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Journal Articles

Formation of NaCl-type monodeuteride LaD by the disproportionation reaction of LaD$$_{2}$$

Machida, Akihiko; Honda, Mitsunori*; Hattori, Takanori; Sano, Asami; Watanuki, Tetsu; Katayama, Yoshinori; Aoki, Katsutoshi; Komatsu, Kazuki*; Arima, Hiroshi*; Oshita, Hidetoshi*; et al.

Physical Review Letters, 108(20), p.205501_1 - 205501_5, 2012/05

 Times Cited Count:10 Percentile:58.4(Physics, Multidisciplinary)

Hydrogen atoms absorbed in a metal occupy the interstitial sites of the metal lattice. In an fcc metal lattice, each metal atom has two tetrahedral (T) and one octahedral (O) sites that can accommodate hydrogen. Rare-earth metal La forms T-site occupied LaH$$_2$$ and fully occupied LaH$$_3$$. O-site occupied or NaCl-type monohydride has yet to be reported for rare-earth metals. Previous X-ray diffraction measurements revealed the pressure-induced decomposition of an fcc-LaH$$_{2.3}$$ into H-rich and H-poor phases around 11 GPa. The present neutron diffraction measurements on LaD$$_{2}$$ confirm the formation of NaCl-type LaD as a counterpart of the D-rich LaD$$_{2+delta}$$ by disproportionation. First-principle calculations demonstrate that the NaCl-type LaH is stabilized at high pressures. Finding the NaCl-type LaH will pave the way for investigations on the site-dependent nature of hydrogen-metal interactions.

Journal Articles

Development of Nondestructive Measurement Techniques for Uranium-contaminated Waste in Containers

Oki, Koichi; Aoyama, Yasuhiro; Sukegawa, Yasuhiro*; Suzuki, Satoshi*; Sagawa, Hiroshi*; Hideo, Doi,*; Endo, Yasumi*

Waste Management 2005 Proceeding, CD-ROM, 8p., 8 Pages, 2005/03

We developed as a new technique to remove the influence of distance between radionuclides and detectors. We named the technique "the Facing Couple Method (FCM)". Partcality inspection which uses uranium source was parformed.Furthermore, the application possibility to a system was confirmed.

Journal Articles

Development of Technique for Measuring Uranium Quantity within Containers Using the Passive Gamma Method

Oki, Koichi; Aoyama, Yasuhiro; Sukegawa, Yasuhiro*; Suzuki, Satoshi*; Sagawa, Hiroshi*; Hideo, Doi,*; Endo, Yasumi*

Saikuru Kiko Giho, (25), p.57 - 68, 2004/00

The system which measures and evaluates the quantity of uranium in the uranium contaminated waste in a large-sized container by NDA technology was manufactured.Practicality inspection which uses an uranium source was performed. Furthermore, the application possibility to a system was confirmed.

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