Updates to the AMUR code for R-matrix analyses on heavy nuclei

Kunieda, Satoshi; Endo, Shunsuke; Kimura, Atsushi

EPJ Web of Conferences, 281, p.00017_1 - 00017_6, 2023/03

https://doi.org/10.1051/epjconf/202328100017

The AMUR code, which is based on the multi-channel/multi-level R-matrix theory, is under development for the cross-section evaluation with the covariance data in the resolved resonance energy region. Although, the code was initially designed for the analysis of the light-nuclei, the authors extended its capability toward the analysis of heavier nuclei by introducing the Reich-Moore approximation and the free-gas approximation for the Doppler broadening. In this work, we challenge a resonance analysis of neutron cross-section data measured in J-PARC/ANNRI with AMUR, in which the resolution functions and the double-bunching effects were taken into account inside the code. In this presentation, let us show results of resonance analysis on some of the J-PARC/ANNRI measurements together with covariance of the resonance parameters and cross-sections, for the first time. We also plan to discuss differences of correlation matrices among approximations of the R-matrix theory to understand physics underlying on the resonant reaction.

Water contents in aggregates and cement pastes determined by gravimetric analysis and prompt -ray analysis

Kinoshita, Norikazu*; Noto, Takuma*; Nakajima, Hitoshi*; Kosako, Kazuaki*; Kato, Takahiro*; Kuroiwa, Yoichi*; Kurabe, Misako*; Sasaki, Yuki*; Torii, Kazuyuki*; Maeda, Makoto; et al.

Journal of Radioanalytical and Nuclear Chemistry, 332(2), p.479 - 486, 2023/02

https://doi.org/10.1007/s10967-023-08776-w

Measurements of capture cross-section of Nb by activation method and half-life of Nb by mass analysis

Nakamura, Shoji; Shibahara, Yuji*; Endo, Shunsuke; Kimura, Atsushi

Journal of Nuclear Science and Technology, 11 Pages, 2023/00

https://doi.org/10.1080/00223131.2023.2198526

The thermal-neutron capture cross section () and resonance integral (I) for Nb among nuclides for decommissioning were measured by an activation method and the half-life of Nb by mass analysis. Niobium-93 samples were irradiated with a hydraulic conveyer installed in the research reactor in Institute for Integral Radiation and Nuclear Science, Kyoto University. Gold-aluminum, cobalt-aluminum alloy wires were used to monitor thermal-neutron fluxes and epi-thermal Westcott's indexes at an irradiation position. A 25-m-thick gadolinium foil was used to sort out reactions ascribe to thermal-and epi-thermal neutrons. Its thickness provided a cut-off energy of 0.133 eV. In order to attenuate radioactivity of Ta due to impurities, the Nb samples were cooled for nearly 2 years. The induced radio activity in the monitors and Nb samples were measured by -ray spectroscopy. In analysis based on Westcott's convention, the and I values were derived as 1.110.04 barn and 10.50.6 barn, respectively. After the -ray measurements, mass analysis was applied to the Nb sample to obtain the reaction rate. By combining data obtained by both -ray spectroscopy and mass analysis, the half-life of Nb was derived as (2.000.15)10 years.

Measurement of the transverse asymmetry of rays in the Sn()Sn reaction

Endo, Shunsuke; Okudaira, Takuya*; Abe, Ryota*; Fujioka, Hiroyuki*; Hirota, Katsuya*; Kimura, Atsushi; Kitaguchi, Masaaki*; Oku, Takayuki; Sakai, Kenji; Shima, Tatsushi*; et al.

Physical Review C, 106(6), p.064601_1 - 064601_7, 2022/12

https://doi.org/10.1103/PhysRevC.106.064601

no abstracts in English

Thermal-neutron capture cross-section measurements of neptunium-237 with graphite thermal column in KUR

Nakamura, Shoji; Shibahara, Yuji*; Endo, Shunsuke; Kimura, Atsushi

Journal of Nuclear Science and Technology, 59(11), p.1388 - 1398, 2022/11

https://doi.org/10.1080/00223131.2022.2058639

The present study selected Np among radioactive nuclides and aimed to measure the thermal-neutron capture cross-section for Np in a well-thermalized neutron field by an activation method. A Np standard solution was used for irradiation samples. A thermal-neutron flux at an irradiation position was measured with neutron flux monitors: Sc, Co, Mo, Ta and Au. The Np sample and flux monitors were irradiated together for 30 minutes in the graphite thermal column equipped with the Kyoto University Research Reactor. The similar irradiation was carried out twice. After the irradiations, the Np samples were quantified using 312-keV gamma ray emitted from Pa in a radiation equilibrium with Np. The reaction rates of Np were obtained from gamma-ray peak net counts given by Np, and then the thermal-neutron capture cross-section of Np was found to be 173.84.4 barn by averaging the results obtained by the two irradiations. The present result was in agreement with the reported data given by a time-of-flight method within the limit of uncertainty.

Evaluation of analyzing power of gamma-ray polarimeter

Endo, Shunsuke; Shizuma, Toshiyuki*; Zen, H.*; Taira, Yoshitaka*; Omer, M.; Kawamura, Shiori*; Abe, Ryota*; Okudaira, Takuya*; Kitaguchi, Masaaki*; Shimizu, Hirohiko*

UVSOR-49, P. 38, 2022/08

Effect of sample density in prompt -ray analysis

Maeda, Makoto; Segawa, Mariko; Toh, Yosuke; Endo, Shunsuke; Nakamura, Shoji; Kimura, Atsushi

Scientific Reports (Internet), 12(1), p.6287_1 - 6287_8, 2022/06

https://doi.org/10.1038/s41598-022-08594-2

Angular distribution of rays from the -wave resonance of Sn

Koga, Jun*; Takada, Shusuke*; Endo, Shunsuke; Fujioka, Hiroyuki*; Hirota, Katsuya*; Ishizaki, Kohei*; Kimura, Atsushi; Kitaguchi, Masaaki*; Niinomi, Yudai*; Okudaira, Takuya*; et al.

Physical Review C, 105(5), p.054615_1 - 054615_5, 2022/05

https://doi.org/10.1103/PhysRevC.105.054615

no abstracts in English

Development of a neutron beam monitor for nuclear data measurement using spallation neutron source

Nakano, Hideto*; Katabuchi, Tatsuya*; Rovira Leveroni, G.*; Kodama, Yu*; Terada, Kazushi*; Kimura, Atsushi; Nakamura, Shoji; Endo, Shunsuke

JAEA-Conf 2021-001, p.166 - 170, 2022/03

https://doi.org/10.11484/jaea-conf-2021-001

Neutron capture and total cross-section measurements and resonance parameter analysis of niobium-93 below 400 eV

Endo, Shunsuke; Kimura, Atsushi; Nakamura, Shoji; Iwamoto, Osamu; Iwamoto, Nobuyuki; Rovira Leveroni, G.; Terada, Kazushi*; Meigo, Shinichiro; Toh, Yosuke; Segawa, Mariko; et al.

Journal of Nuclear Science and Technology, 59(3), p.318 - 333, 2022/03

https://doi.org/10.1080/00223131.2021.1970040