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Journal Articles

Role of advection in atmospheric ammonia; A Case study at a Japanese lake basin influenced by agricultural ammonia sources

Kubota, Tomohiro; Kuroda, Hisao*; Watanabe, Mirai*; Takahashi, Akiko*; Nakazato, Ryoji*; Tarui, Mika*; Matsumoto, Shunichi*; Nakagawa, Keita*; Numata, Yasuko*; Ouchi, Takao*; et al.

Atmospheric Environment, 243, p.117856_1 - 117856_9, 2020/12

 Times Cited Count:3 Percentile:15.82(Environmental Sciences)

The dry and wet depositions of atmospheric ammonia (NH$$_{3}$$) is one of the important pathways of nitrogen loads to aquatic ecosystems. Crop and livestock agriculture, one of the largest emitters of NH$$_{3}$$ in Asian countries, are known to cause high spatial and seasonal variation of NH$$_{3}$$ and influence the surrounding lake basin areas via its dry and wet deposition. However, the spatial characteristics of the NH$$_{3}$$ concentration in basin scale are not completely understood for regulation in NH$$_{3}$$ emission. Here we aim to clarify dominant factors of spatial and seasonal variations of the NH$$_{3}$$ concentration in a eutrophic lake basin surrounded by agricultural areas in Japan. Passive sampling over various land use categories in the basin was conducted at 36 sites in total from October 2018 to January 2020. Interestingly, the observed NH$$_{3}$$ concentration near the livestock houses were higher in winter than summer, which was inconsistent with knowledge of seasonal changes of current NH$$_{3}$$ emission inventory based on temperature-driven volatilization process. Comparing monthly NH$$_{3}$$ concentrations with various meteorological factors, we suggested the importance of seasonal advection of NH$$_{3}$$ from high emission sources to which has been rarely paid attention by the previous past studies. As for this, should be considered for lake ecosystem management since deposition of NH$$_{3}$$ is known to be closely related to the ecological processes such as phytoplankton blooming.

Journal Articles

Characterization and storage of radioactive zeolite waste

Yamagishi, Isao; Nagaishi, Ryuji; Kato, Chiaki; Morita, Keisuke; Terada, Atsuhiko; Kamiji, Yu; Hino, Ryutaro; Sato, Hiroyuki; Nishihara, Kenji; Tsubata, Yasuhiro; et al.

Journal of Nuclear Science and Technology, 51(7-8), p.1044 - 1053, 2014/07

 Times Cited Count:19 Percentile:78.38(Nuclear Science & Technology)

For safe storage of zeolite wastes generated by treatment of radioactive saline water at the Fukushima Daiichi Nuclear Power Station, properties of the Herschelite adsorbent were studied and its adsorption vessel was evaluated for hydrogen production and corrosion. Hydrogen production depends on its water level and dissolved species because hydrogen is oxidized by radicals in water. It is possible to evaluate hydrogen production rate in Herschelite submerged in seawater or pure water by taking into account of the depth effect of the water. The reference vessel of decay heat 504 W with or without residual pure water was evaluated for the hydrogen concentration by thermal hydraulic analysis using obtained fundamental properties. Maximum hydrogen concentration was below the lower explosive limit (4 %). The steady-state corrosion potential of a stainless steel 316L increased with absorbed dose rate but its increase was repressed by the presence of Herschelite. At 750 Gy/h and $$<$$60$$^{circ}$$C which were values evaluated at the bottom of the vessel of 504 W, the localized corrosion of SUS316L contacted with Herschelite would not immediately occur under 20,000 ppm of Cl$$^{-}$$ concentration.

Journal Articles

Safe storage of zeolite adsorbents used for treatment of accident-generated water at Fukushima Daiichi Power Station

Yamagishi, Isao; Nagaishi, Ryuji; Terada, Atsuhiko; Kamiji, Yu; Kato, Chiaki; Morita, Keisuke; Nishihara, Kenji; Tsubata, Yasuhiro; Ji, W.*; Fukushima, Hisashi*; et al.

IAEA-CN-211 (Internet), 5 Pages, 2013/01

Since the accident at Fukushima Daiichi Nuclear Power Station, a large amount of radioactive contaminated water has been generated to cool damaged reactor cores. Adsorption of cesium with zeolite-like media was employed for treatment of this contaminated saline water. As spent zeolite media are highly radioactive, their safe storage is a pressing issue. Japan Atomic Energy Agency has extensively conducted R&D on the management of secondary wastes produced by the operation of the treatment system. Subjects on the safe storage of spent zeolites include the analysis of their characteristics and the evaluation of effectiveness of the present safety measures in consideration of decay heat emission and hydrogen generation by water radiolysis as well as durability of vessels exposed to saline. Preliminary results obtained are described in the present paper.

JAEA Reports

FY 2003 JNC R&D on HLW disposal technology

Fukushima, Isao; Takeda, Seietsu; Yamazaki, Shinichi; Ishikawa, Hirohisa

JNC TN1400 2003-014, 65 Pages, 2004/02

JNC-TN1400-2003-014.pdf:47.43MB

none

JAEA Reports

None

Fukushima, Mineo; Ojima, Hisao

PNC TN8420 91-012, 22 Pages, 1991/03

PNC-TN8420-91-012.pdf:0.44MB

None

JAEA Reports

Experience and projects for treatment, conditioning and strage of all radioactive wastes from Tokai Reprocessing Plant

Matsumoto, Kenichi*; Miyahara, Kenji; ; Asazuma, Shinichiro; Fukushima, Isao; Shoji, Kenji; Nojima, Yasuo; Kimura; Ikeda; Shibuya, Jun*; et al.

PNC TN8440 87-194, 82 Pages, 1987/08

PNC-TN8440-87-194.pdf:4.92MB

no abstracts in English

JAEA Reports

None

*; Yasu, Takami; Shoji, Kenji; Fukushima, Isao; *; Shibuya, Jun; ; ; Yamamoto, Masao

PNC TN8440 87-190, 35 Pages, 1987/08

PNC-TN8440-87-190.pdf:2.43MB

no abstracts in English

Oral presentation

Thermal conductivity of mordenite from Ayashi and herschelite

Ji, W.*; Fukushima, Hisashi*; Sato, Seichi*; Kozaki, Tamotsu*; Yamagishi, Isao; Nishihara, Kenji

no journal, , 

no abstracts in English

Oral presentation

Thermal conductivity of cement paste containing zeolite

Fukushima, Hisashi*; Ji, W.*; Sato, Seichi*; Kozaki, Tamotsu*; Yamagishi, Isao; Nishihara, Kenji

no journal, , 

no abstracts in English

Oral presentation

Thermal conductivity of granular zeolite in helium atmosphere and under vacuum

Ji, W.*; Fukushima, Hisashi*; Sato, Seichi*; Watanabe, Naoko*; Kozaki, Tamotsu*; Yamagishi, Isao; Nishihara, Kenji; Terada, Atsuhiko

no journal, , 

no abstracts in English

Oral presentation

Feasibility study for disposal of cement waste form containing cesium-adsorbed zeolite

Fukushima, Hisashi*; Sato, Seichi*; Watanabe, Naoko*; Kozaki, Tamotsu*; Yamagishi, Isao; Nishihara, Kenji

no journal, , 

no abstracts in English

Oral presentation

Role of advection in atmospheric ammonia; A Case study at a Japanese lake basin influenced by agricultural ammonia sources

Katata, Genki*; Kubota, Tomohiro; Kuroda, Hisao*; Watanabe, Mirai*; Takahashi, Akiko*; Nakazato, Ryoji*; Tarui, Mika*; Matsumoto, Shunichi*; Nakagawa, Keita*; Numata, Yasuko*; et al.

no journal, , 

no abstracts in English

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