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Nagai, Takayuki; Okamoto, Yoshihiro; Shibata, Daisuke*; Kojima, Kazuo*; Hasegawa, Takehiko*; Sato, Seiichi*; Fukaya, Akane*; Hatakeyama, Kiyoshi*
JAEA-Research 2024-014, 54 Pages, 2025/02
JAEA-Research-2024-014.pdf:7.02MB
XAFS measurements in the soft X-ray region are suitable for evaluating the chemical state of the surface layer of a measurement sample because the X-ray transmittance is low. In this study, the purpose of the study was to confirm the difference between the coagulated surface layer and the inside of the simulated waste glasses by measuring the K-edge of the glass constituent elements boron, oxygen, sodium, and silicon, and the L
edge of the waste component cerium. As a result, the B K-edge XANES spectra showed that the proportion of B-O tetracoordinate sp
structures (BO
) on the surface layer of the coagulated glass samples was higher than that on the cut surface inside the glass samples, which is expected to improve the water resistance of the coagulated surface. On the other hand, the O K-edge XANES spectra suggested that the O abundance in the coagulated surface layer was lower than that in the cut surface inside the glass samples, and that alkali metal elements may be concentrated in the coagulated surface layer. However, no difference was observed in the Na K-edge XANES spectra between the coagulated surface layer and the cut surface, and no difference was observed in the Si K-edge XANES spectra between the solidified surface and the inside of glass samples. In addition, the Ce L-edge XANES spectra confirmed that the Ce valence in the surface layer of coagulated glass samples were oxidized compared to the inside of glass samples.
Fukaya, Yuki
Vacuum and Surface Science, 68(2), p.91 - 96, 2025/02
3-Si phase on Al(111), studied by the multiple usages of positron diffraction and core-level photoemission spectroscopySato, Yusuke*; Fukaya, Yuki; 14 of others*
Physical Review Materials (Internet), 9(1), p.014002_1 - 014002_11, 2025/01
Times Cited Count：0 Percentile：0.00(Materials Science, Multidisciplinary)no abstracts in English
Okita, Shoichiro; Aoki, Takeshi; Fukaya, Yuji; Tachibana, Yukio
Proceedings of 31st International Conference on Nuclear Engineering (ICONE31) (Internet), 5 Pages, 2024/11
Higuchi, Yuki*; Yoshimune, Wataru*; Kato, Satoru*; Hibi, Shogo*; Setoyama, Daigo*; Isegawa, Kazuhisa*; Matsumoto, Yoshihiro*; Hayashida, Hirotoshi*; Nozaki, Hiroshi*; Harada, Masashi*; et al.
Communications Engineering (Internet), 3, p.33_1 - 33_7, 2024/02
Koyama, Shinichi; Ikeuchi, Hirotomo; Mitsugi, Takeshi; Maeda, Koji; Sasaki, Shinji; Onishi, Takashi; Tsai, T.-H.; Takano, Masahide; Fukaya, Hiroyuki; Nakamura, Satoshi; et al.
Hairo, Osensui, Shorisui Taisaku Jigyo Jimukyoku Homu Peji (Internet), 216 Pages, 2023/11
In FY 2021 and 2022, JAEA perfomed the subsidy program for "the Project of Decommissioning and Contaminated Water Management (Development of Analysis and Estimation Technology for Characterization of Fuel Debris (Development of Technologies for Enhanced Analysis Accuracy, Thermal Bahavior Estimation, and Simplified Analysis of Fuel Debris)" started in FY 2021. This presentation material summarized the results of the project, which will be available shortly on the website of Management Office for the Project of Decommissioning, Contaminated Water and Treated Water Management.
Fukaya, Yuki; Entani, Shiro*; Sakai, Seiji*
Physical Review B, 108(15), p.155422_1 - 155422_6, 2023/10
Times Cited Count：2 Percentile：29.03(Materials Science, Multidisciplinary)no abstracts in English
Kobayashi, Fuyumi; Fukaya, Hiroyuki; Izawa, Kazuhiko; Kida, Takashi; Sono, Hiroki; Suyama, Kenya
Proceedings of 12th International Conference on Nuclear Criticality Safety (ICNC2023) (Internet), 7 Pages, 2023/10
In the criticality experiment in the new STACY, pseudo fuel debris samples are used to acquire data for validation of the system used for 1F debris criticality safety assessment. The pseudo fuel debris is a pellet with a diameter of 8 mm and a height of 10 mm containing uranium oxide and structural materials (iron, silicon, zirconium, etc.). The pellets are made by mixing, pressing and sintering uranium dioxide powder and structural materials powder. The UO
powder uses the same composition of uranium as the STACY driver fuel rods, in order to reduce the errors in fuel composition. The pseudo fuel debris fabrication devices and analysis equipment are installed at the BECKY in order to evaluate the critical properties of fuel debris with high accuracy in dimension and analysis. This equipment is located in the same laboratory and can quickly respond to experimental needs such as preparation of the pseudo fuel debris and analysis before and after irradiation.
Nagai, Takayuki; Okamoto, Yoshihiro; Yamagishi, Hirona*; Shibata, Daisuke*; Kojima, Kazuo*; Hasegawa, Takehiko*; Sato, Seiichi*; Fukaya, Akane*; Hatakeyama, Kiyoshi*
JAEA-Research 2023-004, 45 Pages, 2023/09
JAEA-Research-2023-004.pdf:6.07MB
The local structure of glass-forming elements and waste elements in borosilicate glasses varies with its chemical composition. In this study, simulated waste glass samples were prepared and the chemical state regarding boron (B), silicon (Si) and waste elements of iron (Fe), cesium (Cs) were estimated by using XAFS measurement in soft X-ray region. To understand the chemical stability of simulated waste glasses, XANES spectra of B K-edge, Fe L, L-edge, and Cs M
, M-edge were measured on the glass surface exposed to the leachate. As a result, it was found that the glass surface exposed to the leachate was changed and it was difficult to obtain a clear XANES spectrum. From the B K-edge XANES spectra on glass surfaces exposed to the leachate, an increase in three-coordination of B-O (BO) and a decrease in four-coordination of B-O (BO) were observed compared to the glass surfaces before immersion. The XANES spectra of Fe L, L-edge, and Cs M, M-edge show that as the exposure time in the leachate increases, the Cs present on the glass surface dissolves into the leachate. The XANES spectra of Si K-edge were measured on simulated waste glass surfaces before immersion, and it was confirmed that the change in XANES spectra given by NaO concentration had a larger effect than the waste component concentration.
Okita, Shoichiro; Fukaya, Yuji; Sakon, Atsushi*; Sano, Tadafumi*; Takahashi, Yoshiyuki*; Unesaki, Hironobu*
Nuclear Science and Engineering, 197(8), p.2251 - 2257, 2023/08
Times Cited Count：1 Percentile：15.53(Nuclear Science & Technology)Kawamura, Takaaki*; Fukaya, Yuki; Fukutani, Katsuyuki
Surface Science, 722, p.122098_1 - 122098_8, 2022/08
Times Cited Count：1 Percentile：7.01(Chemistry, Physical)no abstracts in English
Fukaya, Yuji; Okita, Shoichiro; Kanda, Shun*; Goto, Masaki*; Nakajima, Kunihiro*; Sakon, Atsushi*; Sano, Tadafumi*; Hashimoto, Kengo*; Takahashi, Yoshiyuki*; Unesaki, Hironobu*
KURNS Progress Report 2021, P. 101, 2022/07
The Japan Atomic Energy Agency (JAEA) started the Research and Development (R&D) to improve nuclear prediction techniques for High Temperature Gas-cooled Reactors (HTGRs) in 2018. The objectives are to intro-duce the generalized bias factor method to avoid full mock-up experiment for the first commercial HTGR and to improve neutron instrumentation system by virtue of the particular characteristics due to a graphite moderation system. For this end, we composed B7/4"G2/8"p8EU(3)+3/8"p38EU in the B-rack of Kyoto University Critical Assembly (KUCA) in 2021.
Sakon, Atsushi*; Hashimoto, Kengo*; Sano, Tadafumi*; Nakajima, Kunihiro*; Kanda, Shun*; Goto, Masaki*; Fukaya, Yuji; Okita, Shoichiro; Fujimoto, Nozomu*; Takahashi, Yoshiyuki*
KURNS Progress Report 2021, P. 100, 2022/07
The R&D of reactor noise analysis to obtain HTGR nuclear characteristics have been performed with Kyoto University Critical Assembly (KUCA). In the last study, a neutron detector located about 55 cm away of fuel assembly measured the auto power spectral density. However, the prompt neutron decay constants obtained by this detector was different from that of other detectors. The objective of this study is experimental study of reactor noise analysis by the power spectrum method using neutron detector placed outside reactor core.
Fukaya, Yuji; Ohashi, Hirofumi; Sato, Hiroyuki; Goto, Minoru; Kunitomi, Kazuhiko
Nihon Genshiryoku Gakkai Wabun Rombunshi (Internet), 21(2), p.116 - 126, 2022/06
An improvement electricity generation cost evaluation method for High Temperature Gas-cooled Reactors (HTGRs) has been performed. Japan Atomic Energy Agency (JAEA) had completed the commercial HTGR concept named Gas Turbine High Temperature Reactor (GTHTR300) and the electricity generation cost evaluation method approximately a decade ago. The cost evaluation was developed based on the method of Federation of Electric Power Companies (FEPC). The FEPC method was drastically revised after the Fukushima Daiichi nuclear disaster. Moreover, the escalation of material and labor cost for the decade should be consider to evaluate the latest cost. Therefore, we revised the cost evaluation method for GTHTR300 and the cost was compared with that of Light Water Reactor (LWR). As a result, it was found that the electricity generation cost of HTGR of 7.9 yen/kWh is cheaper than that of LWR of 11.7 yen/kWh by approximately 30% at the capacity factor of 70%.
Okita, Shoichiro; Fukaya, Yuji; Sakon, Atsushi*; Sano, Tadafumi*; Takahashi, Yoshiyuki*; Unesaki, Hironobu*
Proceedings of International Conference on Physics of Reactors 2022 (PHYSOR 2022) (Internet), 9 Pages, 2022/05
Zhao, Y.*; Suzuki, T.*; Iimori, T.*; Kim, H.-W.*; Ahn, J. R.*; Horio, Masafumi*; Sato, Yusuke*; Fukaya, Yuki; Kanai, T.*; Okazaki, K.*; et al.
Physical Review B, 105(11), p.115304_1 - 115304_8, 2022/03
Times Cited Count：1 Percentile：7.68(Materials Science, Multidisciplinary)no abstracts in English
Takahashi, Tomoyuki*; Fukaya, Yukiko*; Iimoto, Takeshi*; Uni, Yasuo*; Kato, Tomoko; Sun, S.*; Takeda, Seiji; Nakai, Kunihiro*; Nakabayashi, Ryo*; Uchida, Shigeo*; et al.
Hoken Butsuri (Internet), 56(4), p.288 - 305, 2021/12
We report the results of activities related to the Task Group of Parameters Used in Biospheric Dose Assessment Models for Radioactive Waste Disposal at the Japan Health Physics Society.
Fukaya, Yuki; Zhao, Y.*; Kim, H.-W.*; Ahn, J.-R.*; Fukidome, Hirokazu*; Matsuda, Iwao*
Physical Review B, 104(18), p.L180202_1 - L180202_5, 2021/11
Times Cited Count：16 Percentile：72.25(Materials Science, Multidisciplinary)no abstracts in English
Koyama, Shinichi; Nakagiri, Toshio; Osaka, Masahiko; Yoshida, Hiroyuki; Kurata, Masaki; Ikeuchi, Hirotomo; Maeda, Koji; Sasaki, Shinji; Onishi, Takashi; Takano, Masahide; et al.
Hairo, Osensui Taisaku jigyo jimukyoku Homu Peji (Internet), 144 Pages, 2021/08
JAEA performed the subsidy program for the "Project of Decommissioning and Contaminated Water Management (Development of Analysis and Estimation Technology for Characterization of Fuel Debris (Development of Technologies for Enhanced Analysis Accuracy and Thermal Behavior Estimation of Fuel Debris))" in 2020JFY. This presentation summarized briefly the results of the project, which will be available shortly on the website of Management Office for the Project of Decommissioning and Contaminated Water Management.
Takeda, Tetsuaki*; Inagaki, Yoshiyuki; Aihara, Jun; Aoki, Takeshi; Fujiwara, Yusuke; Fukaya, Yuji; Goto, Minoru; Ho, H. Q.; Iigaki, Kazuhiko; Imai, Yoshiyuki; et al.
High Temperature Gas-Cooled Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.5, 464 Pages, 2021/02
As a general overview of the research and development of a High Temperature Gas-cooled Reactor (HTGR) in JAEA, this book describes the achievements by the High Temperature Engineering Test Reactor (HTTR) on the designs, key component technologies such as fuel, reactor internals, high temperature components, etc., and operational experience such as rise-to-power tests, high temperature operation at 950
C, safety demonstration tests, etc. In addition, based on the knowledge of the HTTR, the development of designs and component technologies such as high performance fuel, helium gas turbine and hydrogen production by IS process for commercial HTGRs are described. These results are very useful for the future development of HTGRs. This book is published as one of a series of technical books on fossil fuel and nuclear energy systems by the Power Energy Systems Division of the Japan Society of Mechanical Engineers.
