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Teshigawara, Makoto; Ikeda, Yujiro*; Muramatsu, Kazuo*; Sutani, Koichi*; Fukuzumi, Masafumi*; Noda, Yohei*; Koizumi, Satoshi*; Saruta, Koichi; Otake, Yoshie*
Journal of Neutron Research, 26(2-3), p.69 - 74, 2024/09
Slow neutrons, such as cold neutrons, are important non-destructive probes not only for basic physics but also for the structural genomics advancements in the life sciences and the battery technology advancements needed for the transition to a hydrogen society. Neutron-based science is also known as high-neutron-intensity-dependent science. A new unique method focusing on nanosized particle aggregation has been proposed to increase neutron intensity in that energy region. The method is based on intensity enhancement by multiple coherent scatterings with nanosized particle aggregation. The aggregation of nanosized particles matches the wavelength of below cold neutrons, causing a similar effect to coherent scattering, so-called Bragg scattering, leading to neutron intensity enhancement by several orders of magnitude. Nanodiamonds and magnesium hydride have recently been studied numerically and experimentally. The major challenge with nanodiamonds in practical applications is the molding method. Another carbon structure, graphene is focused on to find a solution to this problem. It is hypothesized that nanosized graphene could aid coherent neutron scattering under particle size conditions similar to nanodiamonds. We report the potential of nanosized graphene as a reflector material below cold neutrons, together with experimental results.
Teshigawara, Makoto; Ikeda, Yujiro*; Yan, M.*; Muramatsu, Kazuo*; Sutani, Koichi*; Fukuzumi, Masafumi*; Noda, Yohei*; Koizumi, Satoshi*; Saruta, Koichi; Otake, Yoshie*
Nanomaterials (Internet), 13(1), p.76_1 - 76_9, 2023/01
Times Cited Count:4 Percentile:60.72(Chemistry, Multidisciplinary)To enhance neutron intensity below cold neutrons, it is proposed that nanosized graphene aggregation could facilitate neutron coherent scattering under particle size conditions similar to nanodiamond. It might also be possible to use it in high neutron radiation conditions due to graphene's strong sp2 bonds. Using the RIKEN accelerator-driven compact neutron source and iMATERIA at J-PARC, we performed neutron measurement experiments, total neutron cross-section, and small-angle neutron scattering on nanosized graphene aggregation. The measured data revealed, for the first time, that nanosized graphene aggregation increased the total cross-sections and small-angle scattering in the cold neutron energy region, most likely due to coherent scattering, resulting in higher neutron intensities, similar to nanodiamond.
Hori, Fuminobu*; Fukuzumi, Masafumi*; Kawasuso, Atsuo; Zushi, Yoshihiro*; Chimi, Yasuhiro; Ishikawa, Norito; Iwase, Akihiro*
Physica Status Solidi (C), 4(10), p.3530 - 3533, 2007/09
Times Cited Count:0 Percentile:0.00(Physics, Atomic, Molecular & Chemical)no abstracts in English
Zushi, Yoshihiro*; Fukuzumi, Masafumi*; Chimi, Yasuhiro; Ishikawa, Norito; Ono, Fumihisa*; Iwase, Akihiro*
Nuclear Instruments and Methods in Physics Research B, 256(1), p.434 - 437, 2007/03
Times Cited Count:23 Percentile:80.90(Instruments & Instrumentation)Fe-50at.%Rh alloys were irradiated with swift heavy ions such as 120 MeV Ni, 150 MeV Kr, 200 MeV Xe, 200 MeV Au, and it is found that low-temperature antiferromagnetic state changes to ferromagnetic state after the irradiations. The ion-fluence dependence and ion-species dependence was investigated. It is found that saturated magnetization evolves as fluence increases, and the evolution behavior for different ion-species differs from each other, but it scales with single universal curve as a function of total energy deposition via elastic collision.
Iwase, Akihiro*; Fukuzumi, Masafumi*; Zushi, Yoshihiro*; Suzuki, Motohiro*; Takagaki, Masafumi*; Kawamura, Naomi*; Chimi, Yasuhiro; Mizuki, Junichiro; Ishikawa, Norito; Ono, Fumihisa*
Nuclear Instruments and Methods in Physics Research B, 256(1), p.429 - 433, 2007/01
Times Cited Count:19 Percentile:75.94(Instruments & Instrumentation)We have studied the effects of swift heavy ion irradiation on the magnetic properties of Fe-Rh intermetallic compound by using Fe K-edge X-ray magnetic circular dichroism (XMCD) at 20 K. For an unirrdaiated specimen, no signal of XMCD spectrum has been observed because Fe-Rh intermetallic compound is intrinsically anti-ferromagnetic below room temperature. For the specimens irradiated with 120-200 MeV Ni, Kr, Xe or Au ions, we have found XMCD spectra which are characterized by a dispersion-type profile with a positive peak and a negative peak near Fe K-edge. The intensity of XMCD spectra remarkably depends on ion-fluence and ion-mass. The experimental result implies that the ferromagnetic state is induced by the swift heavy ion irradiation. The change in magnetic state of Fe element is discussed in terms of energy deposition through the elastic and electronic processes.
Iwase, Akihiro*; Chimi, Yasuhiro; Ishikawa, Norito; Nakatani, Rikizo*; Kato, Yuzaburo*; Fukuzumi, Masafumi*; Tsuchida, Hidetsugu*; Baba, Yuji
Nuclear Instruments and Methods in Physics Research B, 245(1), p.141 - 144, 2006/04
Times Cited Count:0 Percentile:0.00(Instruments & Instrumentation)Diffusion of Si atoms in Pd under energetic ion irradiation is studied in Pd-Si thin layer system using synchrotron radiation photoemission spectroscopy. Specimens are prepared by depositing Pd on Si single crystals. The Pd layer thicknesses are 10-300 nm. Before irradiation, we observe photoemission spectra only for Pd, but do not find any trace of Si. After irradiation with 3-MeV Si ions, 1-MeV O ions or 200-MeV Xe ions, we observe an additional photoemission component at the binding energy about 3 eV higher than that of Si 1s bulk component. The experimental result implies that the energetic ion-irradiation induces the diffusion of Si atoms from the Si-Pd interface to the Pd layer surface. The shift of the binding energy from the value for the Si bulk can be interpreted as arising from electron charge transfer from Si to Pd. The dependences of photoemission spectra and ion-irradiation induced diffusion on ion-species and ion-fluence are discussed.
Fukuzumi, Masafumi*; Chimi, Yasuhiro; Ishikawa, Norito; Suzuki, Motohiro*; Takagaki, Masafumi*; Mizuki, Junichiro; Ono, Fumihisa*; Neumann, R.*; Iwase, Akihiro*
Nuclear Instruments and Methods in Physics Research B, 245(1), p.161 - 165, 2006/04
Times Cited Count:18 Percentile:75.22(Instruments & Instrumentation)We have performed swift heavy ion irradiations in Fe-50at.%Rh alloys at room temperature. Before and after the irradiations, the magnetic properties and the lattice structure are measured using Superconducting QUantum Interference Device (SQUID) and X-Ray Diffractometer (XRD), respectively. We have also performed X-ray Magnetic Circular Dichroism (XMCD) measurement near the Fe K-edge at the synchrotron radiation facility, SPring-8, to examine the irradiation-induced ferromagnetic state near the specimen surface. We have found that the swift heavy ion irradiations induce the ferromagnetic state in Fe-50at.%Rh alloy below the antiferromagnetism-ferromagnetism transition temperature of the unirradiated alloy and the lattice expasion by 0.3%. For the specimens irradiated with swift heavy ions, we observe the XMCD spectra correponding to ferromagnetisim, which depend on the mass of irradiating ions and/or irradiation fluence. Effects of energy loss through electronic excitation and elastic collisions on lattice and magnetic structures of Fe-Rh alloy are discussed.
Teshigawara, Makoto; Ikeda, Yujiro*; Muramatsu, Kazuo*; Sutani, Koichi*; Fukuzumi, Masafumi*; Noda, Yohei*; Koizumi, Satoshi*; Kawamura, Yuji*; Saruta, Koichi; Otake, Yoshie*
no journal, ,
Science using neutrons in the nanometer (nm) wavelength region as probes is expanding into a wide range of fields, from basic research in materials and life science to industrial applications. Dramatic increase in the intensity of the beam source is required to drive such research. To increase the intensity of neutron beams, we have focused on coherent scattering caused by nano-sized particle aggregations. We focused on graphene, which is different from nanodiamond that has been vigorously researched and developed, and started to develop its nano-sized aggregates, which have high van der Waals force of more than one order of magnitude and stronger bonding force between carbons than nanodiamond, so that they can be easily formed into a lump shape and adapted to higher radiation fields. The graphene is expected to be formable into clumps and adaptable to higher radiation fields. By promoting chemical vapor deposition (CVD), we have established a technique to form nano-sized graphene (graphene flower) with a shape similar to a sunflower flower. In this talk, we report on the neutron scattering characteristics that contribute to the coherent scattering of the newly developed graphene flowers.
Muramatsu, Kazuo*; Sutani, Koichi*; Kimishima, Koichi*; Teshigawara, Makoto; Ikeda, Yujiro*; Fukuzumi, Masafumi*; Koizumi, Satoshi*; Kawamura, Yuji*; Saruta, Koichi; Otake, Yoshie*
no journal, ,
The use of nano-diamonds has been vigorously investigated to increase the intensity of neutron beams, focusing on the coherent scattering caused by nano-sized particle aggregations. Sp2 intercarbon-bonded graphene has a larger van der Waals force than sp3 intercarbon-bonded nano-diamonds. It is expected to be more easily formed into a lump shape and adaptability to higher radiation fields. On the other hand, the large cohesive nature of graphene makes it difficult to construct nano-sized three-dimensional structures. To solve this problem, we focused on the Hot Isostatic Pressing (HIP) method, which uses resin powder as a raw material and produces vapor-phase grown graphene. In this talk, we will report on the preparation of graphene flower structures, in which nano-sized graphene is three-dimensionally freestanding, how to control the nano-size of graphene, and a prototype of graphene neutron reflector material.
Hori, Fuminobu*; Fukuzumi, Masafumi*; Kawasuso, Atsuo; Iwase, Akihiro*
no journal, ,
no abstracts in English
Ishikawa, Norito; Chimi, Yasuhiro; Michikami, Osamu*; Ota, Yasuyuki*; Saito, Yuichi; Chiba, Atsuya; Fukuzumi, Masafumi*; Hori, Fuminobu*; Iwase, Akihiro*
no journal, ,
no abstracts in English