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Yakushev, A.*; Gates, J. M.*; Trler, A.*; Sch
del, M.; D
llmann, Ch. E.*; Ackermann, D.*; Andersson, L.-L.*; Block, M.*; Br
chle, W.*; Dvorak, J.*; et al.
Inorganic Chemistry, 53(3), p.1624 - 1629, 2014/02
Times Cited Count:94 Percentile:98.73(Chemistry, Inorganic & Nuclear)We report on a gas-solid chromatography study of the adsorption of element 114 (flerovium, Fl) on a Au surface. Fl was produced in the nuclear fusion reaction Pu(
Ca, 3-4n)
Fl and was isolated in-flight from the primary
beam in a physical recoil separator. The adsorption behavior of Fl, its nuclear
-decay product Cn, their lighter homologues in groups 14 and 12, i.e., Pb and Hg, and the noble gas Rn were studied simultaneously by isothermal gas chromatography and thermochromatography. Two Fl atoms were detected. They adsorbed on a Au surface at room temperature, but not as readily as Pb and Hg. The observed adsorption behavior of Fl points to a higher inertness compared to its nearest homologue in the group, Pb. However, the measured lower limit for the adsorption enthalpy of Fl on a Au surface points to the formation of a metal-metal bond of Fl with Au. Fl is the least reactive element in the group, but still a metal.
Even, J.*; Yakushev, A.*; Dllmann, C. E.*; Dvorak, J.*; Eichler, R.*; Gothe, O.*; Hild, D.*; J
ger, E.*; Khuyagbaatar, J.*; Kratz, J. V.*; et al.
Inorganic Chemistry, 51(12), p.6431 - 6433, 2012/06
Times Cited Count:34 Percentile:83.38(Chemistry, Inorganic & Nuclear)Carbonyl complexes of radioactive transition metals can be easily synthesized with high yields by stopping nuclear fission or fusion products in a gas volume containing CO. Here, we focus on Mo, W, and Os complexes. The reaction takes place at pressures of around 1 bar at room temperature, i.e., at conditions that are easy to accommodate. The formed complexes are highly volatile. They can thus be transported within a gas stream without major losses to setups for their further investigation or direct use. The rapid synthesis holds promise for radiochemical purposes and will be useful for studying, e.g., chemical properties of superheavy elements.
Forsberg, U.*; Golubev, P.*; Sarmiento, L. G.*; Jeppsson, J.*; Rudolph, D.*; Andersson, L.-L.*; Ackermann, D.*; Asai, Masato; Block, M.*; Eberhardt, K.*; et al.
Acta Physica Polonica B, 43(2), p.305 - 311, 2012/02
The atomic numbers and mass numbers of superheavy elements produced in the reactions of Ca beam with actinide targets have not been identified with direct experimental evidences. This causes a little doubt about a new element synthesis. The aim of this study is to identify the atomic numbers of those superheavy elements through characteristic X-ray measurements. To produce and separate superheavy elements, we employed a gas-filled separator TASCA at GSI, and constructed high-efficiency
-
-electron multi-coincidence detector setup at the focal plane of TASCA. Transmission efficiencies and focusing abilities were tested experimentally, and compared with simulations. We achieved a good performance to realize X-ray measurement for the element 115.
Graeger, R.*; Ackermann, D.*; Chelnokov, M.*; Chepigin, V.*; Dllmann, C. E.*; Dvorak, J.*; Even, J.*; Gorshkov, A.*; He
berger, F. P.*; Hild, D.*; et al.
Physical Review C, 81(6), p.061601_1 - 061601_5, 2010/06
Times Cited Count:43 Percentile:90.76(Physics, Nuclear)Dvorak, J.*; Brchle, W.*; D
llmann, Ch. E.*; Dvorakova, Z.*; Eberhardt, K.*; Eichler, R.*; J
ger, E.*; Nagame, Yuichiro; Qin, Z.*; Sch
del, M.*; et al.
Physical Review C, 79(3), p.037602_1 - 037602_4, 2009/05
Times Cited Count:17 Percentile:70.89(Physics, Nuclear)no abstracts in English
Dvorak, J.*; Brchle, W.*; Chelnokov, M.*; D
llmann, Ch. E.*; Dvorakova, Z.*; Eberhardt, K.*; J
ger, E.*; Kr
cken, R.*; Kuznetsov, A.*; Nagame, Yuichiro; et al.
Physical Review Letters, 100(13), p.132503_1 - 132503_4, 2008/04
The analysis of a large body of heavy ion fusion reaction data with medium-heavy projectiles (6Z
18) and actinide targets suggests a disappearance of the 3
exit channel with increasing atomic number of the projectile. Here, we report a measurement of the excitation function of the reaction
Cm(
Mg,
)
Hs and the observation of the new nuclide
Hs produced in the 3
evaporation channel at a beam energy well below the Bass fusion barrier with a cross section comparable to the maxima of the 4
and 5
channels. This indicates the possible discovery of new neutron-rich transactinide nuclei using relatively light heavy ion beams of the most neutron-rich stable isotopes and actinide targets.
Dvorak, J.*; Brchle, W.*; Chelnokov, M.*; D
llmann, Ch. E.*; Dvorakova, Z.*; Eberhardt, K.*; J
ger, E.*; Kr
cken, R.*; Kuznetsov, A.*; Nagame, Yuichiro; et al.
Physical Review Letters, 100(13), p.132503_1 - 132503_4, 2008/04
Times Cited Count:122 Percentile:95.06(Physics, Multidisciplinary)Dvorak, J.*; Brchle, W.*; Chelnokov, M.*; Dressler, R.*; D
llmann, Ch. E.*; Eberhardt, K.*; Gorshkov, V.*; J
ger, E.*; Kr
cken, R.*; Kuznetsov, A.*; et al.
Physical Review Letters, 97(24), p.242501_1 - 242501_4, 2006/12
Times Cited Count:147 Percentile:96.06(Physics, Multidisciplinary)no abstracts in English