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JAEA Reports

Analysis of the radioactivity concentrations in radioactive waste generated from JPDR Facility

Tobita, Minoru*; Haraga, Tomoko; Endo, Tsubasa*; Omori, Hiroyuki*; Mitsukai, Akina; Aono, Ryuji; Ueno, Takashi; Ishimori, Kenichiro; Kameo, Yutaka

JAEA-Data/Code 2021-013, 30 Pages, 2021/12

JAEA-Data-Code-2021-013.pdf:1.47MB

Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed concrete samples generated from JPDR facility. In this report, we summarized the radioactivity concentrations of 21 radionuclides ($$^{3}$$H, $$^{14}$$C, $$^{36}$$Cl, $$^{41}$$Ca, $$^{60}$$Co, $$^{63}$$Ni, $$^{90}$$Sr, $$^{94}$$Nb, $$^{rm 108m}$$Ag, $$^{137}$$Cs, $$^{152}$$Eu, $$^{154}$$Eu, $$^{rm 166m}$$Ho, $$^{234}$$U, $$^{238}$$U, $$^{238}$$Pu, $$^{239}$$Pu, $$^{240}$$Pu, $$^{241}$$Am, $$^{243}$$Am, $$^{244}$$Cm) which were obtained from radiochemical analysis of the samples in fiscal year 2018-2019.

Journal Articles

Development of evaluation method for diffusion and filtration behavior of colloid in compacted bentonites using dendrimers

Endo, Takashi*; Tachi, Yukio; Ishidera, Takamitsu; Terashima, Motoki

Nihon Genshiryoku Gakkai Wabun Rombunshi, 20(1), p.9 - 22, 2021/03

Evaluation method of colloid diffusion and filtration in compacted bentonites was developed using dendrimers. Diffusion and filtration behavior of PAMAM dendrimers with the size of 5.7$$sim$$7.2nm was investigated by the through-diffusion experiment in bentonite compacted to 0.8 Mg/m$$^{3}$$ and saturated with 0.005$$sim$$0.5mol/L NaCl. Effective diffusivities (De) and filtration ratios (Rf) of dendrimers were determined from the breakthrough curves and the depth profiles in compacted bentonite, respectively. The De values of negatively charged dendrimer increased when porewater salinity increased and dendrimer size decreased as influenced by anion exclusion effect in negatively charged clay surfaces. The Rf values increased when porewater salinity decreased and dendrimer size increased, demonstrating significant fractions of dendrimer were filtered by narrow pores in complex pore networks. These trends consistent with the previous studies emphasize the validity of the evaluation method using dendrimer.

Journal Articles

Development and application of a $$^3$$He neutron spin filter at J-PARC

Okudaira, Takuya; Oku, Takayuki; Ino, Takashi*; Hayashida, Hirotoshi*; Kira, Hiroshi*; Sakai, Kenji; Hiroi, Kosuke; Takahashi, Shingo*; Aizawa, Kazuya; Endo, Hitoshi*; et al.

Nuclear Instruments and Methods in Physics Research A, 977, p.164301_1 - 164301_8, 2020/10

 Times Cited Count:4 Percentile:76.41(Instruments & Instrumentation)

Journal Articles

Determination of humic substances in deep groundwater from sedimentary formations by the carbon concentration-based DAX-8 resin isolation technique

Terashima, Motoki; Endo, Takashi*; Miyakawa, Kazuya

Journal of Nuclear Science and Technology, 57(4), p.380 - 387, 2020/04

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

Journal Articles

Measurement of the angular distribution of $$gamma$$-rays after neutron capture by $$^{139}$$La for a T-violation search

Okudaira, Takuya; Shimizu, Hirohiko*; Kitaguchi, Masaaki*; Hirota, Katsuya*; Haddock, C. C.*; Ito, Ikuya*; Yamamoto, Tomoki*; Endo, Shunsuke*; Ishizaki, Kohei*; Sato, Takumi*; et al.

EPJ Web of Conferences, 219, p.09001_1 - 09001_6, 2019/12

Parity violating effects enhanced by up to 10$$^6$$ times have been observed in several neutron induced compound nuclei. There is a theoretical prediction that time reversal (T) violating effects can also be enhanced in these nuclei implying that T-violation can be searched for by making very sensitive measurements. However, the enhancement factor has not yet been measured in all nuclei. The angular distribution of the (n,$$gamma$$) reaction was measured with $$^{139}$$La by using a germanium detector assembly at J-PARC, and the enhancement factor was obtained. From the result, the measurement time to achieve the most sensitive T-violation search was estimated as 1.4 days, and a 40% polarized $$^{139}$$La target and a 70% polarized $$^3$$He spin filter whose thickness is 70 atm$$cdot$$cm are needed. Therefore high quality $$^3$$He spin filter is developed in JAEA. The measurement result of the (n,$$gamma$$) reaction at J-PARC and the development status of the $$^3$$He spin filter will be presented.

Journal Articles

Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex, 2; Neutron scattering instruments

Nakajima, Kenji; Kawakita, Yukinobu; Ito, Shinichi*; Abe, Jun*; Aizawa, Kazuya; Aoki, Hiroyuki; Endo, Hitoshi*; Fujita, Masaki*; Funakoshi, Kenichi*; Gong, W.*; et al.

Quantum Beam Science (Internet), 1(3), p.9_1 - 9_59, 2017/12

The neutron instruments suite, installed at the spallation neutron source of the Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex (J-PARC), is reviewed. MLF has 23 neutron beam ports and 21 instruments are in operation for user programs or are under commissioning. A unique and challenging instrumental suite in MLF has been realized via combination of a high-performance neutron source, optimized for neutron scattering, and unique instruments using cutting-edge technologies. All instruments are/will serve in world-leading investigations in a broad range of fields, from fundamental physics to industrial applications. In this review, overviews, characteristic features, and typical applications of the individual instruments are mentioned.

Journal Articles

A Stencil framework to realize large-scale computations beyond device memory capacity on GPU supercomputers

Shimokawabe, Takashi*; Endo, Toshio*; Onodera, Naoyuki; Aoki, Takayuki*

Proceedings of 2017 IEEE International Conference on Cluster Computing (IEEE Cluster 2017) (Internet), p.525 - 529, 2017/09

Stencil-based applications such as CFD have succeeded in obtaining high performance on GPU supercomputers. The problem sizes of these applications are limited by the GPU device memory capacity, which is typically smaller than the host memory. On GPU supercomputers, a locality improvement technique using temporal blocking method with memory swapping between host and device enables large computation beyond the device memory capacity. Our high-productivity stencil framework automatically applies temporal blocking to boundary exchange required for stencil computation and supports automatic memory swapping provided by a MPI/CUDA wrapper library. The framework-based application for the airflow in an urban city maintains 80% performance even with the twice larger than the GPU memory capacity and have demonstrated good weak scalability on the TSUBAME 2.5 supercomputer.

Journal Articles

Gamma radiation resistance of spin Seebeck devices

Yagmur, A.*; Uchida, Kenichi*; Ihara, Kazuki*; Ioka, Ikuo; Kikkawa, Takashi*; Ono, Madoka*; Endo, Junichi*; Kashiwagi, Kimiaki*; Nakashima, Tetsuya*; Kirihara, Akihiro*; et al.

Applied Physics Letters, 109(24), p.243902_1 - 243902_4, 2016/12

 Times Cited Count:2 Percentile:12.91(Physics, Applied)

Thermoelectric devices based on the spin Seebeck effect (SSE) were irradiated with gamma ($$gamma$$) rays with the total dose of around 3$$times$$10$$^{5}$$ Gy in order to investigate the $$gamma$$-radiation resistance of the devices. To demonstrate this, Pt/Ni$$_{0.2}$$Zn$$_{0.3}$$Fe$$_{2.5}$$O$$_{4}$$/Glass and Pt/Bi$$_{0.1}$$Y$$_{2.9}$$Fe$$_{5}$$O$$_{12}$$/Gd$$_{3}$$Ga$$_{5}$$O$$_{12}$$ SSE devices were used. We confirmed that the thermoelectric, magnetic, and structural properties of the SSE devices are not affected by the $$gamma$$-ray irradiation. This result demonstrates that SSE devices are applicable to thermoelectric generation even in high radiation environments.

Journal Articles

Small-angle neutron scattering study of specific interaction and coordination structure formed by mono-acetyl-substituted dibenzo-20-crown-6-ether and cesium ions

Motokawa, Ryuhei; Kobayashi, Toru; Endo, Hitoshi*; Ikeda, Takashi; Yaita, Tsuyoshi; Suzuki, Shinichi; Narita, Hirokazu*; Akutsu, Kazuhiro*; Heller, W. T.*

Journal of Nuclear Science and Technology, 53(8), p.1205 - 1211, 2016/08

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

Journal Articles

22A beam production of the uniform negative ions in the JT-60 negative ion source

Yoshida, Masafumi; Hanada, Masaya; Kojima, Atsushi; Kashiwagi, Mieko; Grisham, L. R.*; Hatayama, Akiyoshi*; Shibata, Takanori*; Yamamoto, Takashi*; Akino, Noboru; Endo, Yasuei; et al.

Fusion Engineering and Design, 96-97, p.616 - 619, 2015/10

 Times Cited Count:10 Percentile:73.32(Nuclear Science & Technology)

In JT-60 Super Advanced for the fusion experiment, 22A, 100s negative ions are designed to be extracted from the world largest ion extraction area of 450 mm $$times$$ 1100 mm. One of the key issues for producing such as high current beams is to improve non-uniform production of the negative ions. In order to improve the uniformity of the negative ions, a tent-shaped magnetic filter has newly been developed and tested for JT-60SA negative ion source. The original tent-shaped filter significantly improved the logitudunal uniformity of the extracted H$$^{-}$$ ion beams. The logitudinal uniform areas within a $$pm$$10 deviation of the beam intensity were improved from 45% to 70% of the ion extraction area. However, this improvement degrades a horizontal uniformity. For this, the uniform areas was no more than 55% of the total ion extraction area. In order to improve the horizontal uniformity, the filter strength has been reduced from 660 Gasus$$cdot$$cm to 400 Gasus$$cdot$$cm. This reduction improved the horizontal uniform area from 75% to 90% without degrading the logitudinal uniformity. This resulted in the improvement of the uniform area from 45% of the total ion extraction areas. This improvement of the uniform area leads to the production of a 22A H$$^{-}$$ ion beam from 450 mm $$times$$ 1100 mm with a small amount increase of electron current of 10%. The obtained beam current fulfills the requirement for JT-60SA.

JAEA Reports

Evaluation of irradiation behavior on oxide dispersion strengthened (ODS) steel claddings irradiated in Joyo/CMIR-6

Yano, Yasuhide; Otsuka, Satoshi; Yamashita, Shinichiro; Ogawa, Ryuichiro; Sekine, Manabu; Endo, Toshiaki; Yamagata, Ichiro; Sekio, Yoshihiro; Tanno, Takashi; Uwaba, Tomoyuki; et al.

JAEA-Research 2013-030, 57 Pages, 2013/11

JAEA-Research-2013-030.pdf:48.2MB

It is necessary to develop the fast reactor core materials, which can achieve high-burnup operation improving safety and economical performance. Ferritic steels are expected to be good candidate core materials to achieve this objective because of their excellent void swelling resistance. Therefore, oxide dispersion strengthened (ODS) ferritic steel and 11Cr-ferritic/martensitic steel (PNC-FMS) have been respectively developed for cladding and wrapper tube materials in Japan Atomic Energy Agency. In this study, the effects of fast neutron irradiation on mechanical properties and microstructure of 9Cr-and 12Cr-ODS steel claddings for fast reactor were investigated. Specimens were irradiated in the experimental fast reactor Joyo using the CMIR-6 at temperatures between 420 and 835$$^{circ}$$C to fast neutron doses ranging from 16 to 33 dpa. The post-irradiation ring tensile tests were carried out at irradiation temperatures.

Journal Articles

Origin of non-uniformity of the source plasmas in JT-60 negative ion source

Yoshida, Masafumi; Hanada, Masaya; Kojima, Atsushi; Inoue, Takashi; Kashiwagi, Mieko; Grisham, L. R.*; Akino, Noboru; Endo, Yasuei; Komata, Masao; Mogaki, Kazuhiko; et al.

Plasma and Fusion Research (Internet), 8(Sp.1), p.2405146_1 - 2405146_4, 2013/11

Distributions of H$$^{0}$$ and H$$^{+}$$ in the source plasmas produced at the end-plugs of JT-60 negative ions source were measured by Langmuir probes and emission spectroscopy in order to experimentally investigate the cause of lower density of the negative ions extracted from end-plugs in the source. Densities of H$$^{0}$$ and H$$^{+}$$ in end-plugs of the plasma grid in the source were compared with those in the center regions. As a result, lower density of the negative ion at the edge was caused by lower beam optics due to lower and higher density of the H$$^{0}$$ and H$$^{+}$$.

Journal Articles

Utilization of process monitoring data in the Tokai Reprocessing Plant for future nuclear security

Kimura, Takashi; Shimizu, Yasuyuki; Yamazaki, Katsuyuki; Endo, Yuji; Nakamura, Hironobu

Kaku Busshitsu Kanri Gakkai (INMM) Nihon Shibu Dai-34-Kai Nenji Taikai Rombunshu (Internet), 8 Pages, 2013/10

no abstracts in English

Journal Articles

Utilization of process monitoring data in the Tokai Reprocessing Plant for future nuclear security

Shimizu, Yasuyuki; Yamazaki, Katsuyuki; Kimura, Takashi; Endo, Yuji; Nakamura, Hironobu

Proceedings of INMM 54th Annual Meeting (CD-ROM), 7 Pages, 2013/07

Japanese regulation of reprocessing safety and security was revised in March 2012, and almost all requirements except for nuclear material accountancy and control described in the INFCIRC225/rev.5 are included into the regulation. We have many things to do to meet the requirements within 2 years pursuant to the regulation. Separately from the revised regulation, we think that utilizing the process monitoring data not only for the safety control but also for the nuclear material security would be useful in establishing more effective and efficient nuclear material security. Since we observe the process monitoring data to confirm the operational condition including unusual change for the safety purpose, it is though that the various alarm information through the process monitoring data help to detect the risk of sabotage and unauthorized removal. As future challenge, we would like to establish a possible method of utilizing the process monitoring data in combination with the physical protection to make it possible to give more effective and efficient nuclear material security.

Journal Articles

Development of multi-purpose MW gyrotrons for fusion devices

Minami, Ryutaro*; Kariya, Tsuyoshi*; Imai, Tsuyoshi*; Numakura, Tomoharu*; Endo, Yoichi*; Nakabayashi, Hidetaka*; Eguchi, Taku*; Shimozuma, Takashi*; Kubo, Shin*; Yoshimura, Yasuo*; et al.

Nuclear Fusion, 53(6), p.063003_1 - 063003_7, 2013/06

Journal Articles

Development of multi-purpose MW gyrotrons for fusion devices

Minami, Ryutaro*; Kariya, Tsuyoshi*; Imai, Tsuyoshi*; Numakura, Tomoharu*; Endo, Yoichi*; Nakabayashi, Hidetaka*; Eguchi, Taku*; Shimozuma, Takashi*; Kubo, Shin*; Yoshimura, Yasuo*; et al.

Nuclear Fusion, 53(6), p.063003_1 - 063003_7, 2013/06

 Times Cited Count:12 Percentile:54.31(Physics, Fluids & Plasmas)

Journal Articles

Magnetic properties of single crystalline YbFe$$_{2}$$O$$_{4}$$

Yoshii, Kenji; Mizumaki, Masaichiro*; Matsumoto, Keisuke*; Mori, Shigeo*; Endo, Naruki; Saito, Hiroyuki; Matsumura, Daiju; Kambe, Takashi*; Ikeda, Naoshi*

Journal of Physics; Conference Series, 428, p.012032_1 - 012032_5, 2013/04

 Times Cited Count:13 Percentile:97.61

We have investigated a single crystal of multiferroic YbFe$$_{2}$$O$$_{4}$$. Its magnetic transition temperature was 250 K. The magnetization along the c-axis was much larger than that within the ab plane, indicating the Ising character of this system. The field-cooled magnetization became negative below 10 K. This was explained in terms of an antiparallel coupling between Yb and Fe moments. Magnetocaloric effects were also observed. The change of entropy was found to show a broad peak with a width of 100 K, which is favorable to application.

Journal Articles

Neutron irradiation tests for beryllium material selection of neutron reflector in JMTR

Tsuchiya, Kunihiko; Ito, Masayasu; Kitagishi, Shigeru; Endo, Yasuichi; Saito, Takashi; Hanawa, Yoshio; Dorn, C. K.*

JAEA-Conf 2012-002, p.111 - 114, 2012/12

no abstracts in English

Journal Articles

Performance evaluation of friction welded joint of zircaloy-2 to type 316L stainless steel

Kitagishi, Shigeru; Saito, Takashi; Kikuchi, Taiji; Endo, Yasuichi; Tsuchiya, Kunihiko

Nihon Kikai Gakkai Rombunshu, A, 78(788), p.564 - 570, 2012/04

The development of the friction welded joint between Zircaloy-2 (Zry-2) and Type 316L stainless steel (SUS316L) has been carried out for the fabrication of fuel irradiation capsules in Japan Materials Testing Reactor (JMTR). The welding condition was determined from the fabrication test results of total loss and tensile strength. The joint interface was characterized by metallographic observation, elemental analysis and micro-hardness test. It was found that heat-affected zones at the joint interface were different between the center and outside positions. The tensile strength of the joint was equal to that of base Zry-2 metals at 300$$^{circ}$$C. And, the joint performance was good from the results of helium leak test and hydraulic pressure burst test. From the results of these tests, it was obvious that the Zry-2/SUS316L friction welded joints were promised to use for the structural material of irradiation capsules for fuel irradiation tests.

Journal Articles

Progress in development and design of the neutral beam injector for JT-60SA

Hanada, Masaya; Kojima, Atsushi; Tanaka, Yutaka; Inoue, Takashi; Watanabe, Kazuhiro; Taniguchi, Masaki; Kashiwagi, Mieko; Tobari, Hiroyuki; Umeda, Naotaka; Akino, Noboru; et al.

Fusion Engineering and Design, 86(6-8), p.835 - 838, 2011/10

 Times Cited Count:8 Percentile:58.2(Nuclear Science & Technology)

Neutral beam (NB) injectors for JT-60 Super Advanced (JT-60SA) have been designed and developed. Twelve positive-ion-based and one negative-ion-based NB injectors are allocated to inject 30 MW D$$^{0}$$ beams in total for 100 s. Each of the positive-ion-based NB injector is designed to inject 1.7 MW for 100s at 85 keV. A part of the power supplies and magnetic shield utilized on JT-60U are upgraded and reused on JT-60SA. To realize the negative-ion-based NB injector for JT-60SA where the injection of 500 keV, 10 MW D$$^{0}$$ beams for 100s is required, R&Ds of the negative ion source have been carried out. High-energy negative ion beams of 490-500 keV have been successfully produced at a beam current of 1-2.8 A through 20% of the total ion extraction area, by improving voltage holding capability of the ion source. This is the first demonstration of a high-current negative ion acceleration of $$>$$1 A to 500 keV. The design of the power supplies and the beamline is also in progress. The procurement of the acceleration power supply starts in 2010.

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