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Eaton, A. G.*; Weinberger, T. I.*; Popiel, N. J. M.*; Wu, Z.*; Hickey, A. J.*; Cabala, A.*; Posp
il, J.*; Prokle
ka, J.*; Haidamak, T.*; Bastien, G.*; et al.
Nature Communications (Internet), 15, p.223_1 - 223_10, 2024/01
被引用回数:42 パーセンタイル:98.62(Multidisciplinary Sciences)Fermi surfaces (FSs) of the anomalous UTe
were successfully detected using quantum oscillation technique on an ultrapure single crystal. The shape of FS was reproduced from the experimental data revealing two cylindrical quasi-two-dimensional FSs. This analysis suggests that a fairly strong nesting nature possibly leading to magnetic fluctuations responsible for the triplet superconductivity.
)
Jesche, A.*; Winterhalter-Stocker, N.*; Hirschberger, F.*; Bellon, A.*; Bachus, S.*; 常盤 欣文; Tsirlin, A. A.*; Gegenwart, P.*
Physical Review B, 107(10), p.104402_1 - 104402_8, 2023/03
被引用回数:42 パーセンタイル:94.36(Materials Science, Multidisciplinary)スピン-1/2三角反強磁性体KBaGd(BO
)
の結晶構造、熱力学特性、断熱減磁冷凍(ADR)効果を報告する。最近隣交換相互作用が44mKであるこの化合物は、ゼロ磁場で
=263mKの磁気秩序を示す。ADRテストは、
の2倍以上低い
=122mKの温度に達し、PPMSセットアップでは192mJ K
cm
のエントロピー蓄積容量と8時間以上の保持時間を実現した。スピン-
Yb
アナログと比較して改善された。我々は、KBaGd(BO
)
は交換結合と双極子結合のバランスの取れた相互作用を示し、構造的ランダム性と幾何学的フラストレーションとともに
を秩序温度
よりもかなり低い位置にシフトさせ、したがって冷却を促進すると主張する。
Yakushev, A.*; Lens, L.*; D
llmann, Ch. E.*; Khuyagbaatar, J.*; J
ger, E.*; Krier, J.*; Runke, J.*; Albers, H. M.*; 浅井 雅人; Block, M.*; et al.
Frontiers in Chemistry (Internet), 10, p.976635_1 - 976635_11, 2022/08
被引用回数:31 パーセンタイル:82.66(Chemistry, Multidisciplinary)114番元素フレロビウム(Fl)は現在その化学的性質が研究されている最も重い元素である。Flに関する最初の化学実験では、Flは貴ガス的な性質を持つ元素であると報告された。一方、2番目の研究では、Flは揮発性金属の性質を示すと報告された。より信頼性の高い結論を得るため、我々は更なる実験的研究を行い、二酸化ケイ素と金表面におけるFlの吸着挙動を調べた。その結果、Flは揮発性金属の水銀よりも高い揮発性と低い反応性を示し、一方、貴ガスのラドンよりは反応性が高いことを明らかにした。
NoBronis, A.*; He
berger, F. P.*; Antalic, S.*; Andel, B.*; Ackermann, D.*; Heinz, S.*; Hofmann, S.*; Khuyagbaatar, J.*; Kindler, B.*; Kojouharov, I.*; et al.
Physical Review C, 106(1), p.014602_1 - 014602_12, 2022/07
被引用回数:12 パーセンタイル:77.69(Physics, Nuclear)The decay of excited states in
No was investigated by applying the evaporation-residue-conversion-electron correlation technique. Two new isomeric states were observed in
No together with the previously known one. Excitation energies of the isomeric states were estimated based on the energies of conversion electrons and
rays from correlation chains. These results were in accord with theoretical calculations based on the mean-field models. A tentative decay scheme of isomeric states in
No is proposed, and their Nilsson configurations are discussed. The energy decrease of the 11/2
[725] Nilsson level for heavy
=153 isotones as a function of increasing proton number is confirmed.
M
ri, A.*; Mazurek, M.*; 太田 久仁雄; Siitari-Kauppi, M.*; Eichinger, F.*; Leuenberger, M.*
Minerals (Internet), 11(10), p.1072_1 - 1072_17, 2021/10
被引用回数:8 パーセンタイル:45.15(Geochemistry & Geophysics)The porosity and pore geometry of rock samples from a coherent granodioritic rock body at the Grimsel Test Site in Switzerland was characterised by different methods using injection techniques. Results from in situ and laboratory techniques are compared by applying in situ resin impregnation techniques as well as rock impregnation and mercury injection under laboratory conditions. In situ resin impregnation of the rock matrix shows an interconnected pore network throughout the rock body, providing an important reservoir for pore water and solutes, accessible by diffusion. Porosity and pore connectivity do not vary as a function of distance to brittle shear zones. In situ porosity is about half the porosity value that was determined on rock samples in the laboratory. This could be due to that such samples were affected by artefacts created since core recovery. The extrapolation of laboratory measurements to in situ conditions requires great care and may not be feasible in all cases.
-process nucleosynthesisBhattacharyya, A.*; Datta, U.*; Rahaman, A.*; Chakraborty, S.*; Aumann, T.*; Beceiro-Novo, S.*; Boretzky, K.*; Caesar, C.*; Carlson, B. V.*; Catford, W. N.*; et al.
Physical Review C, 104(4), p.045801_1 - 045801_14, 2021/10
被引用回数:8 パーセンタイル:61.53(Physics, Nuclear)中性子過剰核に対する中性子捕獲断面積は、
過程元素合成を理解する上で直接必要なデータであるものの、中性子標的が存在しないことと中性子過剰核の半減期が短いため、その実験を行うことは困難である。その代替手段として、
反応の逆過程である
反応のデータから導出する方法が行われている。本論文では、中性子数20領域の中性子過剰核に対し、クーロン分解反応を用いて
反応の断面積を測定し、そこから
反応の断面積を得た。その結果、
Naと
Alに対する中性子捕獲断面積については、統計模型で予測された値よりも小さく、
Mgに対しては大きな値となることがわかった。
Khuyagbaatar, J.*; Yakushev, A.*; D
llmann, Ch. E.*; Ackermann, D.*; Andersson, L.-L.*; 浅井 雅人; Block, M.*; Boll, R. A.*; Brand, H.*; Cox, D. M.*; et al.
Physical Review C, 102(6), p.064602_1 - 064602_9, 2020/12
被引用回数:98 パーセンタイル:99.26(Physics, Nuclear)原子番号119及び120を持つ超重元素の合成を目指した探索実験を、それぞれ
Ti+
Bk及び
Ti+
Cf核融合-粒子蒸発反応を用いて、ガス充填型反跳分離装置TASCAにて実施した。4ヶ月間におよぶビーム照射実験を行ったが、どちらの元素も検出されず、その生成断面積の上限値は65fb及び200fbであった。119, 120番元素が観測されなかった理由について、安定の島領域の超重元素の核分裂障壁の高さを予測する様々な理論計算値を用いて、核融合-粒子蒸発反応の概念を用いて議論した。
-decay properties of
FrGhys, L.*; Andreyev, A. N.; Huyse, M.*; Van Duppen, P.*; Antalic, S.*; Barzakh, A.*; Capponi, L.*; Cocolios, T. E.*; Cubiss, J.*; Derkx, X.*; et al.
Physical Review C, 100(5), p.054310_1 - 054310_13, 2019/11
被引用回数:15 パーセンタイル:74.31(Physics, Nuclear)The aim of this work was to investigate the
-decay properties of
Fr and daughter products. Neutron-deficient francium nuclei are produced at ISOLDE-CERN bombarding a UCx target with 1.4 GeV protons. Due to the very high statistics and the high beam purity, improved decay data for
Fr and its daughters were obtained. The observation of crossover transitions positioned the isomeric high-spin level of
At at an excitation energy of 265(3) keV. Half-life values of 4.47(5) s and 1.28(10) s were extracted for the ground state and isomeric state of
At and 52(3) ms for the ground-state decay of
Fr.
At revealed by in-source laser spectroscopyBarzakh, A. E.*; Cubiss, J. G.*; Andreyev, A. N.; Seliverstov, M. D.*; Andel, B.*; Antalic, S.*; Ascher, P.*; Atanasov, D.*; Beck, D.*; Biero
, J.*; et al.
Physical Review C, 99(5), p.054317_1 - 054317_9, 2019/05
被引用回数:17 パーセンタイル:77.96(Physics, Nuclear)Hyperfine-structure parameters and isotope shifts for the 795-nm atomic transitions in
At have been measured at CERN-ISOLDE, using the in-source resonance-ionization spectroscopy technique. Magnetic dipole and electric quadrupole moments, and changes in the nuclear mean-square charge radii, have been deduced. A large inverse odd-even staggering in radii, which may be associated with the presence of octupole collectivity, has been observed. Namely, the radius of the odd-odd isotope
At has been found to be larger than the average.
Ca+
Bk leading to formation of the element Ts (Z=117)Khuyagbaatar, J.*; Yakushev, A.*; D
llmann, Ch. E.*; Ackermann, D.*; Andersson, L.-L.*; 浅井 雅人; Block, M.*; Boll, R. A.*; Brand, H.*; Cox, D. M.*; et al.
Physical Review C, 99(5), p.054306_1 - 054306_16, 2019/05
被引用回数:36 パーセンタイル:92.33(Physics, Nuclear)
Ca+
B融合反応を用いて117番元素(Ts)合成実験を行い、117番元素に起因すると思われる4つの
崩壊連鎖を観測した。うち2つは長い崩壊連鎖で、
Tsの
崩壊に起因するものと同定された。他の2つは短い崩壊連鎖で、
Tsの
崩壊に起因すると考えると矛盾しない。今回の結果と過去の文献値を比較したところ、今回の我々の結果は過去の文献値をほぼ再現し、117番元素合成の事実を強く再確認する結果となった。
98 in multi-nucleon transfer reactions of
Ca+
CmDevaraja, H. M.*; Heinz, S.*; Beliuskina, O.*; Hofmann, S.*; Hornung, C.*; M
nzenberg, G.*; Ackermann, D.*; Gupta, M.*; Gambhir, Y. K.*; Henderson, R. A.*; et al.
European Physical Journal A, 55(2), p.25_1 - 25_9, 2019/02
被引用回数:18 パーセンタイル:79.35(Physics, Nuclear)The results for nuclei above curium, produced in multi-nucleon transfer reactions of
Ca+
Cm at the velocity filter SHIP of GSI Darmstadt, are presented. Spontaneous fission and
activities have been used to study the population of nuclei with lifetimes ranging from few milliseconds to several days. We observed several, relatively neutron-rich isotopes with atomic numbers Z
98; among them a weak 224 millisecond activity which we tentatively attributed to
No. The measured cross-sections of the observed nuclei give hope that multi-nucleon transfer reactions are a way to reach new neutron-rich heavy and superheavy nuclei, which are not accessible in other reactions. We compare our results with data from earlier experiments and discuss limitations and future perspectives of the method.
and Au surfaces in preparation for chemical investigations on Cn, Nh, and Fl at TASCALens, L.*; Yakushev, A.*; D
llmann, Ch. E.*; 浅井 雅人; Ballof, J.*; Block, M.*; David, H. M.*; Despotopulos, J.*; Di Nitto, A.*; Eberhardt, K.*; et al.
Radiochimica Acta, 106(12), p.949 - 962, 2018/12
被引用回数:14 パーセンタイル:72.99(Chemistry, Inorganic & Nuclear)半減期4
49秒の短寿命同位体を用いて、水銀(Hg), タリウム(Tl), 鉛(Pb)の単一原子レベルでのSiO
及びAu表面への固体吸着挙動をオンライン気相実験により調べた。超重元素Cn, Nh, Flの吸着エンタルピー測定のためのモデル実験として実施した。短寿命同位体はドイツ重イオン研究所の反跳核分離装置TASCAを用いて生成・分離した。生成核はヘリウムガス中に捕集された後、SiO
あるいはAuで表面を覆われたSi検出器で作製されたガスクロマトグラフィーカラムへと導入した。短寿命Tl及びPb同位体は室温においてSiO
表面に吸着し、Si検出器で測定することに成功した。一方、HgはSiO
表面には吸着せず、Au表面に吸着した。この結果より、本実験のセットアップを用いることで短寿命Hg, Tl, Pb同位体の吸着特性を調べることができると証明され、この手法がCn, Nh, Flの実験にも適用できることが確認された。
-delayed fission of
AmWilson, G. L.*; 武山 美麗*; Andreyev, A. N.; Andel, B.*; Antalic, S.*; Catford, W. N.*; Ghys, L.*; 羽場 宏光*; He
berger, F. P.*; Huang, M.*; et al.
Physical Review C, 96(4), p.044315_1 - 044315_7, 2017/10
被引用回数:12 パーセンタイル:59.47(Physics, Nuclear)The exotic decay process of
-delayed fission has been studied in the neutron-deficient isotope
Am at RIKEN, Japan. The
Am nuclei were produced in the complete fusion reaction
Pb(
Al,4n)
Am and separated by using the GARIS gas-filled recoil ion separator. A lower limit for the
-delayed fission probability larger than 0.30 was deduced, which so far is the highest value among all known nuclei exhibiting this decay mode.
Al via Coulomb breakupChakraborty, S.*; Datta, U.*; Aumann, T.*; Beceiro-Novo, S.*; Boretzky, K.*; Caesar, C.*; Carlson, B. V.*; Catford, W. N.*; Chartier, M.*; Cortina-Gil, D.*; et al.
Physical Review C, 96(3), p.034301_1 - 034301_9, 2017/09
被引用回数:4 パーセンタイル:30.33(Physics, Nuclear)GSIのLAND-FRSセットアップを用いて、
Alの基底状態配位をクーロン分解反応によって調べた。そこで得られた包括的断面積は78(13)mbとなった。単一粒子模型によるクーロン分解反応断面積を大規模殻模型計算による
Al+1中性子系の分光学的因子と組み合わせることによって得られた理論計算の断面積を実験値と比較した。その結果、殻模型計算では
軌道の寄与をいくらか過大評価し、
軌道の寄与を過小評価していることがわかった。これは、
Alの基底状態において中性子数28の殻ギャップが著しく縮まっており、それによって、
殻を占める最後の2個の中性子軌道が
軌道をより多く占有しているためであると考えられる。
Es and
BkKonki, J.*; Khuyagbaatar, J.*; Uusitalo, J.*; Greenlees, P. T.*; Auranen, K.*; Badran, H.*; Block, M.*; Briselet, R.*; Cox, D. M.*; Dasgupta, M.*; et al.
Physics Letters B, 764, p.265 - 270, 2017/01
被引用回数:25 パーセンタイル:84.21(Astronomy & Astrophysics)The new neutron-deficient nuclei
Es and
Bk were synthesised at the gas-filled recoil separator RITU. They were identified by their radioactive decay chains starting from
Es produced in the fusion-evaporation reaction
Bi(
S,3n)
Es. Half-lives of 6(2)s and 22
s were obtained for
Es and
Bk, respectively. Two groups of
particles with energies
=8.19(3) MeV and 8.09(3) MeV were unambiguously assigned to
Es. Electron-capture delayed fission branches with probabilities of 0.16(6) and 0.04(2) were measured for
Es and
Bk, respectively. These new data show a continuation of the exponential increase of ECDF probabilities in more neutron-deficient isotopes.
-fission and recoil-
-
-fission events observed in the reaction
Ca +
AmForsberg, U.*; Rudolph, D.*; Andersson, L.-L.*; Di Nitto, A.*; D
llmann, Ch. E.*; Fahlander, C.*; Gates, J. M.*; Golubev, P.*; Gregorich, K. E.*; Gross, C. J.*; et al.
Nuclear Physics A, 953, p.117 - 138, 2016/09
被引用回数:59 パーセンタイル:94.98(Physics, Nuclear)
Ca +
Am反応による115番元素合成実験で観測された
崩壊連鎖について、最近我々が報告したドイツGSIで測定したデータと過去に報告されたロシアDubna及び米国LBNLで測定されたデータのすべてを使い、その起源を調査した。それらのデータの中に、反跳核-
-(
)-核分裂タイプの短い崩壊連鎖が14事象観測されており、そのうちのいくつかは中性子が2個放出されてできる
Mc起源であるとこれまで解釈されてきた。一方、今回我々は、これらの短い崩壊連鎖のほとんどが、中性子が3個放出されてできる
Mc起源であり、崩壊連鎖の途中でEC崩壊して核分裂したものであろうと再同定した。
-delayed fission and
decay of
AtTruesdale, V. L.*; Andreyev, A. N.; Ghys, L.*; Huyse, M.*; Van Duppen, P.*; Sels, S.*; Andel, B.*; Antalic, S.*; Barzakh, A.*; Capponi, L.*; et al.
Physical Review C, 94(3), p.034308_1 - 034308_11, 2016/09
被引用回数:12 パーセンタイル:60.80(Physics, Nuclear)A nuclear-decay spectroscopy study of the neutron-deficient isotope
At is reported where an isotopically pure beam was produced using the selective Resonance Ionization Laser Ion Source and On-Line Isotope Mass Separator (CERN). The fine-structure
decay of
At allowed the low-energy excited states in the daughter nucleus
Bi to be investigated. A
-delayed fission study of
At was also performed. A mixture of symmetric and asymmetric fission-fragment mass distributions of the daughter isotope
Po (populated by
decay of
At) was deduced based on the measured fission-fragment energies. A
DF probability
(
At) = 9(1)
10
was determined.
Hofmann, S.*; Heinz, S.*; Mann, R.*; Maurer, J.*; M
nzenberg, G.*; Antalic, S.*; Barth, W.*; Burkhard, K. G.*; Dahl, L.*; Eberhardt, K.*; et al.
European Physical Journal A, 52(6), p.180_1 - 180_34, 2016/06
被引用回数:225 パーセンタイル:93.94(Physics, Nuclear)The reaction
Cr+
Cm was investigated at the velocity filter SHIP at GSI with the intention to study production and decay properties of isotopes of element 120. Three correlated signals were measured, which occurred within a period of 279 ms. The heights of the signals correspond with the expectations for a decay sequence starting with an isotope of element 120. However, a complete decay chain cannot be established, since a signal from the implantation of the evaporation residue cannot be identified unambiguously. Measured properties of the event chain are discussed in detail. The result is compared with theoretical predictions. Previously measured decay properties of even element super-heavy nuclei were compiled in order to find arguments for an assignment from the systematics of experimental data. In the course of this review, a few tentatively assigned data could be corrected. New interpretations are given for results which could not be assigned definitely in previous studies. The discussion revealed that the cross-section for production of element 120 could be high enough so that a successful experiment seems possible with presently available techniques. However, a continuation of the experiment at SHIP for a necessary confirmation of the results obtained in a relatively short irradiation of five weeks is not possible at GSI presently. In the summary and outlook section we also present concepts for the continuation of research in the field of super-heavy nuclei.
Po and
PoAndel, B.*; Andreyev, A. N.; Antalic, S.*; He
berger, F. P.*; Ackermann, D.*; Hofmann, S.*; Huyse, M.*; Kalaninov
, Z.*; Kindler, B.*; Kojouharov, I.*; et al.
Physical Review C, 93(6), p.064316_1 - 064316_12, 2016/06
被引用回数:5 パーセンタイル:35.08(Physics, Nuclear)Isomeric states in
Po and
Po were studied at the velocity filter SHIP. The isotopes were produced in the fusion-evaporation reactions
Pr(
Fe,
)
Po and
Sm(
V,
)
Po. Several new
-ray transitions were attributed to the isomers and
-
coincidences for both isomers were studied for the first time. The 459-keV transition earlier, tentatively proposed as de-exciting the isomeric level in
Po, was replaced by a new 248-keV transition, and the spin of this isomer was reassigned from (11
) to (10
). The de-excitation of the (11
) isomeric level in
Po by the 154-keV transition was confirmed and a parallel de-excitation by a 733-keV (E3) transition to (8
) level of the ground-state band was suggested. Moreover, side feeding to the (4
) level of the ground-state band was proposed. The paper also discusses strengths of transitions de-exciting 11
isomers in neighboring Po and Pb isotopes.
Hofmann, S.*; Heinz, S.*; Mann, R.*; Maurer, J.*; M
nzenberg, G.*; Antalic, S.*; Barth, W.*; Dahl, L.*; Eberhardt, K.*; Grzywacz, R.*; et al.
European Physical Journal A, 52(4), p.116_1 - 116_12, 2016/04
被引用回数:35 パーセンタイル:87.57(Physics, Nuclear)Shell-correction energies of super-heavy nuclei are approximated by using Q
values of measured decay chains. Five decay chains were analyzed, which start at the isotopes
Fl,
118,
Lv,
Lv and
Lv. The data are compared with predictions of macroscopic-microscopic models. Fission barriers are estimated that can be used to eliminate uncertainties in partial fission half-lives and in calculations of evaporation-residue cross-sections. In that calculations, fission probability of the compound nucleus is a major factor contributing to the total cross-section. The data also provide constraints on the cross-sections of capture and quasi-fission in the entrance channel of the fusion reaction. Arguments are presented that fusion reactions for synthesis of isotopes of elements 118 and 120 may have higher cross-sections than assumed so far.