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Journal Articles

Crystal-liquid duality driven ultralow two-channel thermal conductivity in $$alpha$$-MgAgSb

Li, J.*; Li, X.*; Zhang, Y.*; Zhu, J.*; Zhao, E.*; Kofu, Maiko; Nakajima, Kenji; Avdeev, M.*; Liu, P.-F.*; Sui, J.*; et al.

Applied Physics Reviews (Internet), 11(1), p.011406_1 - 011406_8, 2024/03

 Times Cited Count:0 Percentile:0.01(Physics, Applied)

Journal Articles

Extreme phonon anharmonicity underpins superionic diffusion and ultralow thermal conductivity in argyrodite Ag$$_{8}$$SnSe$$_{6}$$

Ren, Q.*; Gupta, M. K.*; Jin, M.*; Ding, J.*; Wu, J.*; Chen, Z.*; Lin, S.*; Fabelo, O.*; Rodriguez-Velamazan, J. A.*; Kofu, Maiko; et al.

Nature Materials, 22, p.999 - 1006, 2023/05

 Times Cited Count:21 Percentile:99.22(Chemistry, Physical)

Journal Articles

Two-step Mott transition in Ni(S,Se)$$_2$$; $$mu$$SR studies and charge-spin percolation model

Sheng, Q.*; Kaneko, Tatsuya*; Yamakawa, Kohtaro*; Guguchia, Z.*; Gong, Z.*; Zhao, G.*; Dai, G.*; Jin, C.*; Guo, S.*; Fu, L.*; et al.

Physical Review Research (Internet), 4(3), p.033172_1 - 033172_14, 2022/09

Journal Articles

Strong lattice anharmonicity exhibited by the high-energy optical phonons in thermoelectric material

Wu, P.*; Fan, F.-R.*; Hagihara, Masato*; Kofu, Maiko; Peng, K.*; Ishikawa, Yoshihisa*; Lee, S.*; Honda, Takashi*; Yonemura, Masao*; Ikeda, Kazutaka*; et al.

New Journal of Physics (Internet), 22(8), p.083083_1 - 083083_9, 2020/08

 Times Cited Count:8 Percentile:58.58(Physics, Multidisciplinary)

Thermoelectric material SnSe has aroused world-wide interests in the past years, and its inherent strong lattice anharmonicity is regarded as a crucial factor for its outstanding thermoelectric performance. However, the understanding of lattice anharmonicity in SnSe system remains inadequate, especially regarding how phonon dynamics are affected by this behavior. In this work, we present a comprehensive study of lattice dynamics on Na$$_{0.003}$$Sn$$_{0.997}$$Se$$_{0.9}$$S$$_{0.1}$$ by means of neutron total scattering, inelastic neutron scattering, Raman spectroscopy as well as frozen-phonon calculations. Lattice anharmonicity is evidenced by pair distribution function, inelastic neutron scattering and Raman measurements. By separating the effects of thermal expansion and multi-phonon scattering, we found that the latter is very significant in high-energy optical phonon modes. The strong temperature-dependence of these phonon modes indicate the anharmonicity in this system. Moreover, our data reveals that the linewidths of high-energy optical phonons become broadened with mild doping of sulfur. Our studies suggest that the thermoelectric performance of SnSe could be further enhanced by reducing the contributions of high-energy optical phonon modes to the lattice thermal conductivity via phonon engineering.

Journal Articles

Multiple magnetic bilayers and unconventional criticality without frustration in BaCuSi$$_2$$O$$_6$$

Allenspach, S.*; Biffin, A.*; Stuhr, U.*; Tucker, G. S.*; Kawamura, Seiko; Kofu, Maiko; Voneshen, D. J.*; Boehm, M.*; Normand, B.*; Laflorencie, N.*; et al.

Physical Review Letters, 124(17), p.177205_1 - 177205_7, 2020/05

 Times Cited Count:10 Percentile:65.11(Physics, Multidisciplinary)

Journal Articles

Ultralow thermal conductivity from transverse acoustic phonon suppression in distorted crystalline $$alpha$$-MgAgSb

Li, X.*; Liu, P.-F.*; Zhao, E.*; Zhang, Z.*; Guide, T.*; Le, M. D.*; Avdeev, M.*; Ikeda, Kazutaka*; Otomo, Toshiya*; Kofu, Maiko; et al.

Nature Communications (Internet), 11, p.942_1 - 942_9, 2020/02

 Times Cited Count:36 Percentile:90.35(Multidisciplinary Sciences)

In high-performance thermoelectric materials, there are two main low thermal conductivity mechanisms: the phonon anharmonic and phonon scattering resulting from the dynamic disorder, which have been successfully revealed by inelastic neutron scattering. Using neutron scattering and ab initio calculations, we report here a mechanism of static local structure distortion combined with phonon-anharmonic-induced ultralow lattice thermal conductivity in $$alpha$$-MgAgSb. Since the transverse acoustic phonons are almost fully scattered by the intrinsic distorted rocksalt sublattice in this compound, the heat is mainly transported by the longitudinal acoustic phonons. The ultralow thermal conductivity in $$alpha$$-MgAgSb is attributed to its atomic dynamics being altered by the structure distortion, which presents a possible microscopic route to enhance the performance of similar thermoelectric materials.

Journal Articles

Nitration activates tyrosine toward reaction with the hydrated electron

Shi, W.-Q.*; Fu, H.-Y.*; Bounds, P. L.*; Muroya, Yusa*; Lin, M.; Katsumura, Yosuke*; Zhao, Y.-L.*; Chai, Z.-F.*

Radiation Research, 176(1), p.128 - 133, 2011/07

 Times Cited Count:3 Percentile:17.22(Biology)

3-Nitrotyrosine (3-NT) has been reported as an important biomarker of oxidative stress and potential source of reactive oxygen species (ROSs). In this work, the UV-visible absorption spectra of the transients formed by hydrated electron (e$$_{rm aq}$$$$^{-}$$) reacting with 3-NT and its derivatives were investigated, the spectra showed many characteristics of aromatic nitro anion radical. The reaction rate constants of e$$_{rm aq}$$$$^{-}$$ reacting with 3-NT, N-acetyl-3-nitrotyrosine ethyl ester (NANTE) and nitrotyrosine-containing peptide Gly-nitroTyr-Gly at neutral pH were determined, respectively, which were almost two orders of magnitude higher than that of tyrosine and tyrosine-containing peptides. The pH-dependence of e$$_{rm aq}$$$$^{-}$$ decay rate constants in presence of 3-NT was also studied.

Journal Articles

Sequential variation of atmospheric mercury in Tokai-mura, seaside area of eastern central Japan

Osawa, Takahito; Ueno, Takashi; Fu, F.*

Journal of Geophysical Research, 112(D19), p.D19107_1 - D19107_9, 2007/10

 Times Cited Count:15 Percentile:35.93(Meteorology & Atmospheric Sciences)

Concentrations of gaseous elemental mercury (GEM) were continuously measured from Oct. 2005 to Aug. 2006 in Tokai-mura, a small city on the Pacific side of central Japan. The concentration of atmospheric mercury in summer and autumn is higher than in winter and spring, and an 11-month average of one-hour measurements is 3.78 ng/m$$^{3}$$ (n=7551). Our results showed that changes in the GEM level in Tokai-mura are largely determined by temperature and relative humidity, but are independent of wind speed and direction. Two contrary patterns were observed in the daily-cycle of GEM concentrations: the most frequent pattern of lower concentrations at noon and a pattern of higher concentrations at noon, which was only observed in November. Our results showed that two nearby potential anthropogenic sources of mercury, a coal-fired power plant and incineration facility, have only little effect on the gaseous elemental mercury (GEM) in Tokai-mura based on only GEM measurements.

Journal Articles

Seasonal characteristics of chemical compositions of the atmospheric aerosols collected in urban seaside area at Tokaimura, eastern central Japan

Fu, F.; Watanabe, Kazuo; Yabuki, Sadayo*; Akagi, Tasuku*

Journal of Geophysical Research, 109(20), p.D20212_1 - D20212_9, 2004/10

Size-separated aerosol samples were collected at Tokaimura urban seaside area of Japan using an Andersen type sampler during July 2002 to July 2003. The size-separated aerosols were divided into water-soluble and insoluble fractions, and chemical compositions (Na$$^{+}$$, Cl$$^{-}$$, NH$$_{3}$$$$^{+}$$, NO$$_{3}$$$$^{-}$$, SO$$_{4}$$$$^{2-}$$, Al, Ca, Mg, Fe, Pb, Th and U) in both water-soluble and insoluble fractions were analyzed. Then, the seasonal variations and the size-distribution in mass concentration and chemical composition have been investigated in detail. Our results showed that the atmospheric aerosol in Tokaimura was obviously affected by dust storm in China, and that sea-salt particles were bigger than those in the Antarctic and were deficient in chlorine.

Journal Articles

Rare earth element distribution in the acetic acid soluble fraction of combusted coals; Its implication as a proxy for the original coal-forming plants

Fu, F.; Akagi, Tasuku*; Suzuki, Yuichiro*; Watanabe, Kazuo; Yabuki, Sadayo*

Geochemical Journal, 38(4), p.333 - 343, 2004/08

 Times Cited Count:9 Percentile:20.33(Geochemistry & Geophysics)

no abstracts in English

Journal Articles

Characteristics of Alfv$'e$n eigenmodes, burst modes and chirping modes in the Alfv$'e$n frequency range driven by negative ion based neutral beam injection in JT-60U

Kusama, Yoshinori; Kramer, G. J.; Kimura, Haruyuki; Saigusa, Mikio*; Ozeki, Takahisa; Tobita, Kenji; Oikawa, Toshihiro; Shinohara, Koji; Kondoh, Takashi; Moriyama, Shinichi; et al.

Nuclear Fusion, 39(11Y), p.1837 - 1843, 1999/11

 Times Cited Count:68 Percentile:87.07(Physics, Fluids & Plasmas)

no abstracts in English

Journal Articles

Destabilization of ellipticity-induced Alfven eigenmodes during ICRF heating and stabilization by negative-ion-based neutral beam injection in JT-60U

Kusama, Yoshinori; Fu, G. Y.*; Kramer, G. J.*; Saigusa, Mikio*; Oikawa, Toshihiro; Ozeki, Takahisa; Moriyama, Shinichi; Tchernychev, F. V.*; Nemoto, Masahiro; Kondoh, Takashi; et al.

Plasma Physics and Controlled Fusion, 41(9), p.1167 - 1177, 1999/00

 Times Cited Count:5 Percentile:20.12(Physics, Fluids & Plasmas)

no abstracts in English

Journal Articles

Alfv$'e$n eigenmodes and their impact on plasma characteristics in JT-60U

Kusama, Yoshinori; Nazikian, R.*; Kramer, G. J.*; Kimura, Haruyuki; Saigusa, Mikio*; Ozeki, Takahisa; Fu, G. Y.*; Tobita, Kenji; Oikawa, Toshihiro; Shinohara, Koji; et al.

Fusion Energy 1998, 2, p.537 - 544, 1998/10

no abstracts in English

Oral presentation

Difference of results obtained with high and low Andersen sampler respectively in the research of atmospheric aerosols

Fu, F.; Watanabe, Kazuo; Wu, Y.*; Xiao, L.*; Xu, X.*; Shinohara, Nobuo

no journal, , 

no abstracts in English

Oral presentation

The Physical characteristics and light absorption of black carbon aerosols in the atmosphere

Fu, F.; Watanabe, Kazuo; Shinohara, Nobuo

no journal, , 

no abstracts in English

Oral presentation

Neutron scattering study on all-inorganic Li$$_{2}$$(Li$$_{1-x}$$Fe$$_{x}$$)N exhibiting single-molecule magnet behavior

Kofu, Maiko; Jesche, A.*; Breitner, F.*; H$"o$hn, P.*; Kawamura, Seiko; Nakajima, Kenji; Hiroi, Kosuke; Oishi, Kazuki*; Kawamura, Yukihiko*

no journal, , 

no abstracts in English

Oral presentation

Neutron scattering study on Li$$_{2}$$(Li$$_{1-x}$$Fe$$_{x}$$)N displaying single molecule magnet behavior

Kofu, Maiko; Jesche, A.*; Breitner, F.*; H$"o$hn, P.*; Kawamura, Seiko; Nakajima, Kenji; Hiroi, Kosuke; Oishi, Kazuki*; Kawamura, Yukihiko*

no journal, , 

no abstracts in English

17 (Records 1-17 displayed on this page)
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