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Journal Articles

Incommensurate antiferromagnetism in UTe$$_2$$ under pressure

Knafo, W.*; Thebault, T.*; Raymond, S.*; Manuel, P.*; Khalyavin, D. D.*; Orlandi, F.*; Ressouche, E.*; Beauvois, K.*; Lapertot, G.*; Kaneko, Koji; et al.

Physical Review X, 15(2), p.021075_1 - 021075_16, 2025/05

 Times Cited Count:0

Journal Articles

Ordered graphane nanoribbons synthesized via high-pressure diels-alder polymerization of 2,2'-bipyrazine

Li, F.*; Tang, X.*; Fei, Y.*; Zhang, J.*; Liu, J.*; Lang, P.*; Che, G.*; Zhao, Z.*; Zheng, Y.*; Fang, Y.*; et al.

Journal of the American Chemical Society, 147(17), p.14054 - 14059, 2025/04

 Times Cited Count:1 Percentile:0.00(Chemistry, Multidisciplinary)

We synthesized a crystalline graphane nanoribbon (GANR) via pressure-induced polymerization of 2,2'-bipyrazine (BPZ). By performing Rietveld refinement of in situ neutron diffraction data, nuclear magnetic resonance spectroscopy, infrared spectra, and theoretical calculation, we found that BPZ experienced Diels-Alder polymerization between the $$pi$$ $$cdots$$ $$pi$$ stacked aromatic rings, and formed extended boat-GANR structures with exceptional long-range order. The unreacted -C=N- groups bridge the two ends of the boat, and ready for further functionalization. The GANR has a bandgap of 2.25 eV, with booming photoelectric response ($$I_{rm on}$$/$$I_{rm off}$$ =18.8). Our work highlights that the high-pressure topochemical polymerization is a promising method for the precise synthesis of graphane with specific structure and desired properties.

Journal Articles

High-pressure polymerization of phenol toward degree-4 carbon nanothread

Yang, X.*; Che, G.*; Wang, Y.*; Zhang, P.*; Tang, X.*; Lang, P.*; Gao, D.*; Wang, X.*; Wang, Y.*; Hattori, Takanori; et al.

Nano Letters, 25(3), p.1028 - 1035, 2025/01

 Times Cited Count:1 Percentile:84.76(Chemistry, Multidisciplinary)

Saturated sp$$^3$$-carbon nanothreads (CNTh) have garnered significant interest due to their predicted high Young's modulus and thermal conductivity. While the incorporation of heteroatoms into the central ring has been shown to influence the formation of CNTh and yield chemically homogeneous products, the impact of pendant groups on the polymerization process remains underexplored. In this study, we investigate the pressure-induced polymerization of phenol, revealing two phase transitions occurring below 0.5 and 4 GPa. Above 20 GPa, phenol polymerizes into degree-4 CNThs featuring hydroxyl and carbonyl groups. Hydrogen transfer of hydroxyl groups was found to hinder the formation of degree-6 nanothreads. Our findings highlight the crucial role of the hydroxyl group in halting further intracolumn polymerization and offer valuable insights for future mechanism research and nanomaterial synthesis.

Journal Articles

Pressure-induced polymerization of 1,4-difluorobenzene towards fluorinated diamond nanothreads

Che, G.*; Fei, Y.*; Tang, X.*; Zhao, Z.*; Hattori, Takanori; Abe, Jun*; Wang, X.*; Ju, J.*; Dong, X.*; Wang, Y.*; et al.

Physical Chemistry Chemical Physics, 27(2), p.1112 - 1118, 2025/01

 Times Cited Count:3 Percentile:75.15(Chemistry, Physical)

Pressure-induced polymerization (PIP) of aromatic molecules has emerged as an effective method for synthesizing various carbon-based materials. In this work, PIP of 1,4-difluorobenzene (1,4-DFB) was investigated. ${it In situ}$ high-pressure investigations of 1,4-DFB reveal a phase transition at approximately 12.0 GPa and an irreversible chemical reaction at 18.7 GPa. Structural analysis of the product and the kinetics of the reaction uncovered the formation of pseudohexagonal stacked fluoro-diamond nanothreads with linear growth. Compared to the crystal structures of benzene under high pressure, 1,4-DFB exhibits higher compression along the [001] axis. The anisotropic compression is attributed to the stronger H$$cdot cdot cdot pi$$ interaction along the [01$$overline{1}$$] axis and the potential compression-inhibiting H$$cdot cdot cdot$$F interactions along the [100] and [010] axes, and it facilitates a possible reaction pathway along the [01$$overline{1}$$] axis. This work emphasizes the crucial role of functionalization in modulating molecular stacking and influencing the reaction pathway.

Journal Articles

Si-addition contributes to overcoming the strength-ductility trade-off in high-entropy alloys

Wei, D.*; Gong, W.; Tsuru, Tomohito; Lobzenko, I.; Li, X.*; Harjo, S.; Kawasaki, Takuro; Do, H.-S.*; Bae, J. W.*; Wagner, C.*; et al.

International Journal of Plasticity, 159, p.103443_1 - 103443_18, 2022/12

 Times Cited Count:107 Percentile:99.79(Engineering, Mechanical)

Journal Articles

MIRS: an imaging spectrometer for the MMX mission

Barucci, M. A.*; Reess, J.-M.*; Bernardi, P.*; Doressoundiram, A.*; Fornasier, S.*; Le Du, M.*; Iwata, Takahiro*; Nakagawa, Hiromu*; Nakamura, Tomoki*; Andr$'e$, Y.*; et al.

Earth, Planets and Space (Internet), 73(1), p.211_1 - 211_28, 2021/12

 Times Cited Count:25 Percentile:82.95(Geosciences, Multidisciplinary)

The MMX InfraRed Spectrometer (MIRS) is an imaging spectrometer on board of MMX JAXA mission. MIRS is built at LESIA-Paris Observatory in collaboration with four other French laboratories, collaboration and financial support of CNES and close collaboration with JAXA and MELCO. The instrument is designed to fully accomplish MMX's scientific and measurement objectives. MIRS will remotely provide near-infrared spectral maps of Phobos and Deimos containing compositional diagnostic spectral features that will be used to analyze the surface composition and to support the sampling site selection. MIRS will also study Mars atmosphere, in particular to spatial and temporal changes such as clouds, dust and water vapor.

Journal Articles

Phase transition and chemical reactivity of 1H-tetrazole under high pressure up to 100 GPa

Gao, D.*; Tang, X.*; Wang, X.*; Yang, X.*; Zhang, P.*; Che, G.*; Han, J.*; Hattori, Takanori; Wang, Y.*; Dong, X.*; et al.

Physical Chemistry Chemical Physics, 23(35), p.19503 - 19510, 2021/09

 Times Cited Count:7 Percentile:42.22(Chemistry, Physical)

Pressure-induced phase transition and polymerization of nitrogen-rich molecules are widely focused due to its extreme importance for the development of green high energy density materials. Here, we present a study of the phase transition and chemical reaction of 1H-tetrazole up to 100 GPa by using ${it in situ}$ Raman, IR, X-ray diffraction, neutron diffraction techniques and theoretical calculation. A phase transition above 2.6 GPa was identified and the high-pressure structure was determined with one molecule in a unit cell. The 1H-tetrazole polymerizes reversibly below 100 GPa, probably through a carbon-nitrogen bonding instead of nitrogen-nitrogen bonding. Our studies updated the structure model of the high pressure phase of 1H-tetrazole, and presented the possible intermolecular bonding route for the first time, which gives new insights to understand the phase transition and chemical reaction of nitrogen-rich compounds, and benefit for designing new high energy density materials.

Journal Articles

Search for elements 119 and 120

Khuyagbaatar, J.*; Yakushev, A.*; D$"u$llmann, Ch. E.*; Ackermann, D.*; Andersson, L.-L.*; Asai, Masato; Block, M.*; Boll, R. A.*; Brand, H.*; Cox, D. M.*; et al.

Physical Review C, 102(6), p.064602_1 - 064602_9, 2020/12

 Times Cited Count:78 Percentile:99.01(Physics, Nuclear)

A search for production of the superheavy elements with atomic numbers 119 and 120 was performed in the $$^{50}$$Ti+$$^{249}$$Bk and $$^{50}$$Ti+$$^{249}$$Cf fusion-evaporation reactions, respectively, at the gas-filled recoil separator TASCA. Over four months of irradiation, neither was detected at cross-section sensitivity levels of 65 and 200 fb, respectively. The non-observation of elements 119 and 120 is discussed within the concept of fusion-evaporation reactions including various theoretical predictions on the fission-barrier heights of superheavy nuclei in the region of the island of stability.

Journal Articles

Simultaneous determination of neutron-induced fission and radiative capture cross sections from decay probabilities obtained with a surrogate reaction

P$'e$rez S$'a$nchez, R.*; Jurado, B.*; M$'e$ot, V.*; Roig, O.*; Dupuis, M.*; Bouland, O.*; Denis-Petit, D.*; Marini, P.*; Mathieu, L.*; Tsekhanovich, I.*; et al.

Physical Review Letters, 125(12), p.122502_1 - 122502_5, 2020/09

 Times Cited Count:21 Percentile:76.54(Physics, Multidisciplinary)

Journal Articles

New excited 2$$^+$$ and 3$$^-$$ two-proton states in $$_{84}^{210}$$Po$$_{126}$$ populated by two-proton transfer

Dupont, E.*; Astier, A.*; Petrache, C. M.*; Lv, B. F.*; Deloncle, I.*; Kiener, J.*; Orlandi, R.; Makii, Hiroyuki; Nishio, Katsuhisa; Hirose, Kentaro; et al.

Physical Review C, 101(1), p.014309_1 - 014309_6, 2020/01

 Times Cited Count:2 Percentile:20.23(Physics, Nuclear)

Journal Articles

Search for $$alpha$$ decay of $$^{104}$$Te with a novel recoil-decay scintillation detector

Xiao, Y.*; Go, S.*; Grzywacz, R.*; Orlandi, R.; Andreyev, A. N.; Asai, Masato; Bentley, M. A.*; de Angelis, G.*; Gross, C. J.*; Hausladen, P.*; et al.

Physical Review C, 100(3), p.034315_1 - 034315_8, 2019/09

 Times Cited Count:19 Percentile:83.32(Physics, Nuclear)

Journal Articles

Inverse odd-even staggering in nuclear charge radii and possible octupole collectivity in $$^{217,218,219}$$At revealed by in-source laser spectroscopy

Barzakh, A. E.*; Cubiss, J. G.*; Andreyev, A. N.; Seliverstov, M. D.*; Andel, B.*; Antalic, S.*; Ascher, P.*; Atanasov, D.*; Beck, D.*; Biero$'n$, J.*; et al.

Physical Review C, 99(5), p.054317_1 - 054317_9, 2019/05

 Times Cited Count:15 Percentile:73.32(Physics, Nuclear)

Journal Articles

Fusion reaction $$^{48}$$Ca+$$^{249}$$Bk leading to formation of the element Ts (Z=117)

Khuyagbaatar, J.*; Yakushev, A.*; D$"u$llmann, Ch. E.*; Ackermann, D.*; Andersson, L.-L.*; Asai, Masato; Block, M.*; Boll, R. A.*; Brand, H.*; Cox, D. M.*; et al.

Physical Review C, 99(5), p.054306_1 - 054306_16, 2019/05

AA2019-0039.pdf:5.03MB

 Times Cited Count:33 Percentile:92.64(Physics, Nuclear)

We have performed an experiment to synthesize the element 117 (Ts) with the $$^{48}$$Ca+$$^{249}$$Bk fusion reaction. Four $$alpha$$-decay chains attributed to the element 117 were observed. Two of them were long decay chains which can be assigned to the one originating from the $$alpha$$ decay of $$^{294}$$Ts. The other two were short decay chains which are consistent with the one originating from the $$alpha$$ decay of $$^{293}$$Ts. We have compared the present results with the literature data, and found that our present results mostly confirmed the literature data, leading to the firm confirmation of the synthesis of the element 117.

Journal Articles

EXILL; A High-efficiency, high-resolution setup for $$gamma$$-spectroscopy at an intense cold neutron beam facility

Jentschel, M.*; Blanc, A.*; de France, G.*; K$"o$ster, U.*; Leoni, S.*; Mutti, P.*; Simpson, G.*; Soldner, T.*; Ur, C.*; Urban, W.*; et al.

Journal of Instrumentation (Internet), 12(11), p.P11003_1 - P11003_33, 2017/11

 Times Cited Count:43 Percentile:84.98(Instruments & Instrumentation)

Journal Articles

Shape evolution in neutron-rich krypton isotopes beyond N=60; First spectroscopy of $$^{98,100}$$Kr

Flavigny, F.*; Doornenbal, P.*; Obertelli, A.*; Delaroche, J.-P.*; Girod, M.*; Libert, J.*; Rodriguez, T. R.*; Authelet, G.*; Baba, Hidetada*; Calvet, D.*; et al.

Physical Review Letters, 118(24), p.242501_1 - 242501_6, 2017/06

 Times Cited Count:40 Percentile:86.04(Physics, Multidisciplinary)

Journal Articles

Identification of the crossing point at $$N$$ = 21 between normal and intruder configurations

Lic$u{a}$, R.*; Rotaru, F.*; Borge, M. J. G.*; Gr$'e$vy, S.*; Negoita, F.*; Poves, A.*; Sorlin, O.*; Andreyev, A. N.; Borcea, R.*; Costache, C.*; et al.

Physical Review C, 95(2), p.021301_1 - 021301_6, 2017/02

 Times Cited Count:19 Percentile:79.02(Physics, Nuclear)

Journal Articles

Are there signatures of harmonic oscillator shells far from stability?; First spectroscopy of $$^{110}$$Zr

Paul, N.*; Corsi, A.*; Obertelli, A.*; Doornenbal, P.*; Authelet, G.*; Baba, Hidetada*; Bally, B.*; Bender, M.*; Calvet, D.*; Ch$^a$teau, F.*; et al.

Physical Review Letters, 118(3), p.032501_1 - 032501_7, 2017/01

 Times Cited Count:46 Percentile:88.07(Physics, Multidisciplinary)

Journal Articles

Recoil-$$alpha$$-fission and recoil-$$alpha$$-$$alpha$$-fission events observed in the reaction $$^{48}$$Ca + $$^{243}$$Am

Forsberg, U.*; Rudolph, D.*; Andersson, L.-L.*; Di Nitto, A.*; D$"u$llmann, Ch. E.*; Fahlander, C.*; Gates, J. M.*; Golubev, P.*; Gregorich, K. E.*; Gross, C. J.*; et al.

Nuclear Physics A, 953, p.117 - 138, 2016/09

 Times Cited Count:54 Percentile:95.04(Physics, Nuclear)

Alpha-decay chains observed in the element-115 production reactions of $$^{48}$$Ca + $$^{243}$$Am were investigated using a new data set consisting of our recently reported data obtained at GSI and previously reported ones at Dubna and LBNL. Short decay chains of recoil-$$alpha$$-($$alpha$$)-fission type, fourteen of which were observed, and some of which were interpreted as the 2-neutron evaporation products $$^{289}$$Mc, have been reassigned. It is plausible that most of them were assigned to the 3-neutron evaporation products $$^{288}$$Mc whose decay chain would on the way have branches of EC decays followed by fission.

Journal Articles

Round Robin test for the determination of nitrogen concentration in solid lithium

Favuzza, P.*; Antonelli, A.*; Furukawa, Tomohiro; Groeschel, F.*; Heidinger, R.*; Higashi, Takuma*; Hirakawa, Yasushi; Iijima, Minoru; Ito, Yuzuru; Kanemura, Takuji; et al.

Fusion Engineering and Design, 107, p.13 - 24, 2016/06

 Times Cited Count:10 Percentile:63.56(Nuclear Science & Technology)

Three different partners, ENEA, JAEA and University of Tokyo, have been involved during 2014 and 2015 in the Round Robin experimentation for the assessment of the soundness of the analitycal procedure for the determination of the Nitrogen impurities contained inside a solid Lithium sample. Two different kinds of Lithium samples, differing by about an order of magnitude in Nitrogen concentration (about 230 wppm, about 20-30 wppm), have been selected for this cross analysis. The agreement of the achieved results appears very good for what concerns the most concentrated Lithium and indicates each partner's procedure is appropriate and intrinsically able to lead to meaningful values, characterized by a relative uncertainty of just few %. The smaller agreement in the case of the less concentrated Lithium anyway points out that particular attention must be paid to reduce as much as possible any source of external contamination and highlights the importance of the proper blank subtraction.

Journal Articles

Fast-timing study of the $$l$$-forbidden 1/2$$^+$$ $$rightarrow$$ 3/2$$^+$$ $$M1$$ transition in $$^{129}$$Sn

Lic$u{a}$, R.*; Mach, H.*; Fraile, L. M.*; Gargano, A.*; Borge, M. J. G.*; M$u{a}$rginean, N.*; Sotty, C. O.*; Vedia, V.*; Andreyev, A. N.; Benzoni, G.*; et al.

Physical Review C, 93(4), p.044303_1 - 044303_7, 2016/04

 Times Cited Count:10 Percentile:53.99(Physics, Nuclear)

57 (Records 1-20 displayed on this page)