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Journal Articles

Valence control of charge and orbital frustrated system YbFe$$_{2}$$O$$_{4}$$ with electrochemical Li$$^{+}$$ intercalation

Murase, Satoshi*; Yoshikawa, Yumi*; Fujiwara, Kosuke*; Fukada, Yukimasa*; Teranishi, Takashi*; Kano, Jun*; Fujii, Tatsuo*; Inada, Yasuhiro*; Katayama, Misaki*; Yoshii, Kenji; et al.

Journal of Physics and Chemistry of Solids, 162, p.110468_1 - 110468_6, 2022/03

 Times Cited Count:0 Percentile:0(Chemistry, Multidisciplinary)

We report a trial of the valence control for mixed valence iron triangular oxide YbFe$$_{2}$$O$$_{4}$$ in order to develop an effective technique to control the frustration of charges in strongly correlated electron systems. The electro-chemical doping of Li$$^{+}$$ into YbFe$$_{2}$$O$$_{4}$$ was examined on the cell type sample similar to the Li-ion secondary battery cell. Systematic change of the lattice constant, Fe-Fe and Fe-Yb distance were observed with Li doping. Maximum value of the doping was over 300 mAh/g. An EXAFS experiment indicated that Li positioned between Yb octahedron layer (U-layer) and Fe-bipyramidal layer (W-layer). However, detailed change of iron valence state of YbFe$$_{2}$$O$$_{4}$$ was not clearly observed because of the superimpose of the signal from iron metal nano particles in XANES observation. The results indicate that the electrochemical method might be one of the potential technique to control the frustration of charges in YbFe$$_{2}$$O$$_{4}$$.

Journal Articles

PSTEP: Project for solar-terrestrial environment prediction

Kusano, Kanya*; Ichimoto, Kiyoshi*; Ishii, Mamoru*; Miyoshi, Yoshizumi*; Yoden, Shigeo*; Akiyoshi, Hideharu*; Asai, Ayumi*; Ebihara, Yusuke*; Fujiwara, Hitoshi*; Goto, Tadanori*; et al.

Earth, Planets and Space (Internet), 73(1), p.159_1 - 159_29, 2021/12

 Times Cited Count:6 Percentile:49.29(Geosciences, Multidisciplinary)

The PSTEP is a nationwide research collaboration in Japan and was conducted from April 2015 to March 2020, supported by a Grant-in-Aid for Scientific Research on Innovative Areas from the Ministry of Education, Culture, Sports, Science and Technology of Japan. It has made a significant progress in space weather research and operational forecasts, publishing over 500 refereed journal papers and organizing four international symposiums, various workshops and seminars, and summer school for graduate students at Rikubetsu in 2017. This paper is a summary report of the PSTEP and describes the major research achievements it produced.

Journal Articles

Sm valence determination of Sm-based intermetallics using $$^{149}$$Sm M$"{o}$ssbauer and Sm L$$_{rm III}$$-edge X-ray absorption spectroscopies

Tsutsui, Satoshi; Higashinaka, Ryuji*; Nakamura, Raito*; Fujiwara, Kosuke*; Nakamura, Jin*; Kobayashi, Yoshio*; Ito, Takashi; Yoda, Yoshitaka*; Kato, Kazuo*; Nitta, Kiyofumi*; et al.

Hyperfine Interactions, 242(1), p.32_1 - 32_10, 2021/12

 Times Cited Count:1 Percentile:84.11(Physics, Atomic, Molecular & Chemical)

Journal Articles

Emergence of spin-orbit coupled ferromagnetic surface state derived from Zak phase in a nonmagnetic insulator FeSi

Otsuka, Yusuke*; Kanazawa, Naoya*; Hirayama, Motoaki*; Matsui, Akira*; Nomoto, Takuya*; Arita, Ryotaro*; Nakajima, Taro*; Hanashima, Takayasu*; Ukleev, V.*; Aoki, Hiroyuki; et al.

Science Advances (Internet), 7(47), p.eabj0498_1 - eabj0498_9, 2021/11

 Times Cited Count:8 Percentile:51.2(Multidisciplinary Sciences)

Journal Articles

High temperature gas-cooled reactors

Takeda, Tetsuaki*; Inagaki, Yoshiyuki; Aihara, Jun; Aoki, Takeshi; Fujiwara, Yusuke; Fukaya, Yuji; Goto, Minoru; Ho, H. Q.; Iigaki, Kazuhiko; Imai, Yoshiyuki; et al.

High Temperature Gas-Cooled Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.5, 464 Pages, 2021/02

As a general overview of the research and development of a High Temperature Gas-cooled Reactor (HTGR) in JAEA, this book describes the achievements by the High Temperature Engineering Test Reactor (HTTR) on the designs, key component technologies such as fuel, reactor internals, high temperature components, etc., and operational experience such as rise-to-power tests, high temperature operation at 950$$^{circ}$$C, safety demonstration tests, etc. In addition, based on the knowledge of the HTTR, the development of designs and component technologies such as high performance fuel, helium gas turbine and hydrogen production by IS process for commercial HTGRs are described. These results are very useful for the future development of HTGRs. This book is published as one of a series of technical books on fossil fuel and nuclear energy systems by the Power Energy Systems Division of the Japan Society of Mechanical Engineers.

Journal Articles

Evaluation of change of LSD spikes by long-term storage

Shibano, Koya; Abe, Katsuo; Tsukasa, Kazuo*; Hosogane, Tatsuya; Kayano, Masashi; Sumi, Mika; Fujiwara, Hideki*; Yamaguchi, Kazuya*; Motoki, Chika*

Dai-41-Kai Nihon Kaku Busshitsu Kanri Gakkai Nenji Taikai Kaigi Rombunshu (Internet), 4 Pages, 2020/11

Large-sized dried spikes, called LSD spike, are used as reference material for accountancy analysis for Plutonium and Uranium by Isotope Dilution Mass Spectrometry. LSD spikes preparation is performed each steps as followed (1) Preparing Plutonium and Uranium mix solution, (2) Aliquoting mix solution to vials, and (3) Drying. J-MOX have planned prepared in-house LSD spike and utilized it for accountancy analysis. If LSD spikes are stored for long term, dried material peel off from bottom of vial and it may affect analytical results. In this study, LSD spikes, which have composition suitable for accountancy analysis in J-MOX, had been stored for about 2 years, then long-term stability of LSD spikes had been evaluated.

Journal Articles

Vertical distribution of $$^{90}$$Sr and $$^{137}$$Cs in soils near the Fukushima Daiichi Nuclear Power Station

Sasaki, Takayuki*; Matoba, Daisuke*; Dohi, Terumi; Fujiwara, Kenso; Kobayashi, Taishi*; Iijima, Kazuki

Journal of Radioanalytical and Nuclear Chemistry, 326(1), p.303 - 314, 2020/10

 Times Cited Count:3 Percentile:34.82(Chemistry, Analytical)

Journal Articles

Electron microscopic analysis of radiocaesium-bearing microparticles in lichens collected within 3 km of the Fukushima Dai-ichi Nuclear Power Plant

Dohi, Terumi; Tagomori, Hisaya; Omura, Yoshihito*; Fujiwara, Kenso; Kanaizuka, Seiichi*; Iijima, Kazuki

Environmental Radiochemical Analysis VI, p.58 - 70, 2019/09

In this study we established a separation method for radiocaesium-bearing microparticles (CsMPs) from lichens using electron microscopic analysis. Lichens were first digested within hydrogen peroxide and then an automatic particle analyser system based on FE-EPMA was used for detecting CsMPs within lots of mineral-like and metallic particles quickly. The elemental composition and radiocaesium activities of the separated CsMPs were measured, and the results show that the digestion treatment did not influence the CsMPs characteristics. An inhomogeneous elemental distribution was found in some CsMPs by two-dimensional elemental analysis using FE-EMPA. Our methods for separation of CsMPs and analysing their elemental composition are expected to be useful for grasping the chemical composition trends of CsMPs statistically.

JAEA Reports

Separation of radiocaesium-bearing micro particle from environmental samples; Application to litter samples

Tagomori, Hisaya; Dohi, Terumi; Ishii, Yasuo; Kanaizuka, Seiichi*; Fujiwara, Kenso; Iijima, Kazuki

JAEA-Technology 2019-001, 37 Pages, 2019/03

JAEA-Technology-2019-001.pdf:26.85MB

An efficient methodology for separating the radiocaesium-bearing micro particles (CsMPs) released by the TEPCO's Fukushima Dai-ichi Nuclear Power Station accident is required to investigate their spatial distribution and physicochemical properties. In this report we developed an efficiency separation method for CsMP from litters since the radiocaesium in litter may affect the radiocaesium cycling in forest ecosystem. One CsMP separation from litter containing lots of soil particles was attained within three days using electron microscopic analysis with digestion treatment of organic matter. This methodology is expected as CsMPs efficient separation method for not only forest floor litter but also barks and leaves of living tree, and other organic materials in the forested environment.

Journal Articles

Spatial anisotropy of neutrons emitted from the $$^{56}$$Fe($$gamma$$, n)$$^{55}$$Fe reaction with a linearly polarized $$gamma$$-ray beam

Hayakawa, Takehito; Shizuma, Toshiyuki; Miyamoto, Shuji*; Amano, Sho*; Takemoto, Akinori*; Yamaguchi, Masashi*; Horikawa, Ken*; Akimune, Hidetoshi*; Chiba, Satoshi*; Ogata, Kazuyuki*; et al.

Physical Review C, 93(4), p.044313_1 - 044313_4, 2016/04

 Times Cited Count:7 Percentile:48.93(Physics, Nuclear)

We have measured the azimuthal anisotropy of neutrons emitted from the $$^{56}$$Fe($$gamma$$, n)$$^{55}$$Fe reaction with a linearly polarized $$gamma$$ ray beam generated by laser Compton scattering at NewSUBARU. Neutron yields at the polar angle of 90$$^{circ}$$ have been measured as a function of the azimuthal angle $$phi$$ between the detector and the linear polarization plane of the ray beam. The azimuthal anisotropy of neutrons measured at seven angles has been well reproduced using a theoretically predicted function of $$a$$ + $$b$$cos(2$$phi$$).

Journal Articles

Diffraction of $$gamma$$-rays with energies of 1.17 and 1.33 MeV by a flat Si crystal

Matsuba, Shunya*; Hayakawa, Takehito; Shizuma, Toshiyuki; Nishimori, Nobuyuki; Nagai, Ryoji; Sawamura, Masaru; Angell, C.; Fujiwara, Mamoru; Hajima, Ryoichi

Japanese Journal of Applied Physics, 54(5), p.052203_1 - 052203_5, 2015/05

 Times Cited Count:3 Percentile:13.81(Physics, Applied)

Journal Articles

Compact neutron sources for energy and security

Uesaka, Mitsuru*; Kobayashi, Hitoshi*; Kureta, Masatoshi; Nakatsuka, Shigehiro*; Nishimura, Kazuya*; Igashira, Masayuki*; Hori, Junichi*; Kiyanagi, Yoshiaki*; Tagi, Kazuhiro*; Seki, Toshichika*; et al.

Reviews of Accelerator Science and Technology, 8, p.181 - 207, 2015/00

We choose nuclear data and nuclear material inspection for energy application and nondestructive testing of explosive and hidden nuclear materials for security application. 90 keV electrostatic accelerators of deuterium are commercially available for nondestructive testing. For nuclear data measurement, electrostatic ion accelerators and L-band and S-band electron linear accelerators (linac) are used for the neutron source. Compact or mobile X-band electron linac neutron sources are under development. Compact proton linac neutron source is used for nondestructive testing especially water in solids. Several efforts for more neutron intensity using proton and deuteron accelerators are also introduced.

Journal Articles

Probing strongly correlated 4$$f$$-orbital symmetry of the ground state in Yb compounds by linear dichroism in core-level photoemission

Mori, Takeo*; Kitayama, Satoshi*; Kanai, Yuina*; Naimen, Sho*; Fujiwara, Hidenori*; Higashiya, Atsushi*; Tamasaku, Kenji*; Tanaka, Arata*; Terashima, Kensei*; Imada, Shin*; et al.

Journal of the Physical Society of Japan, 83(12), p.123702_1 - 123702_5, 2014/12

 Times Cited Count:16 Percentile:68.37(Physics, Multidisciplinary)

We show that the strongly correlated 4$$f$$-orbital symmetry of the ground state is revealed by linear dichroism in core-level photoemission spectra, as we have discovered for YbRh$$_{2}$$Si$$_{2}$$ and YbCu$$_{2}$$Si$$_{2}$$. Theoretical analysis shows us that the linear dichroism reflects the anisotropic charge distributions resulting from a crystalline electric field. We have successfully determined the ground-state 4$$f$$ symmetry for both compounds from the polarization-dependent angle resolved core-level spectra at a temperature well below the first excitation energy. The excited-state symmetry is also probed by temperature dependence of the linear dichroism where the high measurement temperatures are on the order of the crystal-field-splitting energies.

Journal Articles

Accurate structure analyses of polymer crystals on the basis of wide-angle X-ray and neutron diffractions

Tashiro, Koji*; Hanesaka, Makoto*; Yamamoto, Hiroko*; Wasanasuk, K.*; Jayaratri, P.*; Yoshizawa, Yoshinori*; Tanaka, Ichiro*; Niimura, Nobuo*; Kusaka, Katsuhiro*; Hosoya, Takaaki*; et al.

Kobunshi Rombunshu, 71(11), p.508 - 526, 2014/11

 Times Cited Count:6 Percentile:22.22(Polymer Science)

The crystal structure analysis of various polymer substances has been reviewed on the basis of wide-angle high-energy X-ray and neutron diffraction data. The progress in structural analytical techniques of polymer crystals have been reviewed at first. The structural models proposed so far were reinvestigated and new models have been proposed for various kinds of polymer crystals including polyethylene, poly(vinyl alcohol), poly(lactic acid) and its stereocomplex etc. The hydrogen atomic positions were also clarified by the quantitative analysis of wide-angle neutron diffraction data, from which the physical properties of polymer crystals have been evaluated theoretically. The bonded electron density distribution has been estimated for a polydiacetylene single crystal on the basis of the so-called X-N method or by the combination of structural information derived from X-ray and neutron diffraction data analysis. Some comments have been added about future developments in the field of structure-property relationship determination.

Journal Articles

Non-destructive measurements of nuclear materials in nuclear security

Hayakawa, Takehito; Fujiwara, Mamoru*

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 56(7), p.448 - 452, 2014/07

It is considered that progress of nuclear security is important in the world. A key technology for nuclear security is non-destructive measurements of hidden nuclear materials and radioactive isotopes in various conditions. For such purpose, we require helps of professional in wide range fields as nuclear physics, accelerator science, laser science, and nuclear fusion science etc. outside of the traditional nuclear engineering.

Journal Articles

Decontamination of school facilities in Fukushima-city

Yoshikawa, Hideki; Iijima, Kazuki; Sasamoto, Hiroshi; Fujiwara, Kenso; Mitsui, Seiichiro; Kitamura, Akira; Kurikami, Hiroshi; Tokizawa, Takayuki; Yui, Mikazu; Nakayama, Shinichi

Materials Research Society Symposium Proceedings, Vol.1518, p.269 - 275, 2013/10

Following the release of radionuclides into the environment as a result of the accident at Fukushima Daiichi Nuclear Power Plant, Japan Atomic Energy Agency (JAEA) had to develop an immediate and effective method of reducing the dose rate received by students in school facilities. A demonstration of a reducing method was carried out by JAEA at a junior high school ground and kindergarten yard in the center of Fukushima-city. Dose rates of the released radionuclides are largely controlled by the ground level contamination and accumulation of mainly cesium-137 ($$^{137}$$Cs) and cesium-134 ($$^{134}$$Cs) in populated areas. An effective means of reducing dose rate was to remove the surface soil and to bury it on-site under fresh uncontaminated soil or soil collected under deep depth at the site for shielding. The dose rate at1 m above ground level was reduced from 2.5 $$mu$$Sv/h to 0.15 $$mu$$Sv/h.

JAEA Reports

The International Atomic Energy Agency Nuclear Energy Management School 2012

Ohgama, Kazuya; Ando, Yoko; Yamaguchi, Mika; Ikuta, Yuko; Shinohara, Nobuo; Murakami, Hiroyuki; Yamashita, Kiyonobu; Uesaka, Mitsuru*; Demachi, Kazuyuki*; Komiyama, Ryoichi*; et al.

JAEA-Review 2013-004, 76 Pages, 2013/05

JAEA-Review-2013-004.pdf:13.53MB

JAEA together with the Japan Nuclear Human Resource Development Network (JN-HRD Net), the University of Tokyo (UT) and the Japan Atomic Industrial Forum (JAIF) cohosted the IAEA-Nuclear Energy Management School in Tokai Village, aiming that Japan will be the center of nuclear HRD in the Asian region. In the school, not only lectures by IAEA experts, but also lectures by Japanese experts and technical visits were included for foreign participants. The school contributed to the internationalization of Japanese young professionals, development of nuclear human resource of other countries, and enhancement of cooperation between IAEA and Japan. Additionally, collaborative relationship within JN-HRD Net was strengthened by the school. In this report, findings obtained during the preparatory work and the school period are reported for future international nuclear HRD activities in Japan.

Journal Articles

Removal of cesium using cobalt-ferrocyanide-impregnated polymer-chain-grafted fibers

Ishihara, Ryo*; Fujiwara, Kunio*; Harayama, Takato*; Okamura, Yusuke*; Uchiyama, Shoichiro*; Sugiyama, Mai*; Someya, Takaaki*; Amakai, Wataru*; Umino, Satoshi*; Ono, Tsubasa*; et al.

Journal of Nuclear Science and Technology, 48(10), p.1281 - 1284, 2011/10

AA2011-0190.pdf:0.45MB

 Times Cited Count:44 Percentile:94.62(Nuclear Science & Technology)

Journal Articles

Proposal for an advanced hybrid K-edge/XRF densitometry (HKED) using a monochromatic photon beam from laser Compton scattering

Shizuma, Toshiyuki; Hajima, Ryoichi; Hayakawa, Takehito; Fujiwara, Mamoru; Sonoda, Takashi; Seya, Michio

Nuclear Instruments and Methods in Physics Research A, 654(1), p.597 - 603, 2011/10

 Times Cited Count:4 Percentile:32.67(Instruments & Instrumentation)

The general purpose Monte Carlo electron-$$gamma$$ shower computer code (EGS5) was used to obtain the U, Np, and Pu X-ray response from the hybrid K-edge/XRF densitometry (HKED). In the present simulation, we adopt a monochromatic, linearly polarized photon beam generated by inverse Compton scattering of laser light with high energy electrons from an energy recovery linac. The simulation has been carried out under various conditions of the U, Np, and Pu concentrations to investigate the effect to counting rates as well as counting precision. The results of the simulation show that the assessment time for low concentration Pu input solutions can be reduced by the improvement of signal-to-background ratios. The Np concentration can also be determined with a counting precision of approximately 1% in standard deviation during the 1 hour measurement for a 3N HNO$$_3$$ sample solution including U (100 g/L), Np (0.1 g/L), and Pu (20 or 100 g/L).

Journal Articles

Event structure and double helicity asymmetry in jet production from polarized $$p + p$$ collisions at $$sqrt{s}$$ = 200 GeV

Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Y.*; Al-Bataineh, H.*; Alexander, J.*; Aoki, K.*; Aphecetche, L.*; Armendariz, R.*; et al.

Physical Review D, 84(1), p.012006_1 - 012006_18, 2011/07

 Times Cited Count:29 Percentile:73.24(Astronomy & Astrophysics)

We report on the event structure and double helicity asymmetry ($$A_{LL}$$) of jet production in longitudinally polarized $$p + p$$ collisions at $$sqrt{s}$$ = 200 GeV. Photons and charged particles were measured by the PHENIX experiment. Event structure was compared with the results from PYTHIA event generator. The production rate of reconstructed jets is satisfactorily reproduced with the next-to-leading-order perturbative QCD calculation. We measured $$A_{LL}$$ = -0.0014 $$pm$$ 0.0037 at the lowest $$P_T$$ bin and -0.0181 $$pm$$ 0.0282 at the highest $$P_T$$ bin. The measured $$A_{LL}$$ is compared with the predictions that assume various $$Delta G(x)$$ distributions.

148 (Records 1-20 displayed on this page)