, Yuki*; Enderle, M.*; Weber, T.*; Winn, B.*; Graves-Brook, M.*; Tranquada, J. M.*; et al.
Physical Review Letters, 125(2), p.027201_1 - 027201_6, 2020/07
Times Cited Count:45 Percentile:94.07(Physics, Multidisciplinary)Sakai, Hironori; Tokunaga, Yo; Haga, Yoshinori; Kambe, Shinsaku; Ramakrishna, S. K.*; Reyes, A. P.*; Rosa, P. F. S.*; Ronning, F.*; Thompson, J. D.*; Fisk, Z.*; et al.
JPS Conference Proceedings (Internet), 30, p.011169_1 - 011169_6, 2020/03
Uranium disulfide -US showing a semimetal-to-semiconductor crossover has been investigated by the nuclear magnetic resonance (NMR) technique for S nuclei with the nuclear spin of . Since the natural concentration 0.76% of NMR active S nuclei is too dilute, the isotopic enrichment to 50% has been carried out for the single crystal growth. The S NMR spectra have been successfully obtained using a single crystal of -US with external fields along the crystallographic axis. The S sites assignments have been made based on these NMR spectra.
Oyanagi, Koichi*; Takahashi, Saburo*; Cornelissen, L. J.*; Shan, J.*; Daimon, Shunsuke*; Kikkawa, Takashi*; Bauer, G. E. W.*; Van Wees, B. J.*; Saito, Eiji
Nature Communications (Internet), 10, p.4740_1 - 4740_6, 2019/10
Times Cited Count:38 Percentile:89.44(Multidisciplinary Sciences)Dioguardi, A. P.*; Yasuoka, Hiroshi*; Thomas, S. M.*; Sakai, Hironori; Cary, S. K.*; Kozimor, S. A.*; Albrecht-Schmitt, T. E.*; Choi, H. C.*; Zhu, J.-X.*; Thompson, J. D.*; et al.
Physical Review B, 99(3), p.035104_1 - 035104_6, 2019/01
Times Cited Count:8 Percentile:37.59(Materials Science, Multidisciplinary)We present a detailed nuclear magnetic resonance (NMR) study of Pu in bulk and powdered single-crystal plutonium tetraboride (PuB), which has recently been investigated as a potential correlated topological insulator. The Pu NMR spectra are consistent with axial symmetry of the shift tensor showing for the first time that Pu NMR can be observed in an anisotropic environment and up to room temperature. The temperature dependence of the Pu shift, combined with a relatively long spin-lattice relaxation time (), indicate that PuB adopts a nonmagnetic state with gaplike behavior consistent with our density functional theory calculations. The temperature dependencies of the NMR Knight shift and imply bulk gaplike behavior confirming that PuB is a good candidate topological insulator.
Sakai, Hironori; Hattori, Taisuke; Tokunaga, Yo; Kambe, Shinsaku; Ghimire, N. J.*; Ronning, F.*; Bauer, E. D.*; Thompson, J. D.*
Journal of Physics; Conference Series, 868(1), p.012012_1 - 012012_5, 2017/07
Times Cited Count:1 Percentile:49.63(Physics, Applied)Al NMR experiments have been performed using a single crystal of CeRhAlSi. In the paramagnetic state, Knight shifts, quadrupolar frequency, and asymmetric parameter of electrical field gradient on the Al sites have been determined, which has a local orthorhombic symmetry. The transferred hyperfine coupling constants are also determined. The relaxation rates suggest that 4 electrons behave as local moments in the high temperatures. From the NMR spectral analyses, the antiferromagnetic structures are discussed.
Sakai, Hironori; Ronning, F.*; Hattori, Takanori; Tokunaga, Yo; Kambe, Shinsaku; Zhu, J.-X.*; Wakeham, N.*; Yasuoka, Hiroshi; Bauer, E. D.*; Thompson, J. D.*
Journal of Physics; Conference Series, 807(3), p.032001_1 - 032001_6, 2017/04
Times Cited Count:3 Percentile:68.62(Physics, Condensed Matter)We have used nuclear quadrupole resonance (NQR) to probe microscopically the response of a prototypical quantum critical metal CeCoIn to substitutions of small amounts of Cd for In. Approximately half of the Cd substituents induce local Ce moments in their close proximity, as observed by site-dependent longitudinal nuclear spin relaxation rates . To reaffirm that localized moments are induced around the Cd substituents, we find a Gaussian spin-echo decay rate of transverse nuclear spin relaxation. Further, for the NQR subpeak is found to be proportional to temperatures, again indicating local moments fluctuations around the Cd substituents, while that for the NQR main peak shows a -dependence. The latter temperature dependence is close to 0.75 in pure CeCoIn and indicates that the bulk electronic state is located close to a two dimensional quantum critical instability.
Kikkawa, Takashi*; Shen, K.*; Flebus, B.*; Duine, R. A.*; Uchida, Kenichi*; Qiu, Z.*; Bauer, G. E. W.*; Saito, Eiji
Physical Review Letters, 117(20), p.207203_1 - 207203_6, 2016/11
Times Cited Count:144 Percentile:97.73(Physics, Multidisciplinary)Hou, D.*; Qiu, Z.*; Iguchi, Ryo*; Sato, Koji*; Vehstedt, E. K.*; Uchida, Kenichi*; Bauer, G. E. W.*; Saito, Eiji
Nature Communications (Internet), 7, p.12265_1 - 12265_6, 2016/07
Times Cited Count:13 Percentile:64.47(Multidisciplinary Sciences)Chen, Y.-T.*; Takahashi, Saburo*; Nakayama, Hiroyasu*; Althammer, M.*; Goennenwein, S. T. B.*; Saito, Eiji; Bauer, G. E. W.*
Journal of Physics; Condensed Matter, 28(10), p.103004_1 - 103004_15, 2016/03
Times Cited Count:81 Percentile:61.66(Physics, Condensed Matter)We review the so-called spin Hall magnetoresistance (SMR) in bilayers of a magnetic insulator and a metal, in which spin currents are generated in the normal metal by the spin Hall effect. The associated angular momentum transfer to the ferromagnetic layer and thereby the electrical resistance is modulated by the angle between the applied current and the magnetization direction. The SMR provides a convenient tool to non-invasively measure the magnetization direction and spin-transfer torque to an insulator. We introduce the minimal theoretical instruments to calculate the SMR, i.e. spin diffusion theory and quantum mechanical boundary conditions. This leads to a small set of parameters that can be fitted to experiments. We discuss the limitations of the theory as well as alternative mechanisms such as the ferromagnetic proximity effect and Rashba spin-orbit torques, and point out new developments.
Geprgs, S.*; Kehlberger, A.*; Coletta, F.*; Qiu, Z.*; Guo, E.-J.*; Schulz, T.*; Mix, C.*; Meyer, S.*; Kamra, A.*; Althammer, M.*; et al.
Nature Communications (Internet), 7, p.10452_1 - 10452_6, 2016/02
Times Cited Count:152 Percentile:97.33(Multidisciplinary Sciences)Sakai, Hironori; Hattori, Taisuke; Tokunaga, Yo; Kambe, Shinsaku; Ghimire, N. J.*; Ronning, F.*; Bauer, E. D.*; Thompson, J. D.*
Physical Review B, 93(1), p.014402_1 - 014402_9, 2016/01
Times Cited Count:2 Percentile:10.64(Materials Science, Multidisciplinary)Al nuclear magnetic resonance (NMR) experiments have been performed on a single crystal of CeRhAlSi, which is an antiferromagnetic Kondo-lattice compound with successive antiferromagnetic transitions of =14 K and =9 K at zero external field. In the paramagnetic state, the Knight shifts, quadrupolar frequency, and asymmetric parameter of electrical field gradient on the Al sites have been determined, which have local orthorhombic symmetry. The transferred hyperfine coupling constants are also determined. Analysis of the NMR spectra indicates that a commensurate antiferromagnetic structure exists below , but an incommensurate modulation of antiferromagnetic moments is present in the antiferromagnetic state between and . The spin-lattice relaxation rate suggests that the electrons behave as local moments at temperatures above .
Sakai, Hironori; Ronning, F.*; Zhu, J.-X.*; Wakeham, N.*; Yasuoka, Hiroshi; Tokunaga, Yo; Kambe, Shinsaku; Bauer, E. D.*; Thompson, J. D.*
Physical Review B, 92(12), p.121105_1 - 121105_5, 2015/09
Times Cited Count:19 Percentile:62.1(Materials Science, Multidisciplinary)Chemical substitutions are used commonly to tune a magnetic transition to zero temperature, but the resulting non-Fermi liquid (NFL) behavior is non-universal. We have used nuclear quadrupole resonance (NQR) to probe microscopically the response of a prototypical quantum-critical metal CeCoIn to substitutions of small amounts of Sn and Cd for In. These substituents induce very different local electronic environments as observed by site dependent spin lattice relaxation rates that influence the NFL behavior. The effects found here illustrate the need for care in interpreting NFL properties determined by macroscopic measurements.
Bottoni, S.*; Leoni, S.*; Fornal, B.*; Raabe, R.*; Rusek, K.*; Benzoni, G.*; Bracco, A.*; Crespi, F. C. L.*; Morales, A. I.*; Bednarczyk, P.*; et al.
Physical Review C, 92(2), p.024322_1 - 024322_8, 2015/08
Times Cited Count:21 Percentile:79.49(Physics, Nuclear)Schreier, M.*; Bauer, G. E. W.*; Vasyuchka, V.*; Flipse, J.*; Uchida, Kenichi*; Lotze, J.*; Lauer, V.*; Chumak, A.*; Serga, A.*; Daimon, Shunsuke*; et al.
Journal of Physics D; Applied Physics, 48(2), p.025001_1 - 025001_5, 2015/01
Times Cited Count:54 Percentile:87.5(Physics, Applied)Sakai, Hironori; Urbano, R. R.*; Tokunaga, Yo; Kambe, Shinsaku; Suzuki, Michito; Kuhns, P. L.*; Reyes, A. P.*; Tobash, P. H.*; Ronning, F.*; Bauer, E. D.*; et al.
Physical Review Letters, 112(23), p.236401_1 - 236401_5, 2014/06
Times Cited Count:7 Percentile:49.06(Physics, Multidisciplinary)Very high field Si-NMR measurements using a fully Si-enriched URuSi single crystal were carried out in order to microscopically investigate the "hidden order" (HO) state and adjacent magnetic phases in the high field limit. At the lowest measured temperature of 0.4 K, a clear anomaly reflecting a Fermi surface instability near 22 T inside the HO state is detected by the Si shift, . Moreover, a strong enhancement of develops near a critical field T, and the Si-NMR signal disappears suddenly at , indicating the total suppression of the HO state. Nevertheless, a weak and shifted Si-NMR signal reappears for fields higher than at 4.2 K, providing evidence for a magnetic structure within the magnetic phase caused by the Ising-type anisotropy of the uranium ordered moments.
Koutroulakis, G.*; Yasuoka, Hiroshi; Chudo, Hiroyuki; Tobash, P. H.*; Mitchell, J. N.*; Bauer, E. D.*; Thompson, J. D.*
New Journal of Physics (Internet), 16, p.053019_1 - 053019_12, 2014/05
Times Cited Count:6 Percentile:44.89(Physics, Multidisciplinary)We report In nuclear quadrupolar resonance (NQR) measurements on the heavy-fermion superconductor PuCoIn, in the temperature range 0.29 K 75 K. The NQR parameters for the two crystallographically inequivalent In sites are determined, and their temperature dependence is investigated. A linear shift of the quadrupolar frequency with lowering temperature below the critical value is revealed, in agreement with the prediction for composite pairing. The nuclear spin-lattice relaxation rate clearly signals a superconducting (SC) phase transition at 2.3 K, with strong spin fluctuations, mostly in-plane, dominating the relaxation process in the normal state near to . Analysis of the data in the SC state suggests that PuCoIn is a strong-coupling -wave superconductor.
Sakai, Hironori; Tokunaga, Yo; Kambe, Shinsaku; Ronning, F.*; Bauer, E. D.*; Thompson, J. D.*
Physical Review Letters, 112(20), p.206401_1 - 206401_5, 2014/05
Times Cited Count:14 Percentile:65.73(Physics, Multidisciplinary)Single crystals of the heavy-fermion antiferromagnet CePtIn with a Nel temperature () of 5.2 K at ambient pressure have been investigated by zero-field In-nuclear magnetic/quadrupole resonance (NMR/NQR) measurements as a function of applied pressure. Within the antiferromagnetic state the character of Ce's electron appears to change from localized to itinerant-like at GPa, approximately the pressure where superconductivity first emerges. With increased pressure, the superconducting transition reaches a maximum just at or slighty before antiferromagnetic order disappears, and not at the pressure GPa where the steeply decreasing Nel boundary extrapolates to zero temperature. For , the spin relaxation rate drops sharply by more than two orders of magnitude at , suggestive of a first order transition.
Chudo, Hiroyuki; Koutroulakis, G.*; Yasuoka, Hiroshi; Bauer, E. D.*; Tobash, P. H.*; Mitchell, J. N.*; Thompson, J. D.*
Journal of Physics; Condensed Matter, 26(3), p.036001_1 - 036001_5, 2014/01
Times Cited Count:5 Percentile:23.98(Physics, Condensed Matter)The results of In nuclear quadrupole resonance (NQR) measurements on PuIn are reported. Three of the four NQR lines of In expected for nuclear spin =9/2 are observed. The equal spacing of these lines at 20 K yields the NQR frequency of =10.45 MHz, and the asymmetry parameter of the electric field gradient, =0. The NQR line profile and the nuclear spin-lattice relaxation rate display an abrupt change at 14 K, which is associated with the onset of long-range antiferromagnetic order. The temperature dependences of the staggered magnetization , extracted from the NQR spectra, and below =14 K are well explained by the self-consistent renormalization (SCR) theory for spin fluctuations. In addition, scaling between and is also consistent with the predictions of SCR theory, providing further evidence that PuIn is a weak itinerant antiferromagnet in which spin fluctuations around the antiferromagnetic wave vector play a major role in the system's behavior at finite temperatures.