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論文

Outcomes of WPEC SG47 on "Use of Shielding Integral Benchmark Archive and Database for Nuclear Data Validation"

Kodeli, I. A.*; Fleming, M.*; Cabellos, O.*; Leal, L.*; Celik, Y.*; Ding, Y.*; Jansky, B.*; Neudecker, D.*; Novak, E.*; Simakov, S.*; et al.

EPJ Web of Conferences, 284, p.15002_1 - 15002_8, 2023/05

経済協力開発機構原子力機関(OECD/NEA)において、放射線遮蔽積分ベンチマークアーカイブ及びデータベース(SINBAD)の利用促進とSINBAD評価活動への還元を目的として、国際核データ評価協力サブグループ47(WPEC SG47)「核データ検証のためのSINBADの利用」が2019年6月に立ち上がった。SINBADでは、核データ及び放射線輸送計算コードの検証と開発におけるニーズに合致した実験データベースの評価と保存を進めている。その中で、WPEC SG47の活動においては、SINBAD評価活動における核データの感度解析の利用、実験体系を再現する形状、放射線源、材料等のCAD情報のSINBADへの格納、OECD/NEAのソフトウェアGitLabを利用した様々な放射線輸送計算コードの入力ファイルの共有等について議論や提案が進められている。この活動中に約8例のベンチマーク実験データが核データの検証に利用され、今後、高崎量子応用研究所イオン照射研究施設(TIARA)で実施された中性子遮蔽実験を含む様々な実験データも核データの検証で利用される予定である。本発表では、WPEC SG47の活動の他、SINBADの核データ評価への利用例と評価活動計画について紹介する。

論文

Extreme phonon anharmonicity underpins superionic diffusion and ultralow thermal conductivity in argyrodite Ag$$_{8}$$SnSe$$_{6}$$

Ren, Q.*; Gupta, M. K.*; Jin, M.*; Ding, J.*; Wu, J.*; Chen, Z.*; Lin, S.*; Fabelo, O.*; Rodriguez-Velamazan, J. A.*; 古府 麻衣子; et al.

Nature Materials, 22, p.999 - 1006, 2023/05

Ultralow thermal conductivity and fast ionic diffusion endow superionic materials with excellent performance both as thermoelectric converters and as solid-state electrolytes. Yet the correlation and interdependence between these two features remain unclear owing to a limited understanding of their complex atomic dynamics. Here we investigate ionic diffusion and lattice dynamics in argyrodite Ag$$_{8}$$SnSe$$_{6}$$ using synchrotron X-ray and neutron scattering techniques along with machine-learned molecular dynamics. We identify a critical interplay of the vibrational dynamics of mobile Ag and a host framework that controls the overdamping of low-energy Ag-dominated phonons into a quasi-elastic response, enabling superionicity. Concomitantly, the persistence of long-wavelength transverse acoustic phonons across the superionic transition challenges a proposed 'liquid-like thermal conduction' picture. Rather, a striking thermal broadening of low-energy phonons, starting even below 50 K, reveals extreme phonon anharmonicity and weak bonding as underlying features of the potential energy surface responsible for the ultralow thermal conductivity ($$<$$ 0.5 Wm$$^{-1}$$K$$^{-1}$$) and fast diffusion. Our results provide fundamental insights into the complex atomic dynamics in superionic materials for energy conversion and storage.

論文

Producing gold at ISOLDE-CERN

Barzakh, A. E.*; Andreyev, A. N.; Atanasov, D.*; Cubiss, J. G.*; Harding, R. D.*; Al Monthery, M.*; Althubiti, N. A.*; Andel, B.*; 他38名*

Nuclear Instruments and Methods in Physics Research B, 513, p.26 - 32, 2022/02

 被引用回数:0 パーセンタイル:0.02(Instruments & Instrumentation)

The yield of 18 beams of radioactive gold nuclei produced by irradiating the ISOLDE uranium target with 1.4-GeV protons was measured. The production-efficiency dependence on the half-life was derived using the in-target production calculations. Three release models were tested to describe the results. Irregularities in the efficiency curve for 3 long-lived high-spin gold isomers ($$^{187,191,193}$$Au$$^m$$) were found, which require further investigation.

論文

Laser-assisted nuclear decay spectroscopy of $$^{176,177,179}$$Au

Harding, R. D.*; Andreyev, A. N.; Barzakh, A. E.*; Cubiss, J. G.*; Van Duppen, P.*; Al Monthery, M.*; Althubiti, N. A.*; Andel, B.*; 他26名*

Physical Review C, 104(2), p.024326_1 - 024326_16, 2021/08

 被引用回数:3 パーセンタイル:48.27(Physics, Nuclear)

A detailed nuclear spectroscopy study of $$^{176,177,179}$$Au was performed at ISOLDE, CERN. This work provides new insights into the low-lying levels in the daughter nuclei $$^{172,173,175}$$Ir. For $$^{176}$$Au, the nuclear magnetic moments of a high spin and low spin state were determined and used to predict the most likely configuration of each level. Their $$alpha$$-decay branching ratios were also extracted: a 58(5)% branching for the low-spin state, and 29(5)% for the high-spin state.

論文

Laser-assisted decay spectroscopy for the ground states of $$^{180,182}$$Au

Harding, R. D.*; Andreyev, A. N.; Barzakh, A. E.*; Atanasov, D.*; Cubiss, J. G.*; Van Duppen, P.*; 他40名*

Physical Review C, 102(2), p.024312_1 - 024312_16, 2020/08

 被引用回数:9 パーセンタイル:74.44(Physics, Nuclear)

A detailed nuclear spectroscopy study of $$^{180}$$Au was performed. An $$alpha$$-decay branching ratio of $$0.58(10)$$% and a half-life of $$7.2(5)$$s have been derived. The first measurement of the hyper fine structure for atomic transitions has been also performed, from which the magnetic dipole moment has been extracted. A spin assignment of $$(1^+)$$ is proposed for the ground state of $$^{180}$$Au, with a $$(pi3/2^-$$[532]$$timesnu5/2^-$$[512]$$)$$ configuration.

論文

In-source laser spectroscopy of dysprosium isotopes at the ISOLDE-RILIS

Chrysalidis, K.*; Barzakh, A. E.*; Ahmed, R.*; Andreyev, A. N.; Ballof, J.*; Cubiss, J. G.*; Fedorov, D. V.*; Fedosseev, V. N.*; Fraile, L. M.*; Harding, R. D.*; et al.

Nuclear Instruments and Methods in Physics Research B, 463, p.472 - 475, 2020/01

 被引用回数:3 パーセンタイル:36.99(Instruments & Instrumentation)

放射壊変によって生成された多数のジスプロシウム同位体について、ISOLDEのレーザー共鳴イオン源(RILIS)を用いてイオン源内レーザー分光法によって研究した。$$^{152}$$Dyに対する相対的な同位体シフトを$$4f^{10}6s^{2}~^{5}I_{8}$$ (gs) $$rightarrow$$ $$4f^{10}6s6p~(8,1)^{o}_{8}$$共鳴遷移を用いて測定した。電子的因子Fとマスシフト因子Mを導出し、それらを使って$$^{rm 145m}$$Dyと$$^{rm 147m}$$Dyの平均自乗荷電半径の変化を初めて決定した。

論文

$$alpha$$-decay branching ratio of $$^{180}$$Pt

Cubiss, J. G.*; Harding, R. D.*; Andreyev, A. N.; Althubiti, N.*; Andel, B.*; Antalic, S.*; Barzakh, A. E.*; Cocolios, T. E.*; Day Goodacre, T.*; Farooq-Smith, G. J.*; et al.

Physical Review C, 101(1), p.014314_1 - 014314_4, 2020/01

 被引用回数:5 パーセンタイル:53.56(Physics, Nuclear)

$$^{180}$$Ptの基底状態から娘核$$^{176}$$Osの基底状態への$$alpha$$崩壊分岐比を0.52(5)%と、過去の値と比較してより高精度で再決定した。$$^{180}$$PtはCERN-ISOLDE実験施設において$$^{180}$$Hgを単離し、その$$beta$$崩壊孫核種として生成した。今回の結果を用いて導出した$$alpha$$崩壊の換算崩壊幅は、中性子欠損Pt同位体の$$alpha$$崩壊幅の系統性について新しい描像を与えることとなった。

論文

Fine structure in the $$alpha$$ decay of $$^{223}$$U

Sun, M. D.*; Liu, Z.*; Huang, T. H.*; Zhang, W. Q.*; Andreyev, A. N.; Ding, B.*; Wang, J. G.*; Liu, X. Y.*; Lu, H. Y.*; Hou, D. S.*; et al.

Physics Letters B, 800, p.135096_1 - 135096_5, 2020/01

 被引用回数:10 パーセンタイル:80.2(Astronomy & Astrophysics)

Fine structure in the $$alpha$$ decay of $$^{223}$$U was observed in the fusion-evaporation reaction $$^{187}$$Re($$^{40}$$Ar,p3n) by using fast digital pulse processing technique. Two $$alpha$$-decay branches of $$^{223}$$U feeding the ground state and 244 keV excited state of $$^{219}$$Th were identified by establishing the decay chain $$^{223}$$U$$rightarrow$$$$^{219}$$Th$$rightarrow$$$$^{215}$$Ra$$rightarrow$$$$^{211}$$Rn. The $$alpha$$-particle energy for the ground-state to ground-state transition of $$^{223}$$U was determined to be 8993(17) keV, 213 keV higher than the previous value, the half-life was updated to be 62$$^{+14}_{-10} mu$$s. Evolution of nuclear structure for $$N$$=131 even-$$Z$$ isotones from Po to U was discussed in the frameworks of nuclear mass and reduced $$alpha$$-decay width, a weakening octupole deformation in the ground state of $$^{223}$$U relative to its lighter isotones $$^{219}$$Ra and $$^{211}$$Th was suggested.

論文

Shell evolution beyond $$Z$$=28 and $$N$$=50; Spectroscopy of $$^{81,82,83,84}$$Zn

Shand, C. M.*; Podoly$'a$k, Zs.*; G$'o$rska, M.*; Doornenbal, P.*; Obertelli, A.*; Nowacki, F.*; Otsuka, T.*; Sieja, K.*; Tostevin, J. A.*; Tsunoda, T.*; et al.

Physics Letters B, 773, p.492 - 497, 2017/10

 被引用回数:23 パーセンタイル:87.56(Astronomy & Astrophysics)

Low-lying states in neutron-rich $$^{81,82.83.84}$$Zn nuclei were measured for the first time via in-beam $$gamma$$-ray spectroscopy at RIKEN. These include the 4$$_1^+$$ to 2$$_1^+$$ in $$^{82}$$Zn and the 2$$_1^+$$ to 0$$_1^+$$ and 4$$_1^+$$ to 2$$_1^+$$ in $$^{84}$$Zn. The reduced E($$2^+$$) energies and increased E(4$$^+$$)/E(2$$^+$$) ratios at $$N$$=52,54 compared to $$^{80}$$Zn attest that the magicity is confined just on the neutron number $$N$$=50 only. The levels observed in $$^{84}$$Zn suggest the onset of deformation towards heavier Zn isotopes. The data were compared to state-of-the-art shell model calculations.

論文

Shape evolution in neutron-rich krypton isotopes beyond N=60; First spectroscopy of $$^{98,100}$$Kr

Flavigny, F.*; Doornenbal, P.*; Obertelli, A.*; Delaroche, J.-P.*; Girod, M.*; Libert, J.*; Rodriguez, T. R.*; Authelet, G.*; 馬場 秀忠*; Calvet, D.*; et al.

Physical Review Letters, 118(24), p.242501_1 - 242501_6, 2017/06

 被引用回数:34 パーセンタイル:86.96(Physics, Multidisciplinary)

The first $$gamma$$-ray spectroscopy of very neutron rich $$^{98,100}$$Kr isotopes was carried out at the RIBF at RIKEN Nishina center. Excited states in these isotopes were populated via (p,2p) reactions using radioactive $$^{99,101}$$Rb beams accelerated to 220 MeV/nucleon. The new data show a significant increase in deformation beyond N=60, as well as competing configurations (shape-coexistence) at low energy. The data were compared with beyond-mean-field calculations which predict level energies in good agreement with observation, and suggest oblate-prolate shape coexistence.

論文

Low-lying structure and shape evolution in neutron-rich Se isotopes

Chen, S.*; Doornenbal, P.*; Obertelli, A.*; Rodriguez, T. R.*; Authelet, G.*; 馬場 秀忠*; Calvet, D.*; Ch$^a$teau, F.*; Corsi, A.*; Delbart, A.*; et al.

Physical Review C, 95(4), p.041302_1 - 041302_6, 2017/04

 被引用回数:23 パーセンタイル:87.56(Physics, Nuclear)

Neutron-rich isotopes of selenium, $$^{88,90,92,94}$$Se, where studied via in beam $$gamma$$-ray spectroscopy after nucleon removal reactions at RIBF in RIKEN. The low-energy excitations of these nuclei were investigated using $$gamma$$-$$gamma$$ coincidences, and the first and second excited 2$$^+$$ states were found at remarkably low energies. The analysis and comparison with self-consistent beyond-mean field calculations suggest that both shape coexistence and triaxiality are needed to describe these isotopes.

論文

Are there signatures of harmonic oscillator shells far from stability?; First spectroscopy of $$^{110}$$Zr

Paul, N.*; Corsi, A.*; Obertelli, A.*; Doornenbal, P.*; Authelet, G.*; 馬場 秀忠*; Bally, B.*; Bender, M.*; Calvet, D.*; Ch$^a$teau, F.*; et al.

Physical Review Letters, 118(3), p.032501_1 - 032501_7, 2017/01

 被引用回数:36 パーセンタイル:88.46(Physics, Multidisciplinary)

The first measurement of $$gamma$$ rays emitted by the very neutron rich nuclei $$^{112}$$Mo (Z=42) and $$^{110}$$Zr (Z=40) was carried out at the RIBF facility at RIKEN. These data shine light on the postulated N=70 harmonic oscillator shell. If the spin-orbit splitting which gives rise to the N=82 shell gap is reduced in very neutron-rich nuclei, the harmonic oscillator gap at N=70 should open instead. However, both the measured energy of the first excited state $$^{112}$$Mo and $$^{110}$$Zr, respectively 235(7) keV and 185(11) keV, and their E(4$$^+$$)/E(2$$^+$$) ratio, indicate that these nuclei are good rotors, and exclude the shell stabilization scenario at Z=40 and N=70. These results were compared to state-of-the-art density functional theoretical calculations using Gogny and Skyrme effective interactions.

論文

Volume-wise destruction of the antiferromagnetic Mott insulating state through quantum tuning

Frandsen, B. A.*; Liu, L.*; Cheung, S. C.*; Guguchia, Z.*; Khasanov, R.*; Morenzoni, E.*; Munsie, T. J. S.*; Hallas, A. M.*; Wilson, M. N.*; Cai, Y.*; et al.

Nature Communications (Internet), 7, p.12519_1 - 12519_8, 2016/08

 被引用回数:31 パーセンタイル:77.41(Multidisciplinary Sciences)

RENiO$$_3$$ (RE = rare-earth element) and V$$_2$$O$$_3$$ are archetypal Mott insulator systems. When tuned by chemical substitution (RENiO$$_3$$) or pressure (V$$_2$$O$$_3$$), they exhibit a quantum phase transition (QPT) between an antiferromagnetic Mott insulating state and a paramagnetic metallic state. Because novel physics often appears near a Mott QPT, the details of this transition, such as whether it is first or second order, are important. Here, we demonstrate through muon spin relaxation/rotation experiments that the QPT in RENiO$$_3$$ and V$$_2$$O$$_3$$ is first order: the magnetically ordered volume fraction decreases to zero at the QPT, resulting in a broad region of intrinsic phase separation, while the ordered magnetic moment retains its full value until it is suddenly destroyed at the QPT. These findings bring to light a surprising universality of the pressure-driven Mott transition, revealing the importance of phase separation and calling for further investigation into the nature of quantum fluctuations underlying the transition.

論文

Overview of plasma-material interaction experiments on EAST employing MAPES

Ding, F.*; Luo, G.-N.*; Pitts, R.*; Litnovsky, A.*; Gong, X.*; Ding, R.*; Mao, H.*; Zhou, H.*; Wampler, W. R.*; Stangeby, P. C.*; et al.

Journal of Nuclear Materials, 455(1-3), p.710 - 716, 2014/12

 被引用回数:24 パーセンタイル:88.28(Materials Science, Multidisciplinary)

A movable material probe system (Material and Plasma Evaluation System: MAPES) with an independent pumping system and a sample exchange chamber has been developed and installed on a horizontal port of the EAST tokamak for studies of plasma material interaction (PMI). In the 2012 experimental campaign, deposition and erosion were studied for three samples: mock-up of the outer first wall panels (FWPs) in ITER, castellated tungsten, and molybdenum mirrors. The FWPs with carbon deposition layer were exposed to helium plasmas. The maximum erosion rate of the carbon was valuated to be 8 nm/s. The castellated tungsten with rectangular cells and roof-like shaped cells was exposed to deuterium plasmas to compare amount of deposits on the gap surface. The amount of carbon and boron impurities on the gap surface of the roof-like shaped cells were reduced to less than 30% compared with that of the rectangular cells. The molybdenum mirrors of which protective ducts are installed in front were exposed to deuterium plasmas in order to investigate effects of length of the ducts. It was found that the reflectivity of the mirrors with 60 mm-long protective ducts is kept the initial reflectivity.

論文

Progress on the heating and current drive systems for ITER

Jacquinot, J.*; Albajar, F.*; Beaumont, B.*; Becoulet, A.*; Bonicelli, T.*; Bora, D.*; Campbell, D.*; Chakraborty, A.*; Darbos, C.*; Decamps, H.*; et al.

Fusion Engineering and Design, 84(2-6), p.125 - 130, 2009/06

 被引用回数:24 パーセンタイル:82.41(Nuclear Science & Technology)

ITER用電子サイクロトロン波(EC),イオンサイクロトロン波(IC),中性ビーム(NB)、そして低域混成波(LH)について、その物理と工学の両面の進展を2007/2008年にレビューした。全体仕様の変更はないものの、以下のような設計変更があった。第一に、DTフェーズの前に全パワーである73MW入射をルーティンに入射可能となるように調整すべきこと。第二に、NBを水素フェーズにもフルパワー入射が可能となるように対向壁を用意する、IC用によりロバスト名アンテナ2式を用意する、またECには2MW容量の伝送系を用意して、増力を容易にする。さらにRF源と計測及び加熱用ポートプラグの試験施設となる付属建屋を用意する。第三に、LHのようにITERの長パルス運転時に適した電流駆動システムを開発するための計画の必要性が認識された。

口頭

Application of CAD/MC interface code MCAM to generate MCNP model for nuclear analysis of ITER port limiter

Lu, L.*; 飯田 浩正; Li, Y.*; Ding, A.*; Zeng, Q.*; Huang, C.*; Wu, Y.*

no journal, , 

ポートリミターはITER(国際熱核融合炉)の重要な機器の一つであり、非常に複雑な形状を持っている。CAD図面から自動的にモンテカルロコードMCNPの入力を作成するプログラムMCAMを用いて、核解析を行うための詳細な入力を作成した。本発表は元図であるCAD図面のpreprocess及び変換された入力のvalidationの詳細なフローについて述べたものである。本作業が成功裏に行われたことは、複雑な機器のモンテカルロコード用入力を作成することにおいて、MCAMが、従来のマニュアル作業による入力作成に比べ、圧倒的に効率を高め、また正確さを増すことができることを示すものである。

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