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Journal Articles

Study on $$^{99m}$$Tc separation/concentration technology from $$^{99}$$Mo by (n, $$gamma$$) method, 2

Fujita, Yoshitaka; Hu, X.*; Yang, Y.*; Kitagawa, Taiga*; Fujihara, Yasuyuki*; Yoshinaga, Hisao*; Hori, Junichi*; Do, T. M. D.*; Suzuki, Tatsuya*; Suematsu, Hisayuki*; et al.

KURNS Progress Report 2023, P. 122, 2024/07

no abstracts in English

Journal Articles

Onset of collectivity for argon isotopes close to $$N=32$$

Linh, B. D.*; Corsi, A.*; Gillibert, A.*; Obertelli, A.*; Doornenbal, P.*; Barbieri, C.*; Duguet, T.*; G$'o$mez-Ramos, M.*; Holt, J. D.*; Hu, B. S.*; et al.

Physical Review C, 109(3), p.034312_1 - 034312_15, 2024/03

https://doi.org/10.1103/PhysRevC.109.034312
 Times Cited Count：1 Percentile：63.95(Physics, Nuclear)

no abstracts in English

Journal Articles

The Role of collision ionization of K-shell ions in nonequilibrium plasmas produced by the action of super strong, ultrashort PW-class laser pulses on micron-scale argon clusters with intensity up to 5 $$times$$ 10$$^{21}$$ W/cm$$^{2}$$

Skobelev, I. Yu.*; Ryazantsev, S. N.*; Kulikov, R. K.*; Sedov, M. V.*; Filippov, E. D.*; Pikuz, S. A.*; Asai, Takafumi*; Kanasaki, Masato*; Yamauchi, Tomoya*; Jinno, Satoshi; et al.

Photonics (Internet), 10(11), p.1250_1 - 1250_11, 2023/11

https://doi.org/10.3390/photonics10111250
 Times Cited Count：1 Percentile：19.28(Optics)

It is challenging to clearly distinguish the impacts of the optical field and collisional ionization in the evolution of the charge state of a plasma produced when matter interacts with high-intensity laser pulses. In this work, time-dependent calculations of plasma kinetics are used to show that it is possible only when low-density gaseous targets with sufficiently small clusters are used. In the case of Ar plasma, the upper limit of the cluster radius was estimated to be $$R_0 = 0.1 mu$$m.

Journal Articles

Validation of the $$^{10}$$Be ground-state molecular structure using $$^{10}$$Be($$p,palpha$$)$$^{6}$$He triple differential reaction cross-section measurements

Li, P. J.*; Beaumel, D.*; Lee, J.*; Assi$'e$, M.*; Chen, S.*; Franchoo, S.*; Gibelin, J.*; Hammache, F.*; Harada, T.*; Kanada-En'yo, Yoshiko*; et al.

Physical Review Letters, 131(21), p.212501_1 - 212501_7, 2023/11

https://doi.org/10.1103/PhysRevLett.131.212501
 Times Cited Count：18 Percentile：91.30(Physics, Multidisciplinary)

The cluster structure of the neutron-rich isotope $$^{10}$$Be has been probed via the ($$p,palpha$$) reaction. The triple differential cross-section was extracted and compared to distorted-wave impulse approximation reaction calculations performed in a microscopic framework using the Tohsaki-Horiuchi-Schuck-R$"o$pke wave function and the wave function deduced from Antisymmetrized Molecular Dynamics calculations. The remarkable agreement between calculated and measured cross-sections in both shape and magnitude validates the description of the $$^{10}$$Be ground-state as a rather compact nuclear molecule.

Journal Articles

Fetal and maternal atomic bomb survivor dosimetry using the J45 pregnant female phantom series; Considerations of the kneeling and lying posture with comparisons to the DS02 system

Domal, S. J.*; Correa-Alfonso, C. M.*; Paulbeck, C. J.*; Griffin, K. T.*; Sato, Tatsuhiko; Funamoto, Sachiyo*; Cullings, H. M.*; Egbert, S. D.*; Endo, Akira; Hertel, N. E.*; et al.

Health Physics, 125(4), p.245 - 259, 2023/10

https://doi.org/10.1097/HP.0000000000001710
 Times Cited Count：0 Percentile：0.00(Environmental Sciences)

The RERF Working Group on Organ Dose (WGOD) has established the J45 (Japan 1945) series of high-resolution voxel phantoms, which were derived from the UF/NCI series of hybrid phantoms and scaled to match mid-1940s Japanese body morphometries. In this present study, we present the J45 pregnant female phantoms in both a kneeling and lying posture, and assess the dosimetric impact of these more anatomically realistic survivor models in comparisons to current organ doses given by the DS02 system. For the kneeling phantoms facing the bomb hypocenter, organ doses from bomb source photon spectra were shown to be overestimated by the DS02 system by up to a factor of 1.45 for certain fetal organs and up to a factor of 1.17 for maternal organs. For lying phantoms with their feet in the direction of the hypocenter, fetal organ doses from bomb source photon spectra were underestimated by the DS02 system by factors as low as 0.77 while maternal organ doses were overestimated by up to a factor of 1.38. Results from this study highlight the degree to which the existing DS02 system can differ from organ dosimetry based upon 3D radiation transport simulations using more anatomically realistic models of those survivors exposed during pregnancy while in a kneeling or lying position.

Journal Articles

Extraction of $$^{99}$$Mo hot atoms made by a neutron capture method from $$alpha$$-MoO$$_{3}$$ to water

Quach, N. M.*; Ngo, M. C.*; Yang, Y.*; Nguyen, T. B.*; Nguyen, V. T.*; Fujita, Yoshitaka; Do, T. M. D.*; Nakayama, Tadachika*; Suzuki, Tatsuya*; Suematsu, Hisayuki*

Journal of Radioanalytical and Nuclear Chemistry, 332(10), p.4057 - 4064, 2023/10

https://doi.org/10.1007/s10967-023-09125-7
 Times Cited Count：3 Percentile：65.16(Chemistry, Analytical)

Technetium-99m ($$^{99m}$$Tc) is the most widely used medical radioisotope in the world and is produced from molybdenum-99 ($$^{99}$$Mo). Production of $$^{99}$$Mo via the neutron capture method draws attention as an alternative to fission-derived $$^{99}$$Mo due to non-proliferation issues, but the specific radioactivity of $$^{99}$$Mo is extremely low. In this work, a porous $$alpha$$-MoO$$_{3}$$ wire was prepared as an irradiation target in order to improve the specific activity by extracting $$^{99}$$Mo. Porous $$alpha$$-MoO$$_{3}$$ wire is synthesized from Mo metal wire by a two-step heating procedure. The hot atom effect of $$^{99}$$Mo was confirmed by activity and isotope measurements of the porous $$alpha$$-MoO$$_{3}$$ wire after neutron irradiation and the water used for extraction. In term of the extraction effectiveness, the effectiveness of $$^{99}$$Mo extraction in the porous $$alpha$$-MoO$$_{3}$$ wire was comparable to that of commercial $$alpha$$-MoO$$_{3}$$ powder.

Journal Articles

PANDORA Project for the study of photonuclear reactions below $$A=60$$

Tamii, Atsushi*; Pellegri, L.*; S$"o$derstr$"o$m, P.-A.*; Allard, D.*; Goriely, S.*; Inakura, Tsunenori*; Khan, E.*; Kido, Eiji*; Kimura, Masaaki*; Litvinova, E.*; et al.

European Physical Journal A, 59(9), p.208_1 - 208_21, 2023/09

https://doi.org/10.1140/epja/s10050-023-01081-w
 Times Cited Count：5 Percentile：77.95(Physics, Nuclear)

no abstracts in English

Journal Articles

$$beta$$-MoO$$_{3}$$ whiskers in $$^{99}$$Mo/$$^{rm 99m}$$Tc radioisotope production and $$^{99}$$Mo/$$^{rm 99m}$$Tc extraction using hot atoms

Ngo, M. C.*; Fujita, Yoshitaka; Suzuki, Tatsuya*; Do, T. M. D.*; Seki, Misaki; Nakayama, Tadachika*; Niihara, Koichi*; Suematsu, Hisayuki*

Inorganic Chemistry, 62(32), p.13140 - 13147, 2023/08

https://doi.org/10.1021/acs.inorgchem.3c02125
 Times Cited Count：4 Percentile：56.38(Chemistry, Inorganic & Nuclear)

Technetium-99m ($$^{rm 99m}$$Tc) is one of the most important radioisotopes for diagnostic radio-imaging applications. $$^{rm 99m}$$Tc is a daughter product of the $$^{99}$$Mo isotope. There are two methods used to produce $$^{99}$$Mo/$$^{rm 99m}$$Tc: the nuclear fission (n,f) and the neutron capture (n,$$gamma$$) methods. Between them, the (n,f) method is the main route, used for approximately 90% of the world's production. However, the (n,f) method faces numerous problems, including the use of highly enriched uranium, the release of highly radioactive waste, and nonproliferation problems. Therefore, the (n,$$gamma$$) method is being developed as a future replacement for the (n,f) method. In this work, $$beta$$-MoO$$_{3}$$ whiskers prepared by the thermal evaporation method and $$alpha$$-MoO$$_{3}$$ particles were irradiated in a nuclear reactor to produce $$^{99}$$Mo/$$^{rm 99m}$$Tc via neutron capture. The irradiated targets were dispersed into water to extract the $$^{99}$$Mo/$$^{rm 99m}$$Tc. As a result, $$beta$$-MoO$$_{3}$$ whisker yielded higher $$^{99}$$Mo extraction rate than that from $$alpha$$-MoO$$_{3}$$. In addition, by comparing the dissolved $$^{98}$$Mo concentrations in water, we clarified a prominent hot-atom of $$beta$$-MoO$$_{3}$$ whiskers. This research is the first demonstration of $$beta$$-MoO$$_{3}$$ being used as an irradiation target in the neutron capture method. On the basis of the results, $$beta$$-MoO$$_{3}$$ is considered a promising irradiation target for producing $$^{99}$$Mo/$$^{rm 99m}$$Tc by neutron capture and using water for the radioisotope extraction process in the future.

Journal Articles

First observation of $$^{28}$$O

Kondo, Yosuke*; Achouri, N. L.*; Al Falou, H.*; Atar, L.*; Aumann, T.*; Baba, Hidetada*; Boretzky, K.*; Caesar, C.*; Calvet, D.*; Chae, H.*; et al.

Nature, 620(7976), p.965 - 970, 2023/08

https://doi.org/10.1038/s41586-023-06352-6
 Times Cited Count：24 Percentile：95.07(Multidisciplinary Sciences)

no abstracts in English

Journal Articles

Level structures of $$^{56,58}$$Ca cast doubt on a doubly magic $$^{60}$$Ca

Chen, S.*; Browne, F.*; Doornenbal, P.*; Lee, J.*; Obertelli, A.*; Tsunoda, Yusuke*; Otsuka, Takaharu*; Chazono, Yoshiki*; Hagen, G.*; Holt, J. D.*; et al.

Physics Letters B, 843, p.138025_1 - 138025_7, 2023/08

https://doi.org/10.1016/j.physletb.2023.138025
 Times Cited Count：7 Percentile：83.07(Astronomy & Astrophysics)

Gamma decays were observed in $$^{56}$$Ca and $$^{58}$$Ca following quasi-free one-proton knockout reactions from $$^{57,59}$$Sc. For $$^{56}$$Ca, a $$gamma$$ ray transition was measured to be 1456(12) keV, while for $$^{58}$$Ca an indication for a transition was observed at 1115(34) keV. Both transitions were tentatively assigned as the $$2^{+}_{1} rightarrow 0^{+}_{gs}$$ decays. A shell-model calculation in a wide model space with a marginally modified effective nucleon-nucleon interaction depicts excellent agreement with experiment for $$2^{+}_{1}$$ level energies, two-neutron separation energies, and reaction cross sections, corroborating the formation of a new nuclear shell above the N = 34 shell. Its constituents, the $$0_{f5/2}$$ and $$0_{g9/2}$$ orbitals, are almost degenerate. This degeneracy precludes the possibility for a doubly magic $$^{60}$$Ca and potentially drives the dripline of Ca isotopes to $$^{70}$$Ca or even beyond.

Journal Articles

Intruder configurations in $$^{29}$$Ne at the transition into the island of inversion; Detailed structure study of $$^{28}$$Ne

Wang, H.*; Yasuda, Masahiro*; Kondo, Yosuke*; Nakamura, Takashi*; Tostevin, J. A.*; Ogata, Kazuyuki*; Otsuka, Takaharu*; Poves, A.*; Shimizu, Noritaka*; Yoshida, Kazuki; et al.

Physics Letters B, 843, p.138038_1 - 138038_9, 2023/08

https://doi.org/10.1016/j.physletb.2023.138038
 Times Cited Count：4 Percentile：62.61(Astronomy & Astrophysics)

Detailed $$gamma$$-ray spectroscopy of the exotic neon isotope $$^{28}$$Ne has been performed using the one-neutron removal reaction from $$^{29}$$Ne. Based on an analysis of parallel momentum distributions, a level scheme with spin-parity assignments has been constructed for $$^{28}$$Ne and the negative-parity states are identified for the first time. The measured partial cross sections and momentum distributions reveal a significant intruder p-wave strength providing evidence of the breakdown of the N = 20 and N = 28 shell gaps. Only a weak, possible f-wave strength was observed to bound final states. Large-scale shell-model calculations with different effective interactions do not reproduce the large p-wave and small f-wave strength observed experimentally, indicating an ongoing challenge for a complete theoretical description of the transition into the island of inversion along the Ne isotopic chain.

Journal Articles

Fetal atomic bomb survivor dosimetry using the J45 series of pregnant female phantoms with realistic survivor exposure scenarios; Comparisons to dose estimates in the DS02 system

Paulbeck, C. J.*; Sato, Tatsuhiko; Funamoto, Sachiyo*; Lee, C.*; Griffin, K. T.*; Cullings, H. M.*; Egbert, S. D.*; Endo, Akira; Hertel, N. E.*; Bolch, W. E.*

Radiation and Environmental Biophysics, 62(3), p.317 - 329, 2023/08

https://doi.org/10.1007/s00411-023-01032-5
 Times Cited Count：2 Percentile：41.11(Biology)

In our prior study [Radiat Res 192, 538-561 (2019)], we presented a new J45 (Japanese 1945) series of high-resolution phantoms of the adult pregnant female at 8-week, 15-week, 25-week, and 38-week post-conception. In this present study, we extend this work using realistic angular fluences from the DS02 system for up to nine different radiation categories and five shielding conditions. General findings are that the current DS02 fetal dose surrogate overestimates values of fetal organ dose seen in the J45 phantoms towards the cranial end of the fetus, especially in the later stages of pregnancy. This work supports our previous findings that the J45 pregnant female phantom series offers significate opportunities for gestational age-dependent assessment of fetal organ dose without the need to invoke the uterine wall as a fetal organ surrogate.

Journal Articles

Multiple mechanisms in proton-induced nucleon removal at $$sim$$100 MeV/nucleon

Pohl, T.*; Sun, Y. L.*; Obertelli, A.*; Lee, J.*; G$'o$mez-Ramos, M.*; Ogata, Kazuyuki*; Yoshida, Kazuki; Cai, B. S.*; Yuan, C. X.*; Brown, B. A.*; et al.

Physical Review Letters, 130(17), p.172501_1 - 172501_8, 2023/04

https://doi.org/10.1103/PhysRevLett.130.172501
 Times Cited Count：12 Percentile：87.89(Physics, Multidisciplinary)

We report on the first proton-induced single proton- and neutron-removal reactions from the neutron deficient $$^{14}$$O nucleus with large Fermi-surface asymmetry at $$sim$$100 MeV/nucleon. Our results provide the first quantitative contributions of multiple reaction mechanisms including the quasifree knockout, inelastic scattering, and nucleon transfer processes. It is shown that the inelastic scattering and nucleon transfer, usually neglected at such energy regime, contribute about 50% and 30% to the loosely bound proton and deeply bound neutron removal, respectively.

Journal Articles

"Southwestern" boundary of the $$N = 40$$ island of inversion; First study of low-lying bound excited states in $$^{59}$$V and $$^{61}$$V

Elekes, Z.*; Juh$'a$sz, M. M.*; Sohler, D.*; Sieja, K.*; Yoshida, Kazuki; Ogata, Kazuyuki*; Doornenbal, P.*; Obertelli, A.*; Achouri, N. L.*; Baba, Hidetada*; et al.

Physical Review C, 106(6), p.064321_1 - 064321_10, 2022/12

https://doi.org/10.1103/PhysRevC.106.064321
 Times Cited Count：2 Percentile：33.33(Physics, Nuclear)

The low-lying level structure of $$^{59}$$V and $$^{61}$$V was investigated for the first time. The neutron knockout reaction and inelastic proton scattering were applied for $$^{61}$$V while the neutron knock-out reaction provided the data for $$^{59}$$V. Four and five new transitions were determined for $$^{59}$$V and $$^{61}$$V, respectively. Based on the comparison to our shell-model calculations using the Lenzi-Nowacki-Poves-Sieja (LNPS) interaction, three of the observed $$gamma$$ rays for each isotope could be placed in the level scheme and assigned to the decay of the first 11/2$$^{-}$$ and 9/2$$^{-}$$ levels. The ($$p$$,$$p'$$) excitation cross sections for $$^{61}$$V were analyzed by the coupled-channels formalism assuming quadrupole plus hexadecapole deformations. Due to the role of the hexadecapole deformation, $$^{61}$$V could not be unambiguously placed on the island of inversion.

Journal Articles

Extended $$p_{3/2}$$ neutron orbital and the $$N = 32$$ shell closure in $$^{52}$$Ca

Enciu, M.*; Liu, H. N.*; Obertelli, A.*; Doornenbal, P.*; Nowacki, F.*; Ogata, Kazuyuki*; Poves, A.*; Yoshida, Kazuki; Achouri, N. L.*; Baba, Hidetada*; et al.

Physical Review Letters, 129(26), p.262501_1 - 262501_7, 2022/12

https://doi.org/10.1103/PhysRevLett.129.262501
 Times Cited Count：16 Percentile：82.72(Physics, Multidisciplinary)

The one-neutron knockout from $$^{52}$$Ca was performed at $$sim$$230 MeV/nucleon combined with prompt $$gamma$$ spectroscopy. The momentum distributions corresponding to the removal of $$1f_{7/2}$$ and $$2p_{3/2}$$ neutrons were measured. The cross sections are consistent with a shell closure at the neutron number $$N = 32$$, found as strong as at $$N = 28$$ and $$N = 34$$ in Ca isotopes from the same observables. The analysis of the momentum distributions leads to a difference of the root-mean-square radii of the neutron $$1_{f7/2}$$ and $$2p_{3/2}$$ orbitals of 0.61(23) fm, in agreement with the modified-shell-model prediction of 0.7 fm suggesting that the large root-mean-square radius of the $$2p_{3/2}$$ orbital in neutron-rich Ca isotopes is responsible for the unexpected linear increase of the charge radius with the neutron number.

Journal Articles

Selective recovery of thorium and uranium from leach solutions of rare earth concentrates in continuous solvent extraction mode with primary amine N1923

Nguyen, T. H.*; Le Ba, T.*; Tran, C. T.*; Nguyen, T. T.*; Doan, T. T. T.*; Do, V. K.; Watanabe, Masayuki; Pham, Q. M.*; Hoang, S. T.*; Nguyen, D. V.*; et al.

Hydrometallurgy, 213, p.105933_1 - 105933_11, 2022/08

https://doi.org/10.1016/j.hydromet.2022.105933
 Times Cited Count：16 Percentile：78.58(Metallurgy & Metallurgical Engineering)

A continuous counter-current extraction for the selective recovery of thorium (Th) and uranium (U) from the Yen Phu (Vietnam) rare earth concentrate leach solutions was systematically studied. The primary amine N1923 was used as an extractant which was prepared in the isoparaffin IP-2028 diluent. Thorium and uranium were selectively recovered in a hydrometallurgical circuit established by continuous mixer-settler extraction, scrubbing, and back-extraction at the laboratory scale. The desired purity of Th and U can be achieved by managing the volume ratio of organic to aqueous phase (O/A ratio) in the corresponding steps. Highly pure Th and U were recovered from the pregnant back-extraction liquor and the raffinate, respectively, which have satisfactory properties for further processing of the subsequent nuclear materials.

Journal Articles

Gaps in topological magnon spectra; Intrinsic versus extrinsic effects

Do, S.-H.*; Paddison, J. A. M.*; Sala, G.*; Williams, T. J.*; Kaneko, Koji; Kuwahara, Keitaro*; May, A. F.*; Yan, J.*; McGuire, M. A.*; Stone, M. B.*; et al.

Physical Review B, 106(6), p.L060408_1 - L060408_6, 2022/08

https://doi.org/10.1103/PhysRevB.106.L060408
 Times Cited Count：16 Percentile：81.88(Materials Science, Multidisciplinary)

Journal Articles

Radiochemical research for the advancement of $$^{99}$$Mo/$$^{rm 99m}$$Tc generator by (n, $$gamma$$) method, 4

Fujita, Yoshitaka; Seki, Misaki; Ngo, M. C.*; Do, T. M. D.*; Hu, X.*; Yang, Y.*; Takeuchi, Tomoaki; Nakano, Hiroko; Fujihara, Yasuyuki*; Yoshinaga, Hisao*; et al.

KURNS Progress Report 2021, P. 118, 2022/07

https://www.rri.kyoto-u.ac.jp/PUB/report/PR/ProgRep2021/ProgressReport2021_online.pdf#page=134

no abstracts in English

Journal Articles

State-of-the-art of WPS in RPV PTS analysis

Zarazovski, M.*; Pistra, V.*; Lauerova, D.*; Obermeier, F.*; Mora, D.*; Dubyk, Y.*; Bolinder, T.*; Cueto-Felgueroso, C.*; Szavai, S.*; Dudra, J.*; et al.

Proceedings of ASME 2022 Pressure Vessels and Piping Conference (PVP 2022) (Internet), 11 Pages, 2022/07

Journal Articles

A First glimpse at the shell structure beyond $$^{54}$$Ca; Spectroscopy of $$^{55}$$K, $$^{55}$$Ca, and $$^{57}$$Ca

Koiwai, Takuma*; Wimmer, K.*; Doornenbal, P.*; Obertelli, A.*; Barbieri, C.*; Duguet, T.*; Holt, J. D.*; Miyagi, Takayuki*; Navr$'a$til, P.*; Ogata, Kazuyuki*; et al.

Physics Letters B, 827, p.136953_1 - 136953_7, 2022/04

AA2021-0775.pdf:0.62MB

https://doi.org/10.1016/j.physletb.2022.136953
 Times Cited Count：6 Percentile：68.58(Astronomy & Astrophysics)

no abstracts in English

111 (Records 1-20 displayed on this page)